arXiv subjects

Arabinda Bera

Publications and source records attributed to Arabinda Bera.

13 recordsLinked to original sources

arXiv2026

The Physics of Topological Defects in Glasses

Topological defects play a central role in the mechanical behavior of crystalline materials, yet their relevance to amorphous solids has only recently begun to emerge. Over the last few years, theoretical, computational, and experimental studies have revealed the presence of well-defined topological invariants in vibrational eigenmodes, non-affine displacement fields, and deformation-induced vector fields of glasses. These defects have been shown to correlate strongly with soft spots, localized plastic rearrangements, yielding, and shear-band formation, suggesting a new perspective on the microscopic origins of plasticity in disordered materials. In this review, we provide a comprehensive overview of recent developments in the rapidly growing field of topological defects in glasses. We discuss the underlying theoretical concepts, including Burgers vectors, non-affine plasticity, vibrational modes, and topological invariants, and review recent numerical and experimental advances. Finally, we assess the current achievements, limitations, and open questions, and discuss future directions toward a unified topological description of plasticity and mechanical failure in amorphous solids.

cond-mat.dis-nn↗

arXiv2025

Microscopic origin of shear bands in 2D amorphous solids from topological defects

The formation of shear bands in amorphous solids such as glasses has remained an open question in our understanding of condensed matter and amorphous materials. Unlike in crystals, well-defined topological defects such as dislocations have been elusive due to the lack of a periodic ordered background at the atomic level. Recently, topological defects have been identified in the displacement field and in the eigenvectors of amorphous solids. Recent work has suggested that shear bands in amorphous solids coincide with an alignment of vortex-antivortex dipoles, with alternating topological charge +1/-1. Here we numerically confirm this hypothesis by means of well-controlled simulations in 2D. Surprisingly, we show that a chain of topological defects (TDs) pre-exists the shear band and is visible already in the non-affine displacement field of the elastic regime. This chain is activated into a flow band concomitantly with the disappearance and possibly annihilation of a dipole at a distance from the TDs chain. The possible underlying mechanism is reminiscent of a soliton-like rarefaction pulse remotely activated by dipole annihilation as observed in superfluid Bose-Einstein condensates.

cond-mat.soft↗

arXiv2025

Burgers rings as topological signatures of Eshelby-like plastic events in glasses

Eshelby-like quadrupolar structures serve as the fundamental microscopic units for characterizing plastic instabilities in amorphous solids and play a crucial role in explaining their mechanical failure, including the formation of shear bands. However, identifying Eshelby-like plastic events in glasses remains challenging due to their inherent structural and dynamical complexity. In this work, we show that Eshelby-like structures can be precisely identified and localized using a topological invariant known as the continuous Burgers vector. By combining analytical and simulation techniques, we reveal the emergence of a topological Burgers ring around Eshelby plastic events, enabling the precise identification of their center of mass and capturing their orientation as well. This proposed method offers a clear and unambiguous framework to locate and characterize the plastic rearrangements that govern plasticity in glasses.

cond-mat.dis-nn↗

arXiv2025

Density-field structures in a few systems undergoing velocity ordering

We consider two (off-lattice) varieties of out-of-equilibrium systems, viz., granular and active matter systems, that, in addition to displaying velocity ordering, exhibit fascinating pattern formation in the density field, similar to those during vapor-liquid phase transitions. In the granular system, velocity ordering occurs due to reduction in the normal components of velocities, arising from inelastic collisions. In the active matter case, on the other hand, velocity alignment occurs because of the inherent tendency of the active particles to follow each other. Inspite of this difference, the patterns, even during density-field evolutions, in these systems can be remarkably similar. This we have quantified via the calculations of the two-point equal time correlation functions and the structure factors. These results have been compared with the well studied case of kinetics of phase separation within the framework of the Ising model. Despite the order-parameter conservation constraint in all the cases, in the density field, the quantitative structural features in the Ising case is quite different from those for the granular and active matters. Interestingly, the correlation function for the latter varieties, particularly for an active matter model, quite accurately describes the structure in a real assembly of biologically active particles.

cond-mat.soft↗

arXiv2025

Experimental identification of topological defects in 2D colloidal glass

Topological defects are singularities within a field that cannot be removed by continuous transformations. The definition of these irregularities requires an ordered reference configuration, calling into question whether they exist in disordered materials, such as glasses. However, recent work suggests that well-defined topological defects emerge in the dynamics of glasses, even if they are not evident in the static configuration. In this study, we reveal the presence of topological defects in the vibrational eigenspace of a two-dimensional experimental colloidal glass. These defects strongly correlate with the vibrational features and spatially correlate with each other and structural "soft spots", more prone to plastic flow. This work experimentally confirms the existence of topological defects in disordered systems revealing the complex interplay between topology, disorder, and dynamics.

