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Ashvin Vishwanath

Publications and source records attributed to Ashvin Vishwanath.

At least 145 records · Page 8Linked to original sources

Magic Angle Hierarchy in Twisted Graphene Multilayers

When two monolayers of graphene are stacked with a small relative twist angle, the resulting band structure exhibits a remarkably flat pair of bands at a sequence of 'magic angles' where correlation effects can induce a host of exotic phases. Here, we study a class of related models of $n$-layered graphene with alternating relative twist angle $\pm θ$ which exhibit magic angle flat bands coexisting with several Dirac dispersing bands at the Moiré K point. Remarkably, we find that the Hamiltonian for the multilayer system can be mapped exactly to a set of decoupled bilayers at {\it different} angles, revealing a remarkable hierarchy mathematically relating all these magic angles to the TBG case. For the trilayer case ($n = 3$), we show that the sequence of magic angle is obtained by multiplying the bilayer magic angles by $\sqrt{2}$, whereas the quadrilayer case ($n = 4$) has two sequences of magic angles obtained by multiplying the bilayer magic angles by the golden ratio $φ= (\sqrt{5} + 1)/2 \approx 1.62$ and its inverse. We also show that for larger $n$, we can tune the angle to obtain several narrow (almost flat) bands simultaneously and that for $n \rightarrow \infty$, there is a continuum of magic angles for $θ\lesssim 2^o$. Furthermore, we show that tuning several perfectly flat bands for a small number of layers is possible if the coupling between different layers is different. The setup proposed here can be readily achieved by repeatedly applying the "tear and stack" method without the need of any extra tuning of the twist angle and has the advantage that the first magic angle is always larger than the bilayer case.

cond-mat.str-el↗

Shift insulators: rotation-protected two-dimensional topological crystalline insulators

We study a two-dimensional (2D) tight-binding model of a topological crystalline insulator (TCI) protected by rotation symmetry. The model is built by stacking two Chern insulators with opposite Chern numbers which transform under conjugate representations of the rotation group, e.g. $p_\pm$ orbitals. Despite its apparent similarity to the Kane-Mele model, it does not host stable gapless surface states. Nevertheless the model exhibits topological responses including the appearance of quantized fractional charge bound to rotational defects (disclinations) and the pumping of angular momentum in response to threading an elementary magnetic flux, which are described by a mutual Chern-Simons coupling between the electromagnetic gauge field and an effective gauge field corresponding to the rotation symmetry. In addition, we show that although the filled bands of the model do not admit a symmetric Wannier representation, this obstruction is removed upon the addition of appropriate atomic orbitals, which implies `fragile' topology. As a result, the response of the model can be derived by representing it as a superposition of atomic orbitals with positive and negative integer coefficients. Following the analysis of the model, which serves as a prototypical example of 2D TCIs protected by rotation, we show that all TCIs protected by point group symmetries which do not have protected surface states are either atomic insulators or fragile phases. Remarkably, this implies that gapless surface states exist in free electron systems if and only if there is a stable Wannier obstruction. We then use dimensional reduction to map the problem of classifying 2D TCIs protected by rotation to a zero-dimensional (0D) problem which is then used to obtain the complete non-interacting classification of such TCIs as well as the reduction of this classification in the presence of interactions.

cond-mat.mes-hall↗

Topological Correspondence between Hermitian and Non-Hermitian Systems: Anomalous Dynamics

The hallmark of symmetry-protected topological (SPT) phases is the existence of anomalous boundary states, which can only be realized with the corresponding bulk system. In this work, we show that for every Hermitian anomalous boundary mode of the ten Altland-Zirnbauer classes, a non-Hermitian counterpart can be constructed, whose long time dynamics provides a realization of the anomalous boundary state. We prove that the non-Hermitian counterpart is characterized by a point-gap topological invariant, and furthermore, that the invariant exactly matches that of the corresponding Hermitian anomalous boundary mode. We thus establish a correspondence between the topological classifications of $(d+1)$-dimensional gapped Hermitian systems and $d$-dimensional point-gapped non-Hermitian systems. We illustrate this general result with a number of examples in different dimensions. This work provides a new perspective on point-gap topological invariants in non-Hermitian systems.

