arXiv subjects

B. A. Brown

Publications and source records attributed to B. A. Brown.

At least 19 recordsLinked to original sources

arXiv2026

Precision $β$-delayed charged-particle emission spectroscopy at FRIB: Proof of principle with the $β$-decay of $^{25}\mathrm{Si}$

We report on the $β$-delayed proton and $γ$-ray emission from $^{25}\mathrm{Si}$, measured at the Facility for Rare Isotope Beams (FRIB). Low-energy $^{25}\mathrm{Si}$ ions extracted from the Advanced Cryogenic Gas Stopper were implanted into a thin carbon foil surrounded by a compact, highly segmented array of silicon detector telescopes and two high-purity germanium detectors. This setup provides high-resolution charged-particle spectroscopy, establishing a proof of principle for precision stopped-beam decay studies at FRIB. We reconstruct the $^{25}\mathrm{Si}$ decay scheme, resolving new high-energy proton transitions and determining the feeding to excited states in $^{24}\mathrm{Mg}$. The observation of spectral interference patterns enables firm spin and parity assignments for highly excited states in $^{25}\mathrm{Al}$. The $^{25}\mathrm{Si}$ $β$-strength distribution is extracted and compared with large-scale shell-model calculations.

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arXiv2026

Core Breaking at Low Spin in $^{68}$Zn from Nuclear Resonance Fluorescence

Low-spin excited states in $^{68}$Zn have been studied at the High Intensity Gamma-Ray Source (HI$γ$S) from the ground state up to the particle emission threshold using the nuclear resonance fluorescence technique (NRF) and the newly developed Clover Array. Low-spin levels were excited by linearly-polarized, $2.90 - 9.79$ MeV photon beams. Spin-parity quantum numbers as well as associated $M1$ and $E1$ decay strengths were determined for a large fraction of the 158 states observed. In addition, long-duration coincidence measurements at 9.46 and 9.79 MeV enabled the investigation of the level scheme near the ground state. The results have been interpreted with shell-model calculations using two different model spaces and several effective interactions often used to describe nuclei in this mass region. While the structure near the ground state can be understood in terms of excitations involving solely valence nucleons, core breaking is required to account for the evolution of the total $M1$ strength at excitation energies above $\sim5$ MeV.

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arXiv2026

Rapid structural evolution of neutron-rich silicon isotopes toward N = 28

Neutron-rich Si isotopes represent a unique case of shell evolution, exhibiting a robust shell closure at $N=20$ and pronounced quadrupole collectivity at $N = 28$. We report lifetime measurements of excited states in $^{40}$Si and the first simultaneous lifetime and heavy-ion inelastic-scattering measurements in $^{41}$Si. In $^{40}$Si, the extracted lifetimes for the $2_1^+$ and $(2_2^+)$ states indicate moderate quadrupole collectivity at $N=26$, together with signatures of triaxiality. In $^{41}$Si, two near-degenerate states at 570 and 658~keV exhibit comparable $B(E2)$ strengths as extracted from inelastic scattering, while the measured lifetimes indicate dominant $M1$ decays. The combined lifetime and inelastic-scattering results suggest an evolution toward oblate shape, consistent with large-scale shell-model predictions.

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arXiv2026

High-Precision Mass Measurements of 52Ni and 51Co Reveal Breakdown of the Isobaric Multiplet Mass Equation in the f p Shell

We performed high-precision mass measurements of the proton-rich nuclei $^{52}$Ni and $^{51}$Co with the LEBIT Penning trap at the Facility for Rare Isotope Beams (FRIB). For $^{52}$Ni, a mass excess of $-22474.8(2.2)$~keV was determined, which is consistent with a recent storage-ring measurement at the Cooler-Storage Ring (CSRe) but has a factor 37 improved precision. For $^{51}$Co, we obtained a mass excess of $-27375.1(5.7)$~keV, agreeing with a recent CSRe result, while reducing the uncertainty by a factor~2. Combining our mass value for $^{52}$Ni with the known two-proton decay energy of $^{54}$Zn, we determined the mass excess of $^{54}$Zn to be $-6463(42)$~keV. These new mass values reveal a substantial breakdown of the isobaric mass multiplet equation for $A=52$ and $A=54$, and provide stringent benchmarks for isospin-symmetry-breaking effects in the proton-rich $fp$-shell, favoring theoretical descriptions that omit the Coulomb-exchange term.

