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Antonio Ramos

Publications and source records attributed to Antonio Ramos.

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Shear-Induced Electrophoretic Migration Perpendicular to the Electric Field

Recent experiments combining electrophoresis with pressure-driven flows in microchannels have revealed that microparticles undergo lateral migration perpendicular to the applied electric field. Although fluid inertia has been proposed as a possible explanation, inertial effects are negligibly small in these regimes, leaving the underlying physical mechanism an open question. In this study, we address these observations by extending previous theoretical work on concentration polarization,i.e., the external-field-induced modification of the ionic concentration field surrounding a dielectric object. We consider a dielectric particle with surface conductance subjected simultaneously to an external electric field and a shear flow. We show that the shear flow breaks the symmetry of the ionic concentration around the particle in the direction perpendicular to the applied field, thereby driving lateral migration. We demonstrate that the resulting migration velocity comprises two distinct contributions: an electrophoretic and a diffusiophoretic component. Our theory yields an explicit expression for the velocity magnitude as a function of the zeta potential and the Dukhin number, predicting typical speeds on the order of $\mathrm{\mu}$m/s for representative experimental parameters. Notably, the model also predicts a reversal in the migration direction for Dukhin numbers of order unity.

cond-mat.soft

Understanding the Origin of a Second Mobility Reversal in Optoelectrically Powered Metallo-Dielectric Janus Particles

While previous studies indicated the mobility reversal of an electrically-powered metallo-dielectric Janus particle (JP) with increasing frequency, here we report an intriguing second mobility reversal observed in optoelectronically-driven JPs. In contrast to the commonly used setup with parallel ITO-coated glass substrates to induce a uniform electric field orthogonal to the velocity direction, this setup incorporates a thin photoconductive layer deposited on the bottom ITO-coated glass substrate. We have found that the reversal is associated with the asymmetry of the bottom substrate's photoconductivity, localized underneath the JP, resulting from the self-shading effect of the metallic hemisphere under top optical illumination. Numerous control tests, including optical illumination from the bottom, along with numerical simulations, support this hypothesized mechanism

cond-mat.mtrl-sci

Dynamics of fixed-volume pinned film -- dealing with a non-self-adjoint thin film problem

The use of thin liquid films has expanded beyond lubrication and coatings, and into applications in actuators and adaptive optical elements. In contrast to their predecessors, whose dynamics can be typically captured by modelling infinite or periodic films, these applications are characterized by a finite amount of liquid in an impermeable domain. The global mass conservation constraint, together with common boundary conditions (e.g., pinning) create quantitatively and qualitatively different dynamics than those of infinite films. Mathematically, this manifests itself as a non-self-adjoint problem. This work presents a combined theoretical and experimental study for this problem. We provide a time-dependent closed-form analytical solution for the linearized non-self-adjoint system that arises from these boundary conditions. We highlight that, in contrast to self-adjoint problems, here special care should be given to deriving the adjoint problem to reconstruct the solution based on the eigenfunctions properly. We compare these solutions with those obtained for permeable and periodic boundary conditions, representing common models for self-adjoint thin-film problems. We show that while the initial dynamics are nearly identical, the boundary conditions eventually affect the film deformation as well as its response time. To experimentally illustrate the dynamics and to validate the theoretical model, we fabricated an experimental setup that subjects a thin liquid film to a prescribed normal force distribution through dielectrophoresis, and used high-frame-rate digital holography to measure the film deformation in real-time. The experiments agree well with the model and confirm that confined films exhibit different behaviour which could not be predicted by existing models.

physics.flu-dyn

FEM modeling and simulation of broadband ultrasonic transducers with randomized inhomogeneous backing material

A FEM application for the accurate design of composite backing of ultrasonic transducers is presented. The idea is to obtain the dependence between the volume ratio of the tungsten powder in an epoxy matrix used as a backing and the final pulsed RF signal emitted by the backed transducer. An inhomogeneous material model for the backing was adopted instead of the classic complex geometrical FEM. The model was developed in Comsol 5.5 using two of its physics interfaces. The first based on classic FEM or continuous Galerkin for ultrasonic propagation in the backing and the second based on a discontinuous Galerkin option for fluid pulsed propagation. In this way it is possible to avoid the use of an impedance-based model. The calculations for the resulting bandwidth are good enough as predicted for Desilets for the 1D case by using the KLM circuital model. We worked in a 2D space, where the transducer face vibration is far away from the assumed piston-like considered by the unidimensional KLM model.

physics.comp-ph

Shaping liquid films by dielectrophoresis

We present a theoretical model and experimental demonstration of thin liquid film deformations due to a dielectric force distribution established by surface electrodes. We model the spatial electric field produced by a pair of parallel electrodes and use it to evaluate the stress on the interface through Maxwell stresses. By coupling this force with the Young-Laplace equation, we obtain the deformation of the interface. To validate our theory, we design an experimental setup which uses microfabricated electrodes to achieve spatial dielectrophoretic actuation of a thin liquid film, while providing measurements of microscale deformations through digital holographic microscopy. We characterize the deformation as a function of the electrode-pair geometry and film thickness, showing very good agreement with the model. Based on the insights from the characterization of the system, we pattern conductive lines of electrode pairs on the surface of a microfluidic chamber and demonstrate the ability to produce complex two-dimensional deformations. The films can remain in liquid form and be dynamically modulated between different configurations or polymerized to create solid structures with high surface quality.

cond-mat.soft

Dielectrophoretic Equilibrium of Complex Particles

In contrast to the commonly used spherical Janus particles, here we used engineered Janus particles that are fabricated using photolithography technique for precise control over their geometry and coated regions. Specifically, we studied a lollipop-shaped complex particle where its head is coated with gold while its tail is left bare. Due to their distinct electrical properties (i.e. electrical polarizability) the particle exhibits force equilibrium where opposite dielectrophoretic forces acting on its head and tail exactly cancel each other to yield a stable equilibrium position. This was realized in a quadrupolar electrode array where the equilibrium position of the engineered particle could be tuned by the frequency. This stands in contrast to the standard dielectrophoretic behavior where the particle shifts positions from either the center of the quad to the very edge of the electrodes when shifting from a negative to positive dielectrophoretic response, respectively. This opens new opportunities for positioning control of such complex particles for self-assembly, biosensing, biomimetic spermatozoa and more.

cond-mat.soft

Effect of the difference in ion mobilities on traveling-wave electro-osmosis

We analyze the AC electro-osmotic motion of a 1:1 aqueous solution, taking into account the difference in mobilities and diffusion coefficients between positive and negative ions. This model serves to understand the behavior of common systems as a solution of NaCl in water. We pay special attention to two cases. First, the case of slightly different mobilities, that can model a KCl solution. Second, the case of a strongly asymmetric solution, with an almost vanishing mobility, applicable to the case of a salt where the negative ion is much more massive than the positive one. For all the cases, we perform the mathematical description and linear analysis of the problem, in order to establish the dependence of the induced velocity with the frequency, wavelength and amplitude of the applied voltage.

physics.flu-dyn