arXiv subjects

Ayman F. Abouraddy

Publications and source records attributed to Ayman F. Abouraddy.

At least 73 records · Page 4Linked to original sources

arXiv2021

Refraction of space-time wave packets: I. Theoretical principles

Space-time (ST) wave packets are pulsed optical beams endowed with precise spatio-temporal structure by virtue of which they exhibit unique and useful characteristics, such as propagation invariance and tunable group velocity. We study in detail here, and in two accompanying papers, the refraction of ST wave packets at planar interfaces between non-dispersive, homogeneous, isotropic dielectrics. We formulate a law of refraction that determines the change in the ST wave-packet group velocity across such an interface as a consequence of a newly identified optical refractive invariant that we call 'the spectral curvature'. Because the spectral curvature vanishes in conventional optical fields where the spatial and temporal degrees of freedom are separable, these phenomena have not been observed to date. We derive the laws of refraction for baseband, X-wave, and sideband ST wave packets that reveal fascinating refractive phenomena, especially for the former class of wave packets. We predict theoretically, and confirm experimentally in the accompanying papers, refractive phenomena such as group-velocity invariance (ST wave packets whose group velocity does not change across the interface), anomalous refraction (group-velocity increase in higher-index media), group-velocity inversion (change in the sign of the group velocity upon refraction but not its magnitude), and the dependence of the group velocity of the refracted ST wave packet on the angle of incidence.

physics.optics↗

arXiv2021

Refraction of space-time wave packets: II. Experiments at normal incidence

The refraction of space-time (ST) wave packets offers many fascinating surprises with respect to conventional pulsed beams. In paper (I) of this sequence, we described theoretically the refraction of all families of ST wave packets at normal and oblique incidence at a planar interface between two non-dispersive, homogeneous, isotropic dielectrics. Here, in paper (II) of this sequence, we present experimental verification of the novel refractive phenomena predicted for `baseband' ST wave packets upon normal incidence on a planar interface. Specifically, we observe group-velocity invariance, normal and anomalous refraction, and group-velocity inversion leading to group-delay cancellation. These phenomena are verified in a set of optical materials with refractive indices ranging from 1.38 to 1.76, including MgF$_2$, fused silica, BK7 glass, and sapphire. We also provide a geometrical representation of the physics associated with anomalous refraction in terms of the dynamics of the spectral support domain for ST wave packets on the surface of the light-cone.

physics.optics↗

arXiv2021

Refraction of space-time wave packets: III. Experiments at oblique incidence

The refraction of space-time (ST) wave packets at planar interfaces between non-dispersive, homogeneous, isotropic dielectrics exhibit fascinating phenomena, even at normal incidence. Examples of such refractive phenomena include group-velocity invariance across the interface, anomalous refraction, and group-velocity inversion. Crucial differences emerge at oblique incidence with respect to the results established at normal incidence. For example, the group velocity of the refracted ST wave packet can be tuned simply by changing the angle of incidence. In paper (III) of this sequence, we present experimental verification of the refractive phenomena exhibited by ST wave packets at oblique incidence that were predicted in paper (I). We also examine a proposal for 'blind synchronization' whereby identical ST wave packets arrive simultaneously at different receivers without \textit{a priori} knowledge of their locations except that they are all located at the same depth beyond an interface between two media. A first proof-of-principle experimental demonstration of this effect is provided.

physics.optics↗

arXiv2021

Broadband Omni-resonant Coherent Perfect Absorption in Graphene

Coherent perfect absorption (CPA) refers to interferometrically induced complete absorption of incident light by a partial absorber independently of its intrinsic absorption (which may be vanishingly small) or its thickness. CPA is typically realized in a resonant device, and thus cannot be achieved over a broad continuous spectrum, which thwarts its applicability to photodetectors and solar cells, for example. Here, we demonstrate broadband omni-resonant CPA by placing a thin weak absorber in a planar cavity and pre-conditioning the incident optical field by introducing judicious angular dispersion. We make use of monolayer graphene embedded in silica as the absorber and boost its optical absorption from ~1.6% to ~60% over a bandwidth of ~70 nm in the visible. Crucially, an analytical model demonstrates that placement of the graphene monolayer at a peak in the cavity standing-wave field is not necessary to achieve CPA, contrary to conventional wisdom.