cond-mat.mes-hall↗

Two-dimensional topological materials discovery by symmetry-indicator method

Two-dimensional (2D) topological materials (TMs) have attracted tremendous attention due to the promise of revolutionary devices with non-dissipative electric or spin currents. Unfortunately, the scarcity of 2D TMs holds back the experimental realization of such devices. In this work, based on our recently developed, highly efficient TM discovery algorithm using symmetry indicators, we explore the possible 2D TMs in all non-magnetic compounds in four recently proposed materials databases for possible 2D materials. We identify hundreds of 2D TM candidates, including 205 topological (crystalline) insulators and 299 topological semimetals. In particular, we highlight MoS, with a mirror Chern number of -4, as a possible experimental platform for studying the interaction-induced modification to the topological classification of materials. Our results winnow out the topologically interesting 2D materials from these databases and provide a TM gene pool which for further experimental studies.

cond-mat.mes-hall↗

Faithful Tight-binding Models and Fragile Topology of Magic-angle Bilayer Graphene

Correlated insulators and superconductivity have been observed in "magic-angle" twisted bilayer graphene, when the nearly flat bands close to neutrality are partially filled. While a momentum-space continuum model accurately describes these flat bands, interaction effects are more conveniently incorporated in tight-binding models. We have previously shown that no fully symmetric tight-binding model can be minimal, in the sense of capturing just the flat bands, so extended models are unavoidable. Here, we introduce a family of tight-binding models that capture the flat bands while simultaneously retaining all symmetries. In particular, we construct three concrete models with five, six, or ten bands per valley and per spin. These models are also faithful, in that the additional degrees of freedom represent energy bands further away from neutrality, and they serve as optimal starting points for a controlled study of interaction effects. Furthermore, our construction demonstrates the "fragile topology" of the nearly flat bands; i.e., the obstruction to constructing exponentially localized Wannier functions can be resolved when a particular set of trivial bands is added to the model.

cond-mat.str-el↗

Flat band in twisted bilayer Bravais lattices

Band engineering in twisted bilayers of the five generic two-dimensional Bravais networks is demonstrated. We first derive symmetry-based constraints on the interlayer coupling, which helps us to predict and understand the shape of the potential barrier for the electrons under the influence of the moiré structure without reference to microscopic details. It is also pointed out that the generic constraints becomes best relevant when the typical length scale of the microscopic interlayer coupling is moderate. The concepts are numerically demonstrated in simple tight-binding models to show the band flattening due to the confinement into the potential profile fixed by the generic constraints. On the basis of the generic theory, we propose the possibility of anisotropic band flattening, in which quasi one-dimensional band dispersion is generated from relatively isotropic original band dispersion. In the strongly correlated regime, anisotropic band flattening leads to a spin-orbital model where intertwined magnetic and orbital ordering can give rise to rich physics.

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Towards ideal topological materials: Comprehensive database searches using symmetry indicators

Topological materials (TMs) showcase intriguing physical properties defying expectations based on conventional materials, and hold promise for the development of devices with new functionalities. While several theoretically proposed TMs have been experimentally confirmed, extensive experimental exploration of topological properties as well as applications in realistic devices have been held back due to the lack of excellent TMs in which interference from trivial Fermi surface states is minimized. We tackle this problem in the present work by applying our recently developed method of symmetry indicators to all non-magnetic compounds in the 230 space groups. An exhaustive database search reveals thousands of TM candidates. Of these, we highlight the excellent TMs, the 258 topological insulators and 165 topological crystalline insulators which have either noticeable full band gap or a considerable direct gap together with small trivial Fermi pockets. We also give a list of 489 topological semimetals with the band crossing points located near the Fermi level. All predictions obtained through standard generalized gradient approximation (GGA) calculations were cross-checked with the modified Becke-Johnson (MBJ) potential calculations, appropriate for narrow gap materials. With the electronic and optical behavior around the Fermi level dominated by the topologically non-trivial bands, these newly found TMs candidates open wide possibilities for realizing the promise of TMs in next-generation electronic devices.

cond-mat.mes-hall↗

From spinon band topology to the symmetry quantum numbers of monopoles in Dirac spin liquids

The interplay of symmetry and topology has been at the forefront of recent progress in quantum matter. Here we uncover an unexpected connection between band topology and the description of competing orders in a quantum magnet. Specifically we show that aspects of band topology protected by crystalline symmetries determine key properties of the Dirac spin liquid (DSL) which can be defined on the honeycomb, square, triangular and kagomé lattices. At low energies, the DSL on all these lattices is described by an emergent Quantum Electrodynamics (QED$_3$) with $N_f=4$ flavors of Dirac fermions coupled to a $U(1)$ gauge field. However the symmetry properties of the magnetic monopoles, an important class of critical degrees of freedom, behave very differently on different lattices. In particular, we show that the lattice momentum and angular momentum of monopoles can be determined from the charge (or Wannier) centers of the corresponding spinon insulator. We also show that for DSLs on bipartite lattices, there always exists a monopole that transforms trivially under all microscopic symmetries owing to the existence of a parent SU(2) gauge theory. We connect our results to generalized Lieb-Schultz-Mattis theorems and also derive the time-reversal and reflection properties of monopoles. Our results indicate that recent insights into free fermion band topology can also guide the description of strongly correlated quantum matter.

