arXiv subjects

Ashley Lyons

Publications and source records attributed to Ashley Lyons.

At least 19 recordsLinked to original sources

arXiv2025

Entangled-photon time- and frequency-resolved optical spectroscopy

Classical time-resolved optical spectroscopy experiments are performed using sequences of ultrashort light pulses, with photon fluxes incident on the sample which are many orders of magnitude higher than real-world conditions corresponding to sunlight illumination. Here we overcome this paradigm by exploiting quantum correlations to perform time-resolved spectroscopy with entangled photons. Starting from spontaneous parametric down-conversion driven by a continuous-wave laser, we exploit the temporal entanglement between randomly generated signal/idler pairs to obtain temporal resolution, and their spectral entanglement to select the excitation frequency. We also add spectral resolution in detection, using a Fourier transform approach which employs a common-path interferometer. We demonstrate the potential of our entangled-photon streak camera by resolving, at the single-photon level, excitation energy transfer cascades from LH2 to LH1 in the photosynthetic membrane and disentangling the lifetimes of two dyes in a mixture. We show that time-resolved spectroscopy with quantum light can be performed without compromising measurement time, recording a fluorescence time trace in less than a minute even for samples with low quantum yield, which can be reduced to sub-second times with acceptable signal-to-noise ratio. Our results provide a new approach to ultrafast optical spectroscopy, where experiments are performed under conditions comparable to real-world sunlight illumination.

quant-ph↗

arXiv2023

Fluorescence Lifetime Hong-Ou-Mandel Sensing

Fluorescence Lifetime Imaging Microscopy in the time domain is typically performed by recording the arrival time of photons either by using electronic time tagging or a gated detector. As such the temporal resolution is limited by the performance of the electronics to 100's of picoseconds. Here, we demonstrate a fluorescence lifetime measurement technique based on photon-bunching statistics with a resolution that is only dependent on the duration of the reference photon or laser pulse, which can readily reach the 1-0.1 picosecond timescale. A range of fluorescent dyes having lifetimes spanning from 1.6 to 7 picoseconds have been here measured with only ~1 second measurement duration. We corroborate the effectiveness of the technique by measuring the Newtonian viscosity of glycerol/water mixtures by means of a molecular rotor having over an order of magnitude variability in lifetime, thus introducing a new method for contact-free nanorheology. Accessing fluorescence lifetime information at such high temporal resolution opens a doorway for a wide range of fluorescent markers to be adopted for studying yet unexplored fast biological processes, as well as fundamental interactions such as lifetime shortening in resonant plasmonic devices.

quant-ph↗

arXiv2022

Two-Photon Interference LiDAR Imaging

Optical Coherence Tomography (OCT) is a key 3D imaging technology that provides micron scale depth resolution for bio-imaging. This resolution substantially surpasses what it typically achieved in Light Detection and Ranging (LiDAR) which is often limited to the millimetre scale due to the impulse response of the detection electronics. However, the lack of coherence in LiDAR scenes, arising from mechanical motion for example, make OCT practically infeasible. Here we present a quantum interference inspired approach to LiDAR which achieves OCT depth resolutions without the need for high levels of stability. We demonstrate depth imaging capabilities with an effective impulse response of 70 {\mu}m, thereby allowing ranging and multiple reflections to be discerned with much higher resolution than conventional LiDAR approaches. This enhanced resolution opens up avenues for LiDAR in 3D facial recognition, and small feature detection/tracking as well as enhancing the capabilities of more complex time-of-flight methods such as imaging through obscurants and non-line-of-sight imaging.

