arXiv subjects

Antti Karjasilta

Publications and source records attributed to Antti Karjasilta.

3 recordsLinked to original sources

arXiv2026

Multiferroic Quantum Dot in an Artificial van der Waals Heterostructure

Quantum dots (QDs) provide a versatile platform for engineering quantum-confined electronic states with functionalities relevant for optoelectronics, spintronics, and quantum technologies. While substantial progress has been achieved in coupling confined states to spin, valley, topological, or ferroelectric degrees of freedom, the realization of a multiferroic QD in which quantum confinement simultaneously intertwines with magnetism and ferroelectricity remains elusive. Here, we engineer a multiferroic QD in an artificial van der Waals heterostructure grown by molecular beam epitaxy under ultra-high-vacuum conditions. The heterostructure consists of ferroelectric SnTe nanoislands deposited on the layered magnet CrBr$_2$ supported on highly oriented pyrolytic graphite. Combining scanning tunneling microscopy and spectroscopy with ab initio calculations and low-energy tight-binding models, we demonstrate the emergence of spin-polarized discretized electronic states confined within the SnTe islands. Remarkably, the spectroscopic response of the QD strongly depends on the ferroelectric domain configuration of the SnTe nanoislands, demonstrating an interplay between quantum confinement, magnetic exchange, and ferroelectric order at the atomic scale. Our results establish engineered van der Waals heterostructures as a platform for multiferroic quantum confinement and open new routes toward electrically tunable quantum spintronic devices.

cond-mat.mes-hall↗

arXiv2026

Observation of electromagnons in a monolayer multiferroic

Van der Waals multiferroics have emerged as a promising platform to explore novel magnetoelectric phenomena. Recently, it has been shown that monolayer NiI$_2$ hosts robust type-II multiferroicity down to the two-dimensional limit, a giant dynamical magnetoelectric coupling at terahertz frequencies, and an electrically switchable spin polarization. These developments present the possibility of engineering ultrafast, low-energy-consumption, and electrically-tunable spintronic devices based on the collective excitations of the multiferroic order, electromagnons. However, the direct visualization of these bosonic modes in real space and within the monolayer limit remains elusive. Here, we report the atomic-scale observation of electromagnons in monolayer NiI$_2$ using low-temperature scanning tunneling microscopy. By tracking the thermal evolution of the multiferroic phase, we establish the energy scale and resolve coherent in-gap excitations of the symmetry-broken multiferroic state. Comparison with first-principles and spin-model calculations reveals that the low-energy modes originate from electromagnon excitations. Spatially resolved inelastic tunneling spectroscopy maps show a stripe-like modulation of the local spectral function at electromagnon energies, matching theoretical predictions. These results provide direct evidence of the internal structure of electromagnons and establish a methodology to probe these modes at the atomic scale, opening avenues for electrically tunable spintronics.

cond-mat.mtrl-sci↗

arXiv2026

Universality of Type-II Multiferroicity in Monolayer Nickel Dihalides

The recent discovery of type-II multiferroicity in monolayer NiI${_2}$ indicated a new pathway for intrinsic magnetoelectric coupling in the two-dimensional limit. However, determining whether this phenomenon is a unique anomaly or a general, chemically tunable property of the material class remains unresolved. Here, we demonstrate the universality of type-II multiferroicity in the transition metal dihalides by visualizing the ferroelectric order in monolayer NiBr${_2}$. Using scanning tunneling microscopy (STM), we resolve atomic-scale ferroelectric domains and confirm their magnetoelectric origin through reciprocal manipulation experiments: reorienting magnetic order via electric fields and suppressing the electric polarization with external magnetic fields. Furthermore, we find that the multiferroic state in NiBr${_2}$ is energetically less robust than in its iodide counterpart, consistent with modified superexchange interactions and the reduced spin-orbit coupling. Our results establish the transition metal dihalides as a versatile platform where the stability of magnetoelectric phases can be engineered through chemical substitution.

cond-mat.mtrl-sci↗