arXiv subjects

B. Buechner

Publications and source records attributed to B. Buechner.

At least 37 records · Page 2Linked to original sources

arXiv2013

Evidence of d-wave Superconductivity in K_(1-x)Na_xFe_2As_2 (x = 0, 0.1) Single Crystals from Low-Temperature Specific Heat Measurements

From the measurement and analysis of the specific heat of high-quality K_(1-x)Na_xFe_2As_2 single crystals we establish the presence of large T^2 contributions with coefficients alpha_sc ~ 30 mJ/mol K^3 at low-T for both x=0 and 0.1. Together with the observed square root field behavior of the specific heat in the superconducting state both findings evidence d-wave superconductivity on almost all Fermi surface sheets with an average gap amplitude of Delta_0 in the range of 0.4 - 0.8 meV. The derived Delta_0 and the observed T_c agree well with the values calculated within the Eliashberg theory, adopting a spin-fluctuation mediated pairing in the intermediate coupling regime.

cond-mat.supr-con↗

arXiv2013

Pressure dependence of the charge density wave in 1T-TaS2 and its relation to superconductivity

We present a state-of-the-art x-ray diffraction study of the charge density wave order in 1T-TaS2 as a function of temperature and pressure. Our results prove that the charge density wave, which we characterize in terms of wave vector, amplitude and the coherence length, indeed exists in the superconducting region of the phase diagram. The data further imply that the ordered charge density wave structure as a whole becomes superconducting at low temperatures, i. e, superconductivity and charge density wave coexist on a macroscopic scale in real space. This result is fundamentally different from a previously proposed separation of superconducting and insulating regions in real space and, instead, provides evidence that the superconducting and the charge density wave gap exist in separate regions of reciprocal space.

cond-mat.str-el↗

arXiv2012

Quasi-ballistic transport of Dirac fermions in a Bi2Se3 nanowire

Quantum coherent transport of Dirac fermions in a mesoscopic nanowire of the 3D topological insulator Bi2Se3 is studied in the weak-disorder limit. At very low temperatures, many harmonics are evidenced in the Fourier transform of Aharonov-Bohm oscillations, revealing the long phase-coherence length of surface states. Remarkably, from their exponential temperature dependence, we infer an unusual 1/T power law for the phase coherence length. This decoherence is typical for quasi-ballistic fermions weakly coupled to the dynamics of their environment.

cond-mat.mes-hall↗

arXiv2012

Incommensurate magnetic fluctuations and Fermi surface topology in LiFeAs

Using the angle-resolved photoemission spectroscopy (ARPES) data accumulated over the whole Brillouin zone (BZ) in LiFeAs we analyze the itinerant component of the dynamic spin susceptibility in this system in the normal and superconducting state. We identify the origin of the incommensurate magnetic inelastic neutron scattering (INS) intensity as scattering between the electron pockets, centered around the $(π,π)$ point of the BZ and the large two-dimensional hole pocket, centered around the $Γ$-point of the BZ. As the magnitude of the superconducting gap within the large hole pocket is relatively small and angle dependent, we interpret the INS data in the superconducting state as a renormalization of the particle-hole continuum rather than a true spin exciton. Our comparison indicates that the INS data can be reasonably well described by both the sign changing symmetry of the superconducting gap between electron and hole pockets as well as sign preserving gap, depending on the assumptions made for the fermionic damping.

cond-mat.supr-con↗

arXiv2012

Magnetic frustration, phase competition and the magneto-electric effect in NdFe3(BO3)4

We present an element selective resonant magnetic x-ray scattering study of NdFe3(BO3)4 as a function of temperature and applied magnetic field. Our measurements show that the magnetic order of the Nd sublattice is induced by the Fe spin order. When a magnetic field is applied parallel to the hexagonal basal plane, the helicoidal spin order is suppressed and a collinear ordering, where the moments are forced to align in a direction perpendicular to the applied magnetic field, is stabilized. This result excludes a non-collinear spin order as the origin of the magnetically induced electric polarization in this compound. Instead our data imply that magnetic frustration results in a phase competition, which is the origin of the magneto-electric response.

