arXiv subjects

Arnaud Gloppe

Publications and source records attributed to Arnaud Gloppe.

10 recordsLinked to original sources

arXiv2026

Sub-nm range momentum-dependent exciton transfer from a 2D semiconductor to graphene

Heterostructures made from atomically thin semiconductors (here MoSe$_2$) and graphene are uniquely poised to investigate photoinduced charge and energy transfer in the 2D limit. Here, using picosecond time-resolved photoluminescence spectroscopy at cryogenic temperatures on two types of MoSe$_2$/graphene heterostrutures, we unveil key features of the underlying mechanisms. First, the shortening of the MoSe$_2$ bright exciton lifetime is marginally affected by the number of graphene layers to which MoSe$_2$ is coupled. Second, exciton transfer vanishes when a sub-nm thick spacer of hexagonal boron nitride decouples MoSe$_2$ from graphene. These results indicate that charge tunneling govern bright exciton relaxation in MoSe$_2$/graphene and that longer-range, Förster-type energy transfer (FRET) does not affect bright excitons. However, sub-ps FRET to graphene accelerates the relaxation of ``hot'' excitons formed upon optical excitation, leading to photoluminescence quenching factors that exceed expectations based on the shortening of the bright exciton lifetime. Our work has direct implications for energy harvesting and funneling using van der Waals heterostructures.

cond-mat.mes-hall↗

arXiv2025

Magnetic excitons in a suspended 2D antiferromagnetic membrane

Layered magnetic and strongly correlated materials present a rich platform for condensed matter physics with intrinsic properties intertwined by magnetism and low-dimensionality. A suspended light-emitting 2D antiferromagnetic membrane forms a highly controllable hybrid system in which the interplay between spin ordering, optical and mechanical degrees of freedom can be uniquely explored. NiPS$_3$ hosts excitons responsible for a puzzling luminescence down to a few atomic layers, linked to its zigzag antiferromagnetic order. The nature of these excitons remains unclear. Here we report on the magnetic excitons of a suspended few-layer NiPS$_3$ membrane. We reveal nematic zigzag states and study the optical transitions induced by the magnon-mediated motion of the excitation in the magnetic lattice, resulting in magnon-dressed excitons. We observe a strain tuning of these emission lines, dependent on their microscopic origin, with rates that sign a strong localization of the magnetic excitons, fading with the number of magnon-mediated hops.

cond-mat.mes-hall↗

arXiv2023

Symmetry-dependent dielectric screening of optical phonons in monolayer graphene

Quantised lattice vibrations (i.e., phonons) in solids are robust and unambiguous fingerprints of crystal structures and of their symmetry properties. In metals and semimetals, strong electron-phonon coupling may lead to so-called Kohn anomalies in the phonon dispersion, providing an image of the Fermi surface in a non-electronic observable. Kohn anomalies become prominent in low-dimensional systems, in particular in graphene, where they appear as sharp kinks in the in-plane optical phonon branches. However, in spite of intense research efforts on electron-phonon coupling in graphene and related van der Waals heterostructures, little is known regarding the links between the symmetry properties of optical phonons at and near Kohn anomalies and their sensitivity towards the local environment. Here, using inelastic light scattering (Raman) spectroscopy, we investigate a set of custom-designed graphene-based van der Waals heterostructures, wherein dielectric screening is finely controlled at the atomic layer level. We demonstrate experimentally and explain theoretically that, depending exclusively on their symmetry properties, the two main Raman modes of graphene react differently to the surrounding environment. While the Raman-active near-zone-edge optical phonons in graphene undergo changes in their frequencies due to the neighboring dielectric environment, the in-plane, zone-centre optical phonons are symmetry-protected from the influence of the latter. These results shed new light on the unique electron-phonon coupling properties in graphene and related systems and provide invaluable guidelines to characterise dielectric screening in van der Waals heterostructures and moiré superlattices.

cond-mat.mes-hall↗

arXiv2021

Magnon-exciton proximity coupling at a van der Waals heterointerface

Spin and photonic systems are at the heart of modern information devices and emerging quantum technologies. An interplay between electron-hole pairs (excitons) in semiconductors and collective spin excitations (magnons) in magnetic crystals would bridge these heterogeneous systems, leveraging their individual assets in novel interconnected devices. Here, we report the magnon-exciton coupling at the interface between a magnetic thin film and an atomically-thin semiconductor. Our approach allies the long-lived magnons hosted in a film of yttrium iron garnet (YIG) to strongly-bound excitons in a flake of a transition metal dichalcogenide, MoSe$_2$. The magnons induce on the excitons a dynamical valley Zeeman effect ruled by interfacial exchange interactions. This nascent class of hybrid system suggests new opportunities for information transduction between microwave and optical regions.

cond-mat.mes-hall↗

arXiv2019

Resonant magnetic induction tomography of a magnetized sphere

We demonstrate the structural imaging of magnetostatic spin-wave modes hosted in a millimeter-sized ferromagnetic sphere. Unlike for low-dimensional magnetic materials, there is no prior technique to image these modes in bulk magnetized solid of revolution. Based on resonant magnetic induction tomography in the microwave range, our approach ensures the robust identification of these non-trivial spin-wave modes by establishing their azimuthal and polar dependences, starting point of magnonic fundamental studies and hybrid systems with complex spin textures well beyond the uniform precession mode.

