arXiv subjects

Arthur Christianen

Publications and source records attributed to Arthur Christianen.

24 records · Page 2Linked to original sources

arXiv2021

From Efimov Physics to the Bose Polaron using Gaussian States

Since the Efimov effect was introduced in 1970, a detailed theoretical understanding of Efimov physics has been developed in the few-body context. However, it has proven to be challenging to describe the role Efimov-type correlations play in many-body systems such as quenched or collapsing Bose-Einstein condensates (BECs). To study the impact the Efimov effect can have in such scenarios, we consider a light impurity immersed in a weakly interacting BEC, forming a Bose polaron. In this case, the higher-order correlations are localized around the impurity, making it more feasible to develop a theoretical description. Specifically, we employ a Gaussian state variational Ansatz in the reference frame of the impurity, capable of both capturing the Efimov effect and the formation of the polaron cloud. We find that the Efimov effect leads to a cooperative binding of bosons to the impurity and the formation of a many-body bound state. As a result, the polaron is not the ground state, but rendered a metastable excited state which can decay into these Efimov clusters. While this decay is slow for small interaction strengths, it becomes more prominent as the attractive scattering length increases, up to the point where the polaron becomes completely unstable. This critical scattering length can be interpreted as a many-body shifted Efimov resonance, where the scattering of two excitations of the bath with the polaron can lead to bound state formation. Compared to the few-body case, the resonance is shifted to smaller attractive scattering lengths due to the participation of the polaron cloud in the cooperative binding process. This corresponds to an intriguing scenario of polaron-assisted chemistry, where many-body effects lead to enhanced signal of the chemical recombination process, which can be directly probed in state-of-the-art experiments.

cond-mat.quant-gas↗

arXiv2021

Chemistry of a light impurity in a Bose-Einstein condensate

In ultracold atomic gases, a unique interplay arises between phenomena known from condensed matter physics, few-body physics and chemistry. Similar to an electron in a solid, an impurity in an ultracold gas can get dressed by excitations from the medium, forming a quasiparticle called the polaron. We study how dressing of an impurity leads to a modification of its chemical reactivity. Using a Gaussian state variational method in the frame of the impurity, we demonstrate that three-body correlations lead to an instability of the polaron. This instability is connected to an Efimov resonance, but shifted to smaller interactions by many-body effects, showing that polaron formation stimulates Efimov physics and the associated chemistry.

cond-mat.quant-gas↗

arXiv2021

Collisions of ultracold molecules in bright and dark optical dipole traps

Understanding collisions between ultracold molecules is crucial for making stable molecular quantum gases and harnessing their rich internal degrees of freedom for quantum engineering. Transient complexes can strongly influence collisional physics, but in the ultracold regime, key aspects of their behavior have remained unknown. To explain experimentally observed loss of ground-state molecules from optical dipole traps, it was recently proposed that molecular complexes can be lost due to photo-excitation. By trapping molecules in a repulsive box potential using laser light near a narrow molecular transition, we are able to test this hypothesis with light intensities three orders of magnitude lower than what is typical in red-detuned dipole traps. This allows us to investigate light-induced collisional loss in a gas of nonreactive fermionic $^{23}$Na$^{40}$K molecules. Even for the lowest intensities available in our experiment, our results are consistent with universal loss, meaning unit loss probability inside the short-range interaction potential. Our findings disagree by at least two orders of magnitude with latest theoretical predictions, showing that crucial aspects of molecular collisions are not yet understood, and provide a benchmark for the development of new theories.

cond-mat.quant-gas↗

arXiv2021

Exploring universal and non-universal regimes of trimers from three-body interactions in one-dimensional lattices

We investigate the formation of trimers in an infinite one-dimensional lattice model of hard-core particles with single-particle hopping $t$ and and nearest-neighbour two-body $U$ and three-body $V$ interactions of relevance to Rydberg atoms and polar molecules. For sufficiently attractive $U\leq-2t$ and positive $V>0$ a large trimer is stabilized, which persists as $V\rightarrow \infty$, while both attractive $U\leq0$ and $V\leq0$ bind a small trimer. The excited state above this small trimer is also bound and has a large extent; its behavior as $V\rightarrow -\infty$ resembles that of the large ground-state trimer. These large bound states appear to admit a continuum description. Furthermore, we find that in the limit $V>>t$, $U<-2t$ the bound-state behavior qualitatively evolves with larger $|U|$ from a state described by the scattering of three far separated particles to a state of a compact dimer scattering with a single particle.

quant-ph↗

arXiv2019

A quasiclassical method for calculating the density of states of ultracold collision complexes

We derive a quasiclassical expression for the density of states (DOS) of an arbitrary, ultracold, $N$-atom collision complex, for a general potential energy surface (PES). We establish the accuracy of our quasiclassical method by comparing to exact quantum results for the K$_2$-Rb and NaK-NaK systems, with isotropic model PESs. Next, we calculate the DOS for an accurate NaK-NaK PES to be 0.124~$μ$K$^{-1}$, with an associated Rice-Ramsperger-Kassel-Marcus (RRKM) sticking time of 6.0~$μ$s. We extrapolate the DOS and sticking times to all other polar bialkali-bialkali collision complexes by scaling with atomic masses, equilibrium bond lengths, dissociation energies, and dispersion coefficients. The sticking times calculated here are two to three orders of magnitude shorter than those reported by Mayle et al. [Phys. Rev. A 85, 062712 (2012)]. We estimate dispersion coefficients and collision rates between molecules and complexes. We find that the sticking-amplified three-body loss mechanism is not likely the cause of the losses observed in the experiments.

cond-mat.quant-gas↗

arXiv2019

Photo-induced two-body loss of ultracold molecules

The lifetime of nonreactive ultracold bialkali gases was conjectured to be limited by sticky collisions amplifying three-body loss. We show that the sticking times were previously overestimated and do not support this hypothesis. We find that electronic excitation of NaK+NaK collision complexes by the trapping laser leads to the experimentally observed two-body loss. We calculate the excitation rate with a quasiclassical, statistical model employing ab initio potentials and transition dipole moments. Using longer laser wavelengths or repulsive box potentials may suppress the losses.

physics.atom-ph↗