arXiv subjects

B. A. Ivanov

Publications and source records attributed to B. A. Ivanov.

At least 19 recordsLinked to original sources

arXiv2025

Photoengineering the Magnon Spectrum in an Insulating Antiferromagnet

Femtosecond optical pulses have opened a new frontier in ultrafast dynamics, enabling direct access to fundamental interactions in quantum materials. In antiferromagnets (AFMs), where the fundamental quantum mechanical exchange interaction governs spin dynamics, this access is especially compelling, enabling the excitation of magnons - collective spin-wave modes - that naturally reach terahertz (THz) frequencies and supersonic velocities. Femtosecond optical pulses provided a route to coherently excite such magnons across the entire Brillouin zone. Controlling their spectral properties - such as the magnon gap and dispersion - represents the next monumental step, enabling dynamic tuning of group velocities, coherence, and interaction pathways. Yet, achieving this remains a challenge, requiring ultrafast and long-lasting manipulation of the underlying exchange interaction. Here, we show that in DyFeO3 - an insulating AFM with strongly coupled electronic and magnetic degrees of freedom - resonant above-bandgap optical excitation leads to a dramatic renormalization of the THz magnon spectrum, including a near-total collapse of the magnon gap. Our analysis reveals this transformation to be consistent with a transient reduction of the exchange interaction by nearly 90% in the near-surface nanoscale region. These findings establish a pathway for light-driven, nanoscale control of AFM spin dynamics, opening opportunities for reconfigurable, high-speed magnonic and spintronic applications.

cond-mat.str-el↗

arXiv2024

Instability in domain wall dynamics in almost compensated ferrimagnets

Nanoscale self-localized topological spin textures, such as domain walls and skyrmions, are of interest for the fundamental physics of magnets and spintronics applications. Ferrimagnets (FiMs), in the region close to the angular momentum compensation point, are promising materials because of their ultrafast spin dynamics at nonzero magnetization. In this work, we study specific features of the FiM domain wall (DW) dynamics, which are absent in both ferromagnets (FM) and antiferromagnets (AFM). In low-damping FMs and AFMs ($α\ll 1$), the non-stationary forced motion of DWs is characterized by slow ($t_{diss}\propto 1/α$) changes of the DW's velocity and internal structure for all accepted values of the DW energy $E$ and its linear momentum $P$ -- a consequence of the stability of DWs for any value of $P$. In contrast, the dispersion law of FiM DWs has specific points, $P=P_{cr}$ and $E_{cr}=E(P_{cr})$, such that stable DWs are only present for $P<P_{cr}$, i.e., $P_{cr}$ and $E_{cr}$ act as endpoints in the $E(P)$ dependence. We show that when a field-like torque driven DW reaches this endpoint, it falls into a highly-non-equilibrium state with the excitation of fast ($t \ll t_{diss}$) and highly-nonlinear intra-wall magnetization dynamics, covering a wide frequency range up until the frequencies of propagating spin waves. The domain wall finally throws off an "excessive" energy by a short "burst" of the propagating spin waves and returns to the stationary state; the full picture of the forced motion is a periodic repetition of such "explosive" events.

cond-mat.mes-hall↗

arXiv2024

Double pulse all-optical coherent control of ultrafast spin-reorientation in antiferromagnetic rare-earth orthoferrite

A pair of circularly polarized laser pulses of opposite helicities are shown to control the route of spin reorientation phase transition in rare-earth antiferromagnetic orthoferrite (Sm$_{0.55}$Tb$_{0.45}$)FeO$_3$. The route can be efficiently controlled by the delay between the pulses and the sample temperature. Simulations employing previously published models of \mbox{laser-induced} spin dynamics in orthoferrites failed to reproduce the experimental results. We suggest that the failure is due to neglected temperature dependence of the antiferromagnetic resonance damping in the material. Taking into account the experimentally deduced temperature dependence of the damping, we obtained good agreement between the simulations and the experiment.

cond-mat.str-el↗

arXiv2024

Emission of fast-propagating spin waves by an antiferromagnetic domain wall driven by spin current

