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Atsushi Miyake

Publications and source records attributed to Atsushi Miyake.

At least 19 recordsLinked to original sources

Discriminating superconducting fluctuations from the pseudogap in Bi$_2$Sr$_2$Ca$_{n-1}$Cu$_n$O$_{2n+4+δ} (n = 2,3)$: A magnetotransport study

Understanding the normal state is essential for uncovering the mechanism of high-$T_c$ superconductivity. We investigate magnetotransport in Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ and Bi$_2$Sr$_2$Ca$_2$Cu$_3$O$_{10+δ}$ single crystals over a wide doping range. While the in-plane resistivity and Hall coefficient show strong pseudogap-induced temperature dependence, the $T^2$ Hall-angle behavior and the modified Kohler's rule remain robust across all dopings. The onset temperatures of the pseudogap are clearly distinct from superconducting fluctuations, although they scale with the pseudogap magnitudes with a factor consistent with a $d$-wave superconductor. These results demonstrate that the pseudogap does not arise from superconducting fluctuations and instead suggest that it may originate from preformed Cooper pairing in the BCS-BEC crossover regime.

cond-mat.supr-con

Search for magnetoacoustic quantum oscillations in the insulating phase of YbB$_{12}$

A highly exotic phenomenon in solid-state physics is the observation of magnetic quantum oscillations in insulators. For instance, in the Kondo insulator YbB$_{12}$ various groups reported the observation of such oscillations seemingly originating from Fermi surfaces, though this contradicts the concept of an insulator having no charged quasiparticles. In this study, we searched for quantum oscillations in YbB$_{12}$ by using bulk-sensitive ultrasonic experiments in high magnetic fields up to 65 T and down to 485 mK. For that, we utilized an YbB$_{12}$ single crystal that, in previous experiments, revealed oscillations in the magnetoresistance in the insulating state. We confirmed oscillation-like behavior of the magnetoresistance as well as field-dependent oscillations in the magnetocaloric effect. However, we could not observe magnetoacoustic quantum oscillations in the insulating state, only in the field-induced metallic state. In the insulating state, we found some anomalies in our ultrasound data, the origin of which remains elusive. Our findings provide further information on the puzzling behavior of the insulating state of YbB$_{12}$.

cond-mat.str-el

Electron-Hole Scattering Dichotomy and Anisotropic Warping in Quasi-Two-Dimensional Fermi Surfaces of UTe2

We present a combined experimental and theoretical study of the detailed Fermi-surface (FS) geometry of UTe2, a heavy-fermion superconductor that has recently attracted considerable attention as a promising candidate for spin-triplet pairing. Using angle-dependent magnetoresistance oscillations, a bulk- and low-energy-sensitive transport probe for quasi-two-dimensional (Q2D) electronic structures, we directly determine the in-plane FS geometry. We found that the Q2D FS exhibits a rectangular cross-sectional shape with strongly anisotropic warping, originating from the hybridization of two orthogonal quasi-one-dimensional bands. Through a quantitative comparison between experiment and theoretical calculations, we further reveal a large electron-hole scattering dichotomy: the quasiparticle lifetime on the electron FS is substantially shorter than that on the hole FS. This dichotomy is naturally explained by anisotropic, low-dimensional antiferromagnetic fluctuations, which selectively enhance scattering on the electron FS. This suggests a dominant role of the electron pockets for the emergence of superconductivity. Our results clarify a direct relation between FS geometry, magnetic fluctuations, and momentum-dependent quasiparticle lifetimes, and thus providing a crucial basis for the microscopic understanding of pairing mechanism, and impose stringent constraints on the gap symmetry of spin-triplet superconductivity in UTe2.