cond-mat.str-el↗

arXiv2012

Specific heat and upper critical field in KFe2As2 single crystals

We report low-temperature specific heat measurements for high-quality single crystalline KFe2As2 (T_c about 3.5 K). The investigated zero-field specific heat data yields an unusually large nominal Sommerfeld coefficient gamma_n of 94(3) mJ/mol K^2 which is however significantly affected by extrinsic contributions as evidenced by a sizable residual linear specific heat and various theoretical considerations including also an analysis of Kadowaki-Woods relations. Then KFe2As2 should be classified as a weak to intermediately strong coupling superconductor with a total electron-boson coupling constant lambda_tot near 1 (including a calculated weak electron-phonon coupling constant of lambda_el-ph =0.17. From specific heat and ac susceptibility studies in external magnetic fields the magnetic phase diagram has been constructed. We confirm the high anisotropy of the upper critical fields B_c2(T) ranging from a factor of 5 near T_c to a slightly reduced value approaching T=0 for fields B || ab$ and || c and show that their ratio Gamma slightly exceeds the mass anisotropy of 4.35 derived from our full-relativistic LDA-band structure calculations. Its slight reduction when approaching T=0 is not a consequence of Pauli-limiting as in less perfect samples but point likely to a multiband effect. We also report irreversibility field data obtained from ac susceptibility measurements. The double-maximum in the T-dependence of its imaginary part for fields B || c indicates a peak-effect in the T-dependence of critical currents.

cond-mat.supr-con↗

arXiv2012

KFe2As2: coexistence of superconductivity and local moment derived spin-glass

High-quality KFe2As2 single crystals have been studied by transport, magnetization and low-T specific heat measurements. Their analysis shows that superconductivity occurs (in some cases coexists) in the vicinity of disordered magnetic phases (Griffiths and spin-glass type) depending of the amount of local magnetic moments (probably excess Fe derived)and sample inhomogeneity. The achieved phenomenological description of our data including also data from the literature provides a consistent explanation of the observed non-Fermi-liquid behavior and of the nominally large experimental Sommerfeld coefficient gamma_n about 94 mJ/mol K^2. We suggest that the intrinsic value (directly related to the itinerant quasi-particles) gamma_el about 60(10)mJ/mol K^2 is significantly reduced compared with gamma_n. Then an enhanced relative jump of the electronic specific heat Delta C_el/gamma_el T_c about 0.8 and a weak total electron-boson coupling constant lambda less or about 1 follow.

cond-mat.supr-con↗

arXiv2012

Anomalously enhanced photoemission from the Dirac point and symmetry of the self-energy variations for the surface states in Bi2Se3

Accurate analysis of the photoemission intensity from the surface states of Bi2Se3 reveals two unusual features: spectral line asymmetry and anomalously enhanced photoemission from the Dirac point. The former indicates a certain symmetry of a scattering process, which results in strongly kω-dependent contribution to the imaginary part of the self-energy that changes sign while crossing both the dispersion curves and the energy of the Dirac point. The latter is hard to describe by one particle spectral function while a final state interference seems to be plausible explanation.

cond-mat.mes-hall↗

arXiv2011

Orthogonal spin arrangement as possible ground state of three - dimensional Shastry - Sutherland network in Ba3Cu3In4O12

