arXiv subjects

Aymeric Delteil

Publications and source records attributed to Aymeric Delteil.

At least 19 recordsLinked to original sources

arXiv2026

Quantum correlations and dissipative blockade of polaritons in a tunable fiber cavity

Cavity exciton--polaritons are quasiparticles that form when quantum well excitons hybridize with a cavity mode. Here, we carry out photon correlation measurements under continuous wave resonant laser excitation to demonstrate quantum correlations between cavity--polaritons. Our experiments reveal an unexpectedly strong dependence of polariton interactions on cavity--exciton detuning. When the polaritons are predominantly exciton-like, we observe a transition from photon antibunching to bunching as the laser is tuned across the polariton resonance, in agreement with a simple Kerr-nonlinearity model. When the lower-branch polariton energy is tuned to induce a two-polariton Feshbach resonance with the biexciton mode, the degree of polariton antibunching becomes independent of the laser detuning: we explain our finding by invoking a dissipative blockade mechanism arising from large biexciton broadening. Our experiments demonstrate that the strong polariton blockade regime would be achieved by reducing the polariton decay rate by a factor of 10.

cond-mat.mes-hall↗

arXiv2025

Photon correlation Fourier spectroscopy of a B center in hBN

The potential of solid-state quantum emitters for applications critically depends on several key figures of merit. One of the most important is the quantum coherence of the emitted single photons, which can be compromised by fast dephasing and spectral diffusion. In hexagonal boron nitride (hBN), blue-emitting color centers (or B centers) are seen as favorable in this regard, in the light of prior studies mainly based on resonant excitation. Yet, their coherence properties in the more accessible regime of non-resonant excitation (or photoluminescence) has not been extensively characterized. Here, we investigate the coherence and spectral diffusion of the photoluminescence from a B center in the continuous wave regime using photon correlation Fourier spectroscopy. We determine that the emission lineshape consists in a homogeneous contribution, whose linewidth increases with the laser power, and which is broadened by spectral diffusion at a timescale of 10 to 100 microseconds. At low power and short time, the emission line is only a factor ~2 above the Fourier limit, while at long times, the inhomogeneous linewidth increases up to more than a gigahertz. Our work deepens the understanding of decoherence processes of this preeminent family of quantum emitters in hBN.

quant-ph↗

arXiv2025

Deterministic generation of single B centers in hBN by one-to-one conversion from UV centers

Among the variety of quantum emitters in hexagonal boron nitride (hBN), blue-emitting color centers, or B centers, have gathered a particular interest owing to their excellent quantum optical properties. Moreover, the fact that they can be locally activated by an electron beam makes them suitable for top-down integration in photonic devices. However, in the absence of a real-time monitoring technique sensitive to individual emitters, the activation process is stochastic in the number of emitters, and its mechanism is under debate. Here, we implement an in-situ cathodoluminescence monitoring setup capable of detecting individual quantum emitters in the blue and ultraviolet (UV) range. We demonstrate that the activation of individual B centers is spatially and temporally correlated with the deactivation of individual UV centers emitting at 4.1 eV, which are ubiquitous in hBN. We then make use of the ability to detect individual B center activation events to demonstrate the controlled creation of an array with only one emitter per irradiation site. Additionally, we demonstrate a symmetric technique for heralded selective deactivation of individual emitters. Our results provide insights into the microscopic structure and activation mechanism of B centers, as well as versatile techniques for their deterministic integration.

cond-mat.other↗

arXiv2025

Resonance fluorescence and indistinguishable photons from a coherently driven B centre in hBN

Optically active defects in hexagonal boron nitride (hBN) have become amongst the most attractive single-photon emitters in the solid state, owing to their high-quality photophysical properties, combined with the unlimited possibilities of integration offered by the host two-dimensional material. In particular, the B centres, with their narrow linewidth, low wavelength spread and controllable positioning, have raised a particular interest for integrated quantum photonics. However, to date, either their excitation or their detection has been performed non-resonantly due to the difficulty of rejecting the backreflected laser light at the same wavelength, thereby preventing to take full benefit from their high coherence in quantum protocols. Here, we make use of a narrow-linewidth emitter integrated in a hybrid metal-dielectric structure to implement crossed-polarisation laser rejection. This allows us to observe resonantly scattered photons, with associated experimental signatures of optical coherence in both continuous-wave (cw) and pulsed regimes, respectively the Mollow triplet and Hong-Ou-Mandel interference from zero-phonon-line emission. The measured two-photon interference visibility of 0.93 +/- 0.21 and 0.92 +/- 0.26 we measured for two emitters demonstrate the potential of B centres in hBN for applications to integrated quantum information.