physics.optics↗

arXiv2022

An all-dielectric metasurface polarimeter

The polarization state of light is a key parameter in many imaging systems. For example, it can image mechanical stress and other physical properties that are not seen with conventional imaging, and can also play a central role in quantum sensing. However, polarization is more difficult to image and polarimetry typically involves several independent measurements with moving parts in the measurement device. Metasurfaces with interleaved designs have demonstrated sensitivity to either linear or circular/elliptical polarization states. Here we present an all-dielectric meta-polarimeter for direct measurement of any arbitrary polarization states from a single unit-cell design. By engineering a completely asymmetric design, we obtained a metasurface that can excite eigenmodes of the nanoresonators, thus displaying a unique diffraction pattern for not only any linear polarization state but all elliptical polarization states (and handedness) as well. The unique diffraction patterns are quantified into Stokes parameters with a resolution of 5$^{\circ}$ and with a polarization state fidelity of up to $99\pm1$%. This holds promise for applications in polarization imaging and quantum state tomography.

physics.optics↗

arXiv2021

Quantum microscopy based on Hong-Ou-Mandel interference

Hong-Ou-Mandel (HOM) interference, the bunching of indistinguishable photons at a beam splitter, is a staple of quantum optics and lies at the heart of many quantum sensing approaches and recent optical quantum computers. Here, we report a full-field, scan-free, quantum imaging technique that exploits HOM interference to reconstruct the surface depth profile of transparent samples. We demonstrate the ability to retrieve images with micrometre-scale depth features with a photon flux as small as 7 photon pairs per frame. Using a single photon avalanche diode camera we measure both the bunched and anti-bunched photon-pair distributions at the HOM interferometer output which are combined to provide a lower-noise image of the sample. This approach demonstrates the possibility of HOM microscopy as a tool for label-free imaging of transparent samples in the very low photon regime.

quant-ph↗

arXiv2021

3D imaging from multipath temporal echoes

Echo-location is a broad approach to imaging and sensing that includes both man-made RADAR, LIDAR, SONAR and also animal navigation. However, full 3D information based on echo-location requires some form of scanning of the scene in order to provide the spatial location of the echo origin-points. Without this spatial information, imaging objects in 3D is a very challenging task as the inverse retrieval problem is strongly ill-posed. Here, we show that the temporal information encoded in the return echoes that are reflected multiple times within a scene is sufficient to faithfully render an image in 3D. Numerical modelling and an information theoretic perspective prove the concept and provide insight into the role of the multipath information. We experimentally demonstrate the concept by using both radio-frequency and acoustic waves for imaging individuals moving in a closed environment.

eess.IV↗

arXiv2021

Pixel super-resolution using spatially-entangled photon pairs

Pixelation occurs in many imaging systems and limits the spatial resolution of the acquired images. This effect is notably present in quantum imaging experiments with correlated photons in which the number of pixels used to detect coincidences is often limited by the sensor technology or the acquisition speed. Here, we introduce a pixel super-resolution technique based on measuring the full spatially-resolved joint probability distribution (JPD) of spatially-entangled photons. Without shifting optical elements or using prior information, our technique increases the pixel resolution of the imaging system by a factor two and enables retrieval of spatial information lost due to undersampling. We demonstrate its use in various quantum imaging protocols using photon pairs, including quantum illumination, entanglement-enabled quantum holography, and in a full-field version of N00N-state quantum holography. The JPD pixel super-resolution technique can benefit any full-field imaging system limited by the sensor spatial resolution, including all already established and future photon-correlation-based quantum imaging schemes, bringing these techniques closer to real-world applications.

quant-ph↗

arXiv2021

Quantum Light Detection and Ranging

Single-photon light detection and ranging (LiDAR) is a key technology for depth imaging through complex environments. Despite recent advances, an open challenge is the ability to isolate the LiDAR signal from other spurious sources including background light and jamming signals. Here we show that a time-resolved coincidence scheme can address these challenges by exploiting spatiotemporal correlations between entangled photon pairs. We demonstrate that a photon-pair-based LiDAR can distill desired depth information in the presence of both synchronous and asynchronous spurious signals without prior knowledge of the scene and the target object. This result enables the development of robust and secure quantum LiDAR systems and paves the way to time-resolved quantum imaging applications.

