arXiv subjects

Artem G. Volosniev

Publications and source records attributed to Artem G. Volosniev.

At least 19 recordsLinked to original sources

arXiv2026

Second-order Raman and anharmonic lattice dynamics in lead-halide perovskites

We explore the microscopic origin of THz-driven lattice dynamics in methylammonium lead bromide CH$_3$NH$_3$PbBr$_3$ using two-dimensional THz Kerr-effect spectroscopy. The analysis of the experiment enables discrimination between competing nonlinear excitation mechanisms and reveals that the dominant pathway is phonon-mediated rather than purely photonic. In particular, we argue that the commonly observed 1.15~THz Raman-active $A_g$ mode is not excited directly by the THz electric field. Instead, it emerges through cubic anharmonic coupling to an infrared-active phonon at 0.68~THz. Furthermore, a satellite feature at 1.36~THz is identified as a two-phonon Raman response of the same infrared-active mode. The observation of strong quadratic coupling involving the infrared-active phonon suggests an unconventional form of electron-phonon dressing present in lead-halide perovskites.

cond-mat.mtrl-sci↗

arXiv2026

Scissors modes in generalized Gross-Pitaevskii equations

We investigate scissors modes in nonlinear systems with arbitrary power-law dependence of the nonlinear term. Through analytical derivation, we establish a general expression demonstrating that, in the Thomas-Fermi regime, the frequency of the scissors mode is independent of the specific form of the nonlinearity. We conclude that the scissors mode is a shear mode that does not probe the compressibility of the system, which depends on nonlinearity. To validate our findings, we perform numerical simulations of experimentally relevant Lee-Huang-Yang (LHY) systems. Our results illustrate the transition of the scissors mode frequency from the non-interacting to the strongly interacting (Thomas-Fermi) regime. Finally, we demonstrate that the scissors mode frequency remains clearly identifiable even under strong quenches, which should facilitate the experimental observation of our findings.

cond-mat.quant-gas↗

arXiv2026

Generalized Gross-Pitaevskii Equation for 2D Bosons with Attractive Interactions

We introduce a generalized Gross-Pitaevskii equation that provides a nonlinear framework for studying two-dimensional (2D) attractive Bose systems. Its defining feature is the logarithmic density dependence of the coupling constant, which breaks the scale invariance inherent in the standard mean-field equations. This framework allows straightforward calculations of the system properties arising from the quantum anomaly. As a first illustration, we study universal bound states in free space, commonly referred to as quantum droplets. Then, we analyze breathing modes and quench dynamics in trapped systems, paving the way for a systematic exploration of non-equilibrium phenomena in 2D attractive Bose systems. Finally, we predict the existence of universal excited states, including vortex configurations, which may be more accessible to experimental investigation than the ground state. Our results provide a robust theoretical foundation for studying both static and dynamical properties of finite systems, and offer guidance for the design of future experiments.

cond-mat.quant-gas↗

arXiv2026

Phenomenological model of decaying Bose polarons

Cold atom experiments show that a mobile impurity particle immersed in a Bose-Einstein condensate forms a well-defined quasiparticle (Bose polaron) for weak to moderate impurity-boson interaction strengths, whereas a significant line broadening is consistently observed for strong interactions. Motivated by this, we introduce a phenomenological theory based on the assumption that the most relevant states are characterized by the impurity correlated with at most one boson, since they have the largest overlap with the uncorrelated states to which the most common experimental probes couple. These experimentally relevant states can however decay to lower energy states characterised by correlations involving multiple bosons, and we model this using a minimal variational wave function combined with a complex impurity-boson interaction strength. We first motivate this approach by comparing to a more elaborate theory that includes correlations with up to two bosons. Our phenomenological model is shown to recover the main results of two recent experiments probing both the spectral and the non-equilibrium properties of the Bose polaron. Our work offers an intuitive framework for analyzing experimental data and highlights the importance of understanding the complicated problem of the Bose polaron decay in a many-body setting.

