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B. D. Esry

Publications and source records attributed to B. D. Esry.

At least 19 recordsLinked to original sources

An optimized absorbing potential for ultrafast, strong-field problems

Theoretical treatments of strong-field physics have long relied on the numerical solution of the time-dependent Schrödinger equation. The most effective such treatments utilize a discrete spatial representation---a grid. Since most strong-field observables relate to the continuum portion of the wave function, the boundaries of the grid---which act as hard walls and thus cause reflection---can substantially impact the observables. Special care thus needs to be taken. While there exist a number of attempts to solve this problem---e.g., complex absorbing potentials and masking functions, exterior complex scaling, and coordinate scaling---none of them are completely satisfactory. The first of these is arguably the most popular, but it consumes a substantial fraction of the computing resources in any given calculation. Worse, this fraction grows with the dimensionality of the problem. And, no systematic way to design such a potential has been used in the strong-field community. In this work, we address these issues and find a much better solution. By comparing with previous widely used absorbing potentials, we find a factor of 3--4 reduction in the absorption range, given the same level of absorption over a specified energy interval.

physics.comp-ph

Ultracold Three-body Recombination in Two Dimensions

We study three-body recombination in two dimensions for systems interacting via short-range two-body interactions in the regime of large scattering lengths. Using the adiabatic hyperspherical representation, we derive semi-analytical formulas for three-body recombination in both weakly and deeply bound diatom states. Our results demonstrate the importance of long-range corrections to the three-body potentials by showing how they alter the low-energy and scattering length dependence of the recombination rate for both bosonic and fermionic systems, which exhibit suppressed recombination if compared to the three-dimensional case. We verify these results through numerical calculations of recombination for systems with finite-range interactions and supporting a few two-body bound states. We also study finite-range effects for the energies of the universal three-identical-bosons states and found a slow approach to universal predictions as a function of the scattering length.

quant-ph

Adiabatic Hyperspherical Representation for the Three-body Problem in Two Dimensions

We explore the three-body problem in two dimensions using the adiabatic hyperspherical representation. We develop the main equations in terms of democratic hyperangular coordinates and determine several symmetry properties and boundary conditions for both interacting and non-interacting solutions. From the analysis of the three-body effective potentials, we determine the threshold laws for low energy three-body recombination, collision-induced dissociation as well as inelastic atom-diatom collisions in two dimensions. Our results show that the hyperspherical representation can offer a simple and conceptually clear physical picture for three-body process in two dimensions which is also suitable for calculations using finite range two-body interactions supporting a number of bound states.

quant-ph

Coherent control at its most fundamental: CEP-dependent electron localization in photodissoziation of a H2+ molecular ion beam target

Measurements and calculations of the absolute carrier-envelope phase (CEP) effects in the photodissociation of the simplest molecule, H2+, with a 4.5-fs Ti:Sapphire laser pulse at intensities up to (4 +- 2)x10^14 Watt/cm^2 are presented. Localization of the electron with respect to the two nuclei (during the dissociation process) is controlled via the CEP of the ultra-short laser pulses. In contrast to previous CEP-dependent experiments with neutral molecules, the dissociation of the molecular ions is not preceded by a photoionization process, which strongly influences the CEP dependence. Kinematically complete data is obtained by time- and position-resolved coincidence detection. The phase dependence is determined by a single-shot phase measurement correlated to the detection of the dissoziation fragments. The experimental results show quantitative agreement with ab inito 3D-TDSE calculations that include nuclear vibration and rotation.

physics.chem-ph

Carrier-envelope phase control over pathway interference in strong-field dissociation of H$_2^+$

The dissociation of an H$_2^+$ molecular-ion beam by linearly polarized, carrier-envelope-phase-tagged 5 fs pulses at 4$\times10^{14} $W/cm$^2$ with a central wavelength of 730 nm was studied using a coincidence 3D momentum imaging technique. Carrier-envelope-phase-dependent asymmetries in the emission direction of H$^+$ fragments relative to the laser polarization were observed. These asymmetries are caused by interference of odd and even photon number pathways, where net-zero photon and 1-photon interference predominantly contributes at H$^+$+H kinetic energy releases of 0.2 -- 0.45 eV, and net-2-photon and 1-photon interference contributes at 1.65 -- 1.9 eV. These measurements of the benchmark H$_2^+$ molecule offer the distinct advantage that they can be quantitatively compared with \textit{ab initio} theory to confirm our understanding of strong-field coherent control via the carrier-envelope phase.