cond-mat.soft↗

arXiv2024

Geometric indicators of local plasticity in glasses measured by scanning small-beam diffraction

The notion of defects in crystalline phases of matter has been extremely powerful for understanding crystal growth, deformation and melting. Many of these discontinuities in the periodic order of crystals are well described by the Burgers vector, derived from the particle displacements, which encapsulates the direction and magnitude of slip relative to the undeformed state. Since the reference structure of the crystal is known a priori, the Burgers vector can be determined experimentally using both imaging and diffraction methods to measure the final lattice distortion, and thus infer the particle displacements. Glasses have structures that lack the periodicity of crystals, and thus a well-defined reference state. Yet, measurable structural parameters can still be obtained from diffraction from a glass. Here we examine the usefulness of these parameters to probe deformation in glasses. We find that co-ordinated transformations in the centrosymmetry of local particle arrangements are a strong marker of plastic events. For a glass, determining the local distortions corresponding to these plastic events requires measurements before and after deformation. We investigate two geometric indicators that can be derived from these distortions, namely the continuous Burgers vector and the quadrupolar strain. We find that the Burgers vector again emerges as a robust and sensitive metric for understanding local structural transformations due to mechanical deformation, even in disordered glasses.

cond-mat.soft↗

arXiv2024

Hedgehog topological defects in 3D amorphous solids

The underlying structural disorder renders the concept of topological defects in amorphous solids difficult to apply and hinders a first-principle identification of the microscopic carriers of plasticity and of the regions more prone to structural rearrangements (``soft spots''). Recently, it has been proposed that well-defined topological defects can still be identified in glasses, and correlated to local and global plasticity, by looking at the eigenvector field or the particle displacement field. Nevertheless, all the existing proposals and analyses are only valid in two spatial dimensions. In this work, we propose the idea of using hedgehog topological defects to characterize the plasticity of 3D glasses and to geometrically predict the location of their soft spots. We corroborate our proposal by simulating a Kremer-Grest 3D polymer glass, and by using both the normal mode eigenvector field and the displacement field around large plastic events. Contrary to the 2D case, the sign of the topological charge defined from the eigenvector field is ambiguous and the geometry of the topological defects, whether radial or hyperbolic, plays a fundamental role in 3D. In fact, we find that the topological hedgehog defects relevant for plasticity are those exhibiting hyperbolic geometry, resembling the saddle-point structure of 2D topological defects with negative winding number (anti-vortices). Our results confirm that a topological characterization of plasticity in glasses is feasible and provide a concrete realization of this program in 3D amorphous systems.

cond-mat.soft↗

arXiv2024

Clustering of negative topological charge precedes plastic failure in 3D glasses

The deformation mechanism in amorphous solids subjected to external shear remains poorly understood because of the absence of well-defined topological defects mediating the plastic deformation. The notion of soft spots has emerged as a useful tool to characterize the onset of irreversible rearrangements and plastic flow, but these entities are not clearly defined in terms of geometry and topology. In this study, we unveil the phenomenology of recently discovered, precisely defined topological defects governing the microscopic mechanical and yielding behavior of a model 3D glass under shear deformation. We identify the existence of vortex-like and anti-vortex-like topological defects within the 3D non-affine displacement field. The number density of these defects exhibits a significant anti-correlation with the plastic events, with defect proliferation-annihilation cycles matching the alternation of elastic-like segments and catastrophic plastic drops, respectively. Furthermore, we observe collective annihilation of these point-like defects via plastic events, with large local topological charge fluctuations in the vicinity of regions that feature strong non-affine displacements. We reveal that plastic yielding is driven by several large sized clusters of net negative topological charge, the massive annihilation of which triggers the onset of plastic flow. These findings suggest a geometric and topological characterization of soft spots and pave the way for the mechanistic understanding of topological defects as mediators of plastic deformation in glassy materials.

cond-mat.soft↗

arXiv2024

Unveiling the Asymmetry in Density within the Shear Bands of Metallic Glasses

Plastic deformation in metallic glasses at room temperature leads to the development of shear bands due to shear localization. In many experiments, shear bands have shown local density variations along their path, with a distinct imbalance in magnitude between local densification and dilation. However, a comprehensive mechanistic understanding or theory to explain this asymmetry has been lacking until now. Here, we introduce a new model that consists of a sequential arrangement of alternating topological 'charges', generating a dipolar field. The resulting microscopic displacement field, when integrated into the deformation gradient tensor, provides an accurate analytical solution for the observed imbalances in the density variations. The implications of this method are discussed, highlighting the potential to elucidate a broader range of observations in shear bands.

