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Ariando

Publications and source records attributed to Ariando.

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Large spectral weight transfer in optical conductivity of SrTiO$_{3}$ induced by intrinsic vacancies

The optical conductivity ($σ_{1}$) of SrTiO$_{3}$ for various vacancies has been systematically studied using a combination of ultraviolet - vacuum ultraviolet (UV-VUV) reflectivity and spectroscopic ellipsometry. For cation (Ti) vacancies, $σ_{1}$ shows large spectral weight transfer over a wide range of energy from as high as 35 eV to as low as 0.5 eV and the presence of mid-gap states, suggesting that strong correlations play an important role. While for anion (O) vacancies $σ_{1}$ shows changes from 7.4 eV up to 35 eV. These unexpected results can be explained in terms of orbital reconstruction.

cond-mat.str-el

Atomically flat interface between a single-terminated LaAlO3 substrate and SrTiO3 thin film is insulating

The surface termination of (100)-oriented LaAlO3 (LAO) single crystals was examined by atomic force microscopy and optimized to produce a single-terminated atomically flat surface by annealing. Then the atomically flat STO film was achieved on a single-terminated LAO substrate, which is expected to be similar to the n-type interface of two-dimensional electron gas (2DEG), i.e., (LaO)-(TiO2). Particularly, that can serve as a mirror structure for the typical 2DEG heterostructure to further clarify the origin of 2DEG. This newly developed interface was determined to be highly insulating. Additionally, this study demonstrates an approach to achieve atomically flat film growth based on LAO substrates.

cond-mat.mtrl-sci

Magnetic-field induced resistivity minimum with in-plane linear magnetoresistance of the Fermi liquid in SrTiO3-x single crystals

We report novel magnetotransport properties of the low temperature Fermi liquid in SrTiO3-x single crystals. The classical limit dominates the magnetotransport properties for a magnetic field perpendicular to the sample surface and consequently a magnetic-field induced resistivity minimum emerges. While for the field applied in plane and normal to the current, the linear magnetoresistance (MR) starting from small fields (< 0.5 T) appears. The large anisotropy in the transverse MRs reveals the strong surface interlayer scattering due to the large gradient of oxygen vacancy concentration from the surface to the interior of SrTiO3-x single crystals. Moreover, the linear MR in our case was likely due to the inhomogeneity of oxygen vacancies and oxygen vacancy clusters, which could provide experimental evidences for the unusual quantum linear MR proposed by Abrikosov [A. A. Abrikosov, Phys. Rev. B 58, 2788 (1998)].

cond-mat.mtrl-sci

Magnetoresistance of 2D and 3D Electron Gas in LaAlO3/SrTiO3 Heterostructures: Influence of Magnetic Ordering, Interface Scattering and Dimensionality

Magnetoresistance (MR) anisotropy in LaAlO3/SrTiO3 (LAO/STO) interfaces is compared between samples prepared in high oxygen partial pressure (PO2) of 10-4 mbar exhibiting quasi-two-dimensional (quasi-2D) electron gas and low PO2 of 10-6 mbar exhibiting 3D conductivity. While MR of an order of magnitude larger was observed in low PO2 samples compared to those of high PO2 samples, large MR anisotropies were observed in both cases. The MR with the out-of-plane field is always larger compared to the MR with in-plane field suggesting lower dissipation of electrons from interface versus defect scattering. The quasi-2D interfaces show a negative MR at low temperatures while the 3D interfaces show positive MR for all temperatures. Furthermore, the angle relationship of MR anisotropy for these two different cases and temperature dependence of in-plane MR are also presented. Our study demonstrates that MR can be used to distinguish the dimensionality of the charge transport and various (defect, magnetic center, and interface boundary) scattering processes in this system.

cond-mat.str-el

Carrier freeze-out induced metal-insulator transition in oxygen deficient SrTiO3 films

We report the optical, electrical transport, and magnetotransport properties of high quality oxygen deficient SrTiO3 (STO) single crystal film fabricated by pulsed laser deposition and reduced in the vacuum chamber. The oxygen vacancy distribution in the thin film is expected to be uniform. By comparing the electrical properties with oxygen deficient bulk STO, it was found that the oxygen vacancies in bulk STO is far from uniform over the whole material. The metal-insulator transition (MIT) observed in the oxygen deficient STO film was found to be induced by the carrier freeze-out effect. The low temperature frozen state can be re-excited by an electric field, Joule heating, and surprisingly also a large magnetic field.

cond-mat.mtrl-sci

Two-dimensional Graphene Superlattice Made with Partial Hydrogenation

Electronic properties of two-dimensional graphene superlattice made with partial hydrogenation were thoroughly studied via Density Functional Tight Binding approach (DFTB) which incorporates the tight-binding method into the density functional formalism. The two-dimensional (2-d) pattern of hydrogen atoms on graphene was found to have great effects on electronic structures of graphene superlattice. In particular, the edges of the 2-d pattern, armchair or zigzag, are essential for the energy band gap opening, and the energy band gap sensitively depends on the shape, size, and the 2-d periodicity of the pattern. Based on these findings, we suggested that the 2-d graphene superlattice may be used in fabricating quantum dots and 2-d heterojunctions on graphene without the need for cutting or etching.

