arXiv subjects

Ashwin A. Tulapurkar

Publications and source records attributed to Ashwin A. Tulapurkar.

11 recordsLinked to original sources

arXiv2026

Reciprocity of Charge-Orbital-Spin Transport in Normal-Metal/Ferromagnet Heterostructures

Orbital angular momentum has recently emerged as an important carrier of angular momentum in solids, offering new pathways for spin orbitronic functionality beyond conventional spin transport. Here, we investigate the orbital Hall effect which generates orbital torques and their reciprocal process viz orbital pumping and the inverse orbital Hall effect (iOHE) in non-magnet/ferromagnet heterostructures. Using two port scattering parameter measurements on Ru/Ni, Ru/Pt/CoFeB and Co/Cu/SiO2 devices, we directly probe both orbital torque driven magnetization dynamics and orbital pumping within the same device platform. We observe that the transmission coefficients satisfy the symmetry relations required by Onsager reciprocity, demonstrating reciprocal conversion between charge, orbital and spin angular momenta. Our results establish orbital pumping as the reciprocal counterpart of orbital torque. Our experimental findings provide a unified framework for orbital transport phenomena.

cond-mat.mes-hall↗

arXiv2025

Out-of-plane angle resolved second harmonic Hall analysis in perpendicular magnetic anisotropy systems

Spin orbit torques (SOT) are used to manipulate magnetization of ferromagnets in heavy metal / ferromagnetic bilayers and thus are technologically relevant from magnetization switching perspective. This necessitates development of methods which give an insight into SOT behaviour and enable SOT efficiency estimation. In this article, we demonstrate an experimental approach of out-of-plane (OOP) angle resolved Second Harmonic Hall (SHH) measurement, in Pt/Co and Ta/CoFeB perpendicular magnetic anisotropy (PMA) systems, for damping-like and field-like SOT efficiency estimation. This method reveals a unique anomalous field-like torque dependent on magnetization direction in Ta/CoFeB system. The damping-like and field-like SOT efficiencies are extracted by solving LLGS equation in the low frequency limit of magnetic susceptibility. Along with SHH measurements, we also experimentally demonstrate anomalous Hall effect (AHE) based spin-torque ferromagnetic resonance (STFMR) technique for SOT efficiency quantification in PMA systems.

cond-mat.mes-hall↗

arXiv2025

Gate Voltage-Controlled Magnetic Anisotropy Effect on Pt-Porphyrin functionalized single-layer graphene

We report a novel approach to engineering large voltage-controlled magnetic anisotropy (VCMA) and enhanced spin-orbit coupling (SOC) at the interface of single-layer graphene (SLG) and NiFe (Py) through non-covalent functionalization with Platinum (II) 5,10,15,20-tetraphenyl porphyrin (Pt-porphyrin). Using chemical vapor deposition (CVD)-grown SLG, we demonstrate that Pt-porphyrin functionalization significantly increases the SOC and enables robust voltage modulation of interfacial magnetic anisotropy, as confirmed by spin-torque ferromagnetic resonance (ST-FMR) measurements. A substantial VCMA coefficient of 375.6 (fJ/(V-m)) is achieved, accompanied by an order-of-magnitude enhancement in spin torque efficiency (θsh) compared to pristine SLG. The resonance field exhibits a clear, reversible shift under applied gate voltage, confirming robust electric-field modulation of interfacial magnetic anisotropy. Raman spectroscopy and X-ray photoelectron spectroscopy (XPS) confirm the structural integrity and effective charge transfer at the functionalized interface. Electrical characterization of back-gated graphene field-effect transistors (GFETs) further reveals tunable electronic properties upon functionalization. Our results establish functionalized graphene/ferromagnet interfaces as a promising platform for low-power, voltage-controlled spintronic devices, paving the way for scalable, energy-efficient memory and logic technologies

