arXiv subjects

Avraham Schiller

Publications and source records attributed to Avraham Schiller.

At least 19 recordsLinked to original sources

arXiv2016

Transient probing of the symmetry and the asymmetry of electron interference

The transient processes of electron transport in nano-scale devices exhibit special phenomena that exist only in the transient regime. Besides how fast the steady states are approached, one interesting aspect of transient transport arises from its strong dependence on the initial state of the system. Here we address the issue of how the symmetries embedded in the initial state interplay with those of the system structure in the course of transient transports. We explicitly explore the transient currents arising from various initial occupations in a double-quantum-dot Aharonov-Bohm interferometer. We find symmetry relations between the transient in-tunneling and out-tunneling dynamics for initially empty or full quantum dots when the energy levels in the electrodes are symmetrically distributed with respect to the energy levels in the QDs. This is true for whatever applied fluxes. We also find the flux-even components of the currents and the flux-odd components of the currents exhibit distinct cross-lead symmetric relations.

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arXiv2014

From thermal equilibrium to nonequilibrium quench dynamics: A conserving approximation for the interacting resonant level

We develop a low-order conserving approximation for the interacting resonant-level model (IRLM), and apply it to (i) thermal equilibrium, (ii) nonequilibrium steady state, and (iii) nonequilibrium quench dynamics. Thermal equilibrium is first used to carefully gauge the quality of the approximation by comparing the results with other well-studied methods, and finding good agreement for small values of the interaction. We analytically show that the power-law exponent of the renormalized level width usually derived using renormalization group approaches can also be correctly obtained in our approach in the weak interaction limit. A closed expression for the nonequilibrium steady-state current is derived and analytically and numerically evaluated. We find a negative differential conductance at large voltages, and the exponent of the power-law suppression of the steady-state current is calculated analytically at zero-temperature. The response of the system to quenches is investigated for a single-lead as well as for two-lead setup at finite voltage bias at particle-hole symmetry using a self-consistent two-times Keldysh Green function approach, and results are presented for the time-dependent current for different bias and contact interaction strength.

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arXiv2014

Single-molecule-mediated heat current between an electronic and a bosonic bath

In molecular devices electronic degrees of freedom are coupled to vibrational modes of the molecule, offering an opportunity to study fundamental aspects of this coupling between at the nanoscale. To this end we consider the nonequilibrium heat exchange between a conduction band and a bosonic bath mediated by a single molecule. For molecules large enough so that on-site interactions can be dropped we carry out an asymptotically exact calculation of the heat current, governed by the smallness of the electron-phonon coupling, and obtain the steady state heat current driven by a finite temperature drop. At low temperatures the heat current is found to have a power-law behavior with respect to the temperature difference with the power depending on the nature of the bosonic bath. At high temperatures, on the other hand, the current is linear in the temperature difference for all types of bosonic baths. The crossover between these behaviors is described. Some of the results are given a physical explanation by comparing to a perturbative Master equation calculation (whose limitation we examine).

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arXiv2013

Crossover from adiabatic to antiadiabatic phonon-assisted tunneling in single-molecule transistors

The crossover between two customary limits of phonon-assisted tunneling, the adiabatic and antiadiabatic regimes, is studied systematically in the framework of a minimal model for molecular devices: a resonant level coupled by displacement to a localized vibrational mode. Conventionally associated with the limits where the phonon frequency is either sufficiently small or sufficiently large as compared to the bare electronic hopping rate, we show that the crossover between the two regimes is governed for strong electron-phonon interactions primarily by the polaronic shift rather than the phonon frequency. In particular, the perturbative adiabatic limit is approached only as the bare hopping rate Γexceeds the polaronic shift, leaving an extended window of couplings where Γwell exceeds the phonon frequency and yet the physics is basically that of the antiadiabatic regime. We term this intermediate regime the extended antiadiabatic regime. The effective low-energy Hamiltonian in the traditional and the extended antiadiabatic regime is shown to be the (purely fermionic) interacting resonant-level model, with parameters that we extract from numerical renormalization-group calculations. The extended antiadiabatic regime is followed in turn by a true crossover region where the polaron gets progressively undressed. The renormalized tunneling rate, which serves as the low-energy scale in the problem and thus sets the width of the tunneling resonance, is found to follow an approximate scaling form on going from the adiabatic to the antiadiabatic regime. Charging properties are governed by two distinct mechanisms at the extended antiadiabatic and into the crossover region, giving rise to distinctive shoulders in the low-temperature conductance as a function of gate voltage.