cond-mat.mes-hall

Nonlinear Insulator in Complex Oxides

The insulating state is one of the most basic electronic phases in condensed matter. This state is characterised by an energy gap for electronic excitations that makes an insulator electrically inert at low energy. However, for complex oxides, the very concept of an insulator must be re-examined. Complex oxides behave differently from conventional insulators such as SiO2, on which the entire semiconductor industry is based, because of the presence of multiple defect levels within their band gap. As the semiconductor industry is moving to such oxides for high-dielectric (high-k) materials, we need to truly understand the insulating properties of these oxides under various electric field excitations. Here we report a new class of material called nonlinear insulators that exhibits a reversible electric-field-induced metal-insulator transition. We demonstrate this behaviour for an insulating LaAlO3 thin film in a metal/LaAlO3/Nb-SrTiO3 heterostructure. Reproducible transitions were observed between a low-resistance metallic state and a high-resistance non-metallic state when applying suitable voltages. Our experimental results exclude the possibility that diffusion of the metal electrodes or oxygen vacancies into the LaAlO3 layer is occurring. Instead, the phenomenon is attributed to the formation of a quasi-conduction band (QCB) in the defect states of LaAlO3 that forms a continuum state with the conduction band of the Nb-SrTiO3. Once this continuum (metallic) state is formed, the state remains stable even when the voltage bias is turned off. An opposing voltage is required to deplete the charges from the defect states. Our ability to manipulate and control these defect states and, thus, the nonlinear insulating properties of complex oxides will open up a new path to develop novel devices.

cond-mat.mtrl-sci

Macroscopic quantum tunneling and quasiparticle-tunneling blockade effect in s-wave/d-wave hybrid junctions

We have theoretically investigated macroscopic quantum tunneling (MQT) and the influence of nodal quasiparticles and zero energy bound states (ZES) on MQT in s-wave/ d-wave hybrid Josephson junctions. In contrast to d-wave/d-wave junctions, the low-energy quasiparticle dissipation resulting from nodal quasiparticles and ZES is suppressed due to a quasiparticle-tunneling blockade effect in an isotropic s-wave superconductor. Therefore, the inherent dissipation in these junctions is found to be very weak. We have also investigated MQT in a realistic s-wave/d-wave (Nb/Au/YBCO) junction in which Ohmic dissipation in a shunt resistance is stronger than the inherent dissipation and find that MQT is observable within the current experimental technology. This result suggests high potential of s-wave/d-wave hybrid junctions for applications in quantum information devices.

cond-mat.supr-con

Imaging of order parameter induced $π$ phase shifts in cuprate superconductors by low-temperature scanning electron microscopy

Low-temperature scanning electron microscopy (LTSEM) has been used to image the supercurrent distribution in ramp-type Josephson junctions between Nb and either the electron-doped cuprate Nd$_{2-x}$Ce$_x$CuO$_{4-y}$ or the hole-doped cuprate YBa$_2$Cu$_3$O$_7$. For zigzag-shaped devices in the short junction limit the critical current is strongly suppressed at zero applied magnetic field. The LTSEM images show, that this is due to the Josephson current counterflow in neighboring 0 and $π$ facets, which is induced by the $d_{x^2-y^2}$ order parameter in the cuprates. Thus, LTSEM provides imaging of the sign change of the superconducting order parameter, which can also be applied to other types of Josephson junctions.

cond-mat.supr-con

Dynamics of single vortices in grain boundaries: I-V characteristics on the femto-volt scale

We employed a scanning Hall probe microscope to detect the hopping of individual vortices between pinning sites along grain boundaries in YBCO thin films in the presence of an applied current. Detecting the motion of individual vortices allowed us to probe the current-voltage (I-V) characteristics of the grain boundary with voltage sensitivity below a femto-volt. We find a very sharp onset of dissipation with V~I^n with an unprecedented high exponent of n~290 that shows essentially no dependence on temperature or grain boundary angle. Our data have no straightforward explanation within the existing grain boundary transport models.

cond-mat.supr-con

Experiments using high-Tc/low-Tc Josephson contacts

Remarkably rich physics is involved in the behavior of hybrid Josephson junctions, connecting high-Tc and low-Tc superconductors. This relates in particular to the different order parameter symmetries underlying the formation of the superconducting states in these materials. Experiments on high-Tc/low-Tc contacts have also played a crucial role in settling the decade-long d-wave versus s-wave debate in cuprate superconductors. Recently, such hybrid junctions have enabled more detailed pairing symmetry tests. Furthermore, with these junctions, complex arrays of pi-rings have been realized, enabling studies on spontaneously generated fractional flux quanta and their mutual interactions. Steps toward novel superconducting electronic devices are taken, utilizing the phase-shifts inherent to the d-wave superconducting order parameter. This paper is intended to reflect the current status of experiments using high-Tc and low-Tc Josephson contacts.

