arXiv subjects

B. Grémaud

Publications and source records attributed to B. Grémaud.

At least 19 recordsLinked to original sources

arXiv2026

Magnetic-field-induced magnon portfolio in a van der Waals magnet

Magnonic excitations are investigated in chromium oxychloride (CrOCl), a van der Waal (vdW) antiferromagnet prone to a multitude of magnetic phase transitions, with absorption experiments in a broad continuous energy range. At low magnetic fields, the magnon spectra show a strong bi-axial anisotropy and inform on the relative weights of the effective exchange coupling and the system anisotropies. As the magnetic field increases, magnons characteristic of a canted phase are first observed, with peculiarities attributed to in-plane anisotropies and magnon-magnon coupling. Subsequently, a hysteretic magnon spectrum appears as the system transitions to a ferrimagnetic state, with two new magnon branches partly coexisting with the lower energy canted phase branch, indicating the formation of spatially separated magnetic phases. Further changes in the magnon spectrum in higher magnetic fields accompany transitions to the different canted magnetic phases previously reported. Our experiments show that competing exchange interactions and ground states broaden the options to generate different kinds of magnonic excitations in the same vdW material upon the variation of external parameters.

cond-mat.mtrl-sci↗

arXiv2026

Magnetic field tuning of modulated magnetic orders in CrOCl at the two-dimensional limit

Chromium oxychloride is a van der Waals magnet with intrinsic competing exchange interactions, including a strong antiferromagnetic one, source of a very rich magnetic phase diagram, with ferrimagnetic, antiferromagnetic, and canted states, up to high magnetic fields. We investigate the sequence of these magnetic phases in thin layers of CrOCl using magneto-Raman scattering spectroscopy. We identify phases whose magnetic order is commensurate with the atomic lattice, and find signatures of strong magneto-striction, presumably of exchange origin. The coupling of the spin and atomic degrees of freedom in the crystal is observed down to the single-layer limit -- phonon modes significantly soften or stiffen, in a complex way due to the competition of interactions. The existence domains of the different phases change with the number of layers.

cond-mat.mes-hall↗

arXiv2025

Magnetic phases and zone-folded phonons in a frustrated van der Waals magnet

2D magnetic materials have attracted extensive research interest due to their potential application in nanospintronics, optospintronics, and in magnonics. Ferromagnetic as well as antiferromagnetic layered materials have been demonstrated and successfully inserted into van der Waals heterostructures. However, the effects of magnetic frustration in van der Waals materials and the possibilities offered by spin configurations characterized by nonlinear spin arrangements have not been fully considered yet. Herein, we establish the magnetic phase diagram of bulk CrOCl, a frustrated van der Waals magnet, using magnetization and magneto-optical spectroscopy techniques. In particular, we use the magnetic superstructures relative to the crystallographic unit cell and the associated rich zone-folded phonon series to describe the magnetic field induced phases. Theoretical calculations taking into account the competing nearest neighbors magnetic exchange interactions provide a unique insight into the lattice vibrations of this class of magnetic system. This study expands the scope of 2D magnetic materials and provides a methodology to characterize frustrated van der Waals magnets.

cond-mat.mes-hall↗

arXiv2024

Finite width of anyons changes their braiding signature

Anyons are particles intermediate between fermions and bosons, characterized by a nontrivial exchange phase, yielding remarkable braiding statistics. Recent experiments have shown that anyonic braiding has observable consequences on edge transport in the fractional quantum Hall effect (FQHE). Here, we study transport signatures of anyonic braiding when the anyons have a finite width. We show that the width of the anyons, even extremely small, can have a tremendous impact on transport properties and braiding signatures. In particular, we find that taking the finite width into account allows us to explain recent experimental results on FQHE at filling factor $2/5$ [Ruelle et al., Phys. Rev. X \textbf{13}, 011031 (2023)]. Our work shows that the finite width of anyons crucially influences setups involving anyonic braiding, especially when the exchange phase is larger than $π/2$.

cond-mat.mes-hall↗

arXiv2024

Nonreciprocal charge transport and subharmonic structure in voltage-biased Josephson diodes