physics.chem-ph

The universality of the Efimov three-body parameter

In this paper we discuss the recent discovery of the universality of the three-body parameter (3BP) from Efimov physics. This new result was identified by recent experimental observations in ultracold quantum gases where the value of the s-wave scattering length, $a=a_-$, at which the first Efimov resonance is created was found to be nearly the same for a range of atomic species --- if scaled as $a_-/r_{\rm vdW}$, where $r_{\rm vdW}$ is the van der Waals length. Here, we discuss some of the physical principles related to these observations that emerge from solving the three-body problem with van der Waals interactions in the hyperspherical formalism. We also demonstrate the strong three-body multichannel nature of the problem and the importance of properly accounting for nonadiabatic effects.

cond-mat.quant-gas

Origin of the Three-body Parameter Universality in Efimov Physics

In recent years extensive theoretical and experimental studies of universal few-body physics have led to advances in our understanding of universal Efimov physics [1]. The Efimov effect, once considered a mysterious and esoteric effect, is today a reality that many experiments in ultracold quantum gases have successfully observed and continued to explore [2-14]. Whereas theory was the driving force behind our understanding of Efimov physics for decades, recent experiments have contributed an unexpected discovery. Specifically, measurements have found that the so-called three-body parameter determining several properties of the system is universal, even though fundamental assumptions in the theory of the Efimov effect suggest that it should be a variable property that depends on the precise details of the short-range two- and three-body interactions. The present Letter resolves this apparent contradiction by elucidating unanticipated implications of the two-body interactions. Our study shows that the three-body parameter universality emerges because a universal effective barrier in the three-body potentials prevents the three particles from simultaneously getting close to each other. Our results also show limitations on this universality, as it is more likely to occur for neutral atoms and less likely to extend to light nuclei.

cond-mat.quant-gas

Scaling laws for the non-linear coupling constant of a Bose-Einstein condensate at the threshold of delocalization

We explore the localization of a quasi-one-, quasi-two-, and three-dimensional ultra-cold gas by a finite-range defect along the corresponding 'free'-direction/s. The time-independent non-linear Schroedinger equation that describes a Bose-Einstein condensate was used to calculate the maximum non-linear coupling constant, g_max, and thus the maximum number of atoms, N_max, that the defect potential can localize. An analytical model, based on the Thomas-Fermi approximation, is introduced for the wavefunction. We show that g_max becomes a function of R_0 sqrt(V_0) for various one-, two-, and three-dimensional defect shapes with depths V_0 and characteristic lengths R_0. Our explicit calculations show surprising agreement with this crude model over a wide range of V_0 and R_0. A scaling rule is also found for the wavefunction for the ground state at the threshold at which the localized states approach delocalization. The implication is that two defects with the same product R_0 sqrt(V_0) will thus be related to each other with the same g_max and will have the same (reduced) density profile in the free-direction/s.

physics.atom-ph

Multiphoton Dissociation of HeH+ below the He+(1s) + H(1s) Threshold

We discuss the strong-field dynamics of HeH+, the simplest stable heteronuclear molecule, focusing on identifying a laser regime for which there is a sufficient dissociation signal for experimental measurement. We numerically solve the time-dependent Schrödinger equation to obtain total dissociation probabilities, kinetic energy release spectra, and momentum distributions for wavelengths from 800 nm to 2400 nm. The suitability of this simple system as a prototype for understanding the strong-field nuclear dynamics of heteronuclear dissociation is discussed.

physics.atom-ph

Enhancing the intense field control of molecular fragmentation

We describe a pump-probe scheme with which the spatial asymmetry of dissociating molecular fragments --- as controlled by the carrier-envelope phase of an intense few-cycle laser pulse --- can be enhanced by an order of magnitude or more. We illustrate the scheme using extensive, full-dimensional calculations for dissociation of H$_2^+$ and include the averaging necessary for comparison with experiment.

quant-ph

A new class of three-body states

We calculate the three-body spectrum for identical bosons interacting via attractive $1/r^2$ potentials. We have found an infinite number of three-body states even when the pair interactions are too weak to support any two-body states. These new states thus share this surprising scenario with the Efimov effect, but are not themselves Efimov states. Our effect occurs for both identical bosons and identical fermions, and it persists in the presence of two-body bound states.

