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Audrey Ngambia

Publications and source records attributed to Audrey Ngambia.

3 recordsLinked to original sources

What makes a useful molecular model of biochar? A community roadmap

Biochars are disordered carbonaceous materials produced by biomass pyrolysis, with applications spanning soil amendment, water remediation, carbon storage, and functional materials. Although they share structural features with other disordered carbons such as coal, kerogen, and activated carbons, the questions posed to biochar models are distinct, and no single model can answer all of them equally well. Model usefulness must be defined relative to a specific question and validated against independent experimental observables. This community roadmap, arising from a CECAM workshop, critically maps current molecular approaches: experimentally guided top-down reconstruction, mimetic bottom-up simulation, and hybrid methods. We argue that first-generation models have been more successful than is often acknowledged, provided they are built at sufficient length scale and with explicit control over microporosity and bulk chemistry. Structural and equilibrium interfacial properties are increasingly tractable with classical force fields, whereas dynamic and reactive behaviours require selective use of reactive methods within multiscale workflows. A parallel, largely unaddressed gap concerns the mineral and ash components of biochar, and the changes the material undergoes during ageing in soil. We identify seven open questions current models cannot yet answer reliably, and five community priorities: force field benchmarking, open model and data repositories, shared classification and metadata standards, ensemble validation, and training in reproducible practice. Across these, sustained interaction with experimentalists is essential to ground models in real observables and document where they fail. Progress will be accelerated by adapting transferable methods from coal, kerogen, and clay-organic matter frameworks rather than repeating trial-and-error development.

cond-mat.mtrl-sci

Decoupling Precipitation and Surface Complexation during Mn(II) Removal by Biochar via Experiments and Atomistic Simulations

Manganese(II) mobilised by mining activity poses a persistent water-quality challenge, yet the mechanisms by which low-cost sorbents, such as biochar, sequester Mn(II) remain poorly resolved. This study identifies the specific chemical drivers of Mn(II) sequestration by combining fixed-bed column and batch experiments with atomistic molecular dynamics simulations. Oilseed rape straw biochars, produced at 350\textdegree C, 550\textdegree C, and 700\textdegree C, removed 20-50% of dissolved Mn from acidic influent (pH 4, 5 ppm). High-temperature biochar achieved the greatest removal ($\sim$50%) and rapidly increased effluent pH to 9, triggering alkaline precipitation. Conversely, lower-temperature biochars removed 20-30% of Mn while maintaining a near-neutral pH (7-7.5). Enhanced \ce{K+} release in these systems indicates significant cation exchange and non-precipitative pathways. Molecular simulations confirmed that while neutral surfaces show weak Mn(II) association, deprotonated sites drive strong adsorption through inner-sphere complexation ($\sim$50% removal) and outer-sphere association ($\sim$10%). These results establish a mechanistic framework to distinguish between precipitation-led and surface-complexation-led removal. By providing specific chemical criteria for Mn-targeted sequestration, this work enables the rational design of engineered biochars for sustainable water remediation.

cond-mat.mtrl-sci

Development of biochar molecular models with controlled porosity

Biochars are an exciting class of environmental materials with a wide range of applications, including carbon storage and sequestration, soil enhancement, and pollution remediation. However, the limited knowledge of their molecular structures and compositions and the lack of comprehensive understanding of the relationship between these structures and biochars' diverse functionality, is hindering advancements in their development. In this work, we further advance the approach, first introduced by Wood et al. (2023), to constructing biochar molecular models; and now include control of microporosity (pores < 2 nm size) within the developed models. We construct biochar models representative of woody biochars which are experimentally produced at 600 -- 650 oC highest heating temperatures. Our models reproduce experimental H/C and O/C atomic ratios, percentage aromatic carbon, true density, cumulative porosity, and pore size distribution. The development of microporous biochar molecular models allows us to identify the importance of chemical structures involved in the assembly of biochar materials, and describe the relationship between these structures and obtained micropores. To facilitate other researchers integrating our approach into their work, we detail the steps taken, including the tests and reasons for each decision, in the construction of the biochar models. Furthermore, we share our developed molecular models in a format that can be easily integrated into other group's work in the form of molecular dynamics simulations.

cond-mat.mtrl-sci