arXiv subjects

Aristide Lemaître

Publications and source records attributed to Aristide Lemaître.

At least 19 recordsLinked to original sources

arXiv2026

Spin-to-polarization mapping with a coherent quantum dot-cavity receiver

Coherent light-matter interfaces controllably modifying the state of a photon upon interaction with a stationary qubit are a key resource for implementing deterministic entangling gates for optical quantum technologies. This requires a one-to-one mapping between the state of the scattered photon and that of the embedded qubit. Here, we present an experimental signature of such a bijection by leveraging the spin-induced Kerr rotation present in a low-noise charged quantum dot-micropillar cavity device. Through time-resolved polarization measurements, we project the electron spin to one of its eigenstates with $95\pm2\%$ fidelity with a single reflected photon detection, and follow the subsequent spin relaxation through the detection of a second reflected photon. We demonstrate that, after a transient regime governed by the trion radiative lifetime, two orthogonal polarization states can be produced, each associated to a given spin eigenstate. While the current results are limited by a timescale competition between electron spin relaxation and trion radiative lifetime, they could be improved using hole spins displaying increased relaxation times. Our work paves the way towards deterministic logic gates exploiting this one-to-one mapping between a spin and the polarization of a scattered photon.

quant-ph↗

arXiv2026

All-optical nonlinear phase modulation in open semiconductor microcavities

We report a significant advancement in ultra low power light-by-light phase modulation using open semiconductor microcavities in the strong light-matter coupling regime. We achieve cross-phase modulation of up to 247$\pm$17 mrad per particle between laser beams attenuated to single-photon average intensities. This breakthrough extends the potential for quantum information processing and nonlinear quantum optics in strongly coupled light-matter systems, setting a new benchmark in the field without relying on atom-like emitters. Our findings suggest promising new avenues for scalable quantum optical technologies.

physics.optics↗

arXiv2026

Industry-ready spin-photon interfaces for hybrid photonic quantum computing

Hybrid photonic quantum computers, combining stationary matter qubits and flying photonic qubits, offer an intrinsically networked and resource-efficient route to large-scale, error-corrected quantum computation. Their core components are cavity-coupled matter qubits that act as light--matter interfaces, enabling: high-efficiency on-demand single-photon generation, stable near-unity photon indistinguishability and spin--multi-photon entanglement. Semiconductor quantum dots in microcavities are a leading platform for realizing such devices. Yet reaching the performance, reproducibility and spin-coherence thresholds for large-scale error correction remains a major challenge requiring industrial fabrication and control. Here we report thousands of monolithic semiconductor quantum-dot devices fabricated using a III--V pilot production-line process compatible with large-scale deployment. Systematic control of source parameters yields state-of-the-art efficiency and supports a path to optical losses below fault-tolerance thresholds. Using field-quadrature state reconstruction as a stringent joint test of efficiency and indistinguishability, we observe near-unity photon quantum purity stable over tens of minutes and a record single-photon Wigner-function negativity. We further demonstrate seven-partite spin--multi-photon entanglement and spin coherence extendable to microsecond timescales in the low-magnetic-field regime. Finally, photons from distant sources are as indistinguishable as photons emitted successively by a single source. These results establish foundry-compatible III--V quantum dots as a scalable platform for hybrid photonic quantum computing.

quant-ph↗

arXiv2026

Boosted Optomechanics with a Fluid of Nonlinear Polaritons

Merging optomechanics and polaritonics opens stimulating perspectives like the giant enhancement of optomechanical interaction and the enrichment of optomechanics with effective nonlinear photons. The experimental implementation of these concepts has however remained elusive. Here we report on the resonant optical control of polaritonic optomechanical resonators constituted of semiconductor disks embedding quantum wells. Whispering gallery photons and quantum well excitons strongly couple, leading to the emergence of polaritons that couple to the mechanical vibrations of the disk. We perform resonant optomechanical frequency response experiments on these resonators, modeled introducing a minimal set of constitutive equations, from which we extract the polariton-modified optomechanical coupling $g_0$ and the polariton nonlinearities. We observe a boost of $g_0$ by more than a decade compared to bare photons, reaching to a record $g_0$ for whispering gallery resonators of $22$ MHz, and analyze experimentally and theoretically its evolution as function of the polariton's composition. We also measure a clear hierarchy of three polaritonic nonlinearities, again analyzed as function of polariton composition, establishing a bridge between past unconciliated reports in polaritonics. Grounded on experimental and theoretical foundations, resonant polaritonic optomechanics is set ready for an optomechanical exploration of quantum fluids of polaritons.

