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Arne Keller

Publications and source records attributed to Arne Keller.

At least 37 records · Page 2Linked to original sources

Classification of Dark States in Multi-level Dissipative Systems

Dark states are eigenstates or steady-states of a system that are decoupled from the radiation. Their use, along with associated techniques such as Stimulated Raman Adiabatic Passage, has extended from atomic physics where it is an essential cooling mechanism, to more recent versions in condensed phase where it can increase the coherence times of qubits. These states are often discussed in the context of unitary evolution and found with elegant methods exploiting symmetries, or via the Bruce-Shore transformation. However, the link with dissipative systems is not always transparent, and distinctions between classes of CPT are not always clear. We present a detailed overview of the arguments to find stationary dark states in dissipative systems, and examine their dependence on the Hamiltonian parameters, their multiplicity and purity. We find a class of dark states that depends not only on the detunings of the lasers but also on their relative intensities. We illustrate the criteria with the more complex physical system of the hyperfine transitions of $^{87}$Rb and show how a knowledge of the dark state manifold can inform the preparation of pure states.

quant-ph↗

On the ubiquity of Beutler-Fano profiles: from scattering to dissipative processes

Fano models - consisting of a Hamiltonian with discrete-continuous spectrum - are one of the basic toy models in spectroscopy. They have been succesfull in explaining the lineshape of experiments in atomic physics and condensed matter. These models however have largely been out of the scope of dissipative dynamics, with ony a handful of works considering the effect of a thermal bath. Yet in nanostructures and condensed matter systems, dissipation strongly modulates the dynamics. In this article, we present an overview of the theoretical works dealing with Fano interferences coupled to a thermal bath and compare them to the scattering formalism. We provide the solution to any discrete-continuous Hamiltonian structure within the wideband approximation coupled to a Markovian bath. In doing so, we update the toy models that have been available for unitary evolution since the 1960s. We find that the Fano lineshape is preserved as long as we allow a rescaling of the parameters, and an additional Lorentzian contribution that reflects the destruction of the interference by dephasings. We discuss the pertinence of each approach - dissipative and unitary - to different experimental setups: scattering, transport and spectroscopy of dissipative systems. We finish by discussing the current limitations of the theories due to the wideband approximation and the memory effects of the bath.

quant-ph↗

Connecting measurement invasiveness to optimal metrological scenarios

The connection between the Leggett-Garg inequality and optimal scenarios from the point of view of quantum metrology is investigated for perfect and noisy general dichotomic measurements. In this context, we show that the Fisher information can be expressed in terms of quantum temporal correlations. This connection allows us to associate scenarios with relatively high Fisher information to scenarios in which the Leggett-Garg inequality is violated. We thus demonstrate a qualitative and, to some extent, quantitative link between measurement invasiveness and metrological performance. Finally, we illustrate our results by using a specific model for spin systems.

quant-ph↗

Non-linear Fano Interferences in Open Quantum Systems: an Exactly Solvable Model

We obtain an explicit solution for the stationary state populations of a dissipative Fano model, where a discrete excited state is coupled to a continumm set of states; both excited set of states are reachable by photo-excitation from the ground state. The dissipative dynamic is described by a Liouville equation in Lindblad form and the field intensity can take arbitrary values within the model. We show that the continuum states population as a function of laser frequency can always be expressed as a Fano profile plus a Lorentzian function with effective parameters whose explicit expressions are given in the case of a closed system coupled to a bath as well as for the original Fano scattering framework. Although the solution is intricate, it can be elegantly expressed as a linear transformation of the kernel of a $4\times 4$ matrix which has the meaning of an effective Liouvillian. We unveil key notable processes related to the optical nonlinearity and which had not been reported to date: electromagnetic induced-transparency, population inversions, power narrowing and broadening, as well as an effective reduction of the Fano asymmetry parameter.

quant-ph↗

Generalized spin squeezing inequalities for particles number with quantum fluctuations

Particle number fluctuations, no matter how small, are present in experimental set-ups. One should rigorously take these fluctuations into account, especially, for entanglement detection. In this context, we generalize the spin squeezing inequalities introduced by Tóth et al. in Phys. Rev. Lett. 99, 250405 (2007). These new inequalities are fulfilled by all separable states even when the number of particle is not constant, and may present quantum fluctuations. These inequalities are useful for detecting entanglement in many-body systems when the super-selection rule does not apply, or when only a subspace of the total systems Hilbert space is considered. We also define general dichotomic observables for which we obtain a coordinate independent form of the generalized spin squeezing inequalities. We give an example where our generalized coordinate independent spin squeezing inequalities present a clear advantage over the original ones.