quant-ph↗

arXiv2021

Polarization entanglement-enabled quantum holography

Holography is a cornerstone characterisation and imaging technique that can be applied to the full electromagnetic spectrum, from X-rays to radio waves or even particles such as neutrons. The key property in all these holographic approaches is coherence that is required to extract the phase information through interference with a reference beam - without this, holography is not possible. Here we introduce a holographic imaging approach that operates on intrinsically incoherent and unpolarised beams, so that no phase information can be extracted from a classical interference measurement. Instead, the holographic information is encoded in the second order coherence of entangled states of light. Using spatial-polarisation hyper-entangled photons pairs, we remotely reconstruct phase images of complex objects. Information is encoded into the polarisation degree of the entangled state, allowing us to image through dynamic phase disorder and even in the presence of strong classical noise, with enhanced spatial resolution compared to classical coherent holographic systems. Beyond imaging, quantum holography quantifies hyper-entanglement distributed over 10^4 modes via a spatially-resolved Clauser-Horne-Shimony-Holt inequality measurement, with applications in quantum state characterisation.

quant-ph↗

arXiv2020

The role of late photons in diffuse optical imaging

The ability to image through turbid media such as organic tissues, is a highly attractive prospect for biological and medical imaging. This is challenging however, due to the highly scattering properties of tissues which scramble the image information. The earliest photons that arrive at the detector are often associated with ballistic transmission, whilst the later photons are associated with complex paths due to multiple independent scattering events and are therefore typically considered to be detrimental to the final image formation process. In this work we report on the importance of these highly diffuse, "late" photons for computational time-of-flight diffuse optical imaging. In thick scattering materials, >80 transport mean free paths, we provide evidence that including late photons in the inverse retrieval enhances the image reconstruction quality. We also show that the late photons alone have sufficient information to retrieve images of a similar quality to early photon gated data. This result emphasises the importance in the strongly diffusive regime discussed here, of fully time-resolved imaging techniques.

physics.optics↗

arXiv2020

Imaging entanglement correlations with a single-photon avalanche diode camera

Spatial correlations between two photons are the key resource in realising many quantum imaging schemes. Measurement of the bi-photon correlation map is typically performed using single-point scanning detectors or single-photon cameras based on CCD technology. However, both approaches are limited in speed due to the slow scanning and the low frame-rate of CCD-based cameras, resulting in data acquisition times on the order of many hours. Here we employ a high frame rate, single photon avalanche diode (SPAD) camera, to measure the spatial joint probability distribution of a bi-photon state produced by spontaneous parametric down-conversion, with statistics taken over $10^7$ frames acquired in just 140 seconds. We verified the presence of spatial entanglement between our photon pairs through the violation of an Einstein-Podolsky-Rosen criterion, with a confidence level of 227 sigmas. Our work demonstrates the potential of SPAD cameras in the rapid characterisation of photon correlations, leading the way towards quantum imaging in real-time.

quant-ph↗

arXiv2020

Spatial images from temporal data

Traditional paradigms for imaging rely on the use of a spatial structure, either in the detector (pixels arrays) or in the illumination (patterned light). Removal of the spatial structure in the detector or illumination, i.e., imaging with just a single-point sensor, would require solving a very strongly ill-posed inverse retrieval problem that to date has not been solved. Here, we demonstrate a data-driven approach in which full 3D information is obtained with just a single-point, single-photon avalanche diode that records the arrival time of photons reflected from a scene that is illuminated with short pulses of light. Imaging with single-point time-of-flight (temporal) data opens new routes in terms of speed, size, and functionality. As an example, we show how the training based on an optical time-of-flight camera enables a compact radio-frequency impulse radio detection and ranging transceiver to provide 3D images.

eess.IV↗

arXiv2020

Computational time-of-flight diffuse optical tomography

Imaging through a strongly diffusive medium remains an outstanding challenge in particular in association with applications in biological and medical imaging. Here we propose a method based on a single-photon time-of-flight camera that allows, in combination with computational processing of the spatial and full temporal photon distribution data, to image an object embedded inside a strongly diffusive medium over more than 80 transport mean free paths. The technique is contactless and requires one second acquisition times thus allowing Hz frame rate imaging. The imaging depth corresponds to several cm of human tissue and allows one to perform deep-body imaging, here demonstrated as a proof-of-principle.

