SearcharxivSearch

arXiv subjects

Arata Mitsuzuka

Publications and source records attributed to Arata Mitsuzuka.

3 recordsLinked to original sources

Tellurium Metasurface Beam Splitter with Pulse Laser-Controlled Anisotropy

Laser-programmable optical anisotropy offers a new route to developing reconfigurable metasurfaces without conventional nanofabrication processes. Here, we demonstrate a lithography-free approach based on spatial control of the crystallographic $c$ axis orientation in tellurium (Te) using pulse laser irradiation. As a proof of concept, we demonstrate a Te metasurface beam splitter by laser-written optical-axis patterning and experimentally confirm that its optical response is in good agreement with theoretical predictions and numerical simulations. By directly programming the local optical anisotropy, this method enables a simple fabrication process while offering the possibility of rewriting and dynamically reconfiguring device functionality. These features make this approach a promising platform for non-resonant active metasurfaces and other reconfigurable flat-optics applications.

cond-mat.mes-hall

Photo-thermal origin of pulse laser induced orientation of crystallographic c axis in Tellurium thin films

Recent studies have shown that the orientation of crystallographic c axis of Tellurium thin films can be controlled using picosecond long laser pulses. This method provides spatially programmable control of the crystal orientation and is therefore highly attractive for practical applications in functional optical and electronic devices. Previously, it was suggested that laser-induced selective melting and recrystallization can cause the laser-induced reorientation. However, this interpretation remains inconclusive due to limited data. To clarify the mechanism, here we systematically study Te samples under different irradiation conditions. We find that the threshold fluence for inducing optical reorientation depends on the number of laser pulses. The results agrees well with a minimal kinetic model based on the Arrhenius law. Using the model developed, we investigate the condition required to control the optic axis in other two-dimensional materials, such as black phosphorus, WTe2, and SnSe. These findings provide a guide for developing functional electro-optical devices based on anisotropic materials.

cond-mat.mes-hall

Light-programmable reorientation of the crystallographic c-axis of Tellurium thin films

Tellurium (Te), a two-dimensional material with pronounced structural anisotropy, exhibits exceptional electrical and optical properties that are highly sensitive to its crystallographic orientation. However, conventional synthesis techniques offer limited control over the in-plane alignment of Te's crystallographic c-axis, hindering large-scale integration. Here, we report a novel, non-contact method to dynamically manipulate the c-axis orientation of Te thin films using linearly polarized picosecond laser pulses. We show that the c-axis can be omnidirectionally reoriented perpendicular to the laser polarization, even in initially polycrystalline films. This reorientation is fully reversible, allowing for rewritable and spatially selective control of the c-axis orientation post-deposition. Our light-driven approach enables programmable anisotropy in Te, opening new avenues for reconfigurable optoelectronic and photonic devices, such as active metasurfaces and CMOS-compatible architectures.

cond-mat.mes-hall