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Arno Rauschenbeutel

Publications and source records attributed to Arno Rauschenbeutel.

At least 19 recordsLinked to original sources

High-optical-depth, sub-Doppler-width absorption lines at telecom wavelengths in hot, optically driven rubidium vapor

Doppler broadening presents a major limitation for high-resolution spectroscopy and nonlinear optics in room-temperature atomic vapors. Here, we demonstrate the suppression of Doppler broadening accompanied by pronounced absorption on the upper transition of a three-level ladder system, achieved by dressing the intermediate state with a strong control field. As a concrete realization, we study a hot vapor of $^{87}$Rb where the lower transition is driven by a strong control field resonant with the D2 line at a wavelength of 780 nm, while a weak counter-propagating probe field at the telecom C-band wavelength of 1529 nm ($5P_{(3/2)}\leftrightarrow 4D_{(5/2)}$) interrogates the dressed states. We observe absorption features with a resonant optical depth of approximately 4 and a full width at half maximum of about 17 MHz. Remarkably, this corresponds to an order-of-magnitude reduction relative to the Doppler width, while the optical depth on the upper transition of the ladder scheme exceeds that of the Doppler-broadened lower transition. The measured spectra are in good agreement with theoretical modeling. Combining high optical density with sub-Doppler-width absorption lines typically requires laser-cooled atoms, while our approach profits from the experimental simplicity of a hot-vapor platform.

physics.atom-ph

$Λ$-enhanced gray-molasses loading and EIT cooling of neutral atoms in nanophotonic traps

Nanophotonic traps for cold atoms typically have trap volumes that are orders of magnitude smaller than, e.g., free-space optical tweezers. This makes efficient loading of these traps challenging, thereby limiting the total number of atoms coupled to the nanophotonic waveguide. Here, we demonstrate that $Λ$-enhanced gray-molasses ($Λ$GM) can substantially increase the number of trapped atoms in a nanofiber-based cold-atom setup. Specifically, we observe a six-fold increase in the number of loaded atoms compared to conventional red-detuned polarization gradient cooling. Despite the unusually small depth of our optical trap of only 24 $μ$K, we load about 4000 individual Cesium atoms, achieving optical depths exceeding 140 and reaching the collisional blockade regime over a length of approximately 1 mm. After loading, we perform efficient EIT-assisted cooling that is found to increase the trap storage time to 400(9) ms. This is a 5-fold improvement over the passive storage time. Remarkably, EIT-cooling also works with two co-propagating nanofiber-guided light fields and requiries only about a few hundred picowatt of optical power. Our results provide an efficient method to boost both the number of loaded atoms and the storage time of nanophotonic atom traps.

physics.atom-ph

Limits of Stable Near-Field Probing in Nanophotonic Traps

Near-fields around nanophotonic structures and waveguides can be used to optically interface particles ranging from atoms and molecules to microscopic biological and synthetic particles. Due to the strong, non-linear dependence of the near-field coupling strength on the particles' position, a change of the spread of the particles' position will change their mean coupling strength. When the particles are trapped, this position spread depends on their temperature, generally leading to temperature-dependent coupling. Here, we experimentally demonstrate that this effect renders optical probing of trapped particles with near fields an inherently transient process. Specifically, we trap cold atoms in a two-color dipole trap surrounding an optical nanofiber and probe them with the evanescent field of guided, resonant light. The scattering of this probe light heats up the atoms, leading to a decrease of the coupling strength as well as loss of atoms. We observe both effects via a concurrent decrease of the absorption signal. In addition, we demonstrate that the coupling strength can be recovered by cooling the atoms back to their initial temperature. Our findings are relevant for numerous situations where stable coupling of trapped particles to a nanophotonic structure is required.

quant-ph

On the Relationship Between Antibunching and Entanglement in Resonance Fluorescence

Photon antibunching in resonance fluorescence - the emission from a single, resonantly driven two-level quantum emitter - is a paradigmatic signature of nonclassical light. Photon entanglement, by contrast, manifests as correlations that can defy any classical description and is typically regarded as a distinct quantum effect. Here, we experimentally extract pairs of narrowband, time-bin-entangled photons from the antibunched resonance fluorescence of a single trapped atom. We verify entanglement via violation of the CHSH Bell inequality and by reconstructing the two-photon density matrix. The observed correlations vanish when the coincidence time window exceeds the antibunching timescale, revealing underlying multimode entanglement in the emitted field. Our results establish a direct link between photon antibunching and photon-photon entanglement, unifying two canonical signatures of nonclassical light.

