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Arno Rauschenbeutel

Publications and source records attributed to Arno Rauschenbeutel.

At least 55 records · Page 3Linked to original sources

Correlating photons using the collective nonlinear response of atoms weakly coupled to an optical mode

Photons in a nonlinear medium can repel or attract each other, resulting in a strongly correlated quantum many-body system. Typically, such strongly correlated states of light arise from the extreme nonlinearity granted by quantum emitters that are strongly coupled to a photonic mode. However, in these approaches, unavoidable dissipation, like photon loss, blurs nonlinear quantum effects. Here, we generate strongly correlated photon states using only weak coupling and taking advantage of dissipation. We launch light through an ensemble of non-interacting waveguide-coupled atoms, which induce correlations between simultaneously arriving photons through collectively enhanced nonlinear interactions. These correlated photons then experience less dissipation than the uncorrelated ones. Depending on the number of atoms, we experimentally observe strong photon bunching or anti-bunching of the transmitted light. This realization of a collectively enhanced nonlinearity may turn out transformational for quantum information science and opens new avenues for generating nonclassical light, covering frequencies from the microwave to the X-ray regime.

quant-ph↗

Heating in Nanophotonic Traps for Cold Atoms

Laser-cooled atoms that are trapped and optically interfaced with light in nanophotonic waveguides are a powerful platform for fundamental research in quantum optics as well as for applications in quantum communication and quantum information processing. Ever since the first realization of such a hybrid quantum nanophotonic, heating rates of the atomic motion observed in various experimental settings have typically been exceeding those in comparable free-space optical microtraps by about three orders of magnitude. This excessive heating is a roadblock for the implementation of certain protocols and devices. Its origin has so far remained elusive and, at the typical atom-surface separations of less than an optical wavelength encountered in nanophotonic traps, numerous effects may potentially contribute to atom heating. Here, we theoretically describe the effect of mechanical vibrations of waveguides on guided light fields and provide a general theory of particle-phonon interaction in nanophotonic traps. We test our theory by applying it to the case of laser-cooled cesium atoms in nanofiber-based two-color optical traps. We find excellent quantitative agreement between the predicted heating rates and experimentally measured values. Our theory predicts that, in this setting, the dominant heating process stems from the optomechanical coupling of the optically trapped atoms to the continuum of thermally occupied flexural mechanical modes of the waveguide structure. Beyond unraveling the long-standing riddle of excessive heating in nanofiber-based atom traps, we also study the dependence of the heating rates on the relevant system parameters. Our findings allow us to propose several strategies for minimizing the heating. Finally, our findings are also highly relevant for optomechanics experiments with dielectric nanoparticles that are optically trapped close to nanophotonic waveguides.

quant-ph↗

Wavelength-scale errors in optical localization due to spin-orbit coupling of light

The precise determination of the position of point-like emitters and scatterers using far-field optical imaging techniques is of utmost importance for a wide range of applications in medicine, biology, astronomy, and physics. Although the optical wavelength sets a fundamental limit to the image resolution of unknown objects, the position of an individual emitter can in principle be estimated from the image with arbitrary precision. This is used, e.g., in stars' position determination and in optical super-resolution microscopy. Furthermore, precise position determination is an experimental prerequisite for the manipulation and measurement of individual quantum systems, such as atoms, ions, and solid state-based quantum emitters. Here we demonstrate that spin-orbit coupling of light in the emission of elliptically polarized emitters can lead to systematic, wavelength-scale errors in the estimate of the emitter's position. Imaging a single trapped atom as well as a single sub-wavelength-diameter gold nanoparticle, we demonstrate a shift between the emitters' measured and actual positions which is comparable to the optical wavelength. Remarkably, for certain settings, the expected shift can become arbitrarily large. Beyond their relevance for optical imaging techniques, our findings apply to the localization of objects using any type of wave that carries orbital angular momentum relative to the emitter's position with a component orthogonal to the direction of observation.

quant-ph↗

Observation of Multimode Strong Coupling of Cold Atoms to a 30-m Long Optical Resonator

We report on the observation of multimode strong coupling of a small ensemble of atoms interacting with the field of a 30-m long fiber resonator containing a nanofiber section. The collective light--matter coupling strength exceeds the free spectral range and the atoms couple to consecutive longitudinal resonator modes. The measured transmission spectra of the coupled atom-resonator system provide evidence of this regime, realized with a few hundred atoms with an intrinsic single-atom cooperativity of 0.26. These results are the starting point for studies in a new setting of light-matter interaction, with strong quantum non-linearities and a new type of dynamics.