quant-ph↗

arXiv2026

Emission of time-ordered photon pairs from a coherently-driven Kerr microcavity

Weakly-interacting many-body systems possess remarkable quantum properties that are essential components of quantum technologies, and constitute a topic of fundamental interest. Here we show that in a solid-state nonlinear microcavity embedding discrete modes of exciton-dressed photons, we can isolate a single eigenmode of quantum fluctuations from the much brighter coherent fraction of the field. In this regime, we perform frequency- and time-resolved correlations measurements between photons on the red and blue side of the fluctuations spectrum. When the average number of fluctuation quanta is smaller than one, we observe the formation of large pairwise time-ordered correlations: red photon first and blue photon second. We show that this peculiar time-ordering correlation emerges spontaneously from the interplay between frequency-resolved detection, and the non-trivial internal quantum structure of the elementary fluctuations.

cond-mat.quant-gas↗

arXiv2026

Near-identical photons from distant quantum dot-cavity devices

Scalable optical quantum technologies require interference between large numbers of indistinguishable single-photons emitted by independent sources. Semiconductor quantum dots are known to be excellent on-demand sources of single-photons. They show record efficiency when inserted into optical cavities to control their spontaneous emission and generate trains of near identical photons over microsecond timescales. However, generating perfectly identical photons from distant cavity-based sources has remained a long-standing challenge. It requires precise matching of the emission wavelengths and emission dynamics, while simultaneously minimizing spectral noise across all time scales for distant emitters in uncorrelated environments. Here, we report on the nanofabrication of a large number of quantum dot-cavity sources with ultra-low spectral noise and wavelength dispersion. The high source efficiency and the use of two tuning mechanisms enable precise optimization of the spectral overlap between distant sources. With this approach, we demonstrate a two-photon indistinguishability of $88\pm1$ % between photons emitted from two distant sources. Remarkably, this value reaches the upper bound set by the intrinsic indistinguishability of photons emitted successively by each source. These results represent a key milestone for scaling photon-based quantum technologies.

quant-ph↗

arXiv2026

Measuring non-Abelian quantum geometry and topology in a multi-gap photonic lattice

Recent discoveries in semi-metallic multi-gap systems featuring band singularities have galvanized enormous interest in particular due to the emergence of non-Abelian braiding properties of band nodes. This previously uncharted set of topological phases necessitates novel approaches to probe them in laboratories, a pursuit that intricately relates to evaluating non-Abelian generalizations of the Abelian quantum geometric tensor (QGT) that characterizes geometric responses. Here, we pioneer the direct measurement of the non-Abelian QGT. We achieve this by implementing a novel orbital-resolved polarimetry technique to probe the full Bloch Hamiltonian of a six-band two-dimensional (2D) synthetic lattice, which grants direct experimental access to non-Abelian quaternion charges, the Euler curvature, and the non-Abelian quantum metric associated with all bands. Quantum geometry has been highlighted to play a key role on macroscopic phenomena ranging from superconductivity in flat-bands, to optical responses, transport, metrology, and quantum Hall physics. Therefore, our work unlocks the experimental probing of a wide phenomenology of multi-gap systems, at the confluence of topology, geometry and non-Abelian physics.

cond-mat.mes-hall↗

arXiv2026

Tensor-driven geometric phase in nonlinear AlGaAs metasurfaces

Dielectric metasurfaces provide a unique platform for efficient harmonic generation and optical wavefront manipulation at the nanoscale. While several approaches are available for performing wavefront shaping, the one exploiting geometric phase streamlines significantly the design and fabrication process. It has been recently shown that, in III-V semiconductor alloys, the rotation of the crystal axes affects the phase and amplitude of second-harmonic generation (SHG) induced by circularly polarized light [1]. Based on this notion, we fabricated and characterized two aluminum gallium arsenide metasurfaces displaying the versatility of the geometric phase design approach through nonlinear beam steering and structured-light generation on the harmonic field.

physics.optics↗

arXiv2025

Optomechanical disk resonator in the quantum ground state of motion

Although they have enabled several advances in the field of optomechanics, optomechanical disk resonators have not yet been operated in the quantum regime. We present the first experimental demonstration of an optomechanical disk resonator prepared in the quantum ground state. With a gigahertz frequency, the mechanical breathing mode of the investigated semiconductor disk reaches a level of excitation below a single phonon when cooled in a dilution refrigerator. We quantify the phonon occupancy of the mechanical mode by performing Brillouin sideband spectroscopy: a conical optical fiber is evanescently coupled to the disk optical whispering-gallery mode, and Stokes and anti-Stokes photons scattered by phonon emission and absorption are counted on a single-photon detector. We measure a suppression of the absorption process corresponding to a phonon occupancy of $0.66\pm0.20$. We experimentally investigate the mechanisms ruling laser-induced heating, which limits the lowest measurable phonon occupancy, and notably witness an extra-cavity heating effect.

