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B. Buechner

Publications and source records attributed to B. Buechner.

108 records · Page 6Linked to original sources
arXiv2005

Orbital polaron lattice formation in lightly doped La1-xSrxMnO3

By resonant x-ray scattering at the Mn K-edge on La7/8Sr1/8MnO3, we show that an orbital polaron lattice (OPL) develops at the metal-insulator transition of this compound. This orbital reordering explains consistently the unexpected coexistence of ferromagnetic and insulating properties at low temperatures, the quadrupling of the lattice structure parallel to the MnO2-planes, and the observed polarization and azimuthal dependencies. The OPL is a clear manifestation of strong orbital-hole interactions, which play a crucial role for the colossal magnetoresistance effect and the doped manganites in general.

cond-mat.str-el↗
arXiv2005

Parity of the Pairing Bosons in a High-Temperature Superconductor

We report the observation of a novel effect in the bilayer Pb-Bi2212 high-TC superconductor by means of angle-resolved photoemission with circularly polarized excitation. Different scattering rates, determined as a function of energy separately for the bonding and antibonding copper-oxygen bands, strongly imply that the dominating scattering channel is odd with respect to layer exchange within a bilayer. This is inconsistent with a phonon-mediated scattering and favours the participation of the odd collective spin excitations in the scattering mechanism in near-nodal regions of the k-space, suggesting a magnetic nature of the pairing mediator.

cond-mat.supr-con↗
arXiv2004

Crystal and magnetic structure of La_{1-x}Sr_{1+x}MnO_{4} : role of the orbital degree of freedom

The crystal and magnetic structure of La_{1-x}Sr_{1+x}MnO_4 (0<x<0.7) has been studied by diffraction techniques and high resolution capacitance dilatometry. There is no evidence for a structural phase transition like those found in isostructural cuprates or nickelates, but there are significant structural changes induced by the variation of temperature and doping which we attribute to a rearrangement of the orbital occupation.

cond-mat.mtrl-sci↗
arXiv2004

Manifestation of the magnetic resonance mode in the nodal quasiparticle lifetime in superconducting cuprates

Studying the nodal quasiparticles in superconducting cuprates by photoemission with highly improved momentum resolution, we show that a new "kink" feature in the scattering rate is a key to uncover the nature of electron correlations in these compounds. Our data provide evidence that the main doping independent contribution to the scattering can be well understood in terms of the conventional Fermi liquid model, while the additional doping dependent contribution has a magnetic origin. This sheds doubt on applicability of a phonon-mediated pairing mechanism to high temperature superconductors.

cond-mat.supr-con↗
arXiv2003

Dzyaloshinsky-Moriya Spin Canting in the LTT Phase of La2-x-yEuySrxCuO4

The Cu spin magnetism in La2-x-yEuySrxCuO4 (x<=0.17; y<=0.2) has been studied by means of magnetization measurements up to 14 T. Our results clearly show that in the antiferromagnetic phase Dzyaloshinsky-Moriya (DM)superexchange causes Cu spin canting not only in the LTO phase but also in the LTLO and LTT phases. In La1.8Eu0.2CuO4 the canted DM-moment is about 50% larger than in pure La2CuO4 which we attribute to the larger octahedral tilt angle. We also find clear evidence that the size of the DM-moment does not change significantly at the structural transition at T_LT from LTO to LTLO and LTT. The most important change induced by the transition is a significant reduction of the magnetic coupling between the CuO2 planes. As a consequence, the spin-flip transition of the canted Cu spins which is observed in the LTO phase for magnetic field perpendicular to the CuO2 planes disappears in the LTT phase. The shape of the magnetization curves changes from the well known spin-flip type to a weak-ferromagnet type. However, no spontaneous weak ferromagnetism is observed even at very low temperatures, which seems to indicate that the interlayer decoupling in our samples is not perfect. Nonetheless, a small fraction (<15%) of the DM-moments can be remanently magnetized throughout the entire antiferromagnetically ordered LTT/LTLO phase, i.e. for T<T_LT and x<0.02. It appears that the remanent DM-moment is perpendicular to the CuO2 planes. For magnetic field parallel to the CuO2 planes we find that the critical field of the spin-flop transition decreases in the LTLO phase, which might indicate a competition between different in-plane anisotropies. To study the Cu spin magnetism in La2-x-yEuySrxCuO4, a careful analysis of the Van Vleck paramagnetism of the Eu3+ ions was performed.

cond-mat.str-el↗
arXiv2003

Interplay between Freezing and Superconductivity in the Optimally Doped LaEu0.20Sr0.15CuO4 under Hydrostatic Pressure

We study the electronic properties of a LaEu0.20Sr0.15CuO4 single crystal under hydrostatic pressure up to 2.9 GPa. Both the freezing of the Cu 3d moments and the structural transition from the orthorhombic (LTO) to the tetragonal (LTT) phase are observed via the relaxation of the nuclear magnetization of La nuclei. Resistivity and magnetic susceptibility measurements have been carried out under pressure on the same sample. The combination of all data reveals the connection between glassy dynamics, charge localization and the disappearance of superconductivity in the LTT phase.