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Superconductivity from Valley Fluctuations and Approximate SO(4) Symmetry in a Weak Coupling Theory of Twisted Bilayer Graphene

We develop a weak coupling approach to superconductivity in twisted bilayer graphene, starting from the Fermi liquid regime. A key observation is that near half filling, the fermiology consists of well nested Fermi pockets derived from opposite valleys, leading to enhanced valley fluctuation, which in turn can mediate superconductivity. This scenario is studied within the random phase approximation. We find that inter-valley electron pairing with either chiral ($d+i d$ mixed with $p-i p$) or helical form factor is the dominant instability. An approximate SO(4) spin-valley symmetry implies a near degeneracy of spin-singlet and triplet pairing. On increasing interactions, commensurate inter-valley coherence wave (IVCW) order can arise, with simultaneous condensation at the three M points in the Brillouin Zone, and a $2\times2$ pattern in real space. In simple treatments though, this leads to a full gap at fillings $\pm (1/2+1/8)$, slightly away from half-filling. An SO(4) symmetry breaking "anti-Hunds" coupling favors the spin-singlet order both for the IVCW and the superconductor, consistent with observations. Mott insulators derived from phase fluctuating superconductors are also discussed, which exhibit both symmetry protected and intrinsic topological orders.

cond-mat.str-el↗

Spin-polarized Correlated Insulator and Superconductor in Twisted Double Bilayer Graphene

Ferromagnetism and superconductivity typically compete with each other since the internal magnetic field generated in a magnet suppresses the formation of spin-singlet Cooper pairs in conventional superconductors. Only a handful of ferromagnetic superconductors are known in heavy fermion systems, where many-body electron interactions promoted by the narrow energy bands play a key role in stabilizing these emergent states. Recently, interaction-driven superconductivity and ferromagnetism have been demonstrated as separate phenomena in different density regimes of flat bands enabled by graphene moire superlattices. Combining superconductivity and magnetism in a single ground state may lead to more exotic quantum phases. Here, employing van der Waals heterostructures of twisted double bilayer graphene (TDBG), we realize a flat electron band that is tunable by perpendicular electric fields. Similar to the magic angle twisted bilayer graphene, TDBG exhibits energy gaps at the half and quarter filled flat bands, indicating the emergence of correlated insulating states. We find that the gaps of these insulating states increase with in-plane magnetic field, suggesting a ferromagnetic order. Upon doping the ferromagnetic half-filled insulator, superconductivity emerges with a critical temperature controlled by both density and electric fields. We observe that the in-plane magnetic field enhances the superconductivity in the low field regime, suggesting spin-polarized electron pairing. Spin-polarized superconducting states discovered in TDBG provide a new route to engineering interaction-driven topological superconductivity.

cond-mat.mes-hall↗

Stable Luttinger liquids and emergent $U(1)$ symmetry in constrained quantum chains

We explore the effect of local constraints on one-dimensional bosonic and fermionic ground state phases. Motivated by recent experiments on Rydberg chains, we constrain the occupation of neighboring sites in known phases of matter. Starting from Kitaev's topological superconductor wire, we find that a soft constraint induces a stable gapless Luttinger liquid phase. While Luttinger and Fermi liquids are usually unstable to superconducting proximity effects, the constraint suppresses pair creations, allowing for an emergent $U(1)$ symmetry and gaplessness. We substantiate this intuitive picture using field theoretical and Bethe ansatz methods. In particular, in the hard constraint limit, the model is explicitly $U(1)$-symmetric and integrable. For the corresponding spin-$1/2$ chains related by a Jordan-Wigner transformation, the Luttinger liquid is stabilized by the $\mathbb Z_2$ spin flip symmetry. Longer-range constraints stabilize gapless phases even without $\mathbb Z_2$ symmetry, connecting to the seminal work by Fendley, Sengupta and Sachdev [Physical Review B 69, 075106 (2004)], clarifying how the gapless floating phase observed therein can be vastly extended.