Antiferromagnets (AFMs) have great benefits for spintronic applications such as high frequencies (up to THz), high speeds (up to tens of km/s) of magnetic excitations, and field-free operation. Advanced devices will require high-speed propagating spin waves (SWs) as signal carriers, i.e., SWs with high k-vectors, the excitation of which remains challenging. We show that a domain wall (DW) in anisotropic AFM driven by the spin current can be a source of such propagating SWs with high frequencies and group velocities. In the proposed generator, the spin current, with polarization directed along the easy anisotropy axis, excites the precession of the Néel vector within the DW. The threshold current is defined by the value of the anisotropy in the hard plane, and the frequency of the DW precession is tuneable by the strength of the spin current. We show that the above precession of spins inside the DW leads to robust emission of high-frequency propagating SWs into the AFM strip with very short wavelengths comparable to the exchange length, which is hard to achieve by any other method.

cond-mat.mes-hall↗

arXiv2024

Optical read-out and control of antiferromagnetic Neel vector in altermagnets and beyond

Finding methods for the most efficient and fastest detection and control of magnetic domains in antiferromagnets is presently among the main challenges of magnetic research at large. We analyse the problem of optical read-out and control of the antiferromagnetic Neel vector using symmetry analysis and the principles of equilibrium thermodynamics. Following the pioneering approach of Dzyaloshinksii, we divide all antiferromagnets in three classes. It is shown that, using the magneto-optical Faraday effect or other effects which scale linearly with the antiferromagnetic Neel vector, it is possible to distinguish antiferromagnetic domains with mutually opposite Néel vectors in two of the three classes. Symmetry properties of one of these two classes are similar to those of altermagnets. The analysis also reveals multiple mechanisms to directly excite spins with light for practically every type of antiferromagnet.

cond-mat.mtrl-sci↗

arXiv2023

Antiferromagnetic Bloch line driven by spin current as room-temperature analog of a fluxon in a long Josephson junction

Antiferromagnets (AFMs) are promising materials for future high-frequency field-free spintronic applications. Self-localized spin structures can enhance their capabilities and introduce new functionalities to AFM-based devices. Here we consider a domain wall (DW), a topological soliton that bridges a connection between two ground states, similar to a Josephson junction (JJ) link between two superconductors. We demonstrate the similarities between DWs in bi-axial AFM with easy-axis primary anisotropy, driven by a spin current, and long Josephson junctions (LJJs). We found that the Bloch line (BL) in DWs resembles the fluxon state of JJs, creating a close analogy between the two systems. We propose a scheme that allows us to create, move, read, and delete such BLs. This transmission line operates at room temperature and can be dynamically reconfigured in contrast to superconductors. Results of a developed model were confirmed by micromagnetic simulations for Cr$_2$O$_3$ and DyFeO$_3$, i.e., correspondingly with weak and strong in-plane anisotropy. Overall, the proposed scheme has significant potential for use in magnetic memory and logic devices.

cond-mat.mes-hall↗

arXiv2023

Empowering Control of Antiferromagnets by THz-induced Spin Coherence

Finding efficient and ultrafast ways to control antiferromagnets is believed to be instrumental in unlocking their potential for magnetic devices operating at THz frequencies. Still, it is challenged by the absence of net magnetization in the ground state. Here, we show that the magnetization emerging from a state of coherent spin precession in antiferromagnetic iron borate FeBO$_3$ can be used to enable the nonlinear coupling of light to another, otherwise weakly susceptible, mode of spin precession. This nonlinear mechanism can facilitate conceptually new ways of controlling antiferromagnetism.

cond-mat.mtrl-sci↗

arXiv2023

Ultrafast laser-induced spin-lattice dynamics in the van der Waals antiferromagnet CoPS3

CoPS3 stands out in the family of the van der Waals antiferromagnets XPS3 (X=Mn, Ni, Fe, Co) due to the unquenched orbital momentum of the magnetic Co2+ ions which is known to facilitate the coupling of spins to both electromagnetic waves and lattice vibrations. Here, using a time-resolved magneto-optical pump-probe technique we experimentally study the ultrafast laser-induced dynamics of mutually correlated spins and lattice. It is shown that a femtosecond laser pulse acts as an ultrafast heater and thus results in the melting of the antiferromagnetic order. At the same time, the resonant pumping of the 4T1g - 4T2g electronic transition in Co2+ ions effectively changes their orbital momentum, giving rise to a mechanical force that moves the ions in the direction parallel to the orientation of their spins, thus generating a coherent Bg phonon mode at the frequency of about 4.7 THz.