cond-mat.str-el↗
arXiv2002

Ising magnets with mobile defects

Motivated by recent experiments on cuprates with low-dimensional magnetic interactions, a new class of two-dimensional Ising models with short-range interactions and mobile defects is introduced and studied. The non-magnetic defects form lines, which, as temperature increases, first meander and then become unstable. Using Monte Carlo simulations and analytical low- and high-temperature considerations, the instability of the defect stripes is monitored for various microscopic and thermodynamic quantities in detail for a minimal model, assuming some of the couplings to be indefinitely strong. The robustness of the findings against weakening the interactions is discussed as well.

cond-mat↗
arXiv2001

Magnetic excitations in two-leg spin 1/2 ladders: experiment and theory

Magnetic excitations in two-leg S=1/2 ladders are studied both experimentally and theoretically. Experimentally, we report on the reflectivity, the transmission and the optical conductivity sigma(omega) of undoped La_x Ca_14-x Cu_24 O_41 for x=4, 5, and 5.2. Using two different theoretical approaches (Jordan-Wigner fermions and perturbation theory), we calculate the dispersion of the elementary triplets, the optical conductivity and the momentum-resolved spectral density of two-triplet excitations for 0.2 <= J_parallel/J_perpendicular <= 1.2. We discuss phonon-assisted two-triplet absorption, the existence of two-triplet bound states, the two-triplet continuum, and the size of the exchange parameters.

cond-mat.str-el↗
arXiv2001

ESR study of (Sr,La,Ca)_{14}Cu_{24}O_{41}

We report an electron spin resonance (ESR) study of single crystals of the spin-chain spin-ladder compound (Sr,La,Ca)_{14}Cu_{24}O_{41}. The data suggest that in intrinsically hole doped Sr_{14-x}Ca_xCu_{24}O_{41} only a small amount of holes is transferred from the chains to the ladders with increasing x, resulting in a crossover from spin dimerized to uniform spin chains. In the samples of La_{14-x}Ca_xCu_{24}O_{41} with reduced hole content a very broad signal is observed in the paramagnetic state, indicative of a surprisingly strong anisotropy of the nearest neighbor exchange in the chains.

cond-mat.str-el↗
arXiv2001

Optical spectroscopy of (La,Ca)14Cu24O41 spin ladders: comparison of experiment and theory

Transmission and reflectivity of La_x Ca_14-x Cu_24 O_41 two-leg spin-1/2 ladders were measured in the mid-infrared regime between 500 and 12000 1/cm. This allows us to determine the optical conductivity sigma_1 directly and with high sensitivity. Here we show data for x=4 and 5 with the electrical field polarized parallel to the rungs (E||a) and to the legs (E||c). Three characteristic peaks are identified as magnetic excitations by comparison with two different theoretical calculations.

cond-mat.str-el↗
arXiv2001

Observation of two-magnon bound states in the two-leg ladders of (Ca,La)14Cu24O41

Phonon-assisted 2-magnon absorption is studied at T=4 K in the spin-1/2 two-leg ladders of Ca_14-x La_x Cu_24 O_41 (x=5 and 4) for polarization of the electrical field parallel to the legs and the rungs, respectively. Two peaks at about 2140 and 2800 1/cm reflect van-Hove singularities in the density of states of the strongly dispersing 2-magnon singlet bound state, and a broad peak at about 4000 1/cm is identified with the 2-magnon continuum. Two different theoretical approaches (Jordan-Wigner fermions and perturbation theory) describe the data very well for J_parallel = 1050 - 1100 1/cm and J_parallel / J_perp = 1 - 1.1. A striking similarity of the high-energy continuum absorption of the ladders and of the undoped high T_c cuprates is observed.

cond-mat.str-el↗
arXiv2000

Voltage and temperature dependence of the grain boundary tunneling magnetoresistance in manganites

We have performed a systematic analysis of the voltage and temperature dependence of the tunneling magnetoresistance (TMR) of grain boundaries (GB) in the manganites. We find a strong decrease of the TMR with increasing voltage and temperature. The decrease of the TMR with increasing voltage scales with an increase of the inelastic tunneling current due to multi-step inelastic tunneling via localized defect states in the tunneling barrier. This behavior can be described within a three-current model for magnetic tunnel junctions that extends the two-current Julliere model by adding an inelastic, spin-independent tunneling contribution. Our analysis gives strong evidence that the observed drastic decrease of the GB-TMR in manganites is caused by an imperfect tunneling barrier.

cond-mat.str-el↗
arXiv1999

4f-spin dynamics in La(2-x-y)Sr(x)Nd(y)CuO(4)