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arXiv2012

Hybrid NRG-DMRG approach to real-time dynamics of quantum impurity systems

A hybrid approach to nonequilibrium dynamics of quantum impurity systems is presented. The numerical renormalization group serves as a means to generate a suitable low-energy Hamiltonian, allowing for an accurate evaluation of the real-time dynamics of the problem up to exponentially long times using primarily the time-adaptive density-matrix renormalization group. We extract the decay time of the interaction-enhanced oscillations in the interacting resonant-level model and show their quadratic divergence with the interaction strength U. Our numerical analysis is in excellent agreement with analytic predictions based on an expansion in 1/U.

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arXiv2012

Coherent control of correlated nanodevices: A hybrid time-dependent numerical renormalization-group approach to periodic switching

The time-dependent numerical renormalization-group approach (TD-NRG), originally devised for tracking the real-time dynamics of quantum-impurity systems following a single quantum quench, is extended to multiple switching events. This generalization of the TD-NRG encompasses the possibility of periodic switching, allowing for coherent control of strongly correlated systems by an external time-dependent field. To this end, we have embedded the TD-NRG in a hybrid framework that combines the outstanding capabilities of the numerical renormalization group to systematically construct the effective low-energy Hamiltonian of the system with the prowess of complementary approaches for calculating the real-time dynamics derived from this Hamiltonian. We demonstrate the power of our approach by hybridizing the TD-NRG with the Chebyshev expansion technique in order to investigate periodic switching in the interacting resonant-level model. Although the interacting model shares the same low-energy fixed point as its noninteracting counterpart, we surprisingly find the gradual emergence of damped oscillations as the interaction strength is increased. Focusing on a single quantum quench and using a strong-coupling analysis, we reveal the origin of these interaction-induced oscillations and provide an analytical estimate for their frequency. The latter agrees well with the numerical results.

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arXiv2011

Quantum quenches and driven dynamics in a single-molecule device

The nonequilibrium dynamics of molecular devices is studied in the framework of a generic model for single-molecule transistors: a resonant level coupled by displacement to a single vibrational mode. In the limit of a broad level and in the vicinity of the resonance, the model can be controllably reduced to a form quadratic in bosonic operators, which in turn is exactly solvable. The response of the system to a broad class of sudden quenches and ac drives is thus computed in a nonperturbative manner, providing an asymptotically exact solution in the limit of weak electron-phonon coupling. From the analytic solution we are able to (1) explicitly show that the system thermalizes following a local quantum quench, (2) analyze in detail the time scales involved, (3) show that the relaxation time in response to a quantum quench depends on the observable in question, and (4) reveal how the amplitude of long-time oscillations evolves as the frequency of an ac drive is tuned across the resonance frequency. Explicit analytical expressions are given for all physical quantities and all nonequilibrium scenarios under study.

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arXiv2011

Quantum phase transitions, frustration, and the Fermi surface in the Kondo lattice model

The quantum phase transition from a spin-Peierls phase with a small Fermi surface to a paramagnetic Luttinger-liquid phase with a large Fermi surface is studied in the framework of a one-dimensional Kondo-Heisenberg model that consists of an electron gas away from half filling, coupled to a spin-1/2 chain by Kondo interactions. The Kondo spins are further coupled to each other with isotropic nearest-neighbor and next-nearest-neighbor antiferromagnetic Heisenberg interactions which are tuned to the Majumdar-Ghosh point. Focusing on three-eighths filling and using the density-matrix renormalization-group (DMRG) method, we show that the zero-temperature transition between the phases with small and large Fermi momenta appears continuous, and involves a new intermediate phase where the Fermi surface is not well defined. The intermediate phase is spin gapped and has Kondo-spin correlations that show incommensurate modulations. Our results appear incompatible with the local picture for the quantum phase transition in heavy fermion compounds, which predicts an abrupt change in the size of the Fermi momentum.

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arXiv2007

Adiabatic pumping through a quantum dot in the Kondo regime: Exact results at the Toulouse limit

Transport properties of ultrasmall quantum dots with a single unpaired electron are commonly modeled by the nonequilibrium Kondo model, describing the exchange interaction of a spin-1/2 local moment with two leads of noninteracting electrons. Remarkably, the model possesses an exact solution when tuned to a special manifold in its parameter space known as the Toulouse limit. We use the Toulouse limit to exactly calculate the adiabatically pumped spin current in the Kondo regime. In the absence of both potential scattering and a voltage bias, the instantaneous charge current is strictly zero for a generic Kondo model. However, a nonzero spin current can be pumped through the system in the presence of a finite magnetic field, provided the spin couples asymmetrically to the two leads. Tunneling through a Kondo impurity thus offers a natural mechanism for generating a pure spin current. We show, in particular, that one can devise pumping cycles along which the average spin pumped per cycle is closely equal to $\hbar$. By analogy with Brouwer's formula for noninteracting systems with two driven parameters, the pumped spin current is expressed as a geometrical property of a scattering matrix. However, the relevant %Alex: I replaced topological with geometrical in the sentence above scattering matrix that enters the formulation pertains to the Majorana fermions that appear at the Toulouse limit rather than the physical electrons that carry the current. These results are obtained by combining the nonequilibrium Keldysh Green function technique with a systematic gradient expansion, explicitly exposing the small parameter controlling the adiabatic limit.