cond-mat.mtrl-sci↗

arXiv2023

Oscillatory Exchange Bias Controlled by RKKY in Magnetic Multilayers

Ferromagnetic/antiferromagnetic bilayers are interfaced with normal metal/ferromagnetic bilayers to form F*/AF/N/F valves. The N-spacer thickness is chosen such that it mediates strong indirect exchange (RKKY) between the outer magnetic layers, which varies in strength/direction depending on the N thickness and in direction on switching F. The system exhibits a strong modulation of the F*/AF exchange bias, oscillating in strength syncronously with the oscillation in the interlayer RKKY exchange across the normal metal spacer. The effect is explained as due to a superposition taking place within the antiferromagnetic layer of the direct-exchange proximity effect from the F*/AF interface and the indirect RKKY exchange from F penetrating AF via N. The modulation, expressed via the strength of the F*/AF bias field, reaches 400% at the first RKKY peak.

cond-mat.mes-hall↗

arXiv2021

Coherent spin-wave transport in an antiferromagnet

Magnonics is a research field complementary to spintronics, in which the quanta of spin waves (magnons) replace electrons as information carriers, promising less energy dissipation. The development of ultrafast nanoscale magnonic logic circuits calls for new tools and materials to generate coherent spin waves with frequencies as high, and wavelengths as short, as possible. Antiferromagnets can host spin waves at THz frequencies and are therefore seen as a future platform for the fastest and the least dissipative transfer of information. However, the generation of short-wavelength coherent propagating magnons in antiferromagnets has so far remained elusive. Here we report the efficient emission and detection of a nanometer-scale wavepacket of coherent propagating magnons in antiferromagnetic DyFeO3 using ultrashort pulses of light. The subwavelength nanoscale confinement of the laser field due to large absorption creates a strongly non-uniform spin excitation profile, thereby enabling the propagation of a broadband continuum of coherent THz spin waves. The wavepacket features magnons with detected wavelengths down to 125 nm and supersonic velocities up to 13 km/s that propagate over macroscopic distances. The long-sought source of coherent short-wavelength spin carriers demonstrated here opens up new prospects for THz antiferromagnetic magnonics and coherence mediated logic devices at THz frequencies.

cond-mat.mes-hall↗

arXiv2020

Controlling the anisotropy of a van der Waals antiferromagnet with light

Magnetic van der Waals materials provide an ideal playground for exploring the fundamentals of low-dimensional magnetism and open new opportunities for ultrathin spin processing devices. The Mermin-Wagner theorem dictates that as in reduced dimensions isotropic spin interactions cannot retain long-range correlations; the order is stabilized by magnetic anisotropy. Here, using ultrashort pulses of light, we demonstrate all-optical control of magnetic anisotropy in the two-dimensional van der Waals antiferromagnet NiPS$_3$. Tuning the photon energy in resonance with an orbital transition between crystal-field split levels of the nickel ions, we demonstrate the selective activation of a sub-THz two-dimensional magnon mode. The pump polarization control of the magnon amplitude confirms that the activation is governed by the instantaneous magnetic anisotropy axis emergent in response to photoexcitation of orbital states with a lowered symmetry. Our results establish pumping of orbital resonances as a universal route for manipulating magnetic order in low-dimensional (anti)ferromagnets.

cond-mat.mtrl-sci↗

arXiv2019

Light-driven ultrafast phonomagnetism

Exciting atomic oscillations with light is a powerful technique to control the electronic properties of materials, leading to remarkable phenomena such as light-induced superconductivity and ultrafast insulator to metal transitions. Here we show that light-driven lattice vibrations can be utilised to encode efficiently spin information in a magnetic medium. Intense mid-infrared electric field pulses, tuned to resonance with a vibrational normal mode of antiferromagnetic DyFeO3, drive the emergence of long-living weak ferromagnetic order. Light-driven phonon displacements promptly lower the energy barrier separating competing magnetic states, allowing the alignment of spins to occur within a few picoseconds, via non-equilibrium dynamics of the magnetic energy landscape.

cond-mat.str-el↗

arXiv2018

Giant resonant nonlinear damping in nanoscale ferromagnets

Magnetic damping is a key metric for emerging technologies based on magnetic nanoparticles, such as spin torque memory and high-resolution biomagnetic imaging. Despite its importance, understanding of magnetic dissipation in nanoscale ferromagnets remains elusive, and the damping is often treated as a phenomenological constant. Here we report the discovery of a giant frequency-dependent nonlinear damping that strongly alters the response of a nanoscale ferromagnet to spin torque and microwave magnetic field. This novel damping mechanism originates from three-magnon scattering that is strongly enhanced by geometric confinement of magnons in the nanomagnet. We show that the giant nonlinear damping can invert the effect of spin torque on a nanomagnet leading to a surprising current-induced enhancement of damping by an antidamping torque. Our work advances understanding of magnetic dynamics in nanoscale ferromagnets and spin torque devices.