We study charge transport in voltage-biased single-channel junctions involving helical superconductors with finite Cooper pair momentum. For a Josephson junction, the equilibrium current-phase relation shows a superconducting diode effect: the critical current depends on the propagation direction. We formulate a scattering theory for voltage-biased Josephson diodes and show that multiple Andreev reflection processes cause a rich subharmonic structure in the DC current-voltage curve at low temperatures and small voltages due to Doppler shifts of the spectral gap. In the current-biased case, the diode efficiency has maximal rectification efficiency $η_0\approx 0.4$ for this model. In the voltage-biased case, however, the rectification efficiency can reach the ideal value $η=1$. We also discuss charge transport for NS junctions between a normal metal and a helical superconductor and comment on related models with spin-orbit interactions and magnetic Zeeman fields.

cond-mat.supr-con↗

arXiv2024

Levitons in correlated nano-scale systems

in nanoscale systems in the presence of single-electron excitations generated by Lorentzian voltage drives, termed \textit{Levitons}. These excitations allow to realize the analog of quantum optics experiments using electrons instead of photons. Importantly, electrons in condensed matter systems are strongly affected by the presence of different types of non-trivial correlations, with no counterpart in the domain of photonic quantum optics. After providing a short introduction about Levitons in non-interacting systems, we focus on how they operate in the presence of two types of strong electronic correlations in nanoscale systems, such as those arising in the fractional quantum Hall effect or in superconducting systems. Specifically, we consider Levitons in a quantum Hall bar of the fractional quantum Hall effect, pinched by a quantum point contact, where anyons with fractional charge and statistics tunnel between opposite edges. In this case, a Leviton-Leviton interaction can be induced by the strongly correlated background. Concerning the effect of superconducting correlations on Levitons, we show that, in a normal metal system coupled to BCS superconductors, half integer Levitons minimize the excess noise in the Andreev regime. Interestingly, energy-entangled electron states can be realized on-demand in this type of hybrid setups by exploiting crossed Andreev reflection. The results exposed in this review have potential applications in the context of quantum information and computation with single-electron flying qubits.

cond-mat.mes-hall↗

arXiv2024

Approaching ideal rectification in superconducting diodes through multiple Andreev reflections

We analyze the rectification properties of voltage-biased Josephson junctions exhibiting the superconducting diode effect. Taking into account multiple Andreev reflection (MAR) processes in our scattering theory, we consider a short weak link of arbitrary transparency between two superconductors with finite Cooper pair momentum $2q$. In equilibrium, the diode efficiency is bounded from above in this model, with maximal efficiency $η_0\approx 0.4$. Out of equilibrium, we find a rich subharmonic structure in the current-voltage curve. For high transparency and low bias voltage $V$, the rectification efficiency $η(V)$ approaches the ideal value $η=1$ for $qξ\to 1$ (with coherence length $ξ$).

cond-mat.supr-con↗

arXiv2023

Anyonic statistics revealed by the Hong-Ou-Mandel dip for fractional excitations

The fractional quantum Hall effect (FQHE) is known to host anyons, quasiparticles whose statistics is intermediate between bosonic and fermionic. We show here that Hong-Ou-Mandel (HOM) interferences between excitations created by narrow voltage pulses on the edge states of a FQHE system at low temperature show a direct signature of anyonic statistics. The width of the HOM dip is universally fixed by the thermal time scale, independently of the intrinsic width of the excited fractional wavepackets. This universal width can be related to the anyonic braiding of the incoming excitations with thermal fluctuations created at the quantum point contact. We show that this effect could be realistically observed with periodic trains of narrow voltage pulses using current experimental techniques.

cond-mat.mes-hall↗

arXiv2023

Photo-assisted current in the fractional quantum Hall effect as a probe of the quasiparticle operator scaling dimension

We study photo-assisted transport for the edge states of a two dimensional electron gas in the fractional quantum Hall regime, pinched by a single quantum point contact. We provide a general expression of the photo-assisted current using a Keldysh-Floquet approach, when the AC drive is applied either directly to the edge states, or when it modulates the tunneling amplitude at the quantum point contact. Strikingly, for a simple cosine modulation of the tunneling amplitude, the phase shift of the second harmonic of the photoassisted current is directly related to the scaling dimension of the quasiparticle operators describing the fractional excitations. As the scaling dimension is intimately related to the statistics, our proposal of a gate modulation of the backscattered current provides a diagnosis of the statistics of Laughlin quasiparticles using a simple quantum point contact geometry.

