arXiv subjects

Ashley M. Cook

Publications and source records attributed to Ashley M. Cook.

25 records · Page 2Linked to original sources

arXiv2023

Multiplicative topological semimetals

Exhaustive study of topological semimetal phases of matter in equilibriated electonic systems and myriad extensions has built upon the foundations laid by earlier introduction and study of the Weyl semimetal, with broad applications in topologically-protected quantum computing, spintronics, and optical devices. We extend recent introduction of multiplicative topological phases to find previously-overlooked topological semimetal phases of electronic systems in equilibrium, with minimal symmetry-protection. We show these multiplicative topological semimetal phases exhibit rich and distinctive bulk-boundary correspondence and response signatures that greatly expand understanding of consequences of topology in condensed matter settings, such as the limits on Fermi arc connectivity and structure, and transport signatures such as the chiral anomaly. Our work therefore lays the foundation for extensive future study of multiplicative topological semimetal phases.

cond-mat.mes-hall↗

arXiv2022

Multiplicative topological phases

Symmetry-protected topological phases of matter have challenged our understanding of condensed matter systems and harbour exotic phenomena promising to address major technological challenges. Considerable understanding of these phases of matter has been gained recently by considering additional protecting symmetries, different types of quasiparticles, and systems out of equilibrium. Here, we show that symmetries could be enforced not just on full Hamiltonians, but also on their components. We construct a large class of previously unidentified multiplicative topological phases of matter characterized by tensor product Hilbert spaces similar to the Fock space of multiple particles. To demonstrate our methods, we introduce multiplicative topological phases of matter based on the foundational Hopf and Chern insulator phases, the multiplicative Hopf and Chern insulators (MHI and MCI), respectively. The MHI shows the distinctive properties of the parent phases as well as non-trivial topology of a child phase. We also comment on a similar structure in topological superconductors as these multiplicative phases are protected in part by particle-hole symmetry. The MCI phase realizes topologically-protected gapless states that do not extend from the valence bands to the conduction bands for open boundary conditions, which respect the symmetries protecting topological phase. The band connectivity discovered in the MCI could serve as a blueprint for potential multiplicative topology with exotic properties.

cond-mat.str-el↗

arXiv2019

Higher-Order Topology in Bismuth

The mathematical field of topology has become a framework to describe the low-energy electronic structure of crystalline solids. A typical feature of a bulk insulating three-dimensional topological crystal are conducting two-dimensional surface states. This constitutes the topological bulk-boundary correspondence. Here, we establish that the electronic structure of bismuth, an element consistently described as bulk topologically trivial, is in fact topological and follows a generalized bulk-boundary correspondence of higher-order: not the surfaces of the crystal, but its hinges host topologically protected conducting modes. These hinge modes are protected against localization by time-reversal symmetry locally, and globally by the three-fold rotational symmetry and inversion symmetry of the bismuth crystal. We support our claim theoretically and experimentally. Our theoretical analysis is based on symmetry arguments, topological indices, first-principle calculations, and the recently introduced framework of topological quantum chemistry. We provide supporting evidence from two complementary experimental techniques. With scanning-tunneling spectroscopy, we probe the unique signatures of the rotational symmetry of the one-dimensional states located at step edges of the crystal surface. With Josephson interferometry, we demonstrate their universal topological contribution to the electronic transport. Our work establishes bismuth as a higher-order topological insulator.

cond-mat.mtrl-sci↗

arXiv2018

Topology in the Sierpiński-Hofstadter problem

Using the Sierpiński carpet and gasket, we investigate whether fractal lattices embedded in two-dimensional space can support topological phases when subjected to a homogeneous external magnetic field. To this end, we study the localization property of eigenstates, the Chern number, and the evolution of energy level statistics when disorder is introduced. Combining these theoretical tools, we identify regions in the phase diagram of both the carpet and the gasket, for which the systems exhibit properties normally associated to gapless topological phases with a mobility edge.

cond-mat.mes-hall↗

arXiv2018

Higher-Order Topological Insulators

Three-dimensional topological (crystalline) insulators are materials with an insulating bulk, but conducting surface states which are topologically protected by time-reversal (or spatial) symmetries. Here, we extend the notion of three-dimensional topological insulators to systems that host no gapless surface states, but exhibit topologically protected gapless hinge states. Their topological character is protected by spatio-temporal symmetries, of which we present two cases: (1) Chiral higher-order topological insulators protected by the combination of time-reversal and a four-fold rotation symmetry. Their hinge states are chiral modes and the bulk topology is $\mathbb{Z}_2$-classified. (2) Helical higher-order topological insulators protected by time-reversal and mirror symmetries. Their hinge states come in Kramers pairs and the bulk topology is $\mathbb{Z}$-classified. We provide the topological invariants for both cases. Furthermore we show that SnTe as well as surface-modified Bi$_2$TeI, BiSe, and BiTe are helical higher-order topological insulators and propose a realistic experimental setup to detect the hinge states.

cond-mat.mes-hall↗

arXiv2017

Magnetic Weyl and Dirac Kondo semimetal phases in heterostructures

We study a layered three-dimensional heterostructure in which two types of Kondo insulators are stacked alternatingly. One of them is the topological Kondo insulator SmB 6 , the other one an isostructural Kondo insulator AB 6 , where A is a rare-earth element, e.g., Eu, Yb, or Ce. We find that if the latter orders ferromagnetically, the heterostructure generically becomes a magnetic Weyl Kondo semimetal, while antiferromagnetic order can yield a magnetic Dirac Kondo semimetal. We detail both scenarios with general symmetry considerations as well as concrete tight-binding calcu-lations and show that type-I as well as type-II magnetic Weyl/Dirac Kondo semimetal phases are possible in these heterostructures. Our results demonstrate that Kondo insulator heterostructures are a versatile platform for design of strongly correlated topological semimetals.

cond-mat.str-el↗

arXiv2017

Design principles for shift current photovoltaics

While the basic principles and limitations of conventional solar cells are well understood, relatively little attention has gone toward maximizing the potential efficiency of photovoltaic devices based on shift currents. In this work, we outline simple design principles for the optimization of shift currents for frequencies near the band gap, derived from the analysis of a general effective model. The use of a novel sum rule allows us to express the band edge shift current in terms of a few model parameters and to show it depends explicitly on wavefunctions via Berry connections in addition to standard band structure. We use our approach to identify two new classes of shift current photovoltaics, ferroelectric polymer films and single-layer orthorhombic monochalcogenides such as GeS. We introduce tight-binding models for these systems, and show that they exhibit the largest shift current responsivities at the band edge reported so far. Moreover, exploring the parameter space of these models we find photoresponsivities that can exceed $100$ mA/W. Our results show how the study of the shift current via effective models allows one to improve the possible efficiency of devices based on this mechanism and better grasp their potential to compete with conventional solar cells.

cond-mat.mes-hall↗