quant-ph↗

Modeling Leggett-Garg-inequality violation

The Leggett-Garg inequality is a widely used test of the "quantumness" of a system, and involves correlations between measurements realized at different times. According to its widespread interpretation, a violation of the Legget-Garg inequality disproofs macroscopic realism and non-invasiveness. Nevertheless, recent results point out that macroscopic realism is a model dependent notion and that one should always be able to attribute to invasiveness a violation of a Legget-Garg inequality. This opens some natural questions: how to provide such an attribution in a systematic way? How can apparent macroscopic realism violation be recast into a dimensional independent invasiveness model? The present work answers these questions by introducing an operational model where the effects of invasiveness are controllable through a parameter associated with what is called the {\it measurability} of the physical system. Such a parameter leads to different generalized measurements that can be associated with the dimensionality of a system, to measurement errors or to back action.

quant-ph↗

Fano-Liouville Spectral Signatures in Open Quantum Systems

The scattering amplitude from a set of discrete states coupled to a continuum became known as the Fano profile, characteristic for its asymmetric lineshape and originally investigated in the context of photoionization. The generality of the model, and the proliferation of engineered nanostructures with confined states gives immense success to the Fano lineshape, which is invoked whenever an asymmetric lineshape is encountered. However, many of these systems do not conform to the initial model worked out by Fano in that i) they are subject to dissipative processes and ii) the observables are not entirely analogous to the ones measured in the original photoionization experiments. In this letter, we work out the full optical response of a Fano model with dissipation. We find that the exact result for absorption, Raman, Rayleigh and fluorescence emission is a modified Fano profile where the typical lineshape has an additional Lorentzian contribution. Expressions to extract model parameters from a set of relevant observables are given.

quant-ph↗

A general dichotomization procedure to provide qudits entanglement criteria

We present a general strategy to derive entanglement criteria which consists in performing a mapping from qudits to qubits that preserves the separability of the parties and SU(2) rotational invariance. Consequently, it is possible to apply the well known positive partial transpose criterion to reveal the existence of quantum correlations between qudits. We discuss some examples of entangled states that are detected using the proposed strategy. Finally, we demonstrate, using our scheme, how some variance-based entanglement witnesses can be generalized from qubits to higher dimensional spin systems.

quant-ph↗

Toolbox for continuous variable entanglement production and measurement using spontaneous parametric down conversion

We provide a toolbox for continuous variables quantum state engineering and characterization of biphoton states produced by spontaneous parametric down conversion in a transverse pump configuration. We show that the control of the pump beam's incidence spot and angle corresponds to phase space displacements of conjugate collective continuous variables of the biphoton. In particular, we illustrate with numerical simulations on a semiconductor device how this technique can be used to engineer and characterize arbitrary states of the frequency and time degrees of freedom.

quant-ph↗

Bell states generation on a III-V semiconductor chip at room temperature

We demonstrate the generation of polarization-entangled photon pairs at room temperature and telecom wavelength in a AlGaAs semiconductor waveguide. The source is based on spontaneous parametric down conversion with a counterpropagating phase-matching scheme. The quality of the two-photon state is assessed by the reconstruction of the density matrix giving a raw fidelity to a Bell state of 0.83; a theoretical model, taking into account the experimental parameters, provides ways to understand and control the amount of entanglement. Its compatibility with electrical injection, together with the high versatility of the generated two-photon state, make this source an attractive candidate for completely integrated quantum photonics devices.

quant-ph↗

Direct measurement of the biphoton Wigner function through two-photon interference

The Hong-Ou-Mandel (HOM) experiment was a benchmark in quantum optics, evidencing the quantum nature of the photon. In order to go deeper, and obtain the complete information about the quantum state of a system, for instance, composed by photons, the direct measurement or reconstruction of the Wigner function or other quasi--probability distribution in phase space is necessary. In the present paper, we show that a simple modification in the well-known HOM experiment provides the direct measurement of the Wigner function. We apply our results to a widely used quantum optics system, consisting of the biphoton generated in the parametric down conversion process. In this approach, a negative value of the Wigner function is a sufficient condition for non-gaussian entanglement between two photons. In the general case, the Wigner function provides all the required information to infer entanglement using well known necessary and sufficient criteria. We analyze our results using two examples of parametric down conversion processes taken from recent experiments. The present work offers a new vision of the HOM experiment that further develops its possibilities to realize fundamental tests of quantum mechanics involving decoherence and entanglement using simple optical set-ups.