The Ba3Cu3In4O12 stands for unique topology of the magnetic subsystem. It consists of rotated by 90\Box$^b$ relative to each other "paper-chain" columns made of vertex-sharing CuIO4 and CuIIO4 planar units. The overall pattern of the copper ions is that of a three-dimensional Shastry-Sutherland network. At high temperatures, the magnetic susceptibility follows the Curie-Weiss law with positive Weiss temperature indicating strong predominance of ferromagnetic coupling. At low temperatures, however, this compound reaches the antiferromagnetically ordered state and experiences non-trivial succession of two spin-flop and two spin-flip transitions reaching full saturation in modest magnetic fields. Here we show that the possible ground state in Ba3Cu3In4O12 can be three-dimensional orthogonal arrangement of the Cu2+ (S = 1/2) magnetic moments forming three virtually independent antiferromagnetic subsystems. In this arrangement, favored by anisotropic exchange interactions, the quantum fluctuations provide the coupling between three mutually orthogonal magnetic subsystems resulting in an impressive "order by disorder" effect.

cond-mat.mtrl-sci↗

arXiv2011

Electronic band structure of ferro-pnictide superconductors from ARPES experiment

ARPES experiments on iron based superconductors show that the differences between the measured and calculated electronic band structures look insignificant but can be crucial for understanding of the mechanism of high temperature superconductivity. Here we focus on those differences for 111 and 122 compounds and discuss the observed correlation of the experimental band structure with the superconductivity.

cond-mat.supr-con↗

arXiv2011

Calorimetric study of the superconducting and normal state properties of Ca(Fe1-xCox)2As2

We present a calorimetric study on single crystals of Ca(Fe1-xCox)2As2 (x = 0, 0.032, 0.051, 0.056, 0.063, and 0.146). The combined first order spin-density wave/structural transition occurs in the parent CaFe2As2 compound at 168 K and gradually shifts to lower temperature for low doping levels (x = 0.032 and x = 0.051). It is completely suppressed upon higher doping x = 0.056. Simultaneously, superconductivity appears at lower temperature with a transition temperature around Tc = 14.1 K for Ca(Fe0.937Co0.063)2As2. The phase diagram of Ca(Fe0.937Co0.063)2As2 has been derived and the upper critical field is found to be H(c) c2 = 11.5

cond-mat.supr-con↗

arXiv2011

Resistivity and Hall effect of LiFeAs: Evidence for electron-electron scattering

LiFeAs is unique among the broad family of FeAs-based superconductors, because it is superconducting with a rather large $T_c\simeq 18$ K under ambient conditions although it is a stoichiometric compound. We studied the electrical transport on a high-quality single crystal. The resistivity shows quadratic temperature dependence at low temperature giving evidence for strong electron-electron scattering and a tendency towards saturation around room temperature. The Hall constant is negative and changes with temperature, what most probably arises from a van Hove singularity close to the Fermi energy in one of the hole-like bands. Using band structure calculations based on angular resolved photoemission spectra we are able to reproduce all the basic features of both the resistivity as well as the Hall effect data.

cond-mat.supr-con↗

arXiv2011

Disorder-induced Spin Gap in the Zigzag Spin-1/2 Chain Cuprate Sr_{0.9}Ca_{0.1}CuO_2

We report a comparative study of 63Cu Nuclear Magnetic Resonance spin lattice relaxation rates, T_1^{-1}, on undoped SrCuO_2 and Ca doped Sr_{0.9}Ca_{0.1}CuO_2 spin chain compounds. A temperature independent T_1^{-1} is observed for SrCuO_2 as expected for an S=1/2 Heisenberg chain. Surprisingly, we observe an exponential decrease of T_1^{-1} for T < 90,K in the Ca-doped sample evidencing the opening of a spin gap. The data analysis within the J_1-J_2 Heisenberg model employing density-matrix renormalization group calculations suggests an impurity driven small alternation of the J_2-exchange coupling as a possible cause of the spin gap.

cond-mat.str-el↗

arXiv2011

Saturation field of frustrated chain cuprates: broad regions of predominant interchain coupling