cond-mat.supr-con

Hall effect on nontrivial quadrupole order in quasi-kagome compound URhSn

This study focuses on the transport properties of the quasi-kagome compound URhSn, which exhibits successive phase transitions at TC =16 K (ferromagnetic phase) and TO =54 K (intermediate phase). A large anomalous Hall component is present along the easy-magnetization axis (H|| [0001]), and the Hall resistivity shows very complex temperature- and field-dependence, with a sign reversal at low temperatures. The Hall resistivity exhibits a nonlinear and unusual field-dependence. Interestingly, there exists an unusual Hall component that is not proportional to the magnetic susceptibility for H || [0001] in both the intermediate and ferromagnetic states. These results reveal unconventional transport properties of URhSn, providing important insights into nontrivial multipolar phases in 5f- electron systems.

cond-mat.str-el

Nodal Superconductivity of UTe$_2$ Probed by Field-Angle-Resolved Specific Heat on a Crystal with $T_{\rm c}=2.1$ K

Field-angle-resolved specific-heat measurements were performed on a clean single crystal of a spin-triplet superconductor UTe$_2$ with $T_{\rm c}=2.1$ K and a low residual electronic specific heat. At low temperatures, the specific heat exhibits a linear dependence on the magnetic field when the field is applied precisely along the $b$ axis, in stark contrast to its rapid increase at low fields for other orientations. This pronounced anisotropy suggests the presence of nodal quasiparticle excitations with the Fermi velocity predominantly aligned along the $b$ axis. Considering the characteristic field-angle dependences of both the specific heat and the upper critical field, these observations are broadly compatible with theoretical models that assume a superconducting gap structure featuring either point nodes consistent with $B_{\rm 2u}$ symmetry, allowed in the infinitely strong spin-orbit coupling scheme, or line nodes confined to flat regions of the quasi-two-dimensional Fermi surface, consistent with $^3B_{\rm 3u}$ symmetry in the finite spin-orbit classification scheme. These results yield crucial hints for resolving the pairing symmetry of UTe$_2$, paving the way for a deeper understanding of its spin-triplet superconductivity.

cond-mat.supr-con

Intimate relationship between spin configuration in the triplet pair and superconductivity in UTe$_2$

Spin-triplet superconductivity is an intriguing quantum coherent state with both spin and orbital degrees of freedom, which holds significant potential for future applications in quantum technology. However, how the spin of the triplet pairs responds to an external magnetic field remains poorly understood. This is mainly due to the absence of suitable spin-triplet superconductors. Here, we report results of Knight-shift and ac-susceptibility measurements on UTe$_2$. We demonstrate that the spin susceptibility, which slightly decreases compared to the normal-state value below the superconducting (SC) transition temperature $T_{\rm c}$, is rapidly restored and nearly recovers to the normal-state values around 5 T, well below the SC upper critical field $H_{c2}$ when the magnetic field is applied along the $c$ axis ($H \parallel c$). In addition, we found that $H_{\rm c2}$ of superconductivity becomes larger when the SC spin aligns with the magnetic field. By considering the results on $H \parallel b$, our results suggest the presence of a close relationship between the spin configuration of the triplet pair and $H_{\rm c2}$, as well as the anisotropic pinning interaction acting on the triplet pairs. These phenomena, which have never been observed in spin-singlet superconductors, represent characteristic features unique to spin-triplet superconductors. We discuss the similarities between superconductivity in UTe$_2$ and superfluid $^3$He, focusing on their spin-triplet pairing states.

cond-mat.supr-con

Ultrasonic observation of small Fermi surfaces in La$T$In$_5$ ($T$ = Co, Rh, Ir)

We performed high-field ultrasonic measurements on La$T$In$_5$ ($T$ = Co, Rh, Ir) to reveal the origin of the small Fermi surface that was recently observed in LaRhIn$_5$ with an oscillation frequency of 6.8 T. We observed quantum oscillations originating from this Fermi surface in LaRhIn$_5$. In addition, we revealed that LaCoIn$_5$ and LaIrIn$_5$ exhibit quantum osciilations with frequencies below 100 T, indicating hidden Fermi surfaces in these compounds. Furthermore, Co-substituted LaRhIn$_5$ exhibited quantum oscillations with a frequency of 10 T. Our results suggest that the small Fermi surface originates from bulk properties and that $3d$ electrons of the transition metal contribute to its formation.