physics.optics↗

arXiv2025

Reproducible generation of green-emitting color centers in hBN using oxygen annealing

The ability to generate quantum emitters with reproducible properties in solid-state matrices is crucial for quantum technologies. Here, we show that a high density of close-to-identical single-photon emitters can be created in commercial hexagonal boron nitride using annealing under oxygen atmosphere. This simple procedure yields a uniform in-plane distribution of color centers consistently emitting around 539.4 nm, with a wavelength spread smaller than 1 nm. We present an extensive characterization of their photophysical properties, showing that the emitters are bright and stable, and exhibit narrow lines at low temperatures with minimal spectral diffusion. These characteristics make this family of quantum emitters highly appealing for applications to quantum information science.

quant-ph↗

arXiv2024

Crossover from inhomogeneous to homogeneous response of a resonantly driven hBN quantum emitter

We experimentally investigate a solid-state quantum emitter - a B center in hexagonal boron nitride (hBN) - that has lifetime-limited coherence at short times, and experiences inhomogeneous broadening due to spectral diffusion at longer times. By making use of power broadening in resonant laser excitation, we explore the crossover between the inhomogeneous and the homogeneous broadening regimes. With the support of numerical simulations, we show that the lineshape, count rate, second-order correlations and long-time photon statistics evolve from a regime where they are dictated by spectral diffusion to a regime where they are simply given by the homogeneous response of the emitter, yielding restored Lorentzian shape and Poissonian photon statistics. Saturation of the count rate and line broadening occur not at the onset of the Rabi oscillations, but when the power-broadened homogeneous response becomes comparable with the inhomogeneous linewidth. Moreover, we identify specific signatures in both the second-order correlations and long-time photon statistics that are well explained by a microscopic spectral diffusion model based on discrete jumps at timescales of micro- to milliseconds. Our work provides an extensive description of the photophysics of B-centers under resonant excitation, and can be readily extended to a wide variety of solid-state quantum emitters.

physics.optics↗

arXiv2024

N-qubit universal quantum logic with a photonic qudit and O(N) linear optics elements

High-dimensional quantum units of information, or qudits, can carry more than one quantum bit of information in a single degree of freedom, and can therefore be used to boost the performance of quantum communication and quantum computation protocols. A photon in a superposition of $2^N$ time bins - a time-bin qudit - contains as much information as N qubits. Here, we show that N-qubit states encoded in a single time-bin qudit can be arbitrarily and deterministically generated, manipulated and measured using a number of linear optics elements that scales linearly with N, as opposed with prior proposals of single-qudit implementation of N-qubit logic, which typically requires $O(2^N)$ elements. The simple and cost-effective implementation we propose can be used as a small-scale quantum processor. We then demonstrate a path towards scalability by interfacing distinct qudit processors to a matter qubit (atom or quantum dot spin) in an optical resonator. Such a cavity QED system allows for more advanced functionalities, such as single-qubit nondemolition measurement and two-qubit gates between distinct qudits. It could also enable quantum interfaces with other matter quantum nodes in the context of quantum networks and distributed quantum computing.

quant-ph↗

arXiv2024

Quantum efficiency and vertical position of quantum emitters in hBN determined by Purcell effect in hybrid metal-dielectric planar photonic structures

Color centers in hexagonal boron nitride (hBN) advantageously combine excellent photophysical properties with a potential for integration in highly compact devices. Progress towards scalable integration necessitates a high quantum efficiency and an efficient photon collection. In this context, we compare the optical characteristics of individual hBN color centers generated by electron irradiation, in two different electromagnetic environments. We keep track of well-identified emitters that we characterize before and after dry transfer of exfoliated crystals. This comparison provides information about their quantum efficiency - which we find close to unity - as well as their vertical position in the crystal with nanometric precision, which we find away from the flake surfaces. Our work suggests hybrid dielectric-metal planar structures as an efficient tool for characterizing quantum emitters in addition to improving the count rate, and can be generalized to other emitters in 2D materials or in planar photonic structures.

physics.optics↗

arXiv2024

Photon statistics of resonantly driven spectrally diffusive quantum emitters

In the solid state, a large variety of single-photon emitters present high quality photophysical properties together with a potential for integration. However, in many cases, the host matrix induces fluctuations of the emission wavelength in time, limiting the potential applications based on indistinguishable photons. A deep understanding of the underlying spectral diffusion processes is therefore of high importance for improving the stability of the light emission. Here, we theoretically investigate the photon statistics of an emitter driven by a resonant laser, and subject to either of two qualitatively different stationary spectral diffusion processes - a continuous diffusion process and a process based on discrete spectral jumps, both of which being known to model the spectral diffusion of various solid-state emitters. We show that the statistics of light emission carries several experimentally accessible signatures that allow to discriminate between the two classes of models, both at short times in the intensity correlation function, and at long times in the fluctuations of the integrated intensity. These results establish that resonant excitation combined with photon statistics offers a rich access to the spectral diffusion processes, yielding information that goes beyond the bare characterization of the inhomogeneous shape and noise correlation time. Incidentally, our findings shed a new light on recent experimental results of spectral diffusion of B centers in hexagonal boron nitride, providing more insight in their spectral diffusion mechanisms.