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arXiv2007

Strong-to-weak-coupling duality in the nonequilibrium interacting resonant-level model

A strong-to-weak-coupling duality is established for the nonequilibrium interacting resonant-level model, describing tunneling through a single spinless level, capacitively coupled to two leads by a contact interaction. For large capacitive coupling, U, and in the presence of a finite voltage bias, the model maps onto an equivalent model with a small capacitive coupling ρU' \sim 1/ ρU. Here ρis the conduction-electron density of states. This duality is generic to all high-energy cutoff schemes, however its details may vary from one regularization scheme to another. In particular, it has the status of an exact mapping within Abelian bosonization, applicable to all repulsive interactions whether weak, intermediate or strong. On a lattice the mapping is restricted to large U, and is controlled by the small parameter 1/ρU. Explicit expressions are given for the low-energy scale, differential conductance, and occupancy of the level in the limit where U is large.

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arXiv2006

Unified description of correlations in double quantum dots

The two-level model for a double quantum dot coupled to two leads, which is ubiquitously used to describe charge oscillations, transmission-phase lapses and correlation-induced resonances, is considered in its general form. The model features arbitrary tunnelling matrix elements among the two levels and the leads and between the levels themselves (including the effect of Aharonov-Bohm fluxes), as well as inter-level repulsive interactions. We show that this model is exactly mapped onto a generalized Anderson model of a single impurity, where the electrons acquire a pseudo-spin degree of freedom, which is conserved by the tunnelling but not within the dot. Focusing on the local-moment regime where the dot is singly occupied, we show that the effective low-energy Hamiltonian is that of the anisotropic Kondo model in the presence of a tilted magnetic field. For moderate values of the (renormalized) field, the Bethe ansatz solution of the isotropic Kondo model allows us to derive accurate expressions for the dot occupation numbers, and henceforth its zero-temperature transmission. Our results are in excellent agreement with those obtained from the Bethe ansatz for the isotropic Anderson model, and with the functional and numerical renormalization-group calculations of Meden and Marquardt [Phys. Rev. Lett. 96, 146801 (2006)], which are valid for the general anisotropic case. In addition we present highly accurate estimates for the validity of the Schrieffer-Wolff transformation (which maps the Anderson Hamiltonian onto the low-energy Kondo model) at both the high- and low-magnetic field limits. Perhaps most importantly, we provide a single coherent picture for the host of phenomena to which this model has been applied.

cond-mat.mes-hall↗

arXiv2006

Phase diagram of the anisotropic multichannel Kondo Hamiltonian revisited

The phase diagram of the multichannel Kondo Hamiltonian with an XXZ spin-exchange anisotropy is revisited, revealing a far richer fixed-point structure than previously appreciated. For a spin-1/2 impurity and k > 2 conduction-electron channels, a second ferromagnetic-like domain is found deep in the antiferromagnetic regime. The new domain extends above a (typically large) critical longitudinal coupling J_z^{\ast} > 0, and is separated from the antiferromagnetic domain by a second Kosterliz-Thouless line. A similar line of stable ferromagnetic-like fixed points with a residual isospin-1/2 local moment is shown to exist for large J_z >> |J_{\perp}| > 0 and arbitrary k and s obeying |k - 2s| > 1. Here J_z is the longitudinal spin-exchange coupling, J_{\perp} is the transverse coupling, and s is the impurity spin. Near the free-impurity fixed-point, spin-exchange anisotropy is a relevant perturbation for s > 1/2 and arbitrary k. Depending on the sign of J_z^2 - J_{\perp}^2 and the parity of 2s, the system flows either to a conventional Fermi liquid with no residual degeneracy, or to a k-channel, spin-1/2 Kondo effect, or to a line of ferromagnetic-like fixed points with a residual isospin-1/2 local moment. These results are obtained through a combination of perturbative renormalization-group techniques, Abelian bosonization, a strong-coupling expansion in 1/J_z, and explicit numerical renormalization-group calculations.