quant-ph

Efimov physics in heteronuclear four-body systems

We study three- and four-body Efimov physics in a heteronuclear atomic system with three identical heavy bosonic atoms and one light atom. We show that exchange of the light atom between the heavy atoms leads to both three- and four-body features in the low-energy inelastic rate constants that trace to the Efimov effect. Further, the effective interaction generated by this exchange can provide an additional mechanism for control in ultracold experiments. Finally, we find that there is no true four-body Efimov effect - that is, no infinite number of four-body states in the absence of two- and three-body bound states - resolving a decades-long controversy.

physics.atom-ph

Adiabatic Floquet Picture for Hydrogen Atom in an Intense Laser Field

We develop an adiabatic Floquet picture in the length gauge to describe the dynamics of a hydrogen atom in an intense laser field. In this picture, we discuss the roles played by frequency and intensity in terms of adiabatic potentials and the couplings between them, which gives a physical and intuitive picture for quantum systems exposed to a laser field. For simplicity, analyze hydrogen and give the adiabatic potential curves as well as some physical quantities that can be readily calculated for the ground state. Both linearly and circularly polarized laser fields are discussed.

physics.atom-ph

Universal three-body physics at finite energy near Feshbach resonances

We find that universal three-body physics extends beyond the threshold regime to non-zero energies. For ultracold atomic gases with a negative two-body $s$-wave scattering length near a Feshbach resonance, we show the resonant peaks characteristic of Efimov physics persist in three-body recombination to higher collision energies. For this and other inelastic processes, we use the adiabatic hyperspherical representation to derive universal analytical expressions for their dependence on the scattering length, the collision energy, and --- for narrow resonances --- the effective range. These expressions are supported by full numerical solutions of the Schrödinger equation and display log-periodic dependence on energy characteristic of Efimov physics. This dependence is robust and might be used to experimentally observe several Efimov features.

physics.atom-ph

Ultracold three-body collisions near narrow Feshbach resonances

We study ultracold three-body collisions of bosons and fermions when the interatomic interaction is tuned near a narrow Feshbach resonance. We show that the width of the resonance has a substantial impact on the collisional properties of ultracold gases in the strongly interacting regime. We obtain numerical and analytical results that allow us to identify universal features related to the resonance width. For narrow resonances, we have found a suppression of all inelastic processes in boson systems leading to deeply bound states and an enhancement for fermion systems.

quant-ph

Cold three-body collisions in hydrogen-hydrogen-alkali atomic system

We have studied hydrogen-hydrogen-alkali three-body systems in the adiabatic hyperspherical representation. For the spin-stretched case, there exists a single $X$H molecular state when $X$ is one of the bosonic alkali atoms: $^7$Li, $^{23}$Na, $^{39}$K, $^{87}$Rb and $^{133}$Cs. As a result, the {\em only} recombination process is the one that leads to formation of $X$H molecules, H+H+$X$$\rightarrow$$X$H+H, and such molecules will be stable against vibrational relaxation. We have calculated the collision rates for recombination and collision induced dissociation as well as the elastic cross-sections for H+$X$H collisions up to a temperature of 0.5 K, including the partial wave contributions from $J^Π$=$0^+$ to $5^-$. We have also found that there is just one three-body bound state for such systems for $J^Π$=$0^+$ and no bound states for higher angular momenta.

physics.atom-ph

Attosecond pulse trains as multi-color coherent control

We present a general description of the interaction between multi-color laser pulses and atoms and molecules, focusing on the experimentally relevant example of infrared (IR) pulses overlapped with attosecond pulse trains (APTs). This formulation reveals explicitly and analytically the role of the delay between the IR pulse and APT as a coherent control parameter. Our formulation also shows the nearly equivalent roles of the delay and the carrier-envelope phase in controlling the interference between different multiphoton pathways. We illustrate these points by investigating the single ionization of He and introduce dressed adiabatic hyperspherical potentials to aid the discussion. We confirm the predictions with a full-dimensional, two-electron solution of the time-dependent Schrödinger equation.

physics.atom-ph

Magnetically Controlled Exchange Process in an Ultracold Atom-Dimer Mixture

We report on the observation of an elementary exchange process in an optically trapped ultracold sample of atoms and Feshbach molecules. We can magnetically control the energetic nature of the process and tune it from endoergic to exoergic, enabling the observation of a pronounced threshold behavior. In contrast to relaxation to more deeply bound molecular states, the exchange process does not lead to trap loss. We find excellent agreement between our experimental observations and calculations based on the solutions of three-body Schrödinger equation in the adiabatic hyperspherical representation. The high efficiency of the exchange process is explained by the halo character of both the initial and final molecular states.

cond-mat.quant-gas