quant-ph↗

Optical-nanofiber-based interface for single molecules

Optical interfaces for quantum emitters are a prerequisite for implementing quantum networks. Here, we couple single molecules to the guided modes of an optical nanofiber. The molecules are embedded within a crystal that provides photostability and, due to the inhomogeneous broadening, a means to spectrally address single molecules. Single molecules are excited and detected solely via the nanofiber interface without the requirement of additional optical access. In this way, we realize a fully fiber-integrated system that is scalable and may become a versatile constituent for quantum hybrid systems.

physics.optics↗

Nanofiber-mediated chiral radiative coupling between two atoms

We investigate the radiative coupling between two two-level atoms with arbitrarily polarized dipoles in the vicinity of a nanofiber. We present a systematic derivation for the master equation, the single- and cross-atom decay coefficients, and the dipole-dipole interaction coefficients for the atoms interacting with the vacuum of the field in the guided and radiation modes of the nanofiber. We study numerically the case where the atomic dipoles are circularly polarized. In this case, the rate of emission depends on the propagation direction, that is, the radiative interaction between the atoms is chiral. We examine the time evolution of the atoms for different initial states. We calculate the fluxes and mean numbers of photons spontaneously emitted into guided modes in the positive and negative directions of the fiber axis. We show that the chiral radiative coupling modifies the collective emission of the atoms. We observe that the modifications strongly depend on the initial state of the atomic system, the radiative transfer direction, the distance between the atoms, and the distance from the atoms to the fiber surface.

quant-ph↗

Fiber ring resonator with nanofiber section for chiral cavity quantum electrodynamics and multimode strong coupling

We experimentally realize an optical fiber ring resonator that includes a tapered section with subwavelength-diameter waist. In this section, the guided light exhibits a significant evanescent field which allows for efficient interfacing with optical emitters. A commercial tunable fiber beam splitter provides simple and robust coupling to the resonator. Key parameters of the resonator such as its out-coupling rate, free spectral range, and birefringence can be adjusted. Thanks to the low taper- and coupling-losses, the resonator exhibits an unloaded finesse of F=75+/-1, sufficient for reaching the regime of strong coupling for emitters placed in the evanescent field. The system is ideally suited for trapping ensembles of laser-cooled atoms along the nanofiber section. Based on measured parameters, we estimate that the system can serve as a platform for optical multimode strong coupling experiments. Finally, we discuss the possibilities of using the resonator for applications based on chiral quantum optics.

quant-ph↗

Chiral quantum optics with V-level atoms and coherent quantum feedback

We study the dissipative dynamics of an atom in a V-level configuration driven by lasers and coupled to a semi-infinite waveguide. The coupling to the waveguide is chiral, in that each transition interacts only with the modes propagating in a given direction, and this direction is opposite for the two transitions. The waveguide is terminated by a mirror which coherently feeds the photon stream emitted by one transition back to the atom. First, we are interested in the dynamics of the atom in the Markovian limit where the time-delay in the feedback is negligible. Specifically, we study the conditions under which the atom evolves towards a pure "dark" stationary state, where the photons emitted by both transitions interfere destructively thanks to the coherent feedback, and the overall emission vanishes. This is a single-atom analog of the quantum dimer, where a pair of laser-driven two-level atoms is coupled to a unidirectional waveguide and dissipates towards a pure entangled dark state. Our setup should be feasible with current state-of-the-art experiments. Second, we extend our study to non-Markovian regimes and investigate the effect of the feedback retardation on the steady-state.

quant-ph↗

Quantum optical circulator controlled by a single chirally coupled atom

We demonstrate a fiber-integrated quantum optical circulator that is operated by a single atom and that relies on the chiral interaction between emitters and transversally confined light. Like its counterparts in classical optics, our circulator exhibits an inherent asymmetry between light propagation in the forward and the backward direction. However, rather than a magnetic field or a temporal modulation, it is the internal quantum state of the atom that controls the operation direction of the circulator. This working principle is compatible with preparing the circulator in a coherent superposition of its operational states. Such a quantum circulator may thus become a key element for routing and processing quantum information in scalable integrated optical circuits. Moreover, it features a strongly nonlinear response at the single-photon level, thereby enabling, e.g., photon number-dependent routing and novel quantum simulation protocols.