quant-ph

Hybrid Trapping of Cold Atoms with Surface Forces and Blue-Detuned Evanescent Light on a Nanophotonic Waveguide

We demonstrate a novel hybrid nanophotonic trap for cold neutral atoms, leveraging surface forces for attraction and blue-detuned evanescent light for repulsion. We attribute the attractive potential to a combination of Casimir-Polder interactions and electrostatic charges distributed on the waveguide surface. Despite the trap's shallow depth, we efficiently load atoms into it via adiabatic transfer from a conventional two-color dipole trap. Remarkably, the hybrid trap supports a long atomic storage time of 140(9) ms and exhibits a Ramsey coherence time of 16.8(2) ms, the latter exceeding significantly previous reports for nanophotonic systems. Our results pave the way for further exploration of atom-surface interactions at the nanoscale and illustrate the potential of harnessing surface forces to enhance storage and coherence times for atoms coupled to nanophotonic waveguides. This advancement offers new opportunities for neutral-atom quantum technologies.

quant-ph

Magic-wavelength nanofiber-based two-color dipole trap with sub-$λ/2$ spacing

We report on the realization and characterization of a novel magic-wavelength nanofiber-based two-color optical dipole trap for cesium that allows us to generate two diametral periodic one-dimensional arrays of trapping sites with a spacing significantly smaller than half the resonant free-space wavelength of the cesium D2 transition. This is achieved by launching a blue-detuned partial standing wave and two red-detuned light fields through the nanofiber. We trap and optically interface the atoms in the resulting periodic optical potential and characterize the trap by measuring the lifetime of the trapped atoms, the atom-light coupling strength, the filling factor, and the trap frequencies in the radial and axial directions. The implementation of this nanofiber-based optical interface with magic trapping wavelengths and sub-$λ/2$ spacing is an important step towards the exploration of novel collective radiative effects, such as selective radiance.

physics.atom-ph

Few-MHz bandwidth tunable optical filter based on a fiber-ring resonator

We present a fiber-ring resonator that realizes an ultra-narrowband, high-extinction, low-loss, tunable optical filter. It consists of a pair of commercial variable ratio directional couplers that allow precise adjustment of the filter bandwidth and its on-resonance transmission. This design also grants access to multiple modes of operation, such as a simultaneous band-stop and band-pass filter. Our characterization reveals a bandwidth of less than 2 MHz, together with an extinction exceeding 20 dB. The tunability of the filter properties establishes our device as a versatile platform for selective frequency filtering with sub-natural atomic linewidth resolution.

physics.optics

Measuring deviations from a perfectly circular cross-section of an optical nanofiber at the Ångström scale

Tapered optical fibers (TOFs) with sub-wavelength-diameter waists, known as optical nanofibers, are powerful tools for interfacing quantum emitters and nanophotonics. These applications demand stable polarization of the fiber-guided light field. However, the linear birefringence resulting from Ångström-scale deviations in the nanofiber's ideally circular cross-section can lead to significant polarization changes within millimeters of light propagation. Here, we experimentally investigate such deviations using two in-situ approaches. First, we measure the resonance frequencies of hundreds of flexural modes along the nanofiber, which exhibit splitting due to the non-circular cross section. By analyzing the mean resonance frequencies of each pair and the corresponding frequency splitting, we conclude that the nanofiber can be well described as having an elliptical cross-section with a mean radius of 255.6(9) nm, where the semi-axes differ by only about 2Å. Second, we monitor the polarization of the guided light field by imaging the light scattered out of the nanofiber and observe a periodic polarization change along it. From the linear birefringence due to the elliptical cross-section, we infer a comparable difference in the semi-axes as the first method, and determine the orientation of the polarization eigenaxes. Our work is crucial for any fundamental or applied study that requires a well-controlled interaction between guided light and matter, in particular for quantum memories, frequency conversion, or lasing that require a large interaction length.

physics.optics

Simple analytical model describing the collective nonlinear response of an ensemble of two-level emitters weakly coupled to a waveguide