cond-mat.mes-hall↗

arXiv2018

Transient dynamics of strongly coupled spin vortex pairs: effects of anharmonicity and resonant excitation on inertial switching

Spin vortices in magnetic nanopillars are used as GHz oscillators, with frequency however essentially fixed in fabrication. We demonstrate a model system of a two-vortex nanopillar, in which the resonance frequency can be changed by an order of magnitude, without using high dc magnetic fields. The effect is due to switching between the two stable states of the vortex pair, which we show can be done with low-amplitude fields of sub-ns duration. We detail the relevant vortex-core dynamics and explain how field anharmonicity and phase control can be used to enhance the performance.

cond-mat.mes-hall↗

arXiv2018

Resonant pinning spectroscopy with spin-vortex pairs

Vortex pairs in magnetic nanopillars with strongly coupled cores and pinning of one of the cores by a morphological defect, are used to perform resonant pinning spectroscopy, in which a microwave excitation applied to the nanopillar produces pinning or depinning of the cores only when the excitation is in resonance with the rotational or gyrational eigenmodes of the specific initial state of the core-core pair. The shift in the eigenmode frequencies between the pinned and depinned states is determined experimentally and explained theoretically, and illustrates the potential for multi-core spin-vortex memory with resonant writing of information on to various stable vortex pair states. Further, it is shown how the same resonant spectroscopy techniques applied to a vortex pair can be used as a sensitive nanoscale probe for characterizing morphological defects in magnetic films.

cond-mat.mes-hall↗

arXiv2018

Chaotic dynamics in spin-vortex pairs

We report on spin-vortex pair dynamics measured at temperatures low enough to suppress stochastic core motion, thereby uncovering the highly non-linear intrinsic dynamics of the system. Our analysis shows that the decoupling of the two vortex cores is resonant and can be enhanced by dynamic chaos. We detail the regions of the relevant parameter space, in which the various mechanisms of the resonant core-core dynamics are activated. We show that the presence of chaos can reduce the thermally-induced spread in the switching time by up to two orders of magnitude.

cond-mat.mes-hall↗

arXiv2017

THz-Frequency Spin-Hall Auto-Oscillator Based on a Canted Antiferromagnet

We propose a design of a THz-frequency signal generator based on a layered structure consisting of a current-driven platinum (Pt) layer and a layer of an antiferromagnet (AFM) with easy-plane anisotropy, where the magnetization vectors of the AFM sublattices are canted inside the easy plane by the Dzyaloshinskii-Moriya interaction (DMI). The DC electric current flowing in the Pt layer creates, due to the spin-Hall effect, a perpendicular spin current that, being injected in the AFM layer, tilts the DMI-canted AFM sublattices out of the easy plane, thus exposing them to the action of a strong internal exchange magnetic field of the AFM. The sublattice magnetizations, along with the small net magnetization vector $\textbf{m}_{\rm DMI}$ of the canted AFM, start to rotate about the hard anisotropy axis of the AFM with the THz frequency proportional to the injected spin current and the AFM exchange field. The rotation of the small net magnetization $\textbf{m}_{\rm DMI}$ results in the THz-frequency dipolar radiation that can be directly received by an adjacent (e.g. dielectric) resonator. We demonstrate theoretically that the radiation frequencies in the range $f=0.05-2$~THz are possible at the experimentally reachable magnitudes of the driving current density, and evaluate the power of the signal radiated into different types of resonators, showing that this power increases with the increase of frequency $f$, and that it could exceed 1~$μ$W at $f \sim 0.5$~THz for a typical dielectric resonator of the electric permittivity $\varepsilon \sim 10$ and quality factor $Q \sim 750$.

physics.app-ph↗

arXiv2015

Static and dynamic properties of vortex pairs in asymmetric nanomagnets

Stacked spin-vortex pairs in magnetic multilayered nanopillars, with vertical separation between the vortices small compared to the vortex core size, exhibit spin dynamics absent in individual vortices. This dynamics is nonlinear and is due to the strong direct core-core coupling in the system, dominating energetically for small- signal excitation. We observe and explain the appearance of spin resonance modes, forbidden within linear dynamics, and discuss how they depend on the magnetic and morphological asymmetries in the samples.

cond-mat.mes-hall↗