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Anyesh Saraswati

Publications and source records attributed to Anyesh Saraswati.

4 recordsLinked to original sources

Unconventional topological Hall response and anisotropic magnetotransport properties of a helical magnet EuAuAs

Topological magnets with nontrivial spin texture have attracted considerable interest because they display a rich spectrum of emergent quantum phenomena. Here, we present a combined experimental and theoretical investigation of the magnetic and magnetotransport properties of EuAuAs, an antiferromagnet with Néel temperature ($T_\mathrm{N}$) $\sim$ 6 K. The temperature and magnetic field dependence of electrical resistivity and magnetization demonstrate that the charge transport in EuAuAs is strongly influenced by the spin configuration of local Eu moments. Below $T_\mathrm{N}$, both longitudinal magnetoresistance (LMR) and transverse magnetoresistance (TMR) are positive at low fields but large and negative at high fields. With increasing temperature, TMR becomes positive above 60 K, whereas LMR remains negative up to 100 K. The low-field positive LMR and TMR originate from weak antilocalization (WAL). The WAL contribution in TMR is well captured by the Hikami-Larkin-Nagaoka model, whereas the LMR data are described by a generalized Altshuler-Aronov framework. Moreover, we observe a giant topological Hall effect arising from the scalar spin chirality, which is further supported by the helical magnetic structure obtained from the ab-initio calculations. The observed anisotropy in longitudinal resistivity and magnetoresistance underscores the very nature of the Fermi surface of the EuAuAs, as confirmed by first-principles calculations. These results establish EuAuAs as a unique platform for exploring the interplay between electronic structure and noncoplanar spin texture in a centrosymmetric helical magnet.

cond-mat.mtrl-sci

Accessing quasi-flat $\textit{f}$-bands to harvest large Berry curvature in NdGaSi

In typical rare-earth lanthanide compounds, the localized 4\textit{f}-electrons have a weak effect on the electrical conduction, limiting their influence on the Berry curvature and, hence, the intrinsic anomalous Hall effect. A comprehensive study of the magnetic, thermodynamic, and transport properties of single-crystalline NdGaSi, guided by first-principles calculations, reveals a ferromagnetic ground state that induces a splitting of quasi-flat 4\textit{f} electronic bands and positions them near the Fermi energy. The observation of an extraordinarily large intrinsic anomalous Hall conductivity of 1165 $Ω^{-1}$ cm$^{-1}$ implies the direct involvement of localized states in the generation of non-trivial band crossings around the Fermi energy. The angle-resolved photoemission spectroscopy measurements provide direct evidence of non-trivial crossing of the 4\textit{f}-bands with dispersive bands. These results are remarkable when compared to ferrimagnetic NdAlSi, which differs only in a non-magnetic atom (a change in the principal quantum number \textit{n} of the outer \textit{p }orbital) with the same number of valence electrons and does not exhibit any measurable anomalous Hall conductivity.

cond-mat.mtrl-sci

Complex spin dynamics induced metamagnetic phase transitions in Dirac semimetal EuAuBi

We report a comprehensive investigation of the physical properties of the Dirac semimetal compound EuAuBi single crystals, using neutron diffraction, magnetization, electrical transport, and specific heat measurements. EuAuBi crystallizes in a hexagonal structure with space group P63mc (No. 186). First-principles calculations using density functional theory characterize it as a Dirac semimetal, with a notable band-crossing in proximity to the Fermi level (EF ) along the Γ-A direction. The crystal exhibits three distinct magnetic phases at 4 K (TN1), 3.5 K (TN2), and 2.8 K (TN3)as observed from magnetic and specific heat measurements. However, zero-field neutron diffraction resolves only two magnetic phases: a commensurate antiferromagnetic phase and a canted antiferromagnetic phase. Field-dependent ac and dc magnetization measurements uncover field-induced non-trivial spin textures in the magnetic field range 1.5 to 3 T, manifested as a tilted plateau in the magnetization curves. The interplay between conduction carriers and these spin textures is further evidenced by unique features in the magnetic field-dependent longitudinal resistivity in the system. Finally, we present a comprehensive magnetic phase diagram of EuAuBi, highlighting diverse spin alignments present in the material. EuAuBi thus emerges as a rare material system in which both momentum-space and real-space Berry curvature effects may coexist, providing a unique opportunity to investigate their interplay.

cond-mat.mtrl-sci

Giant anisotropic anomalous Hall effect in antiferromagnetic topological metal NdGaSi

The interplay between magnetism and strong electron correlation in magnetic materials discerns a variety of intriguing topological features. Here, we report a systematic investigation of the magnetic, thermodynamic, and electrical transport properties in NdGaSi single crystals. The magnetic measurements reveal a magnetic ordering below T_N (11 K), with spins aligning antiferromagnetically in-plane, and it orders ferromagnetically (FM) out-of-plane. The longitudinal resistivity data and heat capacity exhibit a significant anomaly as a consequence of the magnetic ordering at TN. The magnetoresistance study shows significantly different behavior when measured along either direction, resulting from the complex nature of the magnetic structure, stemming from complete saturation of moments in one direction and subsequent spin flop transitions in the other. Remarkably, we have also noticed an unusual anisotropic anomalous Hall response. We have observed a giant anomalous Hall conductivity (AHC) of 1730 ohm-1 cm-1 and 490 ohm-1 cm-1 at 2 K, with B // [001] and B // [100], respectively. Our scaling analysis of AHC reveals that the anomalous Hall effect in the studied compound is dominated by the Berry phase-driven intrinsic mechanism. These astonishing findings in NdGaSi open up new possibilities for antiferromagnetic spintronics in rare-earth-based intermetallic compounds.

cond-mat.mes-hall