cond-mat.mes-hall↗

arXiv2025

Shape Anisotropy Enabled Field Free Switching of Perpendicular Nanomagnets

Spin Orbit Torque-Magnetic Random Access Memory (SOT-MRAM) is being developed as a successor to the Spin transfer torque MRAM (STT-MRAM) owing to its superior performance on the metrics of reliability and read-write speed. SOT switching of perpendicularly magnetized ferromagnet in the heavy metal/ferromagnet bilayer of SOT-MRAM unit cell requires an additional external magnetic field to support the spin-orbit torque generated by heavy metal to cause deterministic switching. This complexity can be overcome if an internal field can be generated to break the switching symmetry. We experimentally demonstrate that by engineering the shape of ferromagnet, an internal magnetic field capable of breaking the switching symmetry can be generated, which allows for deterministic switching by spin-orbit torques. We fabricated nanomagnets of Cobalt with triangular shape on top of Platinum and showed external magnetic field free switching between the two stable states of magnetization by application of nano-second voltage pulses. The experimental findings are consistent with the micro-magnetic simulation results of the proposed geometry.

cond-mat.mes-hall↗

arXiv2023

Effect of Edge Roughness on resistance and switching voltage of Magnetic Tunnel Junctions

We investigate the impact of edge roughness on the electrical transport properties of magnetic tunnel junctions using non-equilibrium Greens function formalism. We have modeled edge roughness as a stochastic variation in the cross-sectional profile of magnetic tunnel junction characterized by the stretched exponential decay of the correlation function. The stochastic variation in the shape and size changes the transverse energy mode profile and gives rise to the variations in the resistance and switching voltage of the magnetic tunnel junction. We find that the variations are larger as the magnetic tunnel junction size is scaled down due to the quantum confinement effect. A model is proposed for the efficient calculation of edge roughness effects by approximating the cross-sectional geometry to a circle with the same cross-sectional area. Further improvement can be obtained by approximating the cross-sectional area to an ellipse with an aspect ratio determined by the first transverse eigenvalue corresponding to the 2D cross section. These results would be useful for reliable design of the spin transfer torque-magnetic random access memory (STT-MRAM) with ultra-small magnetic tunnel junctions.

cond-mat.mes-hall↗

arXiv2021

Transmission based tomography for spin qubits

We consider a system of static spin qubits embedded in a one-dimensional spin coherent channel and develop a scheme to readout the state of one and two qubits separately. We use unpolarized flying qubits for this purpose that scatter off from the static qubits due to the Heisenberg exchange interaction. Analysing the transmission coefficient as a function of density matrix elements along with additional unitary gates we reconstruct the state of static qubits.

quant-ph↗

arXiv2020

Quantum state preparation of spin eigenstates including the Dicke states with generalized all-coupled interaction in a spintronic quantum computing architecture

There has been an extensive development in the use of multi-partite entanglement as a resource for various quantum information processing tasks. In this paper we focus on preparing arbitrary spin eigenstates whose subset contain important entangled resources like Dicke states as well as some other sub-radiant states that are difficult to prepare. Leveraging on the symmetry of these states we consider uniform pairwise exchange coupling between every pair of qubits. Starting from a product state of a given spin eigenstate with a single qubit state, another spin eigenstate can be prepared using simple time evolutions. This expansion paves a deterministic approach to prepare arbitrary Dicke states in linear steps. We discuss an improvement in this cost building up on a previous work for W states deterministic preparation in logarithmic circuit depth. The modified algorithm requires several iterations of pumping spin angular momentum into the system and is akin to the amplitude amplification in Grover search. As a use case to demonstrate the proposed scheme, we choose a system of non-interacting static spin qubits connected to a ferromagnetic reservoir. The flying qubits emerging from the reservoir locally interact with static qubits successively, mediating an in-direct exchange interaction between all the pairs.

