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Arnold J. Sierk

Publications and source records attributed to Arnold J. Sierk.

At least 19 recordsLinked to original sources

Hauser-Feshbach fission fragment de-excitation with calculated macroscopic-microscopic mass yields

The Hauser-Feshbach statistical model is applied to the de-excitation of primary fission fragments using input mass yields calculated with macroscopic-microscopic models of the potential energy surface. We test the sensitivity of the prompt fission observables to the input mass yields for two important reactions, $^{235}$U$(n_\mathrm{th},f)$ and $^{239}$Pu$(n_\mathrm{th},f)$, for which good experimental data exist. General traits of the mass yields, such as the location of the peaks and their widths, can impact both the prompt neutron and $γ$-ray multiplicities, as well as their spectra. Specifically, we use several mass yields to determine a linear correlation between the calculated prompt neutron multiplicity $\barν$ and the average heavy-fragment mass $\langle A_h\rangle$ of the input mass yields $\partial\barν/\partial\langle A_h\rangle = \pm 0.1\,n/f/\mathrm{u}$. The mass peak width influences the correlation between the total kinetic energy of the fission fragments and the total number of prompt neutrons emitted $\barν_T(\mathrm{TKE})$. Typical biases on prompt particle observables from using calculated mass yields instead of experimental ones are: $δ\barν = 4\%$ for the average prompt neutron multiplicity, $δ\bar{M}_γ= 1\%$ for the average prompt $γ$-ray multiplicity, $δ\barε_n^\mathrm{LAB} = 1\%$ for the average outgoing neutron energy, $δ\barε_γ= 1\%$ for the average $γ$-ray energy, and $δ\langle\mathrm{TKE}\rangle = 0.4\%$ for the average total kinetic energy of the fission fragments.

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Production of Energetic Light Fragments in CEM, LAQGSM, and MCNP6

We extend the cascade-exciton model (CEM), and the Los Alamos version of the quark-gluon string model (LAQGSM), event generators of the Monte-Carlo N-particle transport code version 6 (MCNP6), to describe production of energetic light fragments (LF) heavier than 4He from various nuclear reactions induced by particles and nuclei at energies up to about 1 TeV/nucleon. In these models, energetic LF can be produced via Fermi break-up, preequilibrium emission, and coalescence of cascade particles. Initially, we study several variations of the Fermi break-up model and choose the best option for these models. Then, we extend the modified exciton model (MEM) used by these codes to account for a possibility of multiple emission of up to 66 types of particles and LF (up to 28Mg) at the preequilibrium stage of reactions. Then, we expand the coalescence model to allow coalescence of LF from nucleons emitted at the intranuclear cascade stage of reactions and from lighter clusters, up to fragments with mass numbers A < 8, in the case of CEM, and A < 13, in the case of LAQGSM. Next, we modify MCNP6 to allow calculating and outputting spectra of LF and heavier products with arbitrary mass and charge numbers. The improved version of CEM is implemented into MCNP6. Finally, we test the improved versions of CEM, LAQGSM, and MCNP6 on a variety of measured nuclear reactions. The modified codes give an improved description of energetic LF from particle- and nucleus-induced reactions; showing a good agreement with a variety of available experimental data. They have an improved predictive power compared to the previous versions and can be used as reliable tools in simulating applications involving such types of reactions.

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Energetic Light Fragment Production Capability in MCNP6

The goal of this research is to enable MCNP6 to produce high-energy light fragments. These energetic light fragments may be emitted by our models through three processes: Fermi breakup, preequilibrium, and coalescence. We explore the emission of light fragments through each of these mechanisms and demonstrate an improved agreement with experimental data achieved by extending precompound models to include emission of fragments heavier than $^4$He.

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Comparison of Expanded Preequilibrium CEM Model with CEM03.03 and Experimental Data, FY2013

Emission of light fragments (LF) from nuclear reactions is an open question. Different reaction mechanisms contribute to their production; the relative roles of each, and how they change with incident energy, mass number of the target, and the type and emission energy of the fragments is not completely understood. None of the available models are able to accurately predict emission of LF from arbitrary reactions. However, the ability to describe production of LF (especially at energies $\gtrsim 30$ MeV) from many reactions is important for different applications, such as cosmic-ray-induced Single Event Upsets (SEUs), radiation protection, and cancer therapy with proton and heavy-ion beams, to name just a few. The Cascade-Exciton Model (CEM) version 03.03 and the Los Alamos version of the Quark-Gluon String Model (LAQGSM) version 03.03 event generators in Monte Carlo N-Particle Transport Code version 6 (MCNP6) describe quite well the spectra of fragments with sizes up to $^{4}$He across a broad range of target masses and incident energies (up to $\sim 5$ GeV for CEM and up to $\sim 1$ TeV/A for LAQGSM). However, they do not predict the high-energy tails of LF spectra heavier than $^4$He well. Most LF with energies above several tens of MeV are emitted during the precompound stage of a reaction. The current versions of the CEM and LAQGSM event generators do not account for precompound emission of LF larger than $^{4}$He. The aim of our work is to extend the precompound model in them to include such processes, leading to an increase of predictive power of LF-production in MCNP6. Extending our models to include emission of fragments heavier than $^4$He at the precompound stage has already provided preliminary results that have much better agreement with experimental data.

