arXiv subjects

Arnoud S. Everhardt

Publications and source records attributed to Arnoud S. Everhardt.

3 recordsLinked to original sources

arXiv2022

Dynamic Tilting of Ferroelectric Domain Walls via Optically Induced Electronic Screening

Optical excitation perturbs the balance of phenomena selecting the tilt orientation of domain walls within ferroelectric thin films. The high carrier density induced in a low-strain BaTiO3 thin film by an above-bandgap ultrafast optical pulse changes the tilt angle that 90° a/c domain walls form with respect to the substrate-film interface. The dynamics of the changes are apparent in time-resolved synchrotron x-ray scattering studies of the domain diffuse scattering. Tilting occurs at 298 K, a temperature at which the a/b and a/c domain phases coexist but is absent at 343 K in the better ordered single-phase a/c regime. Phase coexistence at 298 K leads to increased domain-wall charge density, and thus a larger screening effect than in the single-phase regime. The screening mechanism points to new directions for the manipulation of nanoscale ferroelectricity.

cond-mat.mtrl-sci↗

arXiv2021

Unified Framework for Charge-Spin Interconversion in Spin-Orbit Materials

Materials with spin-orbit coupling are of great interest for various spintronics applications due to the efficient electrical generation and detection of spin-polarized electrons. Over the past decade, many materials have been studied, including topological insulators, transition metals, Kondo insulators, semimetals, semiconductors, and oxides; however, there is no unifying physical framework for understanding the physics and therefore designing a material system and devices with the desired properties. We present a model that binds together the experimental data observed on the wide variety of materials in a unified manner. We show that in a material with a given spin-momentum locking, the density of states plays a crucial role in determining the charge-spin interconversion efficiency, and a simple inverse relationship can be obtained. Remarkably, experimental data obtained over the last decade on many different materials closely follow such an inverse relationship. We further deduce two figure-of-merits of great current interest: the spin-orbit torque (SOT) efficiency (for the direct effect) and the inverse Rashba-Edelstein effect length (for the inverse effect), which statistically show good agreement with the existing experimental data on wide varieties of materials. Especially, we identify a scaling law for the SOT efficiency with respect to the carrier concentration in the sample, which agrees with existing data. Such an agreement is intriguing since our transport model includes only Fermi surface contributions and fundamentally different from the conventional views of the SOT efficiency that includes contributions from all the occupied states.

cond-mat.mes-hall↗

arXiv2019

Periodicity doubling cascades: direct observation in ferroelastic materials

Very sensitive responses to external forces are found near phase transitions. However, phase transition dynamics and pre-equilibrium phenomena are difficult to detect and control. We have directly observed that the equilibrium domain structure following a phase transition in BaTiO3, a ferroelectric and ferroelastic material, is attained by halving of the domain periodicity, sequentially and multiple times. The process is reversible, displaying periodicity doubling as temperature is increased. This observation is backed theoretically and can explain the fingerprints of domain period multiplicity observed in other systems, strongly suggesting this as a general model for pattern formation during phase transitions in ferroelastic materials.

cond-mat.mtrl-sci↗