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Dynamical Signature of Fractionalization at the Deconfined Quantum Critical Point

Deconfined quantum critical points govern continuous quantum phase transitions at which fractionalized (deconfined) degrees of freedom emerge. Here we study dynamical signatures of the fractionalized excitations in a quantum magnet (the easy-plane J-Q model) that realize a deconfined quantum critical point with emergent O(4) symmetry. By means of large-scale quantum Monte Carlo simulations and stochastic analytic continuation of imaginary-time correlation functions, we obtain the dynamic spin structure factors in the $S^{x}$ and $S^{z}$ channels. In both channels, we observe broad continua that originate from the deconfined excitations. We further identify several distinct spectral features of the deconfined quantum critical point, including the lower edge of the continuum and its form factor on moving through the Brillouin Zone. We provide field-theoretical and lattice model calculations that explain the overall shapes of the computed spectra, which highlight the importance of interactions and gauge fluctuations to explaining the spectral-weight distribution. We make further comparisons with the conventional Landau O(2) transition in a different quantum magnet, at which no signatures of fractionalization are observed. The distinctive spectral signatures of the deconfined quantum critical point suggest the feasibility of its experimental detection in neutron scattering and nuclear magnetic resonance experiments.

cond-mat.str-el↗

Full Commuting Projector Hamiltonians of Interacting Symmetry-Protected Topological Phases of Fermions

Using the decorated domain wall procedure, we construct Finite Depth Local Unitaries (FDLUs) that realize Fermionic Symmetry-Protected Topological (SPT) phases. This results in explicit 'full' commuting projector Hamiltonians, where 'full' implies the fact that the ground state, as well as all excited states of these Hamiltonians, realizes the nontrivial SPT phase. We begin by constructing explicit examples of 1+1D phases protected by symmetry groups $G=\mathbb Z_2^T \times \mathbb Z_2^F$ , which also has a free fermion realization in class BDI, and $G=\mathbb Z_4 \times \mathbb Z_4^F$, which does not. We then turn to 2+1D, and construct the square roots of the Levin-Gu bosonic SPT phase, protected by $\mathbb Z_2 \times \mathbb Z_2^F$ symmetry, in a concrete model of fermions and spins on the triangular lattice. Edge states and the anomalous symmetry action on them are explicitly derived. Although this phase has a free fermion representation as two copies of $p+ip$ superconductors combined with their $p-ip$ counterparts with a different symmetry charge, the full set of commuting projectors is only realized in the strongly interacting version, which also implies that it admits a many-body localized realization.

cond-mat.str-el↗

Fragile Topology and Wannier Obstructions

Topological phases, such as Chern insulators, are defined in terms of additive indices that are stable against the addition of trivial degrees of freedom. Such topology presents an obstruction to any Wannier representation, namely, the representation of the electronic states in terms of symmetric, exponentially localized Wannier functions. Here, we address the converse question: Do obstructions to Wannier representation imply stable band topology? We answer this in the negative, pointing out that some bands can also display a distinct type of "fragile topology." Bands with fragile topology do not admit any Wannier representation by themselves, but such a representation becomes possible once certain additional trivial degrees of freedom are supplied. We construct a physical model of fragile topology on the honeycomb lattice that also helps resolve a recent puzzle in band theory. This model provides a counterexample to the assumption that splitting of an "elementary band representation" introduced in [Nature 547, 298--305 (2017)] leads to bands that are individually topological. Instead, half of the split bands of our model realizes a trivial band with exponentially localized symmetric Wannier functions, whereas the second half possess fragile topology. Our work highlights an important and previously overlooked connection between band structure and Wannier functions, and is expected to have far reaching consequences given the central role played by Wannier functions in the modeling of real materials.

cond-mat.mes-hall↗

Symmetry indicators and anomalous surface states of topological crystalline insulators

The rich variety of crystalline symmetries in solids leads to a plethora of topological crystalline insulators (TCIs) featuring distinct physical properties, which are conventionally understood in terms of bulk invariants specialized to the symmetries at hand. While isolated examples of TCI have been identified and studied, the same variety demands a unified theoretical framework. In this work, we show how the surfaces of TCIs can be analyzed within a general surface theory with multiple flavors of Dirac fermions, whose mass terms transform in specific ways under crystalline symmetries. We identify global obstructions to achieving a fully gapped surface, which typically lead to gapless domain walls on suitably chosen surface geometries. We perform this analysis for all 32 point groups, and subsequently for all 230 space groups, for spin-orbit-coupled electrons. We recover all previously discussed TCIs in this symmetry class, including those with "hinge" surface states. Finally, we make connections to the bulk band topology as diagnosed through symmetry-based indicators. We show that spin-orbit-coupled band insulators with nontrivial symmetry indicators are always accompanied by surface states that must be gapless somewhere on suitably chosen surfaces. We provide an explicit mapping between symmetry indicators, which can be readily calculated, and the characteristic surface states of the resulting TCIs.

