arXiv subjects
Publications and source records attributed to B. B. Goldberg.
Through the utilization of index-matched GaAs immersion lens techniques we demonstrate a record extinction (12%) of a far-field focused laser by a single InAs/GaAs quantum dot. This contrast level enables us to report for the first time resonant laser transmission spectroscopy on a single InAs/GaAs quantum dot without the need for phase-sensitive lock-in detection.
We theoretically study the problem of detecting dipole radiation in an optical system of high numerical aperture in which the detector is sensitive to \textit{field amplitude}. In particular, we model the phase sensitive detector as a single-mode cylindrical optical fiber. We find that the maximum in collection efficiency of the dipole radiation does not coincide with the optimum resolution for the light gathering instrument. The calculated results are important for analyzing fiber-based confocal microscope performance in fluorescence and spectroscopic studies of single molecules and/or quantum dots.
A mass and spring model is used to calculate the phonon mode dispersion for single wall carbon nanotubes (SWNTs) of arbitrary chirality. The calculated dispersions are used to determine the chirality dependence of the radial breathing phonon mode (RBM) density. Van Hove singularities, usually discussed in the context of the single particle electronic excitation spectrum, are found in the RBM density of states with distinct qualitative differences for zig zag, armchair and chiral SWNTs. The influence the phonon mode density has on the two phonon resonant Raman scattering cross-section is discussed.
We perform tunable resonant Raman scattering on 17 semiconducting and 7 metallic singly resonant single wall carbon nanotubes. The measured scattering cross-section as a function laser energy provides information about a tube's electronic structure, the lifetime of intermediate states involved in the scattering process and also energies of zone center optical phonons. Recording the scattered Raman signal as a function of tube location in the microscope focal plane allows us to construct two-dimensional spatial maps of singly resonant tubes. We also describe a spectral nanoscale artifact we have coined the "nano-slit effect".
We use the Kramers-Heisenberg approach to derive a general expression for the resonant Raman scattering cross section from a one-dimensional (1D) system explicitly accounting for excitonic effects. The result should prove useful for analyzing the Raman resonance excitation profile lineshapes for a variety of 1D systems including carbon nanotubes and semiconductor quantum wires. We apply this formalism to a simple 1D model system to illustrate the similarities and differences between the free electron and correlated electron-hole theories.
Scattering of carriers between spatially separated zero dimensional states has been observed in a system of self-assembled In_{0.55}Al_{0.45}As quantum dots. We believe the interdot tunneling is mediated by localized states below the barrier band edge. The experiment was performed by taking photoluminescence excitation spectra at 4.2K using a near-field scanning optical microscope. Surprisingly, the excitation spectrum from individual dots does not quench to zero at any energy, even when the energy of the exciting light is tuned below the barrier band edge. On top of this continuum, narrow resonances are observed in the emission lines of individual dots. These resonances tend to occur simultaneously in several emission lines, originating from different quantum dots, evincing interdot scattering.
We report an anomalous doublet structure and low-energy satellite in the magneto-photoluminescence spectra of a two-dimensional electron system. The doublet structure moves to higher energy with increasing magnetic field and is most prominent at odd filling factors 5 and 3. The lower-energy satellite peak tunes to lower energy for increasing magnetic field between filling factor 6 and 2. These features occur at energies below the fundamental band of recombination originating from the lowest Landau level and display striking magnetic field and temperature dependence that indicates a many-body origin. Drawing on a recent theoretical description of Hawrylak and Potemski, we show that distinct mechanisms are responsible for each feature.
We observe a dramatic reduction in the degree of spin-polarization of a two-dimensional electron gas in a magnetic field when the Fermi energy moves off the mid-point of the spin-gap of the lowest Landau level, $ν=1$. This rapid decay of spin alignment to an unpolarized state occurs over small changes to both higher and lower magnetic field. The degree of electron spin polarization as a function of $ν$ is measured through the magneto-absorption spectra which distinguish the occupancy of the two electron spin states. The data provide experimental evidence for the presence of Skyrmion excitations where exchange energy dominates Zeeman energy in the integer quantum Hall regime at $ν=1$.