cond-mat.quant-gas↗

arXiv2025

Observation of Analogue Dynamic Schwinger Effect and Non-Perturbative Light Sensing in Lead Halide Perovskites

Dielectric breakdown of physical vacuum (Schwinger effect) is the textbook demonstration of compatibility of Relativity and Quantum theory. Although observing this effect is still practically unachievable, its analogue generalizations have been shown to be more readily attainable. This paper demonstrates that a gapped Dirac semiconductor, methylammonium lead-bromide perovskite (MAPbBr$_3$), exhibits analogue dynamical Schwinger effect. Tunneling ionization under deep sub-gap mid-infrared irradiation leads to intense photoluminescence in the visible range, in full agreement with quasi-adiabatic theory. In addition to revealing a gapped extended system suitable for studying the analogue Schwinger effect, this observation holds great potential for non-perturbative field sensing, i.e., sensing electric fields through non-perturbative light-matter interactions. First, this paper illustrates this by measuring the local deviation from the nominally cubic phase of a perovskite single crystal, which can be interpreted in terms of frozen-in fields. Next, it is shown that analogue dynamic Schwinger effect can be used for nonperturbative amplification of non-parametric upconversion process in perovskites driven simultaneously by multiple optical fields. This discovery demonstrates the potential for material response beyond perturbation theory in the Schwinger regime, offering extremely sensitive light detection and amplification across an ultrabroad spectral range not accessible by conventional devices.

cond-mat.mes-hall↗

arXiv2025

Using optical tweezers to simultaneously trap, charge and measure the charge of a microparticle in air

Optical tweezers are widely used as a highly sensitive tool to measure forces on micron-scale particles. One such application is the measurement of the electric charge of a particle, which can be done with high precision in liquids, air, or vacuum. We experimentally investigate how the trapping laser itself can electrically charge such a particle, in our case a $\sim 1\,\mathrm{μm\;SiO_2}$ sphere in air. We model the charging mechanism as a two-photon process which reproduces the experimental data with high fidelity.

cond-mat.soft↗

arXiv2025

Effective theory for strongly attractive one-dimensional fermions

We study a one-dimensional system of two-component fermions in the limit of strong attractive particle-particle interactions. First, we analyze scattering in the corresponding few-body problem, which is analytically solvable via Bethe ansatz. This allows us to engineer effective interactions between the system's effective degrees of freedom: fermions and bosonic dimers (tightly bound pairs of fermions). We argue that, although these interactions are strong, the resulting effective problem can be mapped onto a weakly interacting one, paving the way for the use of perturbation theory. This finding simplifies studies of many-fermion systems under confinement that are beyond reach of state-of-the-art numerical methods. We illustrate this statement by considering an impurity atom in a Fermi gas.

cond-mat.quant-gas↗

arXiv2025

Two-dimensional bosonic droplets in a harmonic trap

We investigate a system of bosons in a two-dimensional harmonic trap. In the limit of strong attractive interactions, the bosons make a droplet insensitive to external confinement. For weak interactions, in contrast, the ground state is given by the harmonic trap. In this work, we conduct a variational study of the transition between these two limits. We find that this transition occurs abruptly at the critical interaction strength whose value is universal if scaled appropriately with the number of particles. To connect the abrupt change in the properties of the system to the classical description of phase transitions, we analyze the static response of the Bose gas related to the isothermal compressibility. Finally, we perform numerically exact calculations for a few particles to demonstrate the effects of finite range interactions on this transition. We conclude that finite range effects wash out the point of transition.