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Production of Energetic Light Fragments in Spallation Reactions

Different reaction mechanisms contribute to the production of light fragments (LF) from nuclear reactions. Available models cannot accurately predict emission of LF from arbitrary reactions. However, the emission of LF is important for many applications, such as cosmic-ray-induced single event upsets, radiation protection, and cancer therapy with proton and heavy-ion beams, to name just a few. The cascade-exciton model (CEM) and the Los Alamos version of the quark-gluon string model (LAQGSM), as implemented in the CEM03.03 and LAQGSM03.03 event generators used in the Los Alamos transport code MCNP6, describe quite well the spectra of fragments with sizes up to 4He across a broad range of target masses and incident energies. However, they do not predict high-energy tails for LF heavier than 4He. The standard versions of CEM and LAQGSM do not account for preequilibrium emission of LF larger than 4He. The aim of our work is to extend the preequilibrium model to include such processes. We do this by including the emission of fragments heavier than 4He at the preequilibrium stage, and using an improved version of the Fermi Break-up model, providing improved agreement with various experimental data.

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MCNP6 Fission Cross Section Calculations at Intermediate and High Energies

MCNP6 has been Validated and Verified (V&V) against intermediate- and high-energy fission cross-section experimental data. An error in the calculation of fission cross sections of 181Ta and a few nearby target nuclei by the CEM03.03 event generator in MCNP6 and a "bug: in the calculation of fission cross sections with the GENXS option of MCNP6 while using the LAQGSM03.03 event generator were detected during our V&V work. After fixing both problems, we find that MCNP6 using CEM03.03 and LAQGSM03.03 calculates fission cross sections in good agreement with available experimental data for reactions induced by nucleons, pions, and photons on both subactinide and actinide nuclei at incident energies from several tens of MeV to about 1 TeV.

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Preequilibrium Emission of Light Fragments in Spallation Reactions

The ability to describe production of light fragments (LF) is important for many applications, such as cosmic-ray-induced single event upsets (SEUs), radiation protection, and cancer therapy with proton and heavy-ion beams. The Cascade-Exciton Model (CEM) and the Los Alamos version of the Quark-Gluon String Model (LAQGSM) event generators in the LANL transport code MCNP6, describe quite well the spectra of fragments with sizes up to 4He across a broad range of target masses and incident energies (up to ~ 5 GeV for CEM and up to ~ 1 TeV/A for LAQGSM). However, they do not predict the high-energy tails of LF spectra heavier than 4He well. Most LF with energies above several tens of MeV are emitted during the precompound stage of a reaction. The current versions of our event generators do not account for precompound emission of LF larger than 4He. The aim of our work is to generalize the precompound model to include such processes, leading to increased predictive power of LF production. Extending the model in this way provides preliminary results that have much better agreement with experimental data.

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MCNP6 Study of Fragmentation Products from 112Sn + 112Sn and 124Sn + 124Sn at 1 GeV/nucleon

Isotope production cross sections from 112Sn + 112Sn and 124Sn + 124Sn reactions at 1 GeV/nucleon, which were measured recently at GSI using the heavy-ion accelerator SIS18 and the Fragment Separator (FRS), have been analyzed with the latest Los Alamos Monte-Carlo transport code MCNP6 using the LAQGSM03.03 event generator. MCNP6 reproduces reasonably well all the measured cross sections. Comparison of the MCNP6 results with the measured data and with calculations by a modification of the Los Alamos version of the Quark-Gluon String Model allowing for multifragmentation processes in the framework of the Statistical Multifragmentation Model (SMM) by Botvina and coauthors, as realized in the code LAQGSM03.S1, does not suggest unambiguous evidence of a multifragmentation signature.

