arXiv subjects

Arnab Bose

Publications and source records attributed to Arnab Bose.

16 recordsLinked to original sources

arXiv2026

Orbital and Spin Nernst Effects in Monolayers of Transition Metal Dichalcogenides

In recent years, orbitronic effects have attracted growing attention as complementary counterparts to the well-established spintronic phenomena. In this work, we demonstrate that monolayers of transition metal dichalcogenides provide an excellent platform for the observation of the orbital Nernst effect, a relatively less explored phenomenon describing the generation of a transverse orbital current in response to an applied temperature gradient. We show that, similar to its electrical counterpart, viz., the orbital Hall effect, the orbital Nernst effect does not require the presence of spin-orbit coupling. Analytical results based on a low-energy valley model offer key insights into the underlying mechanisms, highlighting in particular the crucial role of electronic states at the Fermi energy for the emergence of this effect. The inclusion of spin-orbit coupling further gives rise to a spin Nernst effect, which scales with the strength of spin-orbit coupling and vanishes in its absence. We substantiate our analytical findings with full Brillouin-zone tight-binding results for two representative systems, monolayer 2H MoS$_2$ and 2H NbS$_2$. Our results show that while both orbital and spin Nernst conductivities in MoS$_2$ require electron or hole doping, both effects are intrinsically present in metallic NbS$_2$. Our work reveals the central role of orbital and spin Berry curvatures, identifies doping as an effective route for tuning orbital and spin Nernst responses, and proposes a possible experimental setup for detecting these effects in monolayer transition metal dichalcogenides.

cond-mat.mes-hall↗

arXiv2025

Non-relativistic spin splitting: Features and Functionalities

Recently, spin splitting of non-relativistic origin in compensated antiferromagnets has drawn growing attention in condensed matter research. Although many materials, now known to exhibit such spin splitting, have been studied for decades, their manifestation along non-high-symmetry momentum directions initially hindered their recognition. In recent years, significant progress has been made in uncovering the symmetry principles that allow non-relativistic spin splitting in the absence of net magnetization, revealing the unconventional physics arising from their coexistence. In this review, we provide a concise overview of non-relativistic spin splitting in compensated antiferromagnets with various spin configurations, including collinear, coplanar, and non-coplanar spin arrangements. We summarize practical identification guidelines, highlight characteristic features in electronic band structures, and discuss the emerging functionalities, with an emphasis on promising directions for future exploration.

cond-mat.mtrl-sci↗

arXiv2025

Identification of orbital pumping from spin pumping and rectification effects

The recently predicted mechanism of orbital pumping enables the generation of pure orbital current from a precessing ferromagnet (FM) without the need for electrical current injection. This orbital current can be efficiently injected into an adjacent nonmagnetic material (NM) without being hampered by electrical conductivity mismatch. However, experimentally identifying this novel effect presents significant challenges due to the substantial background contributions from spin pumping and spin rectification effects (SREs). In this work, we disentangle the effects of orbital pumping from spin pumping in bilayer structures composed of Nb/Ni and Nb/$\mathrm{Fe_{60}Co_{20}B_{20}}$ by observing a sign reversal of the measured voltage. This reversal arises from the competing signs of the spin and orbital Hall effects in the Nb. We establish methods to differentiate the pumping signal from SREs by analyzing the distinct angular dependence of the measured voltage and its spatial dependence relative to the radio frequency excitation source.

cond-mat.mtrl-sci↗

arXiv2024

Fluctuation-mediated spin-orbit torque enhancement in the noncollinear antiferromagnet Mn3Ni0.35Cu0.65N

The role of spin fluctuations near magnetic phase transitions is crucial for generating various exotic phenomena, including anomalies in the extraordinary Hall effect, excess spin-current generation through the spin-Hall effect (SHE), and enhanced spin-pumping, amongst others. In this study, we experimentally investigate the temperature dependence of spin-orbit torques (SOTs) generated by Mn3Ni0.35Cu0.65N (MNCN), a member of the noncollinear antiferromagnetic family that exhibits unconventional magnetotransport properties. Our work uncovers a strong and nontrivial temperature dependence of SOTs, peaking near the Néel temperature of MNCN, which cannot be explained by conventional intrinsic and extrinsic scattering mechanisms of the SHE. Notably, we measure a maximum SOT efficiency of 30%, which is substantially larger than that of commonly studied nonmagnetic materials such as Pt. Theoretical calculations confirm a negligible SHE and a strong orbital Hall effect that can explain the observed SOTs. We propose a previously unidentified mechanism wherein fluctuating antiferromagnetic moments trigger the generation of substantial orbital currents near the Néel temperature due to the emergence of scalar spin chirality. Our findings present an approach for enhancing SOTs, which holds promise for magnetic memory applications by leveraging antiferromagnetic spin fluctuations to amplify both orbital and spin currents.