quant-ph↗

arXiv2025

Biphoton state generation and engineering with bright hybrid III-V/Silicon photonic devices

Hybrid photonic circuits, harnessing the complementary strengths of multiple materials, represent a key resource to enable compact, scalable platforms for quantum technologies. In particular, the availability of bright sources of tunable biphoton states is eagerly awaited to meet the variety of applications currently under development. In this work we demonstrate a heterogeneously integrated device that merges biphoton generation and on-chip quantum state engineering, combining an AlGaAs photon-pair source with a CMOS-compatible silicon-on-insulator (SOI) circuit. Photon pairs are generated in the C telecom band via spontaneous parametric down-conversion and transferred to the SOI chip through a multimode evanescent coupling scheme. This design achieves a pair generation rate above 10$^{6}$ s$^{-1}$mW$^{-1}$ and a coincidence-to-accidental ratio up to 600. Crucially, the coupling design induces strong and predictable transformations of the biphoton joint spectral amplitude, enabling complex quantum state engineering entirely on-chip in a compact device compliant with electrical pumping.

quant-ph↗

arXiv2025

Benchmarking quantum key distribution by mixing single photons and laser light

Quantum key distribution is a key application of quantum mechanics, shaping the future of privacy and secure communications. Many protocols require single photons, often approximated by strongly attenuated laser pulses. Here, we harness the emission of a quantum dot embedded in a micropillar and explore a hybrid approach where the information is encoded on a mixture of single photons and laser pulses. We derive a phenomenological analysis of the configuration where both sources of light are mixed incoherently to perform the BB84 protocol, showing nearly perfect matching between theory and experiment. This provides a flexible technology compensating limited collected brightnesses of single-photon sources as well as a thorough investigation of single-photon statistics advantage scenarios over Poisson-distributed statistics. Explicitly, our model highlights an efficiency threshold for unconditional advantage of single photons over laser along with insights on the interplay between single-photon purity and collected brightness in the performances of BB84.

quant-ph↗

arXiv2025

Dispersion engineered AlGaAs-on-insulator nanophotonics by distributed feedback

Technological advances in the fabrication of nanophotonic circuits have driven the scientific community to increasingly focus on the precise tailoring of their key optical properties, over a broadband spectral domain. In this context, the modulation of the local refractive index can be exploited to customize an effective reflectivity by the use of distributed Bragg mirrors, enabling the on-chip integration of Fabry-Pérot resonators. The resulting cavity length is strongly wavelength-dependent, offering practical solutions to the growing demand of dispersion engineering. Owing to their typically high core-to-cladding refractive index contrast and exceptional nonlinear properties, III-V semiconductor-based platforms represent promising candidates for the fabrication of Bragg reflectors. In this work, we propose an AlGaAs-on-insulator linear resonator based on distributed Bragg mirrors. We discuss the first experimental demonstration of a systematic, shape-constrained inverse design technique which tailors a prescribed dispersion profile, showing a strong agreement between simulations and measurements. In perspective, the proposed approach offers an efficient and general response to the challenge of dispersion engineering in integrated optical circuits.

physics.optics↗

arXiv2025

Measurement-induced back-action in a QD-based coherent spin-photon interface

Polarization-encoded spin-photon interfaces constitute promising candidates for the development of stationary nodes used as photon receivers, for quantum communication and distributed quantum computing. Here we introduce a time-resolved tomography approach which allows observing the dynamics of an electron spin, in a semiconductor quantum dot, mapped onto the dynamics of the polarization state of reflected photons. Through a single tomography experiment, we infer all the relevant spin dynamics timescales, including precession, decoherence and relaxation times. We also demonstrate and quantify the measurement back-action induced, on the embedded spin qubit, by the detection of a single reflected photon. We show that the induced population and coherence of the spin state can be tuned by the chosen polarization basis of the measurement. The control of the photon-induced back-action on the embedded spin qubit constitutes a crucial requirement for the use of spin-photon interfaces as quantum receivers.