cond-mat.str-el

$b$-axis and $c$-axis Knight shift measurements in the superconducting state on ultraclean UTe$_2$ with $T_c$ = 2.1 K

Knight shifts along the $b$ and $c$ axes ($K_b$ and $K_c$) at two crystallographically distinct Te sites were measured down to 70 mK using $^{125}$Te nuclear magnetic resonance (NMR) on an ultraclean UTe$_2$ single crystal with a superconducting (SC) transition temperature $T_{\mathrm{c}}$ = 2.1 K. This was carried out to determine the $\boldsymbol{d}$-vector components, which are the order parameter in the spin-triplet pairing. Although the decrease in $K_b$ and $K_c$ is comparable to the theoretical estimation of the SC diamagnetic shielding effect, it is confirmed, by taking the difference between two Knight shifts at the distinct Te sites, that the spin susceptibility along the $b$ and $c$ axes decreases in the SC state. Taking into account the large decrease in $K_a$ in the SC state, we conclude that the $\boldsymbol{d}$ vector has components along all three crystal axes.

cond-mat.supr-con

Novel Easy-Axis Switching through Metamagnetism in CeSb$_2$

A novel magnetic field-induced switching of the magnetization easy axis has been discovered in the layered compound CeSb$_2$, which crystallizes in an orthorhombic structure with nearly identical lattice constants along the a- and b-axes, giving it a tetragonal-like appearance. When a magnetic field is applied along an orthorhombic in-plane axis at 4.2 K, magnetization increases abruptly around 34 T, followed by a hysteresis loop upon decreasing the field. Subsequent measurements reveal a significantly enhanced magnetization, indicative of a switch of the magnetization easy axis. Conversely, the other orthorhombic in-plane axis becomes the magnetization hard axis. Surprisingly, the easy axis is switchable by changing the field direction to the other orthorhombic in-plane axis. Moreover, this memory effect is stable up to room temperature. Polarized light microscope images have visually revealed domain formation of the as-cast samples and domain rearrangement by magnetic fields. This intriguing axis-conversion phenomenon is a novel magnetic shape memory effect for heat cycles up to room temperature. It is attributed to the specific in-plane Ce-pantograph networks in CeSb$_2$.

cond-mat.str-el

Intrinsic low-temperature magnetic properties on the ultra-clean UTe$_2$ with $T_{\rm c}$ = 2.1 K revealed by $^{125}$Te NMR

To investigate the intrinsic magnetic properties of UTe$_2$, we performed $^{125}$Te-NMR measurements on the ultra-clean single-crystalline UTe$_2$ with superconducting transition temperature $T_{\rm c}$ = 2.1~K and compared the results with those of the $T_{\rm c}$ = 1.6~K sample. The broadening of the linewidth of the NMR spectrum in the $a$-axis magnetic field and the low-temperature magnetic fluctuations observed in the 1.6~K sample are suppressed in the ultra-clean sample, indicating that such magnetic properties originate from a tiny amount of U deficiency. The present results suggest that the magnetic properties in UTe$_2$ are sensitive to the U deficiency. We also observed a peculiar angular dependence of the NMR quantities due to large magnetic anisotropy with the $a$-axis as the magnetic easy axis.

cond-mat.supr-con

Clear Reduction in Spin Susceptibility and Superconducting Spin Rotation for $H \parallel a$ in the Early-Stage Sample of Spin-Triplet Superconductor UTe$_2$