cond-mat.dis-nn↗

arXiv2021

Macroscopic rotation of active colloids in a colloid-polymer mixture confined inside a spherical cavity

From studies via Molecular Dynamics simulations, we report results on structure and dynamics in mixtures of active colloids and passive polymers that are confined inside a spherical container with a repulsive boundary. Such systems mimic the presence of bacteria in the background of bio-polymers. All interactions in the fully passive case are chosen in such a way that in equilibrium coexistence between colloid-rich and polymer-rich phases occurs. For most part of the studies the chosen compositions give rise to Janus structure; one side of the sphere is occupied by the colloids and the rest by the polymers. This partially wet situation mimics nearly a neutral wall in the fully passive scenario. Following the introduction of a velocity-aligning activity to the colloids, the shape of the polymer-rich domain changes to that of an ellipsoid, around the long axis of which the colloid-rich domain attains a macroscopic angular momentum. In the steady state, the orientation of this axis evolves via diffusion, implying that the passive domain is set into motion as well by the active particles.

cond-mat.soft↗

arXiv2020

Active Particles in Explicit Solvent: Dynamics of clustering for alignment interaction

We study dynamics of clustering in systems containing active particles that are immersed in an explicit solvent. For this purpose we have adopted a hybrid simulation method, consisting of molecular dynamics and multi-particle collision dynamics. In our model, overlap-avoiding passive interaction of an active particle with another active particle or a solvent particle has been taken care of via variants of Lennard-Jones potential. Dynamic interaction among the active particles has been incorporated via the Vicsek-like self-propulsion that facilitates clustering. We quantify the effects of activity and importance of hydrodynamics on the dynamics of clustering via variations of relevant system parameters. We work with low overall density of active particles. For this the morphology consists of disconnected clusters, the mechanism of growth switching among particle diffusion, diffusive coalescence and ballistic aggregation, depending upon the presence or absence of active and hydrodynamic interactions. Corresponding growth laws have been quantified and discussed in the background of appropriate theoretical pictures. Our results suggest that multi-particle collision dynamics is an effective method for investigation of hydrodynamic phenomena even in active matter systems.

cond-mat.soft↗

arXiv2020

How Do Clusters in Phase-Separating Active Matter Systems Grow? A study for Vicsek activity in systems undergoing vapor-solid transition

Via molecular dynamics simulations we have studied kinetics of vapor-"solid" phase transition in an active matter model in which self-propulsion is introduced via the well-known Vicsek rule. The overall density of the particles is chosen in such a way that the evolution morphology consists of disconnected clusters that are defined as regions of high density of particles. Our focus has been on understanding the influence of the above mentioned self-propulsion on structure and growth of these clusters by comparing the results with those for the passive limit of the model that also exhibits vapor-"solid" transition. While in the passive case the growth occurs due to standard diffusive mechanism, the Vicsek activity leads to a very rapid growth, via a process that is practically equivalent to the ballistic aggregation mechanism. The emerging growth law in the latter case has been accurately estimated and explained by invoking information on velocity and structural aspects of the clusters into a relevant theory. Some of these results are also discussed with reference to a model for the active Brownian particles.

cond-mat.soft↗

arXiv2019

Aging Phenomena during Phase Separation in Fluids: Decay of autocorrelation for vapor-liquid transitions

We performed molecular dynamics simulations to study relaxation phenomena during vapor-liquid transitions in a single component Lennard-Jones system. Results from two different overall densities are presented; one in the neighborhood of the vapor branch of the coexistence curve and the other being close to the critical density. The nonequilibrium morphologies, growth mechanisms and growth laws in the two cases are vastly different. In the low density case growth occurs via diffusive coalescence of droplets in a disconnected morphology. On the other hand, the elongated structure in the higher density case grows via advective transport of particles inside the tube-like liquid domains. The objective in this work has been to identify how the decay of the order-parameter autocorrelation, an important quantity to understand aging dynamics, differs in the two cases. In the case of the disconnected morphology, we observe a very robust power-law decay, as a function of the ratio of the characteristic lengths at the observation time and at the age of the system, whereas the results for the percolating structure appear rather complex. To quantify the decay in the latter case, unlike standard method followed in a previous study, here we have performed a finite-size scaling analysis. Outcome of this analysis shows the presence of a strong preasymptotic correction, while revealing that in this case also, albeit in the asymptotic limit, the decay follows a power-law. Even though the corresponding exponents in the two cases differ drastically, this study, combined with a few recent ones, suggests that power-law behavior of this correlation function is rather universal in coarsening dynamics.

cond-mat.stat-mech↗