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Operator spreading and the emergence of dissipative hydrodynamics under unitary evolution with conservation laws

We study the scrambling of local quantum information in chaotic many-body systems in the presence of a locally conserved quantity like charge or energy that moves diffusively. The interplay between conservation laws and scrambling sheds light on the mechanism by which unitary quantum dynamics, which is reversible, gives rise to diffusive hydrodynamics, which is a dissipative process. We obtain our results in a random quantum circuit model that is constrained to have a conservation law. We find that a generic spreading operator consists of two parts: (i) a conserved part which comprises the weight of the spreading operator on the local conserved densities, whose dynamics is described by diffusive charge spreading. This conserved part also acts as a source that steadily emits a flux of (ii) non-conserved operators. This emission leads to dissipation in the operator hydrodynamics, with the dissipative process being the conversion of operator weight from local conserved operators to nonconserved, at a rate set by the local diffusion current. The emitted nonconserved parts then spread ballistically at a butterfly speed, thus becoming highly nonlocal and hence essentially non-observable, thereby acting as the "reservoir" that facilitates the dissipation. In addition, we find that the nonconserved component develops a power law tail behind its leading ballistic front due to the slow dynamics of the conserved components. This implies that the out-of-time-order commutator (OTOC) between two initially separated operators grows sharply upon the arrival of the ballistic front but, in contrast to systems with no conservation laws, it develops a diffusive tail and approaches its asymptotic late-time value only as a power of time instead of exponentially. We also derive these results within an effective hydrodynamic description which contains multiple coupled diffusion equations.

cond-mat.stat-mech↗

Band Structure of Twisted Bilayer Graphene: Emergent Symmetries, Commensurate Approximants and Wannier Obstructions

A remarkable feature of the band structure of bilayer graphene at small twist angle is the appearance of isolated bands near neutrality, whose bandwidth can be reduced at certain magic angles (eg. $θ\sim 1.05^\circ$). In this regime, correlated insulating states and superconductivity have been experimentally observed. A microscopic description of these phenomena requires an understanding of universal aspects of the band structure, which we discuss here. First, we point out the importance of emergent symmetries, such as valley conservation, which are excellent symmetries in the limit of small twist angles and dictate qualitative features of the band structure. These have sometimes been overlooked when discussing commensurate approximants to the band structure, which we also review here, and solidify their connection with the continuum theory which incorporates all emergent symmetries. Finally, we discuss obstructions to writing down tight-binding models of just the isolated bands, and in particular a new symmetry based diagnostic of these obstructions, as well as relations to band topology and strategies for resolving the obstruction. Especially, we construct a four-band model where the two lower isolated bands realize all identified Wannier obstructions of the single-valley nearly flat bands of twisted bilayer graphene.

cond-mat.str-el↗

Origin of Magic Angles in Twisted Bilayer Graphene

Twisted Bilayer graphene (TBG) is known to feature isolated and relatively flat bands near charge neutrality, when tuned to special magic angles. However, different criteria for the magic angle such as the vanishing of Dirac speed, minimal bandwidth or maximal band gap to higher bands typically give different results. Here we study a modified continuum model for TBG which has an infinite sequence of magic angles $θ$ at which, we simultaneously find that (i) the Dirac speed vanishes (ii) absolutely flat bands appear at neutrality and (iii) bandgaps to the excited bands are maximized. When parameterized in terms of $α\sim 1/θ, $ they recur with the simple periodicity of $Δα\simeq 3/2$, which, beyond the first magic angle, differs from earlier calculations. Further, in this model we prove that the vanishing of the Dirac velocity ensures the exact flatness of the band and show that the flat band wave functions are related to doubly-periodic functions composed of ratios of theta functions. Also, using perturbation theory up to $α^8$ we capture important features of the first magic angle $θ\approx1.09^{\circ}$ ($α\approx 0.586$), which precisely explains the numerical results. Finally, based on our model we discuss the prospects for observing the second magic angle in TBG.

cond-mat.str-el↗