An efficient and precise thermodynamic method to extract the interchain coupling (IC) of spatially anisotropic 2D or 3D spin-1/2 systems from their empirical saturation field H_s (T=0) is proposed. Using density-matrix renormalization group, hard-core boson, and spin-wave theory we study how H_s is affected by an antiferromagnetic (AFM) IC between frustrated chains described in the J_1-J_2-spin model with ferromagnetic 1st and AFM 2nd neighbor in-chain exchange. A complex 3D-phase diagram has been found. For Li2CuO2 and Y2Ca2Cu5O10, we show that H_s is solely determined by the IC and predict H_s approx 61 T for the latter.Using H_s approx 55 T from our high-field pulsed measurements one reads out a weak IC for Li2CuO2 close to that from neutron scattering.

cond-mat.str-el↗

arXiv2011

Photoemission induced gating of topological insulator

The recently discovered topological insulators exhibit topologically protected metallic surface states which are interesting from the fundamental point of view and could be useful for various applications if an appropriate electronic gating can be realized. Our photoemission study of Cu intercalated Bi2Se3 shows that the surface states occupancy in this material can be tuned by changing the photon energy and understood as a photoemission induced gating effect. Our finding provides an effective tool to investigate the new physics coming from the topological surface states and suggests the intercalation as a recipe for synthesis of the material suitable for electronic applications.

cond-mat.mes-hall↗

arXiv2010

Nanoscale electronic order in iron pnictides

The charge distribution in RFeAsO$_{1-x}$F$_x$ (R=La, Sm) iron pnictides is probed using As nuclear quadrupole resonance. Whereas undoped and optimally-doped or overdoped compounds feature a single charge environment, two charge environments are detected in the underdoped region. Spin-lattice relaxation measurements show their coexistence at the nanoscale. Together with the quantitative variations of the spectra with doping, they point to a local electronic order in the iron layers, where low- and high-doping-like regions would coexist. Implications for the interplay of static magnetism and superconductivity are discussed.

cond-mat.str-el↗

arXiv2010

An ARPES view on the high-Tc problem: phonons vs spin-fluctuations

We review the search for a mediator of high-Tc superconductivity focusing on ARPES experiment. In case of HTSC cuprates, we summarize and discuss a consistent view of electronic interactions that provides natural explanation of both the origin of the pseudogap state and the mechanism for high temperature superconductivity. Within this scenario, the spin-fluctuations play a decisive role in formation of the fermionic excitation spectrum in the normal state and are sufficient to explain the high transition temperatures to the superconducting state while the pseudogap phenomenon is a consequence of a Peierls-type intrinsic instability of electronic system to formation of an incommensurate density wave. On the other hand, a similar analysis being applied to the iron pnictides reveals especially strong electron-phonon coupling that suggests important role of phonons for high-Tc superconductivity in pnictides.

cond-mat.supr-con↗

arXiv2010

Scaling of normal-state transport properties of 1111 iron-pnictide superconductors

We show that the zero field normal-state resistivity above Tc for various levels of electron doping-both for underdoped, optimally, and overdoped LaO1-xFxFeAs, i.e. (x=0.05-0.075 and 0.1-0.2) and underdoped SmO1-xFxFeAs (x=0.06- 0.1) members of the 1111-iron-pnictide superconductor family-can be scaled in a broad temperature range from 20 to 300 K onto a single universal curve. The scaling was performed using the energy scale Delta, the resistivity rho(Delta) and the residual resistivity rho0 as scaling parameters as well as applying a recently proposed model-independent scaling method (H. G. Luo, Y. H. Su, and T. Xiang, Phys. Rev. B 77, 014529 (2008)). The scaling parameters have been calculated and the compositional variation of Delta has been determined. The existence of a universal metallic rho(T) curve is interpreted as an indication of a single mechanism which dominates the scattering of the charge carriers in LaO1-xFxFeAs (x= 0.05 to 0.075 and 0.1 to 0.2) and SmO1-xFxFeAs (x = 0.06 to 0.1) .

cond-mat.supr-con↗