arXiv subjects

B. Deveaud

Publications and source records attributed to B. Deveaud.

18 recordsLinked to original sources

arXiv2017

Spin anisotropic interactions of lower-polaritons in the vicinity of polaritonic Feshbach resonance

We determine experimentally the spinor interaction constants of lower-polaritons $α_1$ and $α_2$ using resonant pump-probe spectroscopy with a spectrally narrow pump pulse. Our experimental findings are analyzed with the Bogoliubov-like theory and mean-field two channel model based on the lower-polariton and biexciton basis. We find an enhancement of the attractive interaction and dissipative nonlinearity of lower-polaritons with anti-parallel spins in the vicinity of the biexciton resonance when the energy of two lower-polaritons approaches energetically that of the biexciton. These observations are consistent with the existence of a scattering resonance between lower-polaritons and biexcitons (polaritonic Feshbach resonance).

cond-mat.mes-hall↗

arXiv2017

2s exciton-polariton revealed in an external magnetic field

We demonstrate the existence of the excited state of an exciton-polariton in a semiconductor microcavity. The strong coupling of the quantum well heavy-hole exciton in an excited 2s state to the cavity photon is observed in non-zero magnetic field due to surprisingly fast increase of Rabi energy of the 2s exciton-polariton in magnetic field. This effect is explained by a strong modification of the wave-function of the relative electron-hole motion for the 2s exciton state.

cond-mat.quant-gas↗

arXiv2017

Doubly dressed bosons - exciton-polaritons in a strong terahertz field

We demonstrate the existence of a novel quasiparticle: an exciton in a semiconductor doubly dressed with two photons of different wavelengths: near infrared cavity photon and terahertz (THz) photon, with the THz coupling strength approaching the ultra-strong coupling regime. This quasiparticle is composed of three different bosons, being a mixture of a matter-light quasiparticle. Our observations are confirmed by a detailed theoretical analysis, treating quantum mechanically all three bosonic fields. The doubly dressed quasiparticles retain the bosonic nature of their constituents, but their internal quantum structure strongly depends on the intensity of the applied terahertz field.

cond-mat.quant-gas↗

arXiv2016

Coherent and incoherent aspects of polariton dynamics in semiconductor microcavities

The interaction between coherent polaritons and incoherent excitons plays an important role in polariton physics. Using resonant pump-probe spectroscopy with selective excitation of single polariton branches, we investigate the different dephasing mechanisms responsible for generating a long-lived exciton reservoir. As expected, pumping the upper polariton results in a strong dephasing process that leads to the generation of a long lived reservoir. Unexpectedly, we observe an efficient reservoir creation while exciting only the lower polariton branch when the detuning is increased towards positive detuning. We propose a simple theoretical model, the polaritonic Bloch equations, to describe the dynamics of the system.

cond-mat.mes-hall↗

arXiv2015

2D Fourier Transform Spectroscopy of exciton-polaritons and their interactions

We investigate polariton-polariton interactions in a semiconductor microcavity through two-dimensional Fourier transform (2DFT) spectroscopy. We observe, in addition to the lower-lower and the upper-upper polariton self-interaction, a lower-upper cross-interaction. This appears as separated peaks in the on-diagonal and off-diagonal part of 2DFT spectra. Moreover, we elucidate the role of the polariton dispersion through a fine structure in the 2DFT spectrum. Simulations, based on lower-upper polariton basis Gross-Pitaevskii equations including both self and cross-interactions, result in a 2DFT spectra in qualitative agreement with experiments.

cond-mat.mes-hall↗

arXiv2015

Spinor Stochastic Resonance

We report on noise-induced-spin-ordering in a collective quasipaticle system: spinor stochastic resonance. Synergetic interplay of a polarization-modulated signal and a polarization-noise allows us to switch coherently between the two metastable states of a microcavity-polariton spin bistable system. Spinor stochastic resonance is demonstrated in a zero-dimensional GaAs based microcavity. The resonance behavior of both the spin amplification and the signal-to-noise ratio are experimentally evidenced as a function of the noise strength for different amplitude modulations. They are theoretically reproduced using a spinor- Gross-Pitaevskii equation driven by a randomly polarized laser field.

cond-mat.mes-hall↗

arXiv2015

The Effect of a Noisy Driving Field on a Bistable Polariton System

We report on the effect of noise on the characteristics of the bistable polariton emission system. The present experiment provides a time resolved access to the polariton emission intensity. We evidence the noise-induced transitions between the two stable states of the bistable polaritons. It is shown that the external noise specifications, intensity and correlation time, can efficiently modify the polariton Kramers time and residence time. We find that there is a threshold noise strength that provokes the collapse of the hysteresis loop. The experimental results are reproduced by numerical simulations using Gross-Pitaeviskii equation driven by a stochastic excitation.

