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Arjun Sapkota

Publications and source records attributed to Arjun Sapkota.

9 recordsLinked to original sources

Rapid supercurrent decay in Mn$_5$Si$_3$ Josephson junctions

Theoretical work predicts that Josephson junctions containing metallic altermagnetic barriers should display $0$-$\pi$ transitions of the critical current as a function of both barrier thickness and temperature, with the decay and oscillation period of the supercurrent depending on the orientation of the crystal axes relative to the transport direction. Motivated by these predictions, and by reports of a compensated magnetic phase attributed to altermagnetism in epitaxial Mn$_5$Si$_3$ thin films, we fabricate and measure Nb/Pt/Mn$_5$Si$_3$/Pt/Nb Josephson junctions varying the thickness of the Mn$_5$Si$_3$ barrier. The critical current decays as a single exponential over more than four orders of magnitude with decay length $\xi_{\text{Mn}_5\text{Si}_3} = 0.31 \pm 0.03$ nm, shorter than reported for Josephson junctions containing the metallic antiferromagnets FeMn, Cr, and NiMn. The Mn$_5$Si$_3$ barrier has an estimated current-perpendicular-to-plane resistivity of $320 \pm 10 \mu\Omega\,$cm. No $0$-$\pi$ transition is resolved at the sampled barrier thicknesses, and the temperature dependence of the critical current of a junction with a 1 nm barrier is smooth and monotonic. We discuss the absence of resolvable transitions in terms of the microstructure of the barrier, its uncertain magnetic phase, and the narrow thickness window imposed by the rapid decay, and identify barriers with well-defined crystalline orientation as the key requirement for future tests of altermagnetic Josephson physics.

cond-mat.supr-con

Large critical current density Josephson $\pi$ junctions with PdNi barriers

We report large $\pi$-state critical current densities, $J_c(\pi)$, in Nb/Pd$_{89}$Ni$_{11}$/Nb Josephson junctions at Pd$_{89}$Ni$_{11}$ thicknesses near the first $\pi$-state. We observe oscillations in the critical current with ferromagnetic barrier thickness consistent with a $0$-$\pi$ transition. For a junction with a 9.4~nm Pd$_{89}$Ni$_{11}$ barrier, we obtain $J_c(\pi) = 410~\mathrm{kA/cm^{2}}$ at 4.2~K, exceeding values reported in prior PdNi-based studies. Magnetization measurements on continuous films, together with coercivity tests on patterned arrays, confirm that Pd$_{89}$Ni$_{11}$ exhibits perpendicular magnetic anisotropy, enabling zero-field operation without magnetic initialization. The combination of large $J_c(\pi)$ and intrinsic anisotropy establishes Pd$_{89}$Ni$_{11}$ as a promising barrier material for passive $\pi$-shifters in superconducting digital logic and qubit architectures.

cond-mat.supr-con

Magnetism and Spin Dynamics in Room-Temperature van der Waals Magnet Fe$_5$GeTe$_2$

Two-dimensional (2D) van der Waals (vdWs) materials have gathered a lot of attention recently. However, the majority of these materials have Curie temperatures that are well below room temperature, making it challenging to incorporate them into device applications. In this work, we synthesized a room-temperature vdW magnetic crystal Fe$_5$GeTe$_2$ with a Curie temperature T$_c = 332$ K, and studied its magnetic properties by vibrating sample magnetometry (VSM) and broadband ferromagnetic resonance (FMR) spectroscopy. The experiments were performed with external magnetic fields applied along the c-axis (H$\parallel$c) and the ab-plane (H$\parallel$ab), with temperatures ranging from 300 K to 10 K. We have found a sizable Landé g-factor difference between the H$\parallel$c and H$\parallel$ab cases. In both cases, the Landé g-factor values deviated from g = 2. This indicates contribution of orbital angular momentum to the magnetic moment. The FMR measurements reveal that Fe$_5$GeTe$_2$ has a damping constant comparable to Permalloy. With reducing temperature, the linewidth was broadened. Together with the VSM data, our measurements indicate that Fe$_5$GeTe$_2$ transitions from ferromagnetic to ferrimagnetic at lower temperatures. Our experiments highlight key information regarding the magnetic state and spin scattering processes in Fe$_5$GeTe$_2$, which promote the understanding of magnetism in Fe$_5$GeTe$_2$, leading to implementations of Fe$_5$GeTe$_2$ based room-temperature spintronic devices.