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arXiv2026

$l$-forbidden $\mathbf{M1}$ strengths near $^{100}$Sn from knockout reactions in Cd and Sn

Neutron knockout reactions on beams of $^{104,102}$Cd, and $^{104}$Sn are presented. States in the residual $^{103,101}$Cd and $^{103}$Sn nuclei are populated, including low-lying $7/2^+$ states of $νg_{7/2}$ character. These states have half-lives $\approx 400$ ps due to their low energy and hindered $B(M1; 7/2^+ \rightarrow 5/2^+)$ strengths. The excited-state half-lives were measured using their Doppler-shifted lineshapes, and the resulting $B(M1)$ strengths are compared to Valence Space In Medium Similarity Renormalization Group (VS-IMSRG) calculations. The VS-IMSRG calculations under-predict the $l$-forbidden $M1$ strengths in the $^{100}$Sn region, as well as in other regions of the nuclear chart near $^{40}$Ca and $^{208}$Pb.

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arXiv2026

Electromagnetic Properties of the N=50 Isotones with the p35-i3 Hamiltonian

The nuclei with 50 neutrons that lie between $^{78}$Ni and $^{100}$Sn have provided benchmark studies of the nuclear shell model for protons in the $\{0f_{5/2}, 1p_{3/2}, 1p_{1/2}, 0g_{9/2}\}$ model space. New Hamiltonians for this model space have recently been obtained based on valence-space in-medium renormalization-group (VS-IMSRG) methods with two- and three-nucleon interactions. The two-body matrix elements (TBME) obtained from these ab-initio methods served as the starting point for singular-value decomposition (SVD) method fits of the TBME to experimental binding energies and excitation energies, resulting in Hamiltonians called p35-i2, p35-i3 and p30-i3. In this paper, magnetic moments, quadrupole moments, $B(M1)$ and $B(E2)$ values obtained with these Hamiltonians are presented and compared to experiment. Results obtained from various Hamiltonians are compared to assess the theoretical uncertainties.

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arXiv2025

Beta-decay Half Lives beyond $^{54}$Ca: A Systematic Survey of Decay Properties approaching the Neutron Dripline

In an experiment performed at the Facility for Rare Isotope Beams (FRIB) using the FRIB Decay Station initiator (FDSi), 15 new half lives of isotopes near $^{54}$Ca were measured. A new method of extracting lifetimes from experimental data, taking into account the unknown $β$-delayed neutron emission branches of very neutron-rich nuclei, was developed to enable systematic uncertainty analysis. The experiment observed a dramatic change in the half-life systematics for the isotopes with neutron number N =34. Beyond N =34, the decline of nuclear lifetime is much slower, leading to longer than anticipated lifetimes for near-dripline nuclei. State-of-the-art shell-model calculations can explain the experimental results for Z$>$19 nuclei, revealing the imprint of shell effects and the need for modification of single-particle neutron states. The results from a newly developed QRPA model with potential for making global predictions were also tested against the experimental results and good agreement was found.

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arXiv2025

Extraction of the non-spin- and spin-transfer isovector responses via the $^{12}\mathrm{C}(^{10}\mathrm{Be},{}^{10}\mathrm{B}+γ)^{12}\mathrm{B}$ reaction

The isovector response in $^{12}$B was investigated via the $^{12}$C($^{10}\mathrm{Be}$,$^{10}\mathrm{B}$+$γ$)$^{12}$B$^\ast$ reaction at $100 A \, \mathrm{MeV}$. By utilizing the $γ$-decay properties of the 1.74 MeV $0^{+}$ and 0.718 MeV $1^{+}$ states in $^{10}\mathrm{B}$, the separate extraction of the non-spin-transfer ($ΔS=0$) and spin-transfer ($ΔS=1$) isovector responses up to an excitation energy of 50 MeV in $^{12}$B in a single measurement is demonstrated. The experimental setup employed the S800 spectrometer to detect and analyze the $^{10}\mathrm{B}$ ejectiles and the Gamma-Ray Energy Tracking In-beam Nuclear Array (GRETINA) for obtaining the Doppler-reconstructed spectrum for $γ$-rays emitted in-flight by $^{10}\mathrm{B}$. A $^{12}$C foil was placed at the pivot point of the spectrograph. The $^{12}$B reaction product was not detected. Contributions from transitions associated with the transfer of different units of angular momentum in the non-spin- and spin-transfer responses were analyzed using a multipole decomposition analysis. The extracted non-spin-dipole ($ΔS=0$, $ΔL=1$) and spin-dipole ($ΔS=1$, $ΔL=1$) responses were found to be consistent with available data from other charge-exchange probes, validating the non-spin- and spin-transfer filters used. While statistical uncertainties and experimental resolutions were relatively large due to the modest intensity of the $^{10}\mathrm{Be}$ secondary beam, the results show that, with the much higher intensities that will be available at new rare-isotope beam facilities, the ($^{10}\mathrm{Be}$,$^{10}\mathrm{B}$+$γ$) reaction and its $ΔT_{z}=-1$ partner, the ($^{10}$C,$^{10}\mathrm{B}$+$γ$) reaction, are powerful tools for elucidating the isovector non-spin- and spin-transfer responses in nuclei.