cond-mat.mes-hall↗

arXiv2014

Magnetic field tuning of exciton polaritons in a semiconductor microcavity

We detail the influence of a magnetic field on exciton-polaritons inside a semiconductor microcavity. Magnetic field can be used as a tuning parameter for exciton and photon resonances. We discuss the change of the exciton energy, the oscillator strength and redistribution of the polariton density along the dispersion curves due to the magnetically-induced detuning. We have observed that field-induced shrinkage of the exciton wave function has a direct influence not only on the exciton oscillator strength, which is observed to increase with the magnetic field, but also on the polariton linewidth. We discuss the effect of the Zeeman splitting on polaritons which magnitude changes with the exciton Hopfield coefficient and can be modelled by independent coupling of the two spin components of excitons with cavity photons.

cond-mat.mes-hall↗

arXiv2013

Polychromatic polariton laser selector switch

Integration of optical elements into scalable chips has been at the center of a large effort in recent years. Concurrently, the separation between the diverse functions, namely switches, detectors or emitters increases significantly the final number of components on chip. Such technical limitations may be overcome by introducing agile devices able, for example, to simultaneously detect, process and emit a coherent signal. Such a pathway has been explored with different approaches that bear advantages and drawbacks. Polaritons have often been proposed as promising candidates for multifunctional devices. Here we present an optical switch based on polariton lasing. An incident monochromatic signal is channeled into several polariton laser beams at different wavelengths by a novel relaxation mechanism which combines bistability, phonon interactions, long polariton lifetime and bosonic stimulation. We demonstrate spin logic operations conserving the original polarization state that is fully imprinted onto the coherently emitted signals.

cond-mat.quant-gas↗

arXiv2013

Spontaneous self-ordered states of vortex-antivortex pairs in a Polariton Condensate

Polariton condensates have proved to be model systems to investigate topological defects, as they allow for direct and non-destructive imaging of the condensate complex order parameter. The fundamental topological excitations of such systems are quantized vortices. In specific configurations, further ordering can bring the formation of vortex lattices. In this work we demonstrate the spontaneous formation of ordered vortical states, consisting in geometrically self-arranged vortex-antivortex pairs. A mean-field generalized Gross-Pitaevskii model reproduces and supports the physics of the observed phenomenology.

cond-mat.quant-gas↗

arXiv2012

Penrose-Onsager Criterion Validation in a One-Dimensional Polariton Condensate

We perform quantum tomography on one-dimensional polariton condensates, spontaneously occurring in linear disorder valleys in a CdTe planar microcavity sample. By the use of optical interferometric techniques, we determine the first-order coherence function and the amplitude and phase of the order parameter of the condensate, providing a full reconstruction of the single particle density matrix for the polariton system. The experimental data are used as input to theoretically test the consistency of Penrose-Onsager criterion for Bose-Einstein condensation in the framework of nonequilibrium polariton condensates. The results confirm the pertinence and validity of the criterion for a non equilibrium condensed gas.

cond-mat.quant-gas↗

arXiv2007

Determination of Trion and Exciton Lineshapes in Modulation-Doped Quantum Wells

We investigate the effect of a two dimensional electron gas on the linear optical properties of CdTe quantum wells. We evidence experimentally the high energy tail of the exciton and charged exciton resonances which depends on electron concentration. Based on that, we show that the scattering of electrons with excitons and charged excitons is needed to be included in the matrix transfer calculations to describe the reflectivity spectra. We demonstrate by time-resolved reflectivity experiments the importance of electron distribution in the resonance lineshapes.

cond-mat.str-el↗

arXiv2007

Dynamics of trion formation in GaAs quantum wells

We propose a double channel mechanism for the formation of charged excitons (trions); they are formed through bi- and tri-molecular processes. This directly implies that both negatively and positively charged excitons coexist in a quantum well, even in the absence of excess carriers. The model is applied to a time-resolved photoluminescence experiment performed on a very high quality InGaAs quantum well sample, in which the photoluminescence contributions at the energy of the trion, exciton and at the band edge can be clearly separated and traced over a broad range of times and densities. The unresolved discrepancy between the theoretical and experimental radiative decay time of the exciton in a doped semiconductor is explained.