physics.optics↗

arXiv2023

Top-down integration of a hBN quantum emitter in a monolithic photonic waveguide

Integrated quantum photonics, with potential applications in quantum information processing, relies on the integration of quantum emitters into on-chip photonic circuits. Hexagonal boron nitride (hBN) is recognized as a material that is compatible with such implementations, owing to its relatively high refractive index and low losses in the visible range, together with advantageous fabrication techniques. Here, we combine hBN waveguide nanofabrication with the recently demonstrated local generation of quantum emitters using electron irradiation to realize a fully top-down elementary quantum photonic circuit in this material, operating at room temperature. This proof of principle constitutes a first step towards deterministic quantum photonic circuits in hBN.

physics.optics↗

arXiv2023

Investigating the fast spectral diffusion of a quantum emitter in hBN using resonant excitation and photon correlations

The ability to identify and characterize homogeneous and inhomogeneous dephasing processes is crucial in solid-state quantum optics. In particular, spectral diffusion leading to line broadening is difficult to evidence when the associated timescale is shorter than the inverse of the photon detection rate. Here, we show that a combination of resonant laser excitation and second-order photon correlations allows to access such fast dynamics. The resonant laser drive converts spectral diffusion into intensity fluctuations, leaving a signature in the second-order coherence function $g^{(2)}(τ)$ of the scattered light that can be characterized using two-photon coincidences -- which simultaneously provides the homogeneous dephasing time. We experimentally implement this method to investigate the fast spectral diffusion of a color center generated by an electron beam in the two-dimensional material hexagonal boron nitride. The $g^{(2)}(τ)$ function of the quantum emitter measured over more than ten orders of magnitude of delay times, at various laser powers, establishes that the color center experiences spectral diffusion at a characteristic timescale of a few tens of microseconds, while emitting Fourier-limited single photons ($T_2/2T_1 \sim 1$) between spectral jumps.

quant-ph↗

arXiv2023

Two-photon interference from a quantum emitter in hexagonal boron nitride

Recently discovered quantum emitters in two-dimensional (2D) materials have opened new perspectives of integrated photonic devices for quantum information. Most of these applications require the emitted photons to be indistinguishable, which has remained elusive in 2D materials. Here, we investigate two-photon interference of a quantum emitter generated in hexagonal boron nitride (hBN) using an electron beam. We measure the correlations of zero-phonon-line photons in a Hong-Ou-Mandel (HOM) interferometer under non-resonant excitation. We find that the emitted photons exhibit a partial indistinguishability of $0.44 \pm 0.11$ in a 3 ns time window, which corresponds to a corrected value of $0.56 \pm 0.11$ after accounting for imperfect emitter purity. The dependence of the HOM visibility on the width of the post-selection time window allows us to estimate the dephasing time of the emitter to be $\sim 1.5$ ns, about half the limit set by spontaneous emission. A visibility above 90 % is under reach using Purcell effect with up-to-date 2D material photonics.

quant-ph↗

arXiv2022

Cathodoluminescence monitoring of quantum emitter activation in hexagonal boron nitride

The ability to locally activate or generate quantum emitters in two-dimensional materials is of major interest for the realization of integrated quantum photonic devices. In particular, hexagonal boron nitride (hBN) has recently been shown to allow a variety of techniques for obtaining quantum emitters at desired locations. Here, we use cathodoluminescence (CL) to monitor in situ the local activation of color centers by an electron beam in hBN. We observe that the CL signal saturates at a given surface dose, independently of the electron current density. Based on photoluminescence and photon correlations, we show that the number of photoactive color centers is proportional to the CL signal, and we estimate the maximum density of quantum emitters that can be generated by our technique. Our results provide insights about the activation mechanism and could help to optimize the controlled generation of single photon sources in hexagonal boron nitride.

physics.app-ph↗

arXiv2022

First-order coherence of light emission from inhomogeneously broadened mesoscopic ensembles