We model and investigate the collective nonlinear optical response of an ensemble of two-level emitters that are weakly coupled to a single-mode waveguide. Our approach generalizes the insight that photon-photon correlations in the light scattered by a single two-level emitter result from two-photon interference to the case of many emitters. Using our model, we study different configurations for probing the nonlinear response of the ensemble, e.g., through the waveguide or via external illumination, and derive analytical expressions for the second-order quantum coherence function, $g^{(2)}(τ)$, as well as for the squeezing spectrum of the output light in the waveguide, $S_θ(ω)$. For the transmission of resonant guided light, we recover the same predictions as previously made with far more involved theoretical models when analyzing experimental results regarding $g^{(2)}(τ)$ (Prasad et al. [1]) and $S_θ(ω)$ (Hinney et al. [2]). We also study the transmission of light that is detuned from the transition of the two-level emitter, a situation that we recently studied experimentally (Cordier et al. [3]). Our model predictions show how the collectively enhanced nonlinear response of weakly coupled emitters can be harnessed to generate non-classical states of light using ensembles ranging from a few to many emitters.

quant-ph

Photon Transport in a Gas of Two-Level Atoms: Unveiling Quantum Light Creation

We present a theoretical analysis of nearly monochromatic light propagation through a gas of two-level atoms using the Heisenberg-Langevin equation method. Our focus is on the evolution of the photon annihilation operator and its impact on the second-order correlation function, $g^{(2)}(τ)$, with particular emphasis on photon antibunching behavior. The model accounts for both open and closed atomic system approximations, including Doppler broadening and the influence of pump field detuning. We derive expressions that reproduce known results from scattering theory and extend the analysis to complex systems, such as inhomogeneously broadened media. The theoretical predictions are compared with experimental data from a waveguide QED platform, which show good agreement and thereby demonstrate the power of our approach. Future work will explore extensions to even more complex systems and other quantum light characteristics for practical applications.

quant-ph

Few-Photon SUPER: Quantum emitter inversion via two off-resonant photon modes

With the realization of controlled quantum systems, exploring excitations beyond the resonant case opens new possibilities. We investigate an extended Jaynes-Cummings model where two photon modes are coupled off-resonantly to a quantum emitter. This allows us to identify few-photon scattering mechanisms that lead to a full inversion of the emitter while transferring off-resonant photons from one mode to another. This behaviour connects to recent measurements of a two-level emitter scattering two off-resonant photons simultaneously. Furthermore, our results can be understood as quantized analogue of the recently developed off-resonant quantum control scheme known as Swing-UP of quantum EmitteR (SUPER). Our intuitive formalism gives a deeper insight into the interaction of a two-level emitter with off-resonant light modes with the prospect of novel photonic applications.

quant-ph

Emergence of second-order coherence in superfluorescence

We experimentally investigate the second-order quantum coherence function of a superradiant burst in a cascaded quantum system. We chirally (i.e. direction-dependently) couple roughly 900 cesium atoms to the forward propagating mode of an optical nanofiber. We then prepare the ensemble in the maximally inverted state, where the subsequent collective emission of a burst is known as superfluorescence. Here, we observe that second-order coherence emerges in the course of the decay. This is a clear feature of the underlying collective dynamics that is also at the origin of the superradiant burst itself. We furthermore study the dynamics of the second-order coherence function of the emission in dependence on the initial average dipole moment of the ensemble. In addition, by correlating the detection of early and late photon emission events, we obtain evidence for fundamental shot-to-shot fluctuations in the delay of the start of the burst emission. Our findings reveal that, despite the fundamentally different coupling Hamiltonian, superradiance in cascaded and symmetrically coupled systems feature a strikingly large number of similarities.

quant-ph

Predicting correlations in superradiant emission from a cascaded quantum system

In recent experiments, a novel type of cascaded quantum system has been realized using nanofiber-coupled cold atomic ensembles. This setup has enabled the study of superradiant decay of highly excited collective spin states of up to a thousand atoms, featuring unidirectional coupling mediated by the waveguide mode. The complexity arising from the large, multi-excited ensemble and the cascaded interactions between atoms makes conventional simulation methods unsuitable for predicting the correlations of superradiant emission beyond the first order. To address this challenge, we developed a new simulation technique based on the truncated Wigner approximation for spins. Our stochastic simulation tool can predict the second-order quantum coherence function, $g^{(2)}$, along with other correlators of the light field emitted by a strongly excited cascaded system of two-level emitters. This approach thus provides an effective and scalable method for analyzing cascaded quantum systems with large numbers of particles.