cond-mat.mes-hall↗

arXiv2023

Higher-order Hall response arises from octupole order and scalar spin chirality in a noncollinear antiferromagnet

Noncollinear antiferromagnets can generate a transverse electrical response known as the anomalous Hall effect, even though they possess almost no net magnetization. The microscopic origin of this behaviour, however, has remained unclear because conventional measurement geometries mix different contributions to the measured response. Here, we show that applying magnetic fields in selected in-plane directions allows us to disentangle the mechanisms underlying the Hall effect in a representative noncollinear antiferromagnet. By suppressing any dipole-related signal, we isolate a purely octupole-driven Hall response that exhibits a characteristic three-fold angular symmetry. At low magnetic fields, we further observe an additional Hall-like contribution that arises from the scalar spin chirality associated with noncoplanar spin textures. Combining symmetry analysis, first-principles calculations, and transport measurements, we reveal that octupole order, dipole moments, and chirality coexist and contribute in distinct field regimes. These findings establish a framework for identifying and controlling complex magnetic order parameters for spintronic applications.

cond-mat.mes-hall↗

arXiv2023

Detection of long-range orbital-Hall torques

We report and quantify a large orbital-Hall torque generated by Nb and Ru, which we identify from a strong dependence of torques on the ferromagnets. This is manifested as a sign reversal and strong enhancement in the damping-like torques measured in Nb (or Ru)/Ni bilayers as compared to Nb (or Ru)/FeCoB bilayers. The long-range nature of orbital transport in the ferromagnet is revealed by the thickness dependences of Ni in Nb (or Ru)/Ni bilayers which are markedly different from the regular spin absorption in the ferromagnet that takes place within a few angstroms and thus it uniquely distinguishes the orbital Hall torque from the spin Hall torque.

cond-mat.mes-hall↗

arXiv2022

Thermally-generated spin current in the topological insulator Bi$_2$Se$_3$

We complete measurements of interconversions among the full triad of thermal gradients, charge currents, and spin currents in the topological insulator Bi$_2$Se$_3$ by quantifying the efficiency with which thermal gradients can generate transverse spin currents. We accomplish this by comparing the spin Nernst magneto-thermopower to the spin Hall magnesistance for bilayers of Bi$_2$Se$_3$/CoFeB. We find that Bi$_2$Se$_3$ does generate substantial thermally-driven spin currents. A lower bound for the ratio of spin current to thermal gradient is $J_s/\nabla_x T$ = (4.9 $\pm$ 0.9) $\times$ 10$^{6}$ ($\hbar/2e$) A m$^{-2}$ / K $μ$m$^{-1}$, and a lower bound for the magnitude of the spin Nernst ratio is $-$0.61 $\pm$ 0.11. The spin Nernst ratio for Bi$_2$Se$_3$ is the largest among all materials measured to date, 2-3 times larger compared to previous measurements for the heavy metals Pt and W.

cond-mat.mes-hall↗

arXiv2022

Origins of transverse voltages generated by applied thermal gradients and applied electric fields in ferrimagnetic-insulator/heavy-metal bilayers

We compare thermal-gradient-driven transverse voltages in ferrimagnetic-insulator/heavy-metal bilayers (Tm3Fe5O12/W and Tm3Fe5O12/Pt) to corresponding electrically-driven transverse resistances at and above room temperature. We find for Tm3Fe5O12/W that the thermal and electrical effects can be explained by a common spin-current detection mechanism, the physics underlying spin Hall magnetoresistance (SMR). However, for Tm3Fe5O12/Pt the ratio of the electrically-driven transverse voltages (planar Hall signal/anomalous Hall signal) is much larger than the ratio of corresponding thermal-gradient signals, a result which is very different from expectations for a SMR-based mechanism alone. We ascribe this difference to a proximity-induced magnetic layer at the Tm3Fe5O12/Pt interface.