quant-ph↗

arXiv2025

A sublattice Stokes polarimeter for bipartite photonic lattices

The concept of pseudo-spin provides a general framework for describing physical systems featuring two-component spinors, including light polarization, sublattice degrees of freedom in bipartite lattices, and valley polarization in 2D materials. In all cases, the pseudo-spin can be mapped to a Stokes vector on the Poincaré sphere. Stokes polarimeters for measuring the polarization of light are a powerful tool with a wide range of applications both in classical and quantum science. Generalizing Stokes polarimetry to other spinor degrees of freedom is thus a challenge of prime importance. Here, we introduce and demonstrate a Stokes polarimeter for the sublattice polarization in a bipartite photonic lattice. Our method relies on k-space photoluminescence intensity measurements under controlled phase shifts and attenuations applied independently to each sublattice. We implement our method using honeycomb arrays of coupled microcavities realizing photonic analogs of graphene and hexagonal boron nitride. Using our sublattice polarimeter, we reconstruct the Bloch modes in amplitude and phase across the Brillouin zone, achieving sub-linewidth precision in the determination of their eigenenergies, including near band touching points. This enables full access to the system Bloch Hamiltonian and quantum geometric tensor. Our approach can readily be extended to more complex systems with additional internal degrees of freedom, enabling experimental investigations of trigonal warping, Chern insulating phases, and Euler-class topology in multigap systems.

cond-mat.mes-hall↗

arXiv2025

Directional transport and nonlinear localization of light in a one-dimensional driven-dissipative photonic lattice

Photonic lattices facilitate band structure engineering, supporting both localized and extended modes through their geometric design. However, greater control over these modes can be achieved by taking advantage of the interference effect between external drives with precisely tuned phases and photonic modes within the lattice. In this work, we build on this principle to demonstrate optical switching, directed light propagation and site-specific localization in a one-dimensional photonic lattice of coupled microresonators by resonantly driving the system with a coherent field of controlled phase. Importantly, our experimental results provide direct evidence that increased driving power acts as a tuning parameter enabling nonlinear localization at frequencies previously inaccessible in the linear regime. These findings open new avenues for controlling light propagation and localization in lattices with more elaborate band structures.

physics.optics↗

arXiv2025

Monitoring the generation of photonic linear cluster states with partial measurements

Quantum states of light with many entangled photons are key resources for photonic quantum computing and quantum communication. In this work, we exploit a highly resource-efficient generation scheme based on a linear optical circuit embedding a fibered delay loop acting as a quantum memory. The single photons are generated with a bright single-photon source based on a semiconductor quantum dot, allowing to perform the entangling scheme up to 6 photons. We demonstrate $2$, $3$, $4$ and $6$-photon entanglement generation at respective rates of $6$kHz, $120$Hz, $2.2$Hz, and $2$mHz, corresponding to an average scaling ratio of $46$. We introduce a method for real-time control of entanglement generation based on partially post-selected measurements. The visibility of such measurements carries faithful information to monitor the entanglement process, an important feature for the practical implementation of photonic measurement-based quantum computation.

quant-ph↗

arXiv2025

Optimizing the quantum interference between single photons and local oscillator with photon correlations

The quantum interference between a coherent state and a single photon is an important tool in continuous variable optical quantum technologies to characterize and engineer non-Gaussian quantum states. Semiconductor quantum dots, which have recently emerged as a key platform for efficient single-photon generation, could become interesting assets in this context. An essential parameter for interfering single photons and classical fields is the mean wavepacket overlap between both fields. Here, we report on two homodyne photon-correlation techniques enabling the precise measurement of the overlap between a single photon generated by a quantum dot-cavity device and pulsed laser light. The different statistics of interfering fields lead to specific signatures of the quantum interference on the photon correlations at the output of the interfering beam splitter. We compare the behavior of maximized overlap, measuring either the Hong-Ou-Mandel visibility between both outputs or the photon bunching at a single output. Through careful tailoring of the laser light in various degrees of freedom, we maximize the overlap to $76\,\%$, with limitations primarily due to mismatched spectral and temporal profiles and low-frequency charge noise in the single-photon source.

quant-ph↗

arXiv2025

Approaching maximal precision of Hong-Ou-Mandel interferometry with non-perfect visibility

In quantum mechanics, the precision achieved in parameter estimation using a quantum state as a probe is determined by the measurement strategy employed. The ultimate quantum limit of precision is bounded by a value set by the state and its dynamics. Theoretical results have revealed that in interference measurements with two possible outcomes, this limit can be reached under ideal conditions of perfect visibility and zero losses. However, in practice, this cannot be achieved, so precision {\it never} reaches the quantum limit. But how do experimental setups approach precision limits under realistic circumstances? In this work we provide a general model for precision limits in two-photon Hong-Ou-Mandel interferometry for non-perfect visibility. We show that the scaling of precision with visibility depends on the effective area in time-frequency phase space occupied by the state used as a probe, and we find that an optimal scaling exists. We demonstrate our results experimentally for different states in a set-up where the visibility can be controlled and reaches up to $99.5\%$. In the optimal scenario, a ratio of $0.97$ is observed between the experimental precision and the quantum limit, establishing a new benchmark in the field.

quant-ph↗