quant-ph

A low-loss and broadband all-fiber acousto-optic circulator

The introduction of low-loss optical fibers probably represents the single most important advance in the growth of our telecommunication system. To meet our needs for secure communications, it is likely that our classical network will soon be operating alongside what is known as a quantum network. The latter is very sensitive to loss and thus poses new constraints to the performance of current fiber components. In particular, recent quantum network prototypes underlined the absence of low-loss non-reciprocal fiber-based devices. Here, we present a solution to this issue by realizing low-loss (0.81 dB), broadband (at least 50 GHz bandwidth) and high-extinction (up to 27 dB) circulators, based on Mach-Zehnder interferometers including so-called fiber null-couplers. The latter are directional couplers, whose splitting-ratio can be controlled by launching acoustic waves along the coupling region. Fabricated from standard single-mode fibers and actuated electrically, these circulators can be made to fit any existing optical fiber networks and could turn out to be key for the transmission and processing of optically encoded quantum information.

physics.optics

Feedback-cooling the fundamental torsional mechanical mode of a tapered optical fiber to 30 mK

Tapered optical fibers (TOFs) are used in many areas of physics and optical technologies ranging from coupling light into nanophotonic components to optical sensing and amplification to interfacing quantum emitters. Here, we study the fundamental torsional mechanical mode of the nanofiber-waist of a TOF using laser light. We find that this oscillator features a quality factor of up to $10^7$ and a $Qf$ product of 1 THz. We damp the thermal motion from room temperature to 28(7) mK by means of active feedback. Our results might enable new types of fiber-based sensors and lay the foundation for a novel hybrid quantum optomechanical platform.

physics.optics

Observation of superradiant bursts in a cascaded quantum system

Dicke superradiance describes the collective radiative decay of a fully inverted ensemble of two-level atoms. We experimentally investigate this effect for a chiral, i.e.,~direction-dependent light--matter coupling. Despite a fundamentally different interaction Hamiltonian which has a reduced symmetry compared to the standard Dicke case, we do observe a superradiant burst emission. The burst occurs above a threshold number of atoms, and its peak power scales faster with the number of atoms than in the case of free-space Dicke superradiance. We measure the first-order coherence of the burst emission and experimentally distinguish two regimes, one dominated by the coherence induced during the excitation process and the other governed by vacuum fluctuations. Our results shed light on the collective radiative dynamics of cascaded quantum many-body systems, i.e., a system in which each quantum emitter is only driven by light radiated by emitters that are further upstream in the cascade. Our findings may turn out useful for generating multi-photon Fock states as a resource for quantum technologies.

quant-ph

Light-matter interaction at the transition between cavity and waveguide QED

Experiments based on cavity quantum electrodynamics (QED) are widely used to study the interaction of a light field with a discrete frequency spectrum and emitters. More recently, the field of waveguide QED has attracted interest due to the strong interaction between propagating photons and emitters that can be obtained in nanophotonic waveguides, where a continuum of frequency modes is allowed. Both cavity and waveguide QED share the common goal of harnessing and deepening the understanding of light-matter coupling. However, they often rely on very different experimental set-ups and theoretical descriptions. Here, we experimentally investigate the transition from cavity to waveguide QED with an ensemble of cold atoms that is coupled to a fiber-ring resonator, which contains a nanofiber section. By varying the length of the resonator from a few meters to several tens of meters, we tailor the spectral density of modes of the resonator while remaining in the strong coupling regime. We demonstrate that for progressively longer resonators, the paradigmatic Rabi oscillations of cavity QED gradually vanish, while non-Markovian features reminiscent of waveguide QED appear.

quant-ph

The Jaynes-Cummings model breaks down when the cavity significantly reduces the emitter's free-space emission rate

Strong coupling between a single resonator mode and a single quantum emitter is key to a plethora of experiments and applications in quantum science and technology and is commonly described by means of the Jaynes-Cummings model. Here, we show that the Jaynes-Cummings model only applies when the cavity does not significantly change the emitter's emission rate into free-space. Most notably, the predictions made by the Jaynes-Cummings model become increasingly wrong when approaching the ideal emitter-resonator systems with no free-space decay channels. We present a Hamiltonian that provides, within the validity range of the rotating wave approximation, a correct theoretical description that applies to all regimes. As minimizing the coupling to free-space modes is paramount for many cavity-based applications, a correct description of strong light-matter interaction is therefore crucial for developing and optimizing quantum protocols.

quant-ph