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The contrasting fission potential-energy structure of actinides and mercury isotopes

Fission-fragment mass distributions are asymmetric in fission of typical actinide nuclei for nucleon number $A$ in the range $228 \lnsim A \lnsim 258$ and proton number $Z$ in the range $90\lnsim Z \lnsim 100$. For somewhat lighter systems it has been observed that fission mass distributions are usually symmetric. However, a recent experiment showed that fission of $^{180}$Hg following electron capture on $^{180}$Tl is asymmetric. We calculate potential-energy surfaces for a typical actinide nucleus and for 12 even isotopes in the range $^{178}$Hg--$^{200}$Hg, to investigate the similarities and differences of actinide compared to mercury potential surfaces and to what extent fission-fragment properties, in particular shell structure, relate to the structure of the static potential-energy surfaces. Potential-energy surfaces are calculated in the macroscopic-microscopic approach as functions of fiveshape coordinates for more than five million shapes. The structure of the surfaces are investigated by use of an immersion technique. We determine properties of minima, saddle points, valleys, and ridges between valleys in the 5D shape-coordinate space. Along the mercury isotope chain the barrier heights and the ridge heights and persistence with elongation vary significantly and show no obvious connection to possible fragment shell structure, in contrast to the actinide region, where there is a deep asymmetric valley extending from the saddle point to scission. The mechanism of asymmetric fission must be very different in the lighter proton-rich mercury isotopes compared to the actinide region and is apparently unrelated to fragment shell structure. Isotopes lighter than $^{192}$Hg have the saddle point blocked from a deep symmetric valley by a significant ridge. The ridge vanishes for the heavier Hg isotopes, for which we would expect a qualitatively different asymmetry of the fragments.

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Five-Dimensional Fission-Barrier Calulations from Se-70 to Cf-252

We present fission-barrier-height calculations for nuclei throught the Periodic Table based on a realistic macroscopic-microscopic model. Compared to other calculations: (1) we use a deformation space of sufficiently high dimension, sampled densely enough to describe the relevant topography of the fission potential, (2) we unambiguously find the physically relevant saddle points in this space, and (3) we formulate our model so that we obtain continuity of the potential energy at the division point between a single system and separated fission fragments or colliding nuclei, allowing us to (4) describe both fission-barrier heights and ground-state masses throughout the Periodic Table.

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Merging the CEM2K and LAQGSM Codes with GEM2 to Describe Fission and Light-fragment Production

We present the current status of the improved Cascade-Exciton Model (CEM) code CEM2k and of the Los Alamos version of the Quark-Gluon String Model code LAQGSM. To describe fission and light-fragment (heavier than He4) production, both CEM2k and LAQGSM have been merged with the GEM2 code of Furihata. We present some results on proton- and deuteron-induced spallation, fission, and fragmentation reactions predicted by these extended versions of CEM2k and LAQGSM. We show that merging CEM2k and LAQGSM with GEM2 allows us to describe many fission and fragmentation reactions in addition to the spallation reactions which are already relatively well described. Nevertheless, the standard version of GEM2 does not provide a completely satisfactory description of complex particle spectra, heavy-fragment emission, and spallation yields, and is not yet a reliable tool for applications. We conclude that we may choose to use a model similar to the GEM2 approach in our codes, but it must be significantly extended and further improved. We observe that it is not sufficient to analyze only A and Z distributions of the product yields when evaluating this type of model, as is often done in the literature; instead it is important to study all the separate isotopic yields as well as the spectra of light particles and fragments.

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Event Generator Benchmarking for Proton Radiography Applications

We have benchmarked the QGSM code and event generators of the MARS and LAHET3 codes as potential candidates for high-energy programs to be used in simulations for the Proton Radiography (PRad) Project. We have compiled from the literature experimental data on spectra of particles emitted from proton-induced reactions at incident energies from 30 GeV to 70 GeV on different nuclei and have performed calculations for all reactions for which we found data with these three codes without any modifications and using only default parameters and standard inputs. Our results (514 plots) show that all three codes describe reasonably most of the studied reactions, though all of them should be further improved before becoming reliable tools for PRad. We present here our conclusions concerning the relative roles of different reaction mechanisms in the production of specific secondary particles. We comment on the strengths and weaknesses of QGSM, MARS, and LAHET3 and suggest further improvements to these codes and to other models.

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Experimental and Theoretical Study of the Residual Product Nuclide Yields in 100-2600 MeV Proton-Irradiated Thin Targets

The work is aimed at experimental determining and computer simulating the independent and cumulative yields of residual product nuclei in the target and structure materials of the transmutation facilities driven by high-current accelerators. The ITEP U-10 accelerator was used in 48 experiments to obtain more than 4000 values of the yields of radioactive residual product nuclei in 0.1-2.6 GeV proton-irradiated thin 182,183,184,186-W, nat-W, 56-Fe, 58-Ni, 93-Nb, 232-Th, nat-U, 99-Tc, 59-Co 63,65-Cu, nat-Hg, 208-Pb, and 27-Al targets. The results of verifying the LAHET, CEM95, CEM2k, CASCADE, CASCADE/INPE, YIELDX, HETC, INUCL, and other simulation codes are presented.