cond-mat.mes-hall↗

arXiv2021

Tilted spin current generated by the collinear antiferromagnet RuO2

We report measurements demonstrating that when the Neel vector of the collinear antiferromagnet RuO2 is appropriately canted relative to the sample plane, the antiferromagnet generates a substantial out of plane damping-like torque. The measurements are in good accord with predictions that when an electric field, E is applied to the spin split band structure of RuO2 it can cause a strong transverse spin current even in the absence of spin-orbit coupling. This produces characteristic changes in all three components of the E induced torque vector as a function of the angle of E relative to the crystal axes, corresponding to a spin current with a well defined tilted spin orientation s approximately (but not exactly) parallel to the Neel vector, flowing perpendicular to both E and S. This angular dependence is the signature of an antiferromagnetic spin Hall effect with symmetries that are distinct from other mechanisms of spin-current generation reported in antiferromagnetic or ferromagnetic materials.

cond-mat.mes-hall↗

arXiv2021

Interfacial and bulk spin Hall contributions to field-like spin-orbit torque generated by Iridium

We present measurements of spin orbit torques generated by Ir as a function of film thickness in sputtered Ir/CoFeB and Ir/Co samples. We find that Ir provides a damping-like component of spin orbit torque with a maximum spin torque conductivity 1.4e5 in SI unit and a maximum spin-torque efficiency of 0.04, which is sufficient to drive switching in an 0.8 nm film of CoFeB with perpendicular magnetic anisotropy. We also observe a surprisingly large field like spin orbit torque. Measurements as a function of Ir thickness indicate a substantial contribution to the FLT from an interface mechanism so that in the ultrathin limit there is a non-zero FLT with a maximum torque conductivity -5.0E4 in the SI unit. When the Ir film thickness becomes comparable to or greater than its spin diffusion length, 1.6 nm, there is also a smaller bulk contribution to the fieldlike torque.

cond-mat.mes-hall↗

arXiv2020

Role of Dirac nodal lines and strain on the high spin Hall conductivity of epitaxial IrO2 thin films

Since the discovery of a 'giant' spin Hall effect (SHE) in certain heavy metal elements there has been an intense effort to identify and develop new and technologically viable, heavy-metal-based thin film materials that could generate spin currents with even greater efficiency to exert spin-orbit torques (SOT) on adjacent ferromagnetic nanostructures. In parallel, there have been wide ranging fundamental studies of the spin currents that can arise from robust, intrinsic spin-orbit interaction (SOI) effects in more exotic systems including topological insulators, transition metal dichalcogenides with broken crystalline symmetry, Weyl and Dirac semimetals where gapless electronic excitations are protected by topology and symmetry. Here we experimentally study strong SOT from the topological semimetal IrO2 in (001) and (110) normal films, which exhibit distinctly different SHE strengths. Angle resolved photoemission spectroscopy studies have shown IrO2 exhibits Dirac nodal lines (DNL) in the band structure, which could enable a very high spin Hall conductivity (SHC). The (001) films exhibit exceptionally high damping like torque efficiency ranging from 0.45 at 293 K to 0.65 at 30 K which sets the lower bound of SHC that is ten times higher and of opposite sign than the theoretical prediction. We observe a substantial reduction of SHC in anisotropically strained (110) films, which suggests that the DNLs that are present in the (001) films and contribute to SHC, are disrupted and gapped due to the large anisotropic strain in (110) films, which in turn significantly lowers SHC. Very large value of SHC at room temperature of this Dirac semimetal could be very promising for the practical application.

cond-mat.mes-hall↗

arXiv2018

Control of magnetization dynamics by spin Nernst torque

Control of magnetization dynamics is one of the primary goals in spintronics. It has been demonstrated using spin Hall effect i.e charge current to spin current conversion in non-magnetic metal which has large spin-orbit coupling such as Pt, W etc. Recently different groups have shown generation of spin current in Pt, W while thermal gradient is created by virtue of spin Nernst effect. In this work we show the evidence of magnetization control by spin Nernst torque in Pt/Py bi-layer. We compared relative strength of spin Nernst Torque and spin Hall torque by measuring the systematic variation of magnetic linewidth on application of constant heat or charge current. Spin-torque ferromagnetic resonance (ST-FMR) technique is adopted to excite the magnet and to measure line-width precisely from the symmetric and anti-symmetric voltage component. Control of magnetization dynamics by spin Nernst torque will emerge as an alternative way to manipulate nano-magnets.