quant-ph↗

Laser induced electron diffraction: a tool for molecular orbital imaging

We explore the laser-induced ionization dynamics of N2 and CO2 molecules subjected to a few-cycle, linearly polarized, 800\,nm laser pulse using effective two-dimensional single active electron time-dependent quantum simulations. We show that the electron recollision process taking place after an initial tunnel ionization stage results in quantum interference patterns in the energy resolved photo-electron signals. If the molecule is initially aligned perpendicular to the field polarization, the position and relative heights of the associated fringes can be related to the molecular geometrical and orbital structure, using a simple inversion algorithm which takes into account the symmetry of the initial molecular orbital from which the ionized electron is produced. We show that it is possible to extract inter-atomic distances in the molecule from an averaged photon-electron signal with an accuracy of a few percents.

physics.atom-ph↗

Bell inequalities with continuous angular variables

We consider bipartite quantum systems characterized by a continuous angular variable θ\in [-π, π[, representing, for instance, the position of a particle on a circle. We show how to reveal non-locality on this type of system using inequalities similar to CHSH ones, originally derived for bipartite spin 1/2 like systems. Such inequalities involve correlated measurement of continuous angular functions and are equivalent to the continuous superposition of CHSH inequalities acting on bidimensional subspaces of the infinite dimensional Hilbert space. As an example, we discuss in detail one application of our results, and we derive inequalities based on orientation correlation measurements. The introduced Bell-type inequalities open the perspective of new and simpler experiments to test non locality on a variety of quantum systems described by continuous variables.

quant-ph↗

Ultrafast Molecular Imaging by Laser Induced Electron Diffraction

We address the feasibility of imaging geometric and orbital structure of a polyatomic molecule on an attosecond time-scale using the laser induced electron diffraction (LIED) technique. We present numerical results for the highest molecular orbitals of the CO2 molecule excited by a near infrared few-cycle laser pulse. The molecular geometry (bond-lengths) is determined within 3% of accuracy from a diffraction pattern which also reflects the nodal properties of the initial molecular orbital. Robustness of the structure determination is discussed with respect to vibrational and rotational motions with a complete interpretation of the laser-induced mechanisms.

quant-ph↗

Thermal entanglement in a molecular chain

We investigate entanglement in a linear chain of $N$ polar molecules coupled by dipole interaction. In our model, nearest neighbour interaction predominate, and we compute entanglement with the help of a two-party correlation entanglement measure. We find that, in this system, only excited states are entangled. Moreover, when an electrostatic field is applied, energy levels crossings occur, changing significantly the system's entanglement properties. We make a systematic study of the entanglement dependency on the inter molecular distance separating pairs of molecules, different partitions of the chain and physical parameters as the temperature and the electrostatic field's intensity, showing that it persists for relatively high temperatures and changes its nature with varying field.

quant-ph↗

Bell-type inequalities for cold heteronuclear molecules

We introduce Bell-type inequalities allowing for non-locality and entanglement tests with two cold heteronuclear molecules. The proposed inequalities are based on correlations between each molecule spatial orientation, an observable which can be experimentally measured with present day technology. Orientation measurements are performed on each subsystem at diferent times. These times play the role of the polarizer angles in Bell tests realized with photons. We discuss the experimental implementations of the proposed tests, which could also be adapted to other high dimensional quantum angular momenta systems.

quant-ph↗

Quantum phase gate and controlled entanglement with polar molecules

We propose an alternative scenario for the generation of entanglement between rotational quantum states of two polar molecules. This entanglement arises from dipole-dipole interaction, and is controlled by a sequence of laser pulses simultaneously exciting both molecules. We study the efficiency of the process, and discuss possible experimental implementations with cold molecules trapped in optical lattices or in solid matrices. Finally, various entanglement detection procedures are presented, and their suitability for these two physical situations is analyzed.

quant-ph↗

Optimally Controlled Field-Free Orientation of the Kicked Molecule

Efficient and long-lived field-free molecular orientation is achieved using only two kicks appropriately delayed in time. The understanding of the mechanism rests upon a molecular target state providing the best efficiency versus persistence compromise. An optimal control scheme is referred to for fixing the free parameters (amplitudes and the time delay between them). The limited number of kicks, the robustness and the transposability to different molecular systems advocate in favor of the process, when considering its experimental feasibility.

physics.chem-ph↗