arXiv subjects

Ashwin K. Boddeti

Publications and source records attributed to Ashwin K. Boddeti.

7 recordsLinked to original sources

arXiv2026

Isotopically enriched epitaxial CaWO$_{4}$ thin films for Er$^{3+}$ spin-photon quantum interfaces

Rare earth ion (REI)-doped oxide thin films are attractive for the application of quantum interconnects due to their stable optical levels and scalability$^{1-3}$. Among them, Er$^{3+}$ doped CaWO$_{4}$ is promising because it possesses narrow optical linewidth transitions and a long spin coherence time$^{4-6}$. The electron spin coherence is limited at high temperatures by paramagnetic impurities and by the presence of the 14.3% $^{183}$W nuclear spin. To further increase the spin coherence time at millikelvin temperatures, where the paramagnetic impurities are frozen out, our approach is to synthesize chemically and isotopically purified thin films as a host material. We first grow non-isotopically enriched Er$^{3+}$ doped CaWO$_{4}$ thin films, which exhibit a 214(13) MHz photoluminescence (PL) inhomogeneous linewidth, indicating the thin film has high crystalline quality. We then grow isotopically enriched CaWO$_{4}$ thin films using an isotopically purified $^{186}$WO$_{3}$ source. Time of flight secondary ion mass spectrometry (ToF-SIMS) was used to measure the relative concentration of W isotopes. $^{183}$W, the only W isotope that has a net nuclear spin and is the major cause of spin decoherence, was at a relative abundance of 1.2%, a factor of 10 lower than natural abundance. We also observed PL emission from single ions after integrating nano-photonic devices with the thin film. These results establish isotopically engineered CaWO$_{4}$ thin films as a promising platform for future studies of nuclear-spin-limited coherence and for scalable rare-earth-ion-based quantum nanophotonic devices.

quant-ph↗

arXiv2025

Coherent control of interacting solid-state spins below the diffraction limit

Optically addressed atomic defects in the solid-state are widely used as single-photon sources and memories for quantum network applications. The solid-state environment allows for a high density of electron and nuclear spins with the potential to form registers for coherent information processing. However, it is challenging to reliably address individual spins at nanometer separations where interactions are large. Rare-earth ions offer a unique solution, as their narrow homogeneous optical linewidth allows frequency-domain resolution of a large number of emitters without regard to their spatial separation. In this work, we realize coherent optical and spin control of a pair of interacting Er$^{3+}$ ions, together with a nearby nuclear spin ancilla. We demonstrate two-qubit electron-electron gates and use them to perform repeated quantum non-demolition measurements on one of the Er$^{3+}$ ions. We also demonstrate electron-nuclear gates to allow coherent storage and retrieval of qubit information in a nuclear spin, and show that the nuclear spin coherence survives readout of the electron spin. These techniques can be readily scaled to larger numbers of electron and nuclear spins, paving the way for massively multiplexed quantum network nodes.

quant-ph↗

arXiv2024

Reducing system dimensionality with long-range collective dipole-dipole interactions

Dimensionality plays a crucial role in long-range dipole-dipole interactions (DDIs). We demonstrate that a resonant nanophotonic structure modifies the apparent dimensionality in an interacting ensemble of emitters, as revealed by population decay dynamics. Our measurements on a dense ensemble of interacting quantum emitters in a resonant nanophotonic structure with long-range DDIs reveal an effective dimensionality reduction to $\bar{d} = 2.20 (12)$, despite the emitters being distributed in 3D. This contrasts the homogeneous environment, where the apparent dimension is $\bar{d} = 3.00$. Our work presents a promising avenue to manipulate dimensionality in an ensemble of interacting emitters.

physics.optics↗

arXiv2024

Computational Kerr-Ellipsometry: Quantifying Broadband Optical Nonreciprocity of Magneto-Optic Materials