We report the re-measurement of the $a$-axis spin susceptibility component in an early-stage sample of the spin-triplet superconductor UTe$_2$ with the transition temperature of $T_{\rm SC}$ = 1.6 K. Using Knight-shift measurements along the $b$ axis and at a 10-degree tilt from the $b$ axis towards the $a$ axis, we accurately determined the $a$-axis component without directly measuring the $a$-axis Knight shift. Our results reveal a decrease of approximately 3\% in the $a$-axis spin susceptibility in the superconducting state under $a$-axis magnetic field $μ_0 H_a \sim 0.1$ T, indicating that the spin susceptibility decreases similarly in both early-stage and ultraclean samples with $T_{\rm SC}$ = 2.1 K. The previously reported absence of the reduction in Knight shift is attributed to the missing of signal from the superconducting region and to the detection of residual signals from the non-superconducting region instead. We also found that the decrease in the $a$-axis spin susceptibility is immediately suppressed with increasing the $a$-axis magnetic field and is estimated to be completely suppressed at around 1.5 T due to superconducting spin rotation.

cond-mat.supr-con

Nernst effect of high-mobility Weyl electrons in NdAlSi enhanced by a Fermi surface nesting instability

The thermoelectric Nernst effect of solids converts heat flow to beneficial electronic voltages. Here, using a correlated topological semimetal with high carrier mobility $μ$ in presence of magnetic fluctuations, we demonstrate an enhancement of the Nernst effect close to a magnetic phase transition. A magnetic instability in NdAlSi modifies the carrier relaxation time on 'hotspots' in momentum space, causing a strong band filling dependence of $μ$. We quantitatively derive electronic band parameters from a novel two-band analysis of the Nernst effect $S_{xy}$, in good agreement with quantum oscillation measurements and band calculations. While the Nernst response of NdAlSi behaves much like conventional semimetals at high temperatures, an additional contribution $ΔS_{xy}$ from electronic correlations appears just above the magnetic transition. Our work demonstrates the engineering of the relaxation time, or the momentum-dependent self energy, to generate a large Nernst response independent of a material's carrier density, i.e. for metals, semimetals, and semiconductors with large $μ$.

cond-mat.mtrl-sci

Quantum liquid states of spin solitons in a ferroelectric spin-Peierls state

In this study, we performed high-magnetic-field magnetization, dielectric, and ultrasound measurements on an organic salt showing a ferroelectric spin-Peierls (FSP) state, which is in close proximity to a quantum critical point. In contrast to the sparsely distributed gas-like spin solitons typically observed in conventional spin-Peierls (SP) states, the FSP state exhibits dense liquid-like spin solitons resulting from strong quantum fluctuations, even at low fields. Nevertheless, akin to conventional SP systems, a magnetic-field-induced transition is observed in the FSP state. In conventional high-field SP states, an emergent wave vector results in the formation of a spin-soliton lattice. However, in the present high-field FSP state, the strong quantum fluctuations preclude the formation of such a soliton lattice, causing the dense solitons to remain in a quantum-mechanically melted state. This observation implies the realization of a quantum liquid--liquid transition of topological particles carrying spin and charge in a ferroelectric insulator.

cond-mat.str-el

High-field phase diagram of the chiral-lattice antiferromagnet Sr(TiO)Cu4(PO4)4

High-field phase diagram of a chiral-lattice antiferromagnet Sr(TiO)Cu4(PO4)4 is studied by means of the ultrasound, dielectric, and magnetocaloric-effect measurements. These experimental techniques reveal two new phase transitions at high fields, which have not been resolved by the previous magnetization experiments. Specifically, the c66 acoustic mode shows drastic changes with hysteresis with applied fields along the c axis, indicating a strong magneto-elastic coupling. Combined with the cluster mean-field theory, we discuss the origins of these phase transitions. By considering the chiral-twist effect of Cu4O12 cupola units, which is inherent to the chiral crystal structure, the phase diagram is reasonably reproduced. The agreement between the experiment and theory suggests that this material is a unique quasi two-dimensional spin system with competing exchange interactions and chirality, leading to the rich phase diagram.