cond-mat.supr-con

Observation of Andreev bound states in YBaCuO/Au/Nb ramp-type Josephson junctions

We report on Josephson and quasiparticle tunneling in YBa2Cu3O7-x(YBCO)/Au/Nb ramp junctions of several geometries. Macroscopically, tunneling occurs in the ab-plane of YBCO either in the (100) and (010) direction, or in the (110) direction. These junctions have a stable and macroscopically well defined geometry. This allows systematic investigations of both quasiparticle and Josephson tunneling over a wide range of temperature and magnetic field. With Nb superconducting, its gap appears in the quasiparticle conductance spectra as Nb coherence peaks and a dip at the center of a broadened zero-bias conductance peak (ZBCP). As we increase the temperature or an applied magnetic field both the Nb coherence peaks and the dip get suppressed and the ZBCP fully develops, while states are conserved. With Nb in the normal state the ZBCP is observed up to about 77 K and is almost unaffected by an increasing field up to 7 T. The measurements are consistent with a convolution of density of states with broadened Andreev bound states formed at the YBCO/Au/Nb junction interfaces. Since junctions with different geometries are fabricated on the same substrate under the same conditions one expects to extract reliable tunneling information that is crystallographic direction sensitive. In high contrast to Josephson tunneling, however, the quasiparticle conductance spectra are crystallographic orientation insensitive: independent whether the tunneling occurs in the (100) or (110) directions, a pronounced ZBCP is always observed, consistent with microscopic roughness of the junction interfaces. Qualitatively, all these particularities regarding quasiparticle spectra hold regardless whether the YBCO thin film is twinned or untwinned.

cond-mat.supr-con

Admixtures to d-wave gap symmetry in untwinned YBa2Cu3O7 superconducting films measured by angle-resolved electron tunneling

We report on an \textit{ab}-anisotropy of $J_{c \parallel b}/J_{c \parallel a}% \cong 1.8$ and $I_{c}R_{n \parallel b}/I_{c}R_{n \parallel a}\cong 1.2$ in ramp-edge junctions between untwinned YBa$_{2}$Cu$_{3}$O$_{7}$ and $s$% -wave Nb. For these junctions, the angle $θ$ with the YBa$_{2}$Cu$_{3}$O$_{7}$ crystal b-axis is varied as a single parameter. The $R_{n}$A($θ$)-dependence presents 2-fold symmetry. The minima in $I_{c}R_{n}$ at $θ\cong 50^{\circ}$ suggest a real s-wave subdominant component and negligible $d_{xy}$-wave or imaginary s-wave admixtures. The $I_{c}R_{n}$($θ$)-dependence is well-fitted by 83% $d_{x^{2}-y^{2}}$-, 15% isotropic $s$- and 2% anisotropic s-wave order parameter symmetry, consistent with $Δ_{b}/Δ_{a} \cong 1.5$.

cond-mat.supr-con

Phase-sensitive order parameter symmetry test experiments utilizing Nd2-xCexCuO4-y/Nb zigzag junctions

Phase-sensitive order parameter symmetry test experiments are presented on the electron-doped high-T_c cuprate Nd2-xCexCuO4-y. These experiments have been conducted using zigzag-shaped thin film Josephson structures, in which the Nd2-xCexCuO4-y is connected to the low-T_c superconductor Nb via a Au barrier layer. For the optimally doped as well as for the overdoped Nd2-xCexCuO4-y a clear predominant dx2-y2-wave behavior is observed at T=4.2K. Both compounds were also investigated at T=1.6K, presenting no indications for a change to a predominant s-wave symmetry with decreasing temperature.

cond-mat.str-el

Anti-ferromagnetic ordering in arrays of superconducting pi-rings

We report experiments in which one dimensional (1D) and two dimensional (2D) arrays of YBa2Cu3O7-x-Nb pi-rings are cooled through the superconducting transition temperature of the Nb in various magnetic fields. These pi-rings have degenerate ground states with either clockwise or counter-clockwise spontaneous circulating supercurrents. The final flux state of each ring in the arrays was determined using scanning SQUID microscopy. In the 1D arrays, fabricated as a single junction with facets alternating between alignment parallel to a [100] axis of the YBCO and rotated 90 degrees to that axis, half-fluxon Josephson vortices order strongly into an arrangement with alternating signs of their magnetic flux. We demonstrate that this ordering is driven by phase coupling and model the cooling process with a numerical solution of the Sine-Gordon equation. The 2D ring arrays couple to each other through the magnetic flux generated by the spontaneous supercurrents. Using pi-rings for the 2D flux coupling experiments eliminates one source of disorder seen in similar experiments using conventional superconducting rings, since pi-rings have doubly degenerate ground states in the absence of an applied field. Although anti-ferromagnetic ordering occurs, with larger negative bond orders than previously reported for arrays of conventional rings, long-range order is never observed, even in geometries without geometric frustration. This may be due to dynamical effects. Monte-Carlo simulations of the 2D array cooling process are presented and compared with experiment.

cond-mat.supr-con