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arXiv2006

Spin Precession and Real Time Dynamics in the Kondo Model: A Time-Dependent Numerical Renormalization-Group Study

A detailed derivation of the recently proposed time-dependent numerical renormalization-group (TD-NRG) approach to nonequilibrium dynamics in quantum impurity systems is presented. We demonstrate that the method is suitable for fermionic as well as bosonic baths. A comparison with exact analytical results for the charge relaxation in the resonant-level model and for dephasing in the spin-boson model establishes the accuracy of the method. The real-time dynamics of a single spin coupled to both types of baths is investigated. We use the TD-NRG to calculate the spin relaxation and spin precession of a single Kondo impurity. The short- and long-time dynamics is studied as a function of temperature in the ferromagnetic and antiferromagnetic regimes. The short-time dynamics agrees very well with analytical results obtained at second order in the exchange coupling $J$. In the ferromagnetic regime, the long-time spin decay is described by the scaling variable $x = 2ρ_F J(T) T t$. In the antiferromagnetic regime it is governed for $T < T_K$ by the Kondo time scale $1/T_K$. Here $ρ_F$ is the conduction-electron density of states and $T_K$ is the Kondo temperature. Results for spin precession are obtained by rotating the external magnetic field from the x axis to the z axis.

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arXiv2005

Coulomb blockade and Non-Fermi-liquid behavior in quantum dots

The non-Fermi-liquid properties of an ultrasmall quantum dot coupled to a lead and to a quantum box are investigated. Tuning the ratio of the tunneling amplitudes to the lead and box, we find a line of two-channel Kondo fixed points for arbitrary Coulomb repulsion on the dot, governing the transition between two distinct Fermi-liquid regimes. The Fermi liquids are characterized by different values of the conductance. For an asymmetric dot, spin and charge degrees of freedom are entangled: a continuous transition from a spin to a charge two-channel Kondo effect evolves. The crossover temperature to the two-channel Kondo effect is greatly enhanced away from the local-moment regime, making this exotic effect accessible in realistic quantum-dot devices.

cond-mat.str-el↗

arXiv2005

Real-time dynamics in Quantum Impurity Systems: A Time-dependent Numerical Renormalization Group Approach

We develop a general approach to the nonequilibrium dynamics of quantum impurity systems for arbitrary coupling strength. The numerical renormalization group is used to generate a complete basis set necessary for the correct description of the time evolution. We benchmark our method with the exact analytical solution for the resonant-level model. As a first application, we investigate the equilibration of a quantum dot subject to a sudden change of the gate voltage and external magnetic field. Two distinct relaxation times are identified for the spin and charge dynamics.

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arXiv2004

Coulomb blockade and Quantum Critical Points in Quantum Dots

An ultrasmall quantum dot coupled to a lead and to a quantum box (a large quantum dot) is investigated. Tuning the tunneling amplitudes to the lead and box, we find a line of unstable non-Fermi-liquid fixed points as function of the gate potentials of the quantum dots, extending to arbitrary charging energies on the small and large quantum dots. These quantum-critical fixed points possess a finite residual entropy. They govern the cross over from one Fermi-liquid regime to another, characterized by distinct (high and low) conductance values.

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arXiv2003

The Coulomb Blockade in Quantum Boxes

The charging of a quantum box connected to a lead by a single-mode point contact is solved for arbitrary temperatures, tunneling amplitudes, and gate voltages, using a variant of Wilson's numerical renormalization group. The charge inside the box and the capacitance of the junction are calculated on equal footing for all physical regimes, including weak tunneling, near perfect transmission, and the crossover regime in between. At the charge plateaus, perturbation theory is found to break down at fairly small tunneling amplitudes. Near perfect transmission, we confirm Matveev's scenario for the smearing of the Coulomb-blockade staircase. A surprising reentrance of the Coulomb-blockade staircase is found for large tunneling amplitudes. At the degeneracy points, we obtain two-channel Kondo behavior directly from the Coulomb-blockade Hamiltonian, without the restriction to two charge configurations or the introduction of an effective cutoff.

cond-mat.mes-hall↗

arXiv2003

Enhancement of the Two-channel Kondo Effect in Single-Electron boxes

The charging of a quantum box, coupled to a lead by tunneling through a single resonant level, is studied near the degeneracy points of the Coulomb blockade. Combining Wilson's numerical renormalization-group method with perturbative scaling approaches, the corresponding low-energy Hamiltonian is solved for arbitrary temperatures, gate voltages, tunneling rates, and energies of the impurity level. Similar to the case of a weak tunnel barrier, the shape of the charge step is governed at low temperatures by the non-Fermi-liquid fixed point of the two-channel Kondo effect. However, the associated Kondo temperature TK is strongly modified. Most notably, TK is proportional to the width of the level if the transmission through the impurity is close to unity at the Fermi energy, and is no longer exponentially small in one over the tunneling matrix element. Focusing on a particle-hole symmetric level, the two-channel Kondo effect is found to be robust against the inclusion of an on-site repulsion on the level. For a large on-site repulsion and a large asymmetry in the tunneling rates to box and to the lead, there is a sequence of Kondo effects: first the local magnetic moment that forms on the level undergoes single-channel screening, followed by two-channel overscreening of the charge fluctuations inside the box.

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