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arXiv2025

Universal Effective Charges in the $sd$ and $fp$ Shells

The 247-keV state in $^{54}$Sc, populated in the $β$ decay of $^{54}$Ca, is reported here as a nanosecond isomer with a half-life of 26.0(22) ns. The state is interpreted as the $1^+$ member of the $πf_{7/2}\otimesνf_{5/2}$ spin-coupled multiplet, which decays to the $3^+,πf_{7/2} \otimes νp_{1/2}$ ground state. The new half-life corresponds to a pure $E2$ transition with a strength of 1.93(16) W.u., providing the most precise, unambiguous $B(E2)$ value in the neutron-rich $fp$ region to date for a nucleus with valence protons above $Z=20$. Notably, it is roughly four times larger than the $B(E2; 1/2^{-} \rightarrow 5/2^{-})$ value in $^{55}$Ca. The results, as compared to semi-empirical and ab initio shell-model calculations, indicate (1) a weak $N=34$ sub-shell gap relative to $N = 32$, (2) a large $E2$ enhancement in Sc as compared to Ca due to $1p-1h$ proton excitations across $Z=28$, and (3) empirical effective proton and neutron charges, $e_π$ = 1.30(8)$e$ and $e_ν$ = 0.452(7)$e$, respectively, that are in contrast to reports of $e_π\approx 1.1-1.15e$ and $e_ν\approx 0.6-0.8e$ for $fp$-shell nuclei near $N = Z$. We demonstrate that these reports are erroneous and that, in fact, a universal set of effective charges can be used across the $sd$ and $fp$ shells.

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arXiv2025

Exploring Isospin Symmetry Breaking in Exotic Nuclei: High-Precision Mass Measurement of 23Si and Shell-Model Calculations of T = 5/2 Nuclei

We present a high-precision mass measurement of the proton-rich nucleus 23Si, performed with the LEBIT Penning trap at the Facility for Rare Isotope Beams (FRIB) utilizing the time-of-flight ion cyclotron resonance (TOF-ICR) technique. We determined a mass excess of 23362.9(5.8) keV, which agrees with a recent storage-ring measurement from CSRe but has a factor 20 improved precision. 23Si is hence the nucleus with the most precisely known mass of all nuclei with an isospin projection of Tz =-5/2. We performed shell-model calculations with the USDC and USDCm Hamiltonians to study binding energy differences and Thomas-Ehrmann shifts in mirror systems with an isospin up to T = 5/2. Our experimental result and other recently reported masses of neutron-deficient sd-shell nuclei agree well with the theoretical predictions, demonstrating that isospin symmetry breaking in sd-shell nuclei, even at high isospin values, is well described by modern shell-model calculations.

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arXiv2025

Extremely large oblate deformation of the first excited state in $^{12}$C: a new challenge to modern nuclear theory

A Coulomb-excitation study of the high-lying first excited state at 4.439 MeV in the nucleus $^{12}$C has been carried out using the $^{208}$Pb($^{12}$C,$^{12}$C$^*$)$^{208}$Pb$^*$ reaction at 56 MeV and the {\sc Q3D} magnetic spectrograph at the Maier-Leibnitz Laboratorium in Munich. High-statistics achieved with an average beam intensity of approximately 10$^{11}$ ions/s together with state-of-the-art {\it ab initio} calculations of the nuclear dipole polarizability permitted the accurate determination of the spectroscopic quadrupole moment, $Q_{_S}(2_{_1}^+) = +0.076(30)$~eb, in agreement with previous measurements. Combined with previous work, a weighted average of $Q_{_S}(2_{_1}^+) = +0.090(14)$ eb is determined, which includes the re-analysis of a similar experiment by Vermeer and collaborators, $Q_{_S}(2_{_1}^+) = +0.103(20)$~eb. Such a large oblate deformation challenges modern nuclear theory and emphasizes the need of $α$ clustering and associated triaxiality effects for full convergence of $E2$ collective properties.