physics.app-ph↗

arXiv2017

Direct Observation of the Reciprocity between Spin Current and Phonon Interconversion

Spin current has emerged as a leading candidate for manipulation of spins in a nano-magnet. We here experimentally show another utility of spin current viz. it can be used for generation of phonons. Within the same experimental setup, we also demonstrate the inverse effect of generation of spin current by phonons. To demonstrate them, we measured the scattering-matrix of a two-port device with interdigital transducers as one port and array of Ni/Pt lines as second port on piezoelectric substrate. The off-diagonal elements which correspond to transmission between the ports, were found to have 180 degree relative phase shift. The transmission of electrical signal from port 2 to 1 corresponds to generation of phonons from spin-current, while transmission from port 1 to 2 corresponds to the inverse effect. These results could be useful for designing spin-current based gyrators.

cond-mat.mes-hall↗

arXiv2017

Sign reversal of field like spin-orbit torque in ultrathin Chromium/Nickel bilayer

In this work report unconventional sign change of field like spin orbit torque in ultra-thin Chromium(1.5nm-5nm)/Nickel(8nm) bi-layer. We performed standard spin-torque ferromagnetic resonance (ST-FMR) experiment in Cr/Ni bi-layer by passing radio frequency current and measuring DC voltage. We observe that when thickness of Cr layer is critically low (<6nm) spin orbit torque by Cr on Ni significantly increases. Most importantly the sign of field like torque is opposite to the Oersted field generated torque. To verify interracial nature of this torque, 2 nm thin Cu is inserted between Cr and Ni and field like torque behaves same as Oersted field induced torque. Hence possible origin of such unconventional sign change of field like torque could be inter-facial Rashba like spin orbit interaction which is present between Cr and Ni but vanishes in Cr/Cu/Ni hetero-structure. From our experiment we can estimate that approximately 35 Oe of effective Rashba like magnetic field is created on 8 nm thicker Ni layer, when 1E12 A/m^2 current flows through Cr layer. All experiments are done at room temperature. So Cr thin film is expected to behave like paramagnet (Neel temperature of bulk Cr is 311K). Hence Cr can be a good choice as a heavy metal to employ large spin orbit torque combining bulk spin Hall effect and inter-facial Rashba interaction.

cond-mat.mes-hall↗

arXiv2017

Observation of anomalous spin-torque generated by a ferromagnet

In this work we report observation of in-plane current induced out-of-plane magnetic field driven torque in spin valve structure. Since ferromagnet has high spin orbit coupling it is expected to be the source of spin-orbit-torque as it possesses anomalous-Hall-effect (AHE: equivalent to spin Hall effect in heavy metal). So we have carried out spin-torque ferromagnetic resonance (ST-FMR) experiment in a spin valve (consists of a fixed magnet and a free magnet which are separated by Cu spacer), passing in-plane radio frequency current and measuring DC voltage. Our experimental results eventually indicate that spin torque exerted on the free magnet is not caused due to the spin current injection by the fixed magnet owing to its AHE, but it is originated from in-plane current driven out-of plane effective magnetic field. This is new class of spin torque which is completely different from Slonczewski-spin transfer torque and Rashba like field like torque. The effective out-of plane magnetic field depends on the direction of current (in-plane) and magnetization (in-plane) of the pinned layer. One possible mechanism behind this unconventional torque could be intefacial spin-scattering which is also origin of current in-plane GMR effect. Most importantly this effective out-of plane torque can be useful to switch out-of plane magnetic bits in spintronic memory application.

cond-mat.mes-hall↗

arXiv2017

Observation of Spin Nernst effect in Platinum

Central focus of spintronics is concentrated on generation of pure spin current and associated spin torque. Pure spin current can be generated by spin Hall effect in heavy metals by passing charge current. By spin Seebeck effect pure spin current can also be generated in ferromagnet. In this work we experimentally demonstrate that if heavy metals like Platinum with high spin orbit coupling carry heat current it can convert it into spin current due to relativistic spin orbit interaction. This conversion of heat current into spin current in non magnet is equivalent of thermally driven spin Hall effect or it is known as spin Nernst effect. We observed spin Nernst effect in Ni/Pt bi-layer experimentally and we confirm that when Pt is replaced by low spin orbit material like Al spin Nernst effect significantly reduces. So we have detected spin Nernst effect unambiguously and compare its strength with electrical spin Hall effect.

cond-mat.mes-hall↗