Characterizing the optical response of magneto-optic and magnetic materials usually relies on semi-classical models (e.g. Lorentz oscillator model) involving few parameters or models based on a detailed quantum mechanical description of the underlying response. These models typically involve a few parameters that are estimated via fitting the experimental data to provide a qualitative understanding of the underlying physics. Such a few-parameters fitting approach falls short of accurately capturing all elements of the complex-valued permittivity tensor across a range of wavelengths. Accurate characterization of the permittivity tensor elements across a broad range of wavelengths is invariably imperative for designing optical elements such as isolators, circulators, etc. Here, we propose and demonstrate a ubiquitous and accessible method based on a combination of spectroscopic ellipsometry and spectroscopic Magneto-Optic Kerr Effect (MOKE) measurements coupled with rigorous numerical parameter extraction techniques. To this end, we use the combined MOKE ellipsometry measurements conducted at different angles of incidence with a gradient-descent minimization algorithm to provide the inverse solution to the complete dielectric permittivity tensor. Further, we demonstrate model re-verification to ensure the estimated dielectric permittivity values reliably predict the measured experimental data. Our method is a simplified bench-top counterpart to the otherwise complex measurement systems.

physics.optics↗

arXiv2023

Optical N-plasmon: Topological hydrodynamic excitations in Graphene from repulsive Hall viscosity

Edge states occurring in Chern and quantum spin-Hall phases are signatures of the topological electronic band structure in two-dimensional (2D) materials. Recently, a new topological electromagnetic phase of graphene characterized by the optical N-invariant has been proposed. Optical N-invariant arises from repulsive Hall viscosity in hydrodynamic many-body electron systems, fundamentally different from the Chern and Z2 invariants. In this paper, we introduce the topologically protected edge excitation -- optical N-plasmon of interacting many-body electron systems in the topological optical N-phase. These optical N-plasmons are signatures of the topological plasmonic band structure in 2D materials. We demonstrate that optical N-plasmons exhibit fundamentally different dispersion relations, stability, and edge profiles from the topologically trivial edge magneto plasmons. Based on the optical N-plasmon, we design an ultra sub-wavelength broadband topological hydrodynamic circulator, which is a chiral quantum radio-frequency circuit component crucial for information routing and interfacing quantum-classical computing systems. Furthermore, we reveal that optical N-plasmons can be effectively tuned by the neighboring dielectric environment without breaking the topological properties. Our work provides a smoking gun signature of repulsive Hall viscosity and opens practical applications of topological electromagnetic phases of two-dimensional materials.

cond-mat.mes-hall↗

arXiv2022

Nonequilibrium Hanbury-Brown-Twiss experiment: Theory and application to binary stars

Intensity-interferometry based on Hanbury-Brown and Twiss's seminal experiment for determining the radius of the star Sirius formed the basis for developing the quantum theory of light. To date, the principle of this experiment is used in various forms across different fields of quantum optics, imaging and astronomy. Though, the technique is powerful, it has not been generalized for objects at different temperatures. Here, we address this problem using a generating functional formalism by employing the P-function representation of quantum-thermal light. Specifically, we investigate the photon coincidences of a system of two extended objects at different temperature using this theoretical framework. We show two unique aspects in the second-order quantum coherence function - interference oscillations and a long-baseline asymptotic value that depends on the observation frequency, temperatures and size of both objects. We apply our approach to the case of binary stars and discuss the advantages of measuring these two features in an experiment. In addition to the estimation of the radii of each star and the distance between them, we also show that the present approach is suitable for the estimation of temperatures as well. To this end, we apply it to the practical case of binary stars Luhman 16 and Spica $α$ Vir. We find that for currently available telescopes, an experimental demonstration is feasible in the near term. Our work contributes to the fundamental understanding of intensity interferometry of quantum-thermal light and can be used as a tool for studying two-body thermal emitters - from binary stars to extended objects.

quant-ph↗

arXiv2019

Spectral domain inverse design for accelerating nanocomposite metamaterials discovery

Inverse design techniques in the context of nanophotonics have helped in discovery of compact and counter-intuitive structures/shapes. We introduce the concept of spectral domain inverse design to search through the optical trade-space (dispersive permittivity) of nanocomposite metamaterials. We develop a hybrid optimization technique that combines genetic algorithms and gradient descent methods. We utilize this technique to inverse design an ultra-thin thermophotovoltaic emitter coating material. Our work can lead to an efficient approach to search for new multi-functional optical/thermal metamaterials with desired complex permittivity.

physics.optics↗