physics.optics↗

arXiv2021

V-Waves: Spatio-temporally induced group-velocity dispersion in free space

Introducing precise spatio-temporal structure into a pulsed optical field can lead to remarkable changes with its free propagation. `Space-time' (ST) wave packets, for example, propagate rigidly at a tunable group velocity in free space by inculcating a one-to-one relationship between the axial wave numbers and the temporal frequencies. Here we introduce a new class of ST wave packets that we call V-waves (so named because of their characteristically V-shaped spatio-temporal spectrum) in which a linear one-to-one relationship is introduced between the temporal frequencies and the transverse wave numbers (or spatial frequencies). We confirm experimentally that V-waves experience anomalous group velocity dispersion in free space, all the while maintaining the group velocity fixed at the speed of light in vacuum. Extremely large values of group velocity dispersion can be easily realized, which are not accessible with traditional optical materials or photonic structures. Moreover, V-waves are the unique optical wave packets whose diffraction and dispersion lengths are intrinsically equal by virtue of the spatio-temporal structure of the field itself. These results are of interest for optical signal processing and nonlinear optics.

physics.optics↗

arXiv2021

Roadmap on multimode light shaping

Our ability to generate new distributions of light has been remarkably enhanced in recent years. At the most fundamental level, these light patterns are obtained by ingeniously combining different electromagnetic modes. Interestingly, the modal superposition occurs in the spatial, temporal as well as spatio-temporal domain. This generalized concept of structured light is being applied across the entire spectrum of optics: generating classical and quantum states of light, harnessing linear and nonlinear light-matter interactions, and advancing applications in microscopy, spectroscopy, holography, communication, and synchronization. This Roadmap highlights the common roots of these different techniques and thus establishes links between research areas that complement each other seamlessly. We provide an overview of all these areas, their backgrounds, current research, and future developments. We highlight the power of multimodal light manipulation and want to inspire new eclectic approaches in this vibrant research community.

physics.optics↗

arXiv2021

Temporal Talbot effect in free space

The temporal Talbot effect refers to the periodic revivals of a pulse train propagating in a dispersive medium, and is a temporal analog of the spatial Talbot effect with group-velocity dispersion in time replacing diffraction in space. Because of typically large temporal Talbot lengths, this effect has been observed to date in only single-mode fibers, rather than with freely propagating fields in bulk dispersive media. Here we demonstrate for the first time the temporal Talbot effect in free space by employing dispersive space-time wave packets, whose spatio-temporal structure induces group-velocity dispersion of controllable magnitude and sign in free space.

physics.optics↗

arXiv2021

Isochronous space-time wave packets

The group delay incurred by an optical wave packet depends on its path length. Therefore, when a wave packet is obliquely incident on a planar homogeneous slab, the group delay upon traversing it inevitably increases with the angle of incidence. Here we confirm the existence of isochronous `space-time' (ST) wave packets: pulsed beams whose spatio-temporal structure enables them to traverse the layer with a fixed group delay over a wide span of incident angles. This unique behavior stems from the dependence of the group velocity of a refracted ST wave packet on its angle of incidence. Isochronous ST wave packets are observed in slabs of optical materials with indices in the range from 1.38 to 2.5 for angles up to $50^{\circ}$ away from normal incidence.

physics.optics↗

arXiv2021

Engineering the optical vacuum: Arbitrary magnitude, sign, and order of dispersion in free space using space-time wave packets

Spatial structuring of an optical pulse can lead in some cases upon free propagation to changes in its temporal profile. For example, introducing conventional angular dispersion into the field results in the pulse encountering group-velocity dispersion in free space. However, only limited control is accessible via this strategy. Here we show that precise and versatile control can be exercised in free space over the dispersion profile of so-called `space-time' wave packets: a class of pulsed beams undergirded by non-differentiable angular dispersion. This abstract mathematical feature allows us to tune the magnitude and sign of the different dispersion orders without introducing losses, thereby realizing arbitrary dispersion profiles, and achieving dispersion values unattainable in optical materials away from resonance. Unlike optical materials and photonic structures in which the values of the different dispersion orders are not independent of each other, these orders are addressable separately using our strategy. These results demonstrate the versatility of space-time wave packets as a platform for structured light and point towards their utility in nonlinear and quantum optics.