Inhomogeneous broadening is well known to hinder individual characteristics of emitters, supplanting the single-particle properties by their broader probability distribution. Here, we present an analysis of the emission spectra of mesoscopic ensembles of inhomogeneously distributed emitters below the thermodynamic limit (10 - 10^4 emitters). Based on a simple analytical model and an extensive numerical analysis, we show that the number and individual linewidths of the emitters can be directly estimated from the ensemble autocorrelation function in spite of an inhomogeneously broadened emission. As an application, we analyze the photoluminescence of colloidal nanocrystal aggregates embedded in a gold shell. Our general method can be applied to a wide range of mesoscopic many-body systems and could provide new insights into their first-order coherence properties.

physics.optics↗

arXiv2021

Position-controlled quantum emitters with reproducible emission wavelength in hexagonal boron nitride

Single photon emitters (SPEs) in low-dimensional layered materials have recently gained a large interest owing to the auspicious perspectives of integration and extreme miniaturization offered by this class of materials. However, accurate control of both the spatial location and the emission wavelength of the quantum emitters is essentially lacking to date, thus hindering further technological steps towards scalable quantum photonic devices. Here, we evidence SPEs in high purity synthetic hexagonal boron nitride (hBN) that can be activated by an electron beam at chosen locations. SPE ensembles are generated with a spatial accuracy better than the cubed emission wavelength, thus opening the way to integration in optical microstructures. Stable and bright single photon emission is subsequently observed in the visible range up to room temperature upon non-resonant laser excitation. Moreover, the low-temperature emission wavelength is reproducible, with an ensemble distribution of width 3 meV, a statistical dispersion that is more than one order of magnitude lower than the narrowest wavelength spreads obtained in epitaxial hBN samples. Our findings constitute an essential step towards the realization of top-down integrated devices based on identical quantum emitters in 2D materials.

physics.optics↗

arXiv2019

Second-order photon correlation measurement with picosecond resolution

The second-order correlation function of light $g^{(2)}(τ)$ constitutes a pivotal tool to quantify the quantum behavior of an emitter and in turn its potential for quantum information applications. The experimentally accessible time resolution of $g^{(2)}(τ)$ is usually limited by the jitter of available single photon detectors. Here, we present a versatile technique allowing to measure $g^{(2)}(τ)$ from a large variety of light signals with a time resolution given by the pulse length of a mode-locked laser. The technique is based on frequency upconversion in a nonlinear waveguide, and we analyze its properties and limitations by modeling the pulse propagation and the frequency conversion process .We measure $g^{(2)}(τ)$ from various signals including light from a quantum emitter - a confined exciton-polariton structure - revealing its quantum signatures at a scale of a few picoseconds and demonstrating the capability of the technique.

quant-ph↗

arXiv2019

Quantum correlations of confined exciton-polaritons

Cavity-polaritons in semiconductor microstructures have emerged as a promising system for exploring nonequilibrium dynamics of many-body systems. Key advances in this field, including the observation of polariton condensation, superfluidity, realization of topological photonic bands, and dissipative phase transitions, generically allow for a description based on a mean-field Gross-Pitaevskii formalism. While observation of polariton intensity squeezing and decoherence of a polarization entangled photon pair by a polariton condensate provide counter-examples, quantum effects in these experiments show up at high polariton occupancy. Going beyond into the regime of strongly correlated polaritons requires the observation of a photon blockade effect where interactions are strong enough to suppress double occupancy of a photonic lattice site. Here, we report the observation of quantum correlations between polaritons in a fiber cavity which spatially confines polaritons into an area of 3 $μ$m$^2$. Photon correlation measurements show that careful tuning of the coupled system allows for a modest photon blockade effect as evidenced by a reduction of simultaneous two-polariton generation probability by 5 %. Concurrently, our experiments provide an unequivocal measurement of the polariton interaction strength, thereby resolving the controversy stemming from recent experimental reports. Our findings constitute a first essential step towards the realization of strongly interacting photonic systems.

cond-mat.mes-hall↗

arXiv2017

Quantum interface between photonic and superconducting qubits

We show that optically active coupled quantum dots embedded in a superconducting microwave cavity can be used to realize a fast quantum interface between photonic and transmon qubits. Single photon absorption by a coupled quantum dot results in generation of a large electric dipole, which in turn ensures efficient coupling to the microwave cavity. Using cavity parameters achieved in prior experiments, we estimate that bi-directional microwave-optics conversion in nanosecond timescales with efficiencies approaching unity is experimentally feasible with current technology. We also outline a protocol for in-principle deterministic quantum state transfer from a time-bin photonic qubit to a transmon qubit. Recent advances in quantum dot based quantum photonics technologies indicate that the scheme we propose could play a central role in connecting quantum nodes incorporating cavity-coupled superconducting qubits.

quant-ph↗