cond-mat.mes-hall↗

arXiv2023

Colored delta-T noise in Fractional Quantum Hall liquids

Photons are emitted or absorbed by a nano-circuit under both equilibrium and non-equilibrium situations. Here, we focus on the non-equilibrium situation arising due to a temperature difference between the leads of a quantum point contact, and study the finite frequency (colored) noise. We explore this delta-$T$ noise in the finite frequency regime for two systems: conventional conductors described by Fermi liquid scattering theory and the fractional quantum Hall system at Laughlin filling fractions, described by the chiral Luttinger liquid formalism. We study the emission noise, its expansion in the temperature difference (focusing on the quadratic component) as well as the excess emission noise defined with respect to a properly chosen equilibrium situation. The behavior of these quantities are markedly different for the fractional quantum Hall system compared to Fermi liquids, signalling the role of strong correlations. We briefly treat the strong backscattering regime of the fractional quantum Hall liquid, where a behavior closer to the Fermi liquid case is observed.

cond-mat.mes-hall↗

arXiv2022

Designer Flat Bands: Topology and Enhancement of Superconductivity

We construct quasi one-dimensional topological and non-topological three-band lattices with tunable band gap and winding number of the flat band. Using mean field (MF) and exact density matrix renormalization group (DMRG) calculations, we show explicitly how the band gap affects pairing and superconductivity (SC) in a Hubbard model with attractive interactions. We show excellent agreement between MF and DMRG. When a phase twist is applied on the system, a phase difference appears between pairing order parameters on different sublattices, and this plays a very important role in the SC density. The SC weight, $D_s$, on the gapped topological, $W\neq0$, flat band increases linearly with interaction strength, $U$, for low values, and with a slope that depends on the details of the compact localized state at $U=0$. As $U\to 0$ for the gapped non-topological flat band ($W=0$), $D_s$ decays with a power law faster than quadratic but slower than exponential. This indicates that isolated non-topological flat bands are less beneficial to SC. In the gapless case (flat band touching the band above it), we find at low $U$ (both for $W=0$ and $W\neq 0$) that $D_s\propto U^φ$ with $φ<1$ contrary to the $U{\rm ln}\, ({\rm const.}/U)$ behavior reported in the literature. In other words, $D_s$ increases faster than linearly for low $U$ thus favoring SC at weak interaction more than the gapped case. For systems with touching bands, we observe that the one-body correlation length, $ξ$, diverges as a power law as $U\rightarrow0$, while for the isolated flat band $ξ(U\to 0)$ is a constant smaller than one lattice spacing. Both behaviors are distinct from the exponential divergence of $ξ$ in the dispersive case. Our results re-establish that the BCS mean field and quantum metric alone are insufficient to characterize SC at weak coupling.

cond-mat.supr-con↗

arXiv2022

Microscopic theory of photo-assisted electronic transport in normal-metal/BCS-superconductor junctions

We investigate photo assisted electronic transport in a normal-metal/BCS-superconductor junction with a microscopic Hamiltonian approach, for several types of periodic voltage drives applied on the normal-metal side. The time-dependent current and the photo-assisted noise are computed to all orders of the tunneling Hamiltonian using a Keldysh-Nambu-Floquet approach. An excess noise analysis allows one to determine to what extent pure electronic excitations with a small number of electrons per period can be generated by the different drives. When the superconducting gap is small compared to the drive frequency, the junction behaves like a normal-metal junction and minimal excess noise is reached for Lorentzian voltage drives carrying an integer charge (levitons). In the opposite regime of a large-gap, the excess noise vanishes for half-quantized levitons, giving rise to the perfect transmission of a Cooper pair on the superconducting side. This microscopic approach also allows us to address the intermediate regime, when the drive frequency is comparable to the gap, allowing us to study the non-trivial interplay between Andreev reflection and quasiparticle-transfer processes. Our analysis also shows the appearance of Tien-Gordon-type relations connecting the current and noise in the AC-driven junction to their DC counterpart, which we investigate in details. Finally, the possibility to build a reliable on-demand source of Cooper pairs with this setup is examined using realistic experimental parameters.

cond-mat.supr-con↗

arXiv2021

Pairing and superconductivity in quasi one-dimensional flat band systems: Creutz and sawtooth lattices