quant-ph↗

arXiv2019

Generation of n-qubit W states using Spin Torque

We examine here a scheme to generate a W state of an n-qubit system with all-to-all pairwise exchange interaction between n qubits. This relies on sharing of superposed excitations of a smaller number of $q$ qubits among others. We present a bound on the maximal jumps from q to n and formalize a scheme to generate $W_n$ state in $\mathcal{O}(\log_4 n)$ stages. We demonstrate this scheme in the context of spin torque based quantum computing architecture that are characterized by repeated interactions between static and flying qubits.

quant-ph↗

arXiv2019

Investigation of the phase separation property in La$_{0.2}$Pr$_{0.4}$Ca$_{0.4}$MnO$_3$ manganite

We report a comprehensive investigation of La0.2Pr0.4Ca0.4MnO3 to clarify the micrometre scale phase separation phenomenon in the mixed valent manganite (La,Pr,Ca)MnO3. The compound shows multiple magnetic transitions, in which the charge-ordered state is converted into a ferromagnetic state in steps with the application of a magnetic field. The ac susceptibility measurements show that the glassy transition at low temperatures does not depend on the frequency, thus indicating the absence of any spin glass behaviour. Magnetization as well as heat capacity measurements indicate that this low temperature transition is magnetic field dependent. The field dependent resistivity at 2K shows a sharp drop indicating that the sample behaviour changes from a high resistive state to a low resistive state, corroborating the conversion of charge-ordered insulating (COI) phase to a ferromagnetic metallic (FMM) phase. Our results point towards the existence of phase separation, rigidity of the low temperature glassy-like phase as well as the conversion of COI phase to FMM phase by the application of magnetic fields.

cond-mat.mtrl-sci↗

arXiv2018

Control of magnetization dynamics by spin Nernst torque

Control of magnetization dynamics is one of the primary goals in spintronics. It has been demonstrated using spin Hall effect i.e charge current to spin current conversion in non-magnetic metal which has large spin-orbit coupling such as Pt, W etc. Recently different groups have shown generation of spin current in Pt, W while thermal gradient is created by virtue of spin Nernst effect. In this work we show the evidence of magnetization control by spin Nernst torque in Pt/Py bi-layer. We compared relative strength of spin Nernst Torque and spin Hall torque by measuring the systematic variation of magnetic linewidth on application of constant heat or charge current. Spin-torque ferromagnetic resonance (ST-FMR) technique is adopted to excite the magnet and to measure line-width precisely from the symmetric and anti-symmetric voltage component. Control of magnetization dynamics by spin Nernst torque will emerge as an alternative way to manipulate nano-magnets.

physics.app-ph↗

arXiv2017

Sign reversal of field like spin-orbit torque in ultrathin Chromium/Nickel bilayer

In this work report unconventional sign change of field like spin orbit torque in ultra-thin Chromium(1.5nm-5nm)/Nickel(8nm) bi-layer. We performed standard spin-torque ferromagnetic resonance (ST-FMR) experiment in Cr/Ni bi-layer by passing radio frequency current and measuring DC voltage. We observe that when thickness of Cr layer is critically low (<6nm) spin orbit torque by Cr on Ni significantly increases. Most importantly the sign of field like torque is opposite to the Oersted field generated torque. To verify interracial nature of this torque, 2 nm thin Cu is inserted between Cr and Ni and field like torque behaves same as Oersted field induced torque. Hence possible origin of such unconventional sign change of field like torque could be inter-facial Rashba like spin orbit interaction which is present between Cr and Ni but vanishes in Cr/Cu/Ni hetero-structure. From our experiment we can estimate that approximately 35 Oe of effective Rashba like magnetic field is created on 8 nm thicker Ni layer, when 1E12 A/m^2 current flows through Cr layer. All experiments are done at room temperature. So Cr thin film is expected to behave like paramagnet (Neel temperature of bulk Cr is 311K). Hence Cr can be a good choice as a heavy metal to employ large spin orbit torque combining bulk spin Hall effect and inter-facial Rashba interaction.

cond-mat.mes-hall↗