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arXiv2025

Extension of the particle x-ray coincidence technique: The lifetimes and branching ratios apparatus

The particle x-ray coincidence technique (PXCT) was originally developed to measure average lifetimes in the $10^{-17}-10^{-15}$~s range for proton-unbound states populated by electron capture (EC). We have designed and built the Lifetimes and Branching Ratios Apparatus (LIBRA) to be used in the stopped-beam area at the Facility for Rare Isotope Beams that extends PXCT to measure lifetimes and decay branching ratios of resonances populated by EC/$β^+$ decay. The first application of LIBRA aims to obtain essential nuclear data from $^{60}$Ga EC/$β^+$ decay to constrain the thermonuclear rates of the $^{59}$Cu$(p,γ)^{60}$Zn and $^{59}$Cu$(p,α)^{56}$Ni reactions, and in turn, the strength of the NiCu nucleosynthesis cycle, which is predicted to significantly impact the modeling of type I x-ray burst light curves and the composition of the burst ashes. Detailed theoretical calculations, Monte Carlo simulations, and performance tests with radioactive sources have been conducted to validate the feasibility of employing LIBRA for the $^{60}$Ga experiment. LIBRA can be utilized to measure most essential ingredients needed for charged-particle reaction rate calculations in a single experiment, in the absence of direct measurements, which are often impractical for radioactive reactants.

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arXiv2025

Improving the predictive power of empirical shell-model Hamiltonians

We present two developments which enhance the predictive power of empirical shell-model Hamiltonians for cases in which calibration data are sparse. A recent improvement in the ab initio derivation of effective Hamiltonians leads to a much better starting point for the optimization procedure. In addition, we introduce a protocol to avoid overfitting, enabling a more reliable extrapolation beyond available data. These developments will enable more robust predictions for exotic isotopes produced at rare isotope beam facilities and in astrophysical environments.

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arXiv2024

In-beam $γ$-ray spectroscopy towards the proton dripline: The curious case of $^{32}$Ar

High-resolution in-beam $γ$-ray spectroscopy was used to study excited states of the neutron-deficient nucleus $^{32}$Ar populated in fast-beam induced four- and six-nucleon removal reactions from $^{36,38}$Ca. One new $γ$-ray transition and indications for an additional two were found, allowing for a glimpse at the level scheme beyond the known $2^+_1$ state. The nature of the new $1900(4)$-keV transition is discussed in the context of the known energy spectrum of the mirror nucleus $^{32}$Si and shell-model calculations using the FSU and SDPF-M cross-shell effective interactions. Its resulting parent state at $3767(5)$ keV, more than $1.3$ MeV above the proton separation energy, is tentatively assigned to have mixed sd-shell and $2p$-$2h$ character. It might either be the mirror of the $J^π=2^+_2$ state of $^{32}$Si at $4230.8(8)$ keV, but with a decay branch favoring a transition to the $2^+_1$ over the ground state, or the mirror of the $4983.9(11)$-keV state with quantum numbers $0^+$. The resulting mirror-energy differences of $-473(5)$ and $-1218(5)$ keV are both sizable when compared to systematics; in the latter case it would, in fact, be among the largest reported to date in the entire nuclear chart or suggest the potential existence of an additional, hitherto unidentified, low-lying $0^+$ state of $^{32}$Si.

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arXiv2024

In-beam $γ$-ray spectroscopy of negative-parity states of $^{37}$K populated in dissipative reactions

In-beam $γ$-ray spectroscopy was used to study excited states of the neutron-deficient nucleus $^{37}$K populated in fast-beam inelastic-scattering and proton-removal reactions at high-momentum loss. New $γ$-ray transitions and $γγ$ coincidence relationships were established using the $γ$-ray tracking array GRETINA. The extension of the level scheme up to the first $(13/2^-)$ state highlights the potential of this recently demonstrated population pathway for studies of isospin symmetry involving mirror-energy differences. The nature of the newly identified states is discussed in comparison to shell-model calculations with the FSU cross-shell effective interaction. The calculated occupation numbers of individual orbitals are shown to offer a consistent explanation of the measured mirror-energy differences between $^{37}$K and $^{37}$Ar.