We study the pairing and superconducting properties of the attractive Hubbard model in two quasi one-dimensional topological lattices: the Creutz and sawtooth lattices. They share two peculiar properties: each of their band structures exhibits a flat band with a non-trivial winding number. The difference, however, is that only the Creutz lattice is genuinely topological, owing to a chiral (sub-lattice) symmetry, resulting in a quantized winding number and zero energy edge modes for open boundary conditions. We use mean field and exact density matrix renormalization group in our work. Our three main results are: (a) For both lattice systems, the superconducting weight, $D_s$, is linear in the coupling strength, $U$, for low values of $U$; (b) for small $U$, $D_s$ is proportional to the quantum metric for the Creutz system but not for the sawtooth system because its sublattices are not equivalent; (c) conventional BCS mean field is not appropriate for such systems with inequivalent sublattices. We show that, for a wide range of densities and coupling strengths, these systems are very well described by a full multi-band mean field method where the pairing parameters and the local particle densities on the inequivalent sublattices are variational mean field parameters.

cond-mat.supr-con↗

arXiv2021

Scattering Theory of Non-Equilibrium Noise and Delta $T$ current fluctuations through a quantum dot

We consider the non-equilibrium zero frequency noise generated by a temperature gradient applied on a device composed of two normal leads separated by a quantum dot. We recall the derivation of the scattering theory for non-equilibrium noise for a general situation where both a bias voltage and a temperature gradient can coexist and put it in a historical perspective. We provide a microscopic derivation of zero frequency noise through a quantum dot based on a tight binding Hamiltonian, which constitutes a generalization of the pioneering work of Caroli et al. for the current obtained in the context of the Keldysh formalism. For a single level quantum dot, the obtained transmission coefficient entering the scattering formula for the non-equilibrium noise corresponds to a Breit-Wigner resonance. We compute the delta-$T$ noise as a function of the dot level position, and of the dot level width, in the Breit-Wigner case, for two relevant situations which were considered recently in two separate experiments. In the regime where the two reservoir temperatures are comparable, our gradient expansion shows that the delta-$T$ noise is dominated by its quadratic contribution, and is minimal close to resonance. In the opposite regime where one reservoir is much colder, the gradient expansion fails and we find the noise to be typically linear in temperature before saturating. In both situations, we conclude with a short discussion of the case where both a voltage bias and a temperature gradient are present, in order to address the potential competition with thermoelectric effects.

cond-mat.mes-hall↗

arXiv2020

Negative delta-$T$ noise in the Fractional Quantum Hall effect

We study the current correlations of fractional quantum Hall edges at the output of a quantum point contact (QPC) subjected to a temperature gradient. This out-of-equilibrium situation gives rise to a form of temperature-activated shot noise, dubbed delta-$T$ noise. We show that the tunneling of Laughlin quasiparticles leads to a negative delta-$T$ noise, in stark contrast with electron tunneling. Moreover, varying the transmission of the QPC or applying a voltage bias across the Hall bar may flip the sign of this noise contribution, yielding signatures which can be accessed experimentally.

cond-mat.mes-hall↗

arXiv2020

Pairing and pair superfluid density in one-dimensional Hubbard models

We use unbiased computational methods to elucidate the onset and properties of pair superfluidity in two-species fermionic and bosonic systems with onsite interspecies attraction loaded in one-dimensional optical lattice. We compare results from quantum Monte Carlo (QMC) and density matrix renormalization group (DMRG), emphasizing the one-to-one correspondence between the Drude weight tensor, calculated with DMRG, and the various winding numbers extracted from the QMC. Our results show that, for any nonvanishing attractive interaction, pairs form and are the sole contributors to superfluidity, there are no individual contributions due to the separate species. For weak attraction, the pair size diverges exponentially, i.e. Bardeen-Cooper-Schrieffer (BCS) pairing requiring huge systems to bring out the pair-only nature of the superfluid. This crucial property is largely overlooked in many studies, thereby misinterpreting the origin and nature of the superfluid. We compare and contrast this with the repulsive case and show that the behavior is very different, contradicting previous claims about drag superfluidity and the symmetry of properties for attractive and repulsive interactions. Finally, our results show that the situation is similar for soft core bosons: superfluidity is due only to pairs, even for the smallest attractive interaction strength compatible with the largest system sizes that we could attain.

cond-mat.quant-gas↗

arXiv2020

Nonlinear two-photon Rabi-Hubbard model: superradiance and photon/photon-pair Bose-Einstein condensate

We study the ground state phase diagram of a nonlinear two-photon Rabi-Hubbard (RH) model in one dimension using quantum Monte Carlo (QMC) simulations and density matrix renormalization group (DMRG) calculations. Our model includes a nonlinear photon-photon interaction term. Absent this term, the RH model has only one phase, the normal disordered phase, and suffers from spectral collapse at larger values of the photon-qubit interaction or inter-cavity photon hopping. The photon-photon interaction