We have performed inelastic magnetic neutron scattering experiments on La(2-x-y)Sr(x)Nd(y)CuO(4) in order to study the Nd 4f-spin dynamics at low energies. In all samples we find at high temperatures a quasielastic line (Lorentzian) with a line width which decreases on lowering the temperature. The temperature dependence of the quasielastic line width Gamma/2(T) can be explained with an Orbach-process, i.e. a relaxation via the coupling between crystal field excitations and phonons. At low temperatures the Nd-4f magnetic response S(Q,omega) correlates with the electronic properties of the CuO(2)-layers. In the insulator La(2-y)Nd(y)CuO(4) the quasielastic line vanishes below 80 K and an inelastic excitation occurs. This directly indicates the splitting of the Nd3+ ground state Kramers doublet due to the static antiferromagnetic order of the Cu moments. In La(1.7-x)Sr(x)Nd(0.3)CuO(4) with x = 0.12, 0.15 and La(1.4-x)Sr(x)Nd(0.6)CuO(4) with x = 0.1, 0.12, 0.15, 0.18 superconductivity is strongly suppressed. In these compounds we observe a temperature independent broad quasielastic line of Gaussian shape below T about 30 K. This suggests a distribution of various internal fields on different Nd sites and is interpreted in the frame of the stripe model. In La(1.8-y)Sr(0.2)Nd(y)CuO(4) (y = 0.3, 0.6) such a quasielastic broadening is not observed even at lowest temperature.

cond-mat.supr-con↗
arXiv1999

Strong enhancement of spin fluctuations in the low-temperature-tetragonal phase of antiferromagnetically ordered La_{2-x-y}Eu_ySr_xCuO_4

Measurements of the static magnetization, susceptibility and ESR of Gd spin probes have been performed to study the properties of antiferromagnetically ordered La_{2-x-y}Eu_ySr_xCuO_4 (x less or equal 0.02) with the low temperature tetragonal structure. According to the static magnetic measurements the CuO_2 planes are magnetically decoupled in this structural phase. The ESR study reveals strong magnetic fluctuations at the ESR frequency which are not present in the orthorhombic phase. It is argued that this drastic enhancement of the spin fluctuations is due to a considerable weakening of the interlayer exchange and a pronounced influence of hole motion on the antiferromagnetic properties of lightly hole doped La_2CuO_4. No evidence for the stripe phase formation at small hole doping is obtained in the present study.

cond-mat.supr-con↗
arXiv1997

Magnetism of the LTT phase of Eu doped La_{2-x}Sr_xCuO_4

The ESR signal of Gd spin probes (0.5 at %) as well as the static normal state susceptibility of Eu (J(Eu^{3+})=0) doped La_{2-x-y}Sr_xEu_yCuO_4 reveal pronounced changes of the Cu magnetism at the structural transition from the orthorhombic to the low temperature tetragonal phase for all non-superconducting compositions. Both a jumplike decrease of χas well as the ESR data show an increase of the in-plane magnetic correlation length in the LTT phase. From the Gd^{3+} ESR linewidth we find that for specific Eu and Sr concentrations in the LTT phase the correlation length increases up to more than 100 lattice constants and the fluctuation frequency of the CuO_2 spin system slows down to 10^{10}- 10^{11}sec^{-1}. However, there is no static order above T ~ 8K in contrast to the LTT phase of Nd doped La_{2-x}Sr_xCuO_4 with pinned stripe correlations.

cond-mat.supr-con↗
arXiv1996

Slow antiferromagnetic dynamics in the low temperature tetragonal phase of La_{2-x}Sr_xCuO_4 as revealed by ESR of Gd spin probes

Measuring the ESR of Gd spin probes we have studied the magnetic properties of the copper oxide planes in the low temperature tetragonal (LTT) phase of Eu doped La_{2-x}Sr_xCuO_4. The data give evidence that at particular levels of Sr and Eu doping the frequency of the antiferromagnetic fluctuations in the LTT phase dramatically decreases at low temperatures by almost three orders of magnitude. However, no static magnetic order has been found for T>8K in contrast to the observation by neutron scattering of stripe ordering of spins below 50K in a Nd doped La_{2-x}Sr_xCuO_4 single crystal. To our opinion static order in the Nd doped compound is induced due to the interaction between the Cu spins with the rare earth magnetic moments. Therefore, a really characteristic property of the magnetism in the LTT structural phase may be not static magnetic order at elevated temperatures but rather extremely slow antiferromagnetic dynamics.

cond-mat.supr-con↗
arXiv1996

Thermodynamic Properties of the Incommensurate Phase of CuGeO_3

We present high resolution measurements of the specific heat and the thermal expansion of the inorganic spin--Peierls cuprate CuGeO_3 in a magnetic field of 16 Tesla. At the transition from the incommensurate to the uniform phase both quantities show pronounced anomalies, which allow to derive the uniaxial pressure dependencies of the transition temperature. In high magnetic fields the specific heat is dominated by magnetic excitations and follows a T^3 law at low temperatures. The thermal expansion measurements show the occurrence of spontaneous strains along all three lattice constants and yield high resolution measurements of the temperature dependence of the incommensurate structural distortion. The sizes of the spontaneous strains in the incommensurate phase are significantly reduced, but both their anisotropy as well as their temperature dependencies are very similar to those in zero field.

cond-mat↗