quant-ph↗

Fictitious magnetic field gradients in optical microtraps as an experimental tool for interrogating and manipulating cold atoms

Optical microtraps provide a strong spatial confinement for laser-cooled atoms. They can, e.g., be realized with strongly focused trapping light beams or the optical near fields of nano-scale waveguides and photonic nanostructures. Atoms in such traps often experience strongly spatially varying AC Stark shifts which are proportional to the magnetic quantum number of the respective energy level. These inhomogeneous fictitious magnetic fields can cause a displacement of the trapping potential that depends on the Zeeman state. Hitherto, this effect was mainly perceived as detrimental. However, it also provides a means to probe and to manipulate the motional state of the atoms in the trap by driving transitions between Zeeman states. Furthermore, by applying additional real or fictitious magnetic fields, the state-dependence of the trapping potential can be controlled. Here, using laser-cooled atoms that are confined in a nanofiber-based optical dipole trap, we employ this control in order to tune the microwave coupling of motional quantum states. We record corresponding microwave spectra which allow us to infer the trap parameters as well as the temperature of the atoms. Finally, we reduce the mean number of motional quanta in one spatial dimension to $\langle n\rangle=0.3 \pm 0.1$ by microwave sideband cooling. Our work shows that the inherent fictitious magnetic fields in optical microtraps expand the experimental toolbox for interrogating and manipulating cold atoms.

physics.atom-ph↗

Chiral Quantum Optics

At the most fundamental level, the interaction between light and matter is manifested by the emission and absorption of single photons by single quantum emitters. Controlling light--matter interaction is the basis for diverse applications ranging from light technology to quantum--information processing. Many of these applications are nowadays based on photonic nanostructures strongly benefitting from their scalability and integrability. The confinement of light in such nanostructures imposes an inherent link between the local polarization and propagation direction of light. This leads to {\em chiral light--matter interaction}, i.e., the emission and absorption of photons depend on the propagation direction and local polarization of light as well as the polarization of the emitter transition. The burgeoning research field of {\em chiral quantum optics} offers fundamentally new functionalities and applications both for single emitters and ensembles thereof. For instance, a chiral light--matter interface enables the realization of integrated non--reciprocal single--photon devices and deterministic spin--photon interfaces. Moreover, engineering directional photonic reservoirs opens new avenues for constructing complex quantum circuits and networks, which may be applied to simulate a new class of quantum many--body systems.

quant-ph↗

Propagation of nanofiber-guided light through an array of atoms

We study the propagation of nanofiber-guided light through an array of atomic cesium, taking into account the transitions between the hyperfine levels $6S_{1/2}F=4$ and $6P_{3/2}F'=5$ of the $D_2$ line. We derive the coupled-mode propagation equation, the input-output equation, the scattering matrix, the transfer matrix, and the reflection and transmission coefficients for the guided field in the linear, quasistationary, weak-excitation regime. We show that, when the initial distribution of populations of atomic ground-state sublevels is flat, the quasilinear polarizations along the principal axes $x$ and $y$, which are parallel and perpendicular, respectively, to the radial direction of the atomic position, are not coupled to each other in the linear coherent scattering process. When the guided probe field is quasilinearly polarized along the major principal axis $x$, forward and backward scattering have different characteristics. We find that, when the array period is far from the Bragg resonance, the backward scattering is weak. Under the Bragg resonance, most of the guided probe light can be reflected back in a broad region of field detunings even though there is an irreversible decay channel into radiation modes. When the atom number is large enough, two different band gaps may be formed, whose properties depend on the polarization of the guided probe field.

quant-ph↗

Chiral nanophotonic waveguide interface based on spin-orbit coupling of light

Controlling the flow of light by means of nanophotonic waveguides has the potential of transforming integrated information processing much in the same way that conventional glass fibers have revolutionized global communication. Owing to the strong transverse confinement of the light, such waveguides give rise to a coupling between the internal spin of the guided photons and their orbital angular momentum. Here, we employ this spin-orbit coupling of light to break the mirror symmetry of the scattering of light by a single gold nanoparticle on the surface of a nanophotonic waveguide. We thereby realize a chiral waveguide coupler in which the handedness of the incident light determines the direction of propagation in the waveguide. Using this effect, we control the directionality of the scattering process and direct up to 94% of the incoupled light into a given direction. This enables novel ways for controlling and manipulating light in optical waveguides and nanophotonic structures as well as for the design of integrated optical sensors.