physics.optics↗

arXiv2021

The space-time Talbot effect

The Talbot effect, epitomized by periodic revivals of a freely evolving periodic field structure, has been observed with waves of diverse physical nature in space and separately in time, whereby diffraction underlies the former and dispersion the latter. To date, a combined spatio-temporal Talbot effect has not been realized in any wave field because diffraction and dispersion are independent physical phenomena, typically unfolding at incommensurable length scales. Here we report the observation of an optical 'space-time' Talbot effect, whereby a spatio-temporal optical lattice structure undergoes periodic revivals after suffering the impact of both diffraction and dispersion. The discovered space-time revivals are governed by a single self-imaging length scale, which encompasses both spatial and temporal degrees of freedom. Key to this effect is the identification of a unique pulsed optical field structure, which we refer to as a V-wave, that is endowed with intrinsically equal diffraction and dispersion lengths in free space, thereby enabling self-imaging to proceed in lockstep in space and time.

physics.optics↗

arXiv2021

Space-time wave packets violate the universal relationship between angular dispersion and pulse-front tilt

Introducing angular dispersion into a pulsed field tilts the pulse front with respect to the phase front. There exists between the angular dispersion and the pulse-front tilt a universal relationship that is device-independent, and also independent of the pulse shape and bandwidth. We show here that this relationship is violated by propagation-invariant space-time (ST) wave packets, which are pulsed beams endowed with precise spatio-temporal structure corresponding to a particular form of angular dispersion. We demonstrate theoretically and experimentally that underlying ST wave packets is -- to the best of our knowledge -- the first example in optics of non-differentiable angular dispersion, resulting in pulse-front tilt that depends on the pulse bandwidth even at fixed angular dispersion.

physics.optics↗

arXiv2020

Coherent perfect absorption in resonant materials

Coherent perfect absorption (CPA) is an interferometric effect that guarantees full absorption in a lossy layer independently of its intrinsic losses. To date, it has been observed only at a single wavelength or narrow bandwidths, whereupon wavelength-dependent absorption can be ignored. Here we produce CPA over a bandwidth of ~ 60 nm in a 2-um-thick polymer film with a low-doping concentration of an organic laser dye. A planar cavity is designed with a spectral `dip' to accommodate the dye resonant linewidth, and CPA is thus achieved even at its absorption edges. This approach allows realizing strong absorption in laser dyes - and resonant materials in general - independently of the intrinsic absorption levels, with a at spectral profile and without suffering absorption quenching due to high doping levels.

physics.optics↗

arXiv2020

Spectrally recycling space-time wave packets

'Space-time' (ST) wave packets are propagation-invariant pulsed optical beams that travel rigidly in linear media without diffraction or dispersion at a potentially arbitrary group velocity. These unique characteristics are a result of spatio-temporal spectral correlations introduced into the field; specifically, each spatial frequency is associated with a single temporal frequency (or wavelength). Consequently, the spatial and temporal bandwidths of ST wave packets are correlated, so that exploiting an optical source with a large temporal bandwidth or achieving an ultralow group velocity necessitate an exorbitantly large numerical aperture. Here we show that `spectral recycling' can help overcome these challenges. 'Recycling' or `reusing' each spatial frequency by associating it with multiple distinct but widely separated temporal frequencies allows one to circumvent the proportionality between the spatial and temporal bandwidths of ST wave packets, which has been one of their permanent characteristics since their inception. We demonstrate experimentally that the propagation invariance, maximum propagation distance, and group velocity of ST wave packets are unaffected by spectral recycling. We also synthesize a ST wave packet with group velocity c/14.3 (c is the speed of light in vacuum) with a reasonable numerical aperture made possible by spectral recycling.