cond-mat.quant-gas↗

arXiv2025

Massive Dirac-Pauli physics in lead-halide perovskites

In standard quantum electrodynamics (QED), the so-called non-minimal (Pauli) coupling is suppressed for elementary particles and has no physical implications. Here, we show that the Pauli term naturally appears in a known family of Dirac materials -- the lead-halide perovskites, suggesting a novel playground for the study of analogue QED effects. We outline measurable manifestations of the Pauli term in the phenomena pertaining to (i) relativistic corrections to bound states (ii) the Klein paradox, and (iii) spin effects in scattering. In particular, we demonstrate that (a) the binding energy of an electron in the vicinity of a positively charged defect is noticeably decreased due to the polarizability of lead ions and the appearance of a Darwin-like term, (b) strong spin-orbit coupling due to the Pauli term affects the exciton states, and (c) scattering of an electron off an energy barrier with broken mirror symmetry produces spin polarization in the outgoing current. Our study adds to understanding of quantum phenomena in lead-halide perovskites, and paves the way for tabletop simulations of analogue Dirac-Pauli equations.

cond-mat.mes-hall↗

arXiv2025

Quantum rotor in a two-dimensional mesoscopic Bose gas

We investigate a molecular quantum rotor in a two-dimensional Bose-Einstein condensate. The focus is on studying the angulon quasiparticle concept in the crossover from few- to many-body physics. To this end, we formulate the problem in real space and solve it with a mean-field approach in the frame co-rotating with the impurity. We show that the system starts to feature angulon characteristics when the size of the bosonic cloud is large enough to screen the rotor. More importantly, we demonstrate the departure from the angulon picture for large system sizes or large angular momenta where the properties of the system are determined by collective excitations of the Bose gas.

cond-mat.quant-gas↗

arXiv2025

Comparison of renormalized interactions using one-dimensional few-body systems as a testbed

Even though the one-dimensional contact interaction requires no regularization, renormalization methods have been shown to improve the convergence of numerical ab initio calculations considerably. In this work, we compare and contrast these methods: `the running coupling constant' where the two-body ground state energy is used as a renormalization condition, and two effective interaction approaches that include information about the ground as well as excited states. In particular, we calculate the energies and densities of few-fermion systems in a harmonic oscillator with the configuration interaction method, and compare the results based upon renormalized and bare interactions. We find that the use of the running coupling constant instead of the bare interaction improves convergence significantly. A comparison with an effective interaction, which is designed to reproduce the relative part of the energy spectrum of two particles, showed a similar improvement. The effective interaction provides an additional improvement if the center-of-mass excitations are included in the construction. Finally, we discuss the transformation of observables alongside the renormalization of the potential, and demonstrate that this might be an essential ingredient for accurate numerical calculations.

cond-mat.quant-gas↗

arXiv2024

Anisotropic potential immersed in a dipolar Bose-Einstein condensate

We study a modified three-dimensional Gross-Pitaevski equation that describes a static impurity in a dipolar Bose-Einstein condensate (BEC). Our focus is on the interplay between the shape of the impurity and the anisotropy of the medium manifested in the energy and the density of the system. Without external confinement, properties of the system are derived with basic analytical approaches. For a system in a harmonic trap, the model is investigated numerically, using the split-step Crank-Nicolson method. Our results demonstrate that the impurity would prefer to change its shape to accommodate the anisotropic character of the bath, in particular it would prefer to align itself with the direction of the dipoles. Our work complements studies of impurities in Bose gases with zero-range interactions, and paves the way for studies of dipolar polarons with a modified Gross-Pitaevski equation.

cond-mat.quant-gas↗

arXiv2024

Classical 'spin' filtering with two degrees of freedom and dissipation

Coupling of angular motion to a spin degree of freedom gives rise to various transport phenomena in quantum systems that are beyond the standard paradigms of classical physics. Here, we discuss features of spin-orbit dynamics that can be visualized using a classical model with two coupled angular degrees of freedom. Specifically, we demonstrate classical 'spin' filtering through our model and show that the interplay between angular degrees of freedom and dissipation can lead to asymmetric 'spin' transport.