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Threshold Reaction Rates and Energy Spectra of Neutrons in the 0.8-1.6 GeV Proton-Irradiated W, Na Targets

Considering the prospects of using the W-Na target assemblies in ADS facilities, the experiments were made to study the nuclear-physics characteristics of W and Na, and the composite structures thereof in their interactions with 0.8-GeV and 1.6-GeV protons. The neutron and proton-induced reaction rates were measured inside, and on the surface of, a cylinder-shaped heterogeneous W-Na assembly together with the double-differential spectra of secondary neutrons emitted from different-depth W and Na discs. The measurement results were simulated by the LAHET, CEM2k, and KASKAD-S codes in terms of the latest versions of nuclear databases.

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Recent Developments of the Cascade-Exciton Model of Nuclear Reactions

Recent developments of the Cascade-Exciton Model (CEM) of nuclear reactions are described. The improved cascade-exciton model as implemented in the code CEM97 differs from the CEM95 version by incorporating new approximations for the elementary cross sections used in the cascade, using more precise values for nuclear masses and pairing energies, using corrected systematics for the level-density parameters, and several other refinements. We have improved algorithms used in many subroutines, decreasing the computing time by up to a factor of 6 for heavy targets. We describe a number of further improvements and changes to CEM97, motivated by new data on isotope production measured at GSI. This leads us to CEM2k, a new version of the CEM code. CEM2k has a longer cascade stage, less preequilibrium emission, and evaporation from more highly excited compound nuclei compared to earlier versions. CEM2k also has other improvements and allows us to better model neutron, radionuclide, and gas production in ATW spallation targets. The increased accuracy and predictive power of the code CEM2k are shown by several examples. Further necessary work is outlined.

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Benchmarking Ten Codes Against the Recent GSI Measurements of the Nuclide Yields from 208Pb, 197Au, and 238U + p Reactions at 1 GeV/nucleon

A qualitative and quantitative comparison of the recent GSI measurements of the nuclide yields from 208Pb and 238U at 1 GeV/nucleon and 197Au at 800 MeV/nucleon interactions with protons with the codes LAHET (with both ISABEL and Bertini options), CEM95, CEM97, CEM2k, CASCADE, CASCADE/INPE, YIELDX, HETC, and INUCL is presented. The predictive power of these codes is reasonable for nuclides in the near spallation region but is worse for deep spallation and much worse in the fission region. None of these codes agree well with the data in the whole mass region of product nuclides and all must be improved to become reliable tools for accelerator-driven applications.

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Complex Particle and Light Fragment Emission in the Cascade-Exciton Model of Nuclear Reactions

A brief description of our improvements and refinements that led from the CEM95 version of the Cascade-Exciton Model (CEM) code to CEM97 and to CEM2k is given. The increased accuracy and predictive power of the code CEM2k are shown by several examples. To describe fission and light-fragment (heavier than 4He) production, the CEM2k code has been merged with the GEM2 code of Furihata. We present some results on proton-induced fragmentation and fission reactions predicted by this extended version of CEM2k. We show that merging CEM2k with GEM2 allows us to describe many fission and fragmentation reactions in addition to the spallation reactions which are already relatively well described. We have initiated another approach to describe fission, complex particles and fragment emission by developing further our CEM2k code addressing specifically these problems. In this effort, we have developed our own universal approximation for inverse cross sections, new routines to calculate Coulomb barriers and widths of emitted particles and to simulate their kinetic energy using arbitrary approximations for the inverse cross sections. To describe fission-fragment production, we have incorporated into CEM2k a thermodynamical model of fission by Stepanov. This extended version of CEM2k allows us to describe much better complex particle emission and many fission fragments, but it is still incomplete and needs further work.

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CEM2k - Recent Developments in CEM

Recent developments of the Cascade-Exciton Model (CEM) of nuclear reactions are briefly described. These changes are motivated by new data on isotope production measured recently in "reverse kinematics" at GSI for interactions of 208-Pb and 238-U at 1 GeV/nucleon and 197-Au at 800 MeV/nucleon with liquid 1-H. This study leads us to CEM2k, which is a new version of the CEM code that is still under development. The increased accuracy and predictive power of the code CEM2k are shown by several examples. Further necessary work is outlined.

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