quant-ph↗

Nonlinear pi phase shift for single fiber-guided photons interacting with a single atom

Realizing a strong interaction between individual optical photons is an important objective of research in quantum science and technology. Since photons do not interact directly, this goal requires, e.g., an optical medium in which the light experiences a phase shift that depends nonlinearly on the photon number. Once the additional phase shift for two photons reaches pi, such an ultra-strong nonlinearity could even enable the direct implementation of high-fidelity quantum logic operations. However, the nonlinear response of standard optical media is many orders of magnitude too weak for this task. Here, we demonstrate the realization of an optical fiber-based nonlinearity that leads to an additional two-photon phase shift close to the ideal value of pi. Our scheme employs a whispering-gallery-mode resonator, interfaced by an optical nanofiber, where the presence of a single rubidium atom in the resonator results in a strongly nonlinear response. We experimentally show that this results in entanglement of initially independent incident photons. The demonstration of this ultra-strong nonlinearity in a fiber-integrated system is a decisive step towards scalable quantum logics with optical photons.

quant-ph↗

Experimental stress-strain analysis of tapered silica optical fibers with nanofiber waist

We experimentally determine tensile force-elongation diagrams of tapered optical fibers with a nanofiber waist. The tapered optical fibers are produced from standard silica optical fibers using a heat and pull process. Both, the force-elongation data and scanning electron microscope images of the rupture points indicate a brittle material. Despite the small waist radii of only a few hundred nanometers, our experimental data can be fully explained by a nonlinear stress-strain model that relies on material properties of macroscopic silica optical fibers. This is an important asset when it comes to designing miniaturized optical elements as one can rely on the well-founded material characteristics of standard optical fibers. Based on this understanding, we demonstrate a simple and non-destructive technique that allows us to determine the waist radius of the tapered optical fiber. We find excellent agreement with independent scanning electron microscope measurements of the waist radius.

physics.class-ph↗

Biprism Electron Interferometry with a Single Atom Tip Source

Experiments with electron or ion matter waves require a coherent, monochromatic and long-term stable source with high brightness. These requirements are best fulfilled by single atom tip (SAT) field emitters. The performance of an iridium covered W(111) SAT is demonstrated and analyzed for electrons in a biprism interferometer. Furthermore we characterize the emission of the SAT in a separate field electron and field ion microscope and compare it with other emitter types. A new method is presented to fabricate the electrostatic charged biprism wire that separates and combines the matter wave. In contrast to other biprism interferometers the source and the biprism size are well defined within a few nanometers. The setup has direct applications in ion interferometry and Aharonov-Bohm physics.

physics.optics↗

Tapered fiber coupling of single photons emitted by a deterministically positioned single nitrogen vacancy center

A diamond nano-crystal hosting a single nitrogen vacancy (NV) center is optically selected with a confocal scanning microscope and positioned deterministically onto the subwavelength-diameter waist of a tapered optical fiber (TOF) with the help of an atomic force microscope. Based on this nano-manipulation technique we experimentally demonstrate the evanescent coupling of single fluorescence photons emitted by a single NV-center to the guided mode of the TOF. By comparing photon count rates of the fiber-guided and the free-space modes and with the help of numerical FDTD simulations we determine a lower and upper bound for the coupling efficiency of (9.5+/-0.6)% and (10.4+/-0.7)%, respectively. Our results are a promising starting point for future integration of single photon sources into photonic quantum networks and applications in quantum information science.

quant-ph↗

Negative azimuthal force of a nanofiber-guided light on a particle

We calculate the force of a quasicircularly polarized guided light field of a nanofiber on a dielectric spherical particle. We show that the orbital parts of the axial and azimuthal components of the Poynting vector are always positive while the spin parts can be either positive or negative. We find that, for appropriate values of the size parameter of the particle, the azimuthal component of the force is directed oppositely to the circulation direction of the energy flow around the nanofiber. The occurrence of such a negative azimuthal force indicates that the particle undergoes a negative torque.

physics.optics↗