cond-mat.mes-hall↗

arXiv2024

Linear rotor in an ideal Bose gas near the threshold for binding

We study a linear rotor in a bosonic bath within the angulon formalism. Our focus is on systems where isotropic or anisotropic impurity-boson interactions support a shallow bound state. To study the fate of the angulon in the vicinity of bound-state formation, we formulate a beyond-linear-coupling angulon Hamiltonian. First, we use it to study attractive, spherically symmetric impurity-boson interactions for which the linear rotor can be mapped onto a static impurity. The well-known polaron formalism provides an adequate description in this limit. Second, we consider anisotropic potentials, and show that the presence of a shallow bound state with pronounced anisotropic character leads to a many-body instability that washes out the angulon dynamics.

cond-mat.quant-gas↗

arXiv2023

Non-equilibrium dynamics of dipolar polarons

We study the out-of-equilibrium quantum dynamics of dipolar polarons, i.e., impurities immersed in a dipolar Bose-Einstein condensate, after a quench of the impurity-boson interaction. We show that the dipolar nature of the condensate and of the impurity results in anisotropic relaxation dynamics, in particular, anisotropic dressing of the polaron. More relevantly for cold-atom setups, quench dynamics is strongly affected by the interplay between dipolar anisotropy and trap geometry. Our findings pave the way for simulating impurities in anisotropic media utilizing experiments with dipolar mixtures.

cond-mat.quant-gas↗

arXiv2023

Achiral dipoles on a ferromagnet can affect its magnetization direction

We demonstrate the possibility of a coupling between the magnetization direction of a ferromagnet and the tilting angle of adsorbed achiral molecules. To illustrate the mechanism of the coupling, we analyze a minimal Stoner model that includes Rashba spin-orbit coupling due to the electric field on the surface of the ferromagnet. The proposed mechanism allows us to study magnetic anisotropy of the system with an extended Stoner-Wohlfarth model, and argue that adsorbed achiral molecules can change magnetocrystalline anisotropy of the substrate. Our research's aim is to motivate further experimental studies of the current-free chirality induced spin selectivity effect involving both enantiomers.

cond-mat.mes-hall↗

arXiv2023

Bond polarizability as a probe of local crystal fields in hybrid lead-halide perovskites

A rotating organic cation and a dynamically disordered soft inorganic cage are the hallmark features of hybrid organic-inorganic lead-halide perovskites. Understanding the interplay between these two subsystems is a challenging problem but it is this coupling that is widely conjectured to be responsible for the unique behavior of photo-carriers in these materials. In this work, we use the fact that the polarizability of the organic cation strongly depends on the ambient electrostatic environment to put the molecule forward as a sensitive probe of local crystal fields inside the lattice cell. We measure the average polarizability of the C/N--H bond stretching mode by means of infrared spectroscopy, which allows us to deduce the character of the motion of the cation molecule, find the magnitude of the local crystal field and place an estimate on the strength of the hydrogen bond between the hydrogen and halide atoms. Our results pave the way for understanding electric fields in lead-halide perovskites using infrared bond spectroscopy.

cond-mat.mes-hall↗

arXiv2023

Emergence of a Bose polaron in a small ring threaded by the Aharonov-Bohm flux

The model of a ring threaded by the Aharonov-Bohm flux underlies our understanding of a coupling between gauge potentials and matter. The typical formulation of the model is based upon a single particle picture, and should be extended when interactions with other particles become relevant. Here, we illustrate such an extension for a particle in an Aharonov-Bohm ring subject to interactions with a weakly interacting Bose gas. We show that the ground state of the system can be described using the Bose polaron concept -- a particle dressed by interactions with a bosonic environment. We connect the energy spectrum to the effective mass of the polaron, and demonstrate how to change currents in the system by tuning boson-particle interactions. Our results suggest the Aharonov-Bohm ring as a platform for studying coherence and few- to many-body crossover of quasi-particles that arise from an impurity immersed in a medium.

cond-mat.quant-gas↗