cond-mat.str-el

Multiple Magnetoelectric Plateaux in Polar Magnet Fe$_2$Mo$_3$O$_8$

The magnetization and electric polarization of a polar antiferromagnet Fe$_2$Mo$_3$O$_8$ are studied up to 66 T for spin-saturation magnetic fields applied along the polar axis. The magnetization process at 1.4 K exhibited multistep structures below the saturation field of 65 T. The electric polarization along the polar axis exhibits a similar multistep behavior with a total change of 1.2 $\rmμC/cm^{2}$. A combined triangular-lattice antiferromagnetic model with strong Ising-type spin anisotropy reproduces this multistep magnetoelectric (ME) effect. The exchange striction mechanism explains the remarkable ME response in the two sub-lattice type-I multiferroic materials. These results and interpretation demonstrate a method for realizing multistage magnetoelectric effects in hybrid spin systems.

cond-mat.str-el

Low-temperature hysteresis broadening emerging from domain-wall creep dynamics in a two-phase competing system

Hysteretic behaviour accompanies any first-order phase transition, forming a basis for many applications. However, its quantitative understanding remains challenging, and even a qualitative understanding of pronounced hysteresis broadening at low temperature, which is often observed in magnetic-field-induced first-order phase transition materials, is unclear. Here, we show that such pronounced hysteresis broadening emerges if the phase-front velocity during the first-order phase transition exhibits an activated behaviour as a function of both temperature and magnetic field. This is demonstrated by using real-space magnetic imaging techniques, for the magnetic-field-induced first-order phase transition between antiferromagnetic and ferrimagnetic phases in (Fe$_{0.95}$Zn$_{0.05}$)$_{2}$Mo$_{3}$O$_{8}$. When combined with the Kolmogorov-Avrami-Ishibashi model, the observed activated temperature- and field-dependences of the growth velocity of the emerging antiferromagnetic domain quantitatively reproduce the pronounced hysteresis broadening. Furthermore, the same approach also reproduces the field-sweep-rate dependence of the transition field observed in the experiment. Our findings thus provide a quantitative and comprehensive understanding of pronounced hysteresis broadening from the microscopic perspective of domain growth.

cond-mat.mtrl-sci

Possible helimagnetic order in Co4+-containing perovskites Sr1-xCaxCoO3

We systematically synthesized perovskite-type oxides Sr1-xCaxCoO3 containing unusually high valence Co4+ ions by a high pressure technique, and investigated the effect of systematic lattice change on the magnetic and electronic properties. As the Ca content x exceeds about 0.6, the structure changes from cubic to orthorhombic, which is supported by the first-principles calculations of enthalpy. Upon the orthorhombic distortion, the ground state remains to be apparently ferromagnetic with a slight drop of the Curie temperature. Importantly, the compounds with x larger than 0.8 show antiferromagnetic behavior with positive Weiss temperatures and nonlinear magnetization curves at lowest temperature, implying that the ground state is noncollinear antiferromagnetic or helimagnetic. Considering the incoherent metallic behavior and the suppression of the electronic specific heat at high x region, the possible emergence of a helimagnetic state in Sr1-xCaxCoO3 is discussed in terms of the band-width narrowing and the double-exchange mechanism with the negative charge transfer energy as well as the spin frustration owing to the next-nearest neighbor interaction.

cond-mat.mtrl-sci

High-Field Ultrasonic Study of CeIrIn$_5$

We performed ultrasonic and temperature measurements under pulsed magnetic fields on CeIrIn$_5$ to investigate whether or not the origin of metamagnetic transition and field-induced Lifshitz transition was described by the anisotropic electronic ordering with crystal symmetry breaking. We observed elastic anomalies with the negative magnetocaloric effects around the field-induced Lifshitz transition and the metamagnetic transition. On the other hand, the elastic anomalies appeared both in the transverse elastic constants $(C_{11} - C_{12})/2$ and $C_{66}$ in CeIrIn$_5$ while $(C_{11} - C_{12})/2$ showed significant elastic anomaly at the crystal symmetry breaking fields in CeRhIn$_5$. These results indicate that the anisotropic electronic ordering with crystal symmetry breaking is absent in high-magnetic fields in CeIrIn$_{5}$.

cond-mat.str-el