cond-mat.mtrl-sci↗

arXiv2004

Photoluminescence of p-doped quantum wells with strong spin splitting

The spectroscopic properties of a spin polarized two-dimensional hole gas are studied in modulation doped (Cd,Mn)Te quantum wells. The giant Zeeman effect induces a significant spin splitting even at very small values of the applied field. Several methods of measuring the carrier density (Hall effect, filling factors of the Landau levels at high field, various manifestations of Moss-Burstein shifts) are described and calibrated. The value of the spin splitting needed to fully polarize the hole gas, evidences a strong enhancement of the spin susceptibility of the hole gas due to carrier-carrier interaction. At small values of the spin splitting, whatever the carrier density (non zero) is, photoluminescence lines are due to the formation of charged excitons in the singlet state. Spectral shifts in photoluminescence and in transmission (including an "excitonic Moss-Bustein shift") are observed and discussed in terms of excitations of the partially or fully polarized hole gas. At large spin splitting, and without changing the carrier density, the singlet state of the charged exciton is destabilized in favour of a triplet state configuration of holes. The binding energy of the singlet state is thus measured and found to be independent of the carrier density (in contrast with the splitting between the charged exciton and the neutral exciton lines). The state stable at large spin splitting is close to the neutral exciton at low carrier density, and close to an uncorrelated electron-hole pair at the largest values of the carrier density achieved. The triplet state gives rise to a characteristic double-line structure with an indirect transition to the ground state (with a strong phonon replica) and a direct transition to an excited state of the hole gas.

cond-mat.mtrl-sci↗

arXiv2004

Interacting many-body systems in quantum wells: Evidence for exciton-trion-electron correlations

We report on the nonlinear optical dynamical properties of excitonic complexes in CdTe modulation-doped quantum wells, due to many-body interactions among excitons, trions and electrons. These were studied by time and spectrally resolved pump-probe experiments. The results reveal that the nonlinearities induced by trions differ from those induced by excitons, and in addition they are mutually correlated. We propose that the main source of these subtle differences comes from the Pauli exclusion-principle through phase-space filling and short-range fermion exchange.

cond-mat.mtrl-sci↗

arXiv2003

Evidence for parametric memory and correlation in semiconductor microcavities

We measured the dynamics of polariton parametric stimulated scattering in semiconductor microcavities, by time-resolving the amplified signal with 250 fs resolution. Our experiments demonstrate that the stimulation process is considerably delayed with respect to the arrival time of both probe and pump pulses. This effect is clearly observable in our high quality sample due to the long lifetime of the microcavity polaritons (about 10 ps), and it is in excellent agreement with the model describing the coherent conversion of two pump polaritons into a signal-idler pair. We demonstrate that the non-instantaneous character of the polariton stimulation occurs because the polariton-wave amplification requires the build up of correlated signal-idler polariton fields.

cond-mat↗

arXiv2003

Direct measure of the exciton formation in quantum wells from time resolved interband luminescence

We present the results of a detailed time resolved luminescence study carried out on a very high quality InGaAs quantum well sample where the contributions at the energy of the exciton and at the band edge can be clearly separated. We perform this experiment with a spectral resolution and a sensitivity of the set-up allowing to keep the observation of these two separate contributions over a broad range of times and densities. This allows us to directly evidence the exciton formation time, which depends on the density as expected from theory. We also evidence the dominant contribution of a minority of excitons to the luminescence signal, and the absence of thermodynamical equilibrium at low densities.

cond-mat↗

arXiv1999

Photoluminescence study of V-groove quantum wires: The influence of disorder on the optical spectra and the carrier thermalization

We report on time-resolved and steady-state photoluminescence studies of GaAs/AlGaAs V-groove quantum wire structures. Steady-state photoluminescence experiments are performed in the temperature range from 8K to 200K. We evaluate the relation between photoluminescence excitation and absorption and determine experimentally an optical density in order to analyze the temperature dependence of the photoluminescence spectra. We find that, at a temperature above 60K, the photoexcited electron-hole pairs reach a thermal equilibrium at the lattice temperature while, at a temperature below about 60K, they do not reach a quasi-equilibrium in the steady-state. Time-resolved photoluminescence studies performed at a carrier density of about 2. 104 cm-1 indicate that, at 60K, a quasi-equilibrium is reached on a time scale of 10 ps. Furthermore, the hot carriers cool in about 100 ps to the lattice temperature. At 8K, however, evidence of a non-thermal carrier distribution is found at the earliest times, which suggests that carriers in extended states are not in thermal equilibrium with carriers in localized states.

cond-mat.mtrl-sci↗