physics.optics↗

arXiv2020

Axial spectral encoding of space-time wave packets

Space-time (ST) wave packets are propagation-invariant pulsed optical beams whose group velocity can be tuned in free space by tailoring their spatio-temporal spectral structure. To date, efforts on synthesizing ST wave packets have striven to maintain their propagation invariance. Here, we demonstrate that one degree of freedom of a ST wave packet -- its on-axis spectrum -- can be isolated and purposefully controlled independently of the others. Judicious spatio-temporal spectral amplitude and phase modulation yields ST wave packets with programmable spectral changes along the propagation axis; including red-shifting or blue-shifting spectra, or more sophisticated axial spectral encoding including bidirectional spectral shifts and accelerating spectra. In all cases, the spectral shift can be larger than the initial on-axis bandwidth, while preserving the propagation-invariance of the other degrees of freedom, including the wave packet spatio-temporal profile. These results may be useful in range-finding in microscopy or remote sensing via spectral stamping.

physics.optics↗

arXiv2020

Veiled Talbot effect

A freely propagating optical field having a periodic transverse spatial profile undergoes periodic axial revivals - a well-known phenomenon known as the Talbot effect or self-imaging. We show here that introducing tight spatio-temporal spectral correlations into an ultrafast pulsed optical field with a periodic transverse spatial profile eliminates all axial dynamics in physical space while revealing a novel space-time Talbot effect that can be observed only when carrying out time-resolved measurements. Indeed, 'time-diffraction' is observed whereupon the temporal profile of the field envelope at a fixed axial plane corresponds to a segment of the spatial propagation profile of a monochromatic field sharing the initial spatial profile and observed at the same axial plane. Time-averaging, which is intrinsic to observing the intensity, altogether veils this effect.

physics.optics↗

arXiv2020

Accelerating and decelerating space-time optical wave packets in free space

Although a plethora of techniques are now available for controlling the group velocity of an optical wave packet, there are very few options for creating accelerating or decelerating wave packets whose group velocity varies controllably along the propagation axis. Here we show that `space-time' wave packets in which each wavelength is associated with a prescribed spatial bandwidth enable the realization of optical acceleration and deceleration in free space. Endowing the field with precise spatio-temporal structure leads to group-velocity changes as high as $\sim c$ observed over a distance of $\sim20$ mm in free space, which represents a boost of at least $\sim4$ orders of magnitude over X-waves and Airy pulses. The acceleration implemented is in principle independent of the initial group velocity, and we have verified this effect in both the subluminal and superluminal regimes.

physics.optics↗

arXiv2020

Space-Time Surface Plasmon Polaritons: A New Propagation-Invariant Surface Wave Packet

We introduce the unique class of propagation-invariant surface plasmon polaritons (SPPs) representing pulsed surface wave packets propagating along unpatterned metal-dielectric interfaces and are localized in all dimensions - with potentially subwavelength transverse spatial widths. The characteristic features of such linear diffraction-free, dispersion-free `plasmonic bullets' stem from tight spatio-temporal correlations incorporated into the SPP spectral support domain, and we thus call them `space-time' SPPs. We show that the group velocity of space-time SPP wave packets can be readily tuned to subluminal, superluminal, and even negative values by tailoring the spatio-temporal field structure independently of any material properties. We present an analytical framework and numerical simulations for the propagation of space-time SPPs in comparison with traditional pulsed SPPs whose spatial and temporal degrees of freedom are separable, thereby verifying the propagation-invariance of the former.

physics.optics↗

arXiv2020

Doubling the near-infrared photocurrent in a solar cell via omni-resonant coherent perfect absorption

Minimizing the material usage in thin-film solar cells can reduce manufacturing costs and enable mechanically flexible implementations, but concomitantly diminishes optical absorption. Coherent optical effects can help alleviate this inevitable drawback at discrete frequencies. For example, coherent perfect absorption guarantees that light is fully absorbed in a thin layer regardless of material or thickness but only on resonance. Here we show that omni resonance delivers such coherent enhancement over a broad bandwidth by structuring the optical field to nullify the angular dispersion intrinsic to resonant structures. After embedding an amorphous-silicon thin film photovoltaic cell in a planar cavity, pre conditioning the incident light using an alignment free optical arrangement severs the link between the resonant bandwidth and the cavity photon lifetime, thereby rendering the cavity omni resonant. Coherently enhanced near infrared absorption doubles the photocurrent over the targeted spectral range 660 to 740 nm where every wavelength resonates. These results may pave the way to transparent solar cells that optimally harvest near infrared light.

physics.optics↗