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arXiv2024

Large quadrupole deformation in $^{20}$Ne challenges rotor model and modern theory: urging for $α$ clusters in nuclei

The spectroscopic quadrupole moment of the first excited state, $Q_{_S}(2^{+}_{1})$, at 1.634 MeV in $^{20}$Ne was determined from sensitive reorientation-effect Coulomb-excitation measurements using a heavy target and safe energies well below the Coulomb barrier. Particle-$γ$ coincidence measurements were collected at iThemba LABS with a digital data-acquisition system using the {\sc AFRODITE} array coupled to an annular, doubled-sided silicon detector. A precise value of $Q_{_S}(2^{+}_{1})=-0.22(2)$ eb was determined at backward angles in agreement with the only safe-energy measurement prior to this work, $Q_{_S}(2^{+}_{1})=-0.23(8)$ eb. This result adopts 1$\hbarω$ shell-model calculations of the nuclear dipole polarizability of the 2$^+_1$ state that contributes to the effective quadrupole interaction and determination of $Q_{_S}(2^{+}_{1})$. It disagrees, however, with the ideal rotor model for axially-symmetric nuclei by almost $3σ$. Larger discrepancies are computed by modern state-of-the-art calculations performed in this and prior work, including {\it ab initio} shell model with chiral effective interactions and the multi-reference relativistic energy density functional ({\sc MR-EDF}) model. The intrinsic nucleon density of the 2$^+_1$ state in $^{20}$Ne calculated with the {\sc MR-EDF} model illustrates the presence of $α$ clustering, which explains the largest discrepancy with the rotor model found in the nuclear chart and motivates the explicit inclusion of $α$ clustering for full convergence of $E2$ collective properties.

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arXiv2024

$^{11}$B states above the $α$-decay threshold studied via $^{10}$B$(d,p){}^{11}$B

The resonance region of $^{11}$B covering excitation energies from 8.4 MeV to 13.6 MeV was investigated with the $(d,p)$ reaction performed on an enriched $^{10}$B target at the Florida State University Super-Enge Split-Pole Spectrograph of the John D. Fox Superconducting Linear Accelerator Laboratory. Complementary measurements were performed with a target enriched in $^{11}$B to identify possible $^{12}$B contaminants in the $(d,p)$ reaction. Four strongly populated $^{11}$B states were observed above the $α$-decay threshold. Angular distributions were measured and compared to DWBA calculations to extract angular momentum transfers and $^{10}\mathrm{B}\left(3^+\right)+n$ spectroscopic factors. The recently observed and heavily discussed resonance at 11.4 MeV in $^{11}$B was not observed in this work. This result is consistent with the interpretation that it is predominantly a $^{10}\mathrm{Be}\left(0^+\right)+p$ resonance with a possible additional $^{7}\mathrm{Li}+α$ contribution. The predicted $^{10}\mathrm{B}\left(3^+\right)+n$ resonance at 11.6 MeV, analogous to the 11.4-MeV proton resonance, was not observed either. Upper limits for the $^{10}\mathrm{B}\left(3^+\right)+n$ spectroscopic factors of the 11.4-MeV and 11.6-MeV states were determined. In addition, supporting configuration interaction shell model calculations with the effective WBP interaction are presented.

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arXiv2024

Proton-unbound states in $^{24}{\rm Al}$ relevant for the $^{23}{\rm Mg}(p,γ)$ reaction in novae

Background: The nucleosynthesis of several proton-rich nuclei is determined by radiative proton-capture reactions on unstable nuclei in nova explosions. One such reaction is $^{23}{\rm Mg}(p,γ)^{24}{\rm Al}$, which links the NeNa and MgAl cycles in oxygen-neon (ONe) novae. Purpose: To extract $^{23}{\rm Mg}(p,γ)$ resonance strengths from a study of proton-unbound states in $^{24}{\rm Al}$, produced via the $^{24}$Mg($^{3}$He,$t$) reaction. Methods: A beam of $^3 {\rm He}^{2+}$ ions at 50.7 MeV was used to produce the states of interest in $^{24}$Al. Proton-triton angular correlations were measured with a $K=600$ QDD magnetic spectrometer and a silicon detector array, located at iThemba LABS, South Africa. Results: We measured the excitation energies of the four lowest proton-unbound states in $^{24}$Al and place lower-limits on $Γ_p/Γ$ values for these four states. Together with shell-model calculations of partial gamma widths, the experimental data are also used to determine resonance strengths for the three lowest $^{23}{\rm Mg}(p,γ)^{24}{\rm Al}$ resonances. Conclusions: The energy of the dominant first $^{23}{\rm Mg}(p,γ)$ resonance is determined to be $E_{r} = 478 \pm 4$ keV, with a resonance strength $ωγ= 19 \pm 9$ meV.

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