physics.optics↗

arXiv2018

Coherent metamaterial absorption of two-photon states with 40% efficiency

Multi-photon absorption processes have a nonlinear dependence on the amplitude of the incident optical field i.e. the number of photons. However, multi-photon absorption is generally weak and multi-photon events occur with extremely low probability. Consequently, it is extremely challenging to engineer quantum nonlinear devices that operate at the single photon level and the majority of quantum technologies have to rely on single photon interactions. Here, we demonstrate experimentally and theoretically that exploiting coherent absorption of N = 2 N00N states makes it possible to enhance the number of two-photon states that are absorbed. An absorbing metasurface placed inside a Sagnac-style interferometer into which we inject an N = 2 N00N state, exhibits two-photon absorption with 40.5% efficiency, close to the theoretical maximum. This high probability of simultaneous absorption of two photons holds the promise for applications in fields that require multi-photon upconversion but are hindered by high peak intensities.

quant-ph↗

arXiv2017

How fast is a twisted photon?

Recent measurements have highlighted that spatially shaped photons travel slower than c, the speed of monochromatic, plane waves in vacuum. Here we investigate the intrinsic delay introduced by `twisting' a photon, i.e. by introducing orbital angular momentum (OAM). In order to do this we use a Hong-Ou-Mandel interferometer to measure the change in delay of single photons when we introduce OAM on a ring-shaped beam that is imaged through a focusing telescope. Our findings show that when all other parameters are held constant the addition of OAM reduces the delay (accelerates) with respect to the same beam with no OAM. We support our results using a theoretical method to calculate the group velocity and gain an intuitive understanding of the measured OAM acceleration by considering a geometrical ray-tracing approach.

physics.optics↗

arXiv2017

Attosecond-Resolution Hong-Ou-Mandel Interferometry

When two indistinguishable photons are each incident on separate input ports of a beamsplitter they `bunch' deterministically, exiting via the same port as a direct consequence of their bosonic nature. This two-photon interference effect has long-held the potential for application in precision measurement of time delays, such as those induced by transparent specimens with unknown thickness profiles. However, the technique has never achieved resolutions significantly better than the few femtosecond (micron)-scale other than in a common-path geometry that severely limits applications. Here we develop the precision of HOM interferometry towards the ultimate limits dictated by statistical estimation theory, achieving few-attosecond (or nanometre path length) scale resolutions in a dual-arm geometry, thus providing access to length scales pertinent to cell biology and mono-atomic layer 2D materials.

quant-ph↗

arXiv2016

Coherent absorption of N00N states

Recent results in deeply subwavelength thickness films demonstrated coherent control and logical gate operations with both classical and single photon light sources. However, quantum processing and devices typically involve more than one photon and non-trivial input quantum states. Here we experimentally investigate two-photon N00N state coherent absorption in a multilayer graphene film. Depending on the N00N state input phase, it is possible to selectively choose between single or two photon absorption of the input state in the graphene film. These results demonstrate that coherent absorption in the quantum regime exhibits unique features opening up applications in multiphoton spectroscopy and imaging.

physics.optics↗

arXiv2015

Observation of image pair creation and annihilation from superluminal scattering sources

The invariance of the speed of light implies a series of consequences related to our perception of simultaneity and of time itself. Whilst these consequences are experimentally well studied for subluminal speeds, the kinematics of superluminal motion lack direct evidence. Using high temporal resolution imaging techniques, we demonstrate that if a source approaches an observer at superluminal speeds, the temporal ordering of events is inverted and its image appears to propagate backwards. If the source changes its speed, crossing the interface between sub- and super-luminal propagation, we observe image pair annihilation and creation. These results show that it is not possible to unambiguously determine the kinematics of an event from imaging and time-resolved measurements alone.

physics.optics↗