cond-mat.mtrl-sci↗

arXiv2019

Hybrid quantum systems based on magnonics

Engineered quantum systems enabling novel capabilities for communication, computation, and sensing have blossomed in the last decade. Architectures benefiting from combining distinct and complementary physical quantum systems have emerged as promising platforms for developing quantum technologies. A new class of hybrid quantum systems based on collective spin excitations in ferromagnetic materials has led to the diverse set of experimental platforms which are outlined in this review article. The coherent interaction between microwave cavity modes and collective spin-wave modes is presented as the backbone of the development of more complex hybrid quantum systems. Indeed, quanta of excitation of the spin-wave modes, called magnons, can also interact coherently with optical photons, phonons, and superconducting qubits in the fields of cavity optomagnonics, cavity magnomechanics, and quantum magnonics, respectively. Notably, quantum magnonics provides a promising platform for performing quantum optics experiments in magnetically-ordered solid-state systems. Applications of hybrid quantum systems based on magnonics for quantum information processing and quantum sensing are also outlined briefly.

quant-ph↗

arXiv2015

Nano-optomechanical measurement in the photon counting regime

Optically measuring in the photon counting regime is a recurrent challenge in modern physics and a guarantee to develop weakly invasive probes. Here we investigate this idea on a hybrid nano-optomechanical system composed of a nanowire hybridized to a single Nitrogen-Vacancy (NV) defect. The vibrations of the nanoresonator grant a spatial degree of freedom to the quantum emitter and the photon emission event can now vary in space and time. We investigate how the nanomotion is encoded on the detected photon statistics and explore their spatio-temporal correlation properties. This allows a quantitative measurement of the vibrations of the nanomechanical oscillator at unprecedentedly low light intensities in the photon counting regime when less than one photon is detected per oscillation period, where standard detectors are dark-noise-limited. These results have implications for probing weakly interacting nanoresonators, for low temperature experiments and for investigating single moving markers.

quant-ph↗

arXiv2015

Observation of a phononic Mollow triplet in a hybrid spin-nanomechanical system

Reminiscent of the bound character of a qubit's dynamics confined on the Bloch sphere, the observation of a Mollow triplet in the resonantly driven qubit fluorescence spectrum represents one of the founding signatures of Quantum Electrodynamics. Here we report on its observation in a hybrid spin-nanomechanical system, where a Nitro-gen Vacancy spin qubit is magnetically coupled to the vibrations of a Silicon Carbide nanowire. A resonant microwave field turns the originally parametric hybrid interac-tion into a resonant process, where acoustic phonons are now able to induce transitions between the dressed qubit states, leading to synchronized spin-oscillator dynamics. We further explore the vectorial character of the hybrid coupling to the bidimensional de-formations of the nanowire. The demonstrated microwave assisted synchronization of the spin-oscillator dynamics opens novel perspectives for the exploration of spin-dependent forces, the key-ingredient for quantum state transfer.

quant-ph↗

arXiv2014

Bidimensional nano-optomechanics and topological backaction in a non-conservative radiation force field

Optomechanics, which explores the fundamental coupling between light and mechanical motion, has made important advances in both exploring and manipulating macroscopic mechanical oscillators down to the quantum level. However, dynamical effects related to the vectorial nature of the optomechanical interaction remain to be investigated. Here we study a nanowire with sub-wavelength dimensions strongly coupled to a tightly focused beam of light, enabling ultrasensitive readout of the nanoresonators dynamics. We experimentally determine the vectorial structure of the optomechanical interaction and demonstrate that bidimensional dynamical backaction governs the nanowire dynamics. Moreover, the non-conservative topology of the optomechanical interaction is responsible for a novel canonical signature of strong coupling between the nanoresonator mechanical modes, leading to a topological instability. These results have a universal character and illustrate the increased sensitivity of nanomechanical devices towards topologically varying interactions, opening fundamental perspectives in nanomechanics, optomechanics, ultrasensitive scanning probe force microscopy and nano-optics.

quant-ph↗

arXiv2013

Strain-mediated coupling in a quantum dot-mechanical oscillator hybrid system

Recent progress in nanotechnology has allowed to fabricate new hybrid systems where a single two-level system is coupled to a mechanical nanoresonator. In such systems the quantum nature of a macroscopic degree of freedom can be revealed and manipulated. This opens up appealing perspectives for quantum information technologies, and for the exploration of quantum-classical boundary. Here we present the experimental realization of a monolithic solid-state hybrid system governed by material strain: a quantum dot is embedded within a nanowire featuring discrete mechanical resonances corresponding to flexural vibration modes. Mechanical vibrations result in a time-varying strain field that modulates the quantum dot transition energy. This approach simultaneously offers a large light extraction efficiency and a large exciton-phonon coupling strength $g_0$. By means of optical and mechanical spectroscopy, we find that $g_0/2π$ is nearly as large as the mechanical frequency, a criterion which defines the ultra-strong coupling regime.

cond-mat.mes-hall↗