cond-mat.mtrl-sci

Magnetic domain wall substructures in Pt/Co/Ni/Ir multi-layers

We examine the substructures of magnetic domain walls (DWs) in [Pt/(Co/Ni)$_M$/Ir]$_N$ multi-layers using a combination of micromagnetic theory and Lorentz transmission electron microscopy (LTEM). Thermal stability calculations of Q=$\pm$1 substructures (2-$π$ vertical Bloch lines (VBLs) and DW skyrmions) were performed using a geodesic nudged elastic band (GNEB) model, which supports their metastability at room temperature. Experimental variation in strength of the interfacial Dzyaloshinskii-Moriya interaction (DMI) and film thickness reveals conditions under which these substructures are present and enables the formation of a magnetic phase diagram. Reduced thickness is found to favor Q=$\pm$1 substructures likely due to the suppression of hybrid DWs. The results from this study provide an important framework for examining 1-D DW substructures in chiral magnetic materials.

cond-mat.mtrl-sci

Formation of zero-field Skyrmion arrays in asymmetric superlattices

We demonstrate the formation of metastable Néel-type skyrmion arrays in Pt/Co/Ni/Ir multi-layers at zero-field following \textit{ex situ} application of an in-plane magnetic field using Lorentz transmission electron microscopy. The resultant skyrmion texture is found to depend on both the strength and misorientation of the applied field as well as the interfacial Dzyaloshinskii-Moriya interaction. To demonstrate the importance of the applied field angle, we leverage bend contours in the specimens which coincide with transition regions between skyrmion and labyrinth patterns. Subsequent application of a perpendicular magnetic field near these regions reveals the unusual situation where skyrmions with opposite magnetic polarities are stabilized in close proximity.

cond-mat.mtrl-sci

Magnetic Damping in Epitaxial Fe Alloyed with Vanadium and Aluminum

To develop low-moment, low-damping metallic ferromagnets for power-efficient spintronic devices, it is crucial to understand how magnetic relaxation is impacted by the addition of nonmagnetic elements. Here, we compare magnetic relaxation in epitaxial Fe films alloyed with light nonmagnetic elements of V and Al. FeV alloys exhibit lower intrinsic damping compared to pure Fe, reduced by nearly a factor of 2, whereas damping in FeAl alloys increases with Al content. Our experimental and computational results indicate that reducing the density of states at the Fermi level, rather than the average atomic number, has a more significant impact in lowering damping in Fe alloyed with light elements. Moreover, FeV is confirmed to exhibit an intrinsic Gilbert damping parameter of $\simeq$0.001, among the lowest ever reported for ferromagnetic metals.

cond-mat.mtrl-sci

Sub-Nanosecond Spin-Transfer Torque in an Ensemble of Superparamagnetic-Like Nanomagnets

Spin currents can exert spin-transfer torques on magnetic systems even in the limit of vanishingly small net magnetization, as is the case for antiferromagnets. Here, we experimentally show that a spin-transfer torque is operative in a material with weak, short-range magnetic order -- namely, a macroscopic ensemble of superparamagnetic-like Co nanomagnets. We employ element- and time-resolved X-ray ferromagnetic resonance (XFMR) spectroscopy to directly detect sub-ns dynamics of the Co nanomagnets, excited into precession with cone angle $\geq$0.003$^{\circ}$ by an oscillating spin current. XFMR measurements reveal that as the net moment of the ensemble decreases, the strength of the spin-transfer torque increases relative to those of magnetic field torques. Our findings point to spin-transfer torque as an effective way to manipulate the state of nanomagnet ensembles at sub-ns timescales.

cond-mat.mes-hall

Conductivity-Like Gilbert Damping due to Intraband Scattering in Epitaxial Iron

Confirming the origin of Gilbert damping by experiment has remained a challenge for many decades, even for simple ferromagnetic metals. In this Letter, we experimentally identify Gilbert damping that increases with decreasing electronic scattering in epitaxial thin films of pure Fe. This observation of conductivity-like damping, which cannot be accounted for by classical eddy current loss, is in excellent quantitative agreement with theoretical predictions of Gilbert damping due to intraband scattering. Our results resolve the longstanding question about a fundamental damping mechanism and offer hints for engineering low-loss magnetic metals for cryogenic spintronics and quantum devices.

cond-mat.mtrl-sci

Magnetic domain wall Skyrmions

It is well established that the spin-orbit interaction in heavy metal/ferromagnet heterostructures leads to a significant interfacial Dzyaloshinskii-Moriya Interaction (DMI) that modifies the internal structure of magnetic domain walls (DWs) to favor Néel over Bloch type configurations. However, the impact of such a transition on the structure and stability of internal DW defects (e.g., vertical Bloch lines) has not yet been explored. We present a combination of analytical and micromagnetic calculations to describe a new type of topological excitation called a DW Skyrmion characterized by a $360^\circ$ rotation of the internal magnetization in a Dzyaloshinskii DW. We further propose a method to identify DW Skyrmions experimentally using Fresnel mode Lorentz TEM; simulated images of DW Skyrmions using this technique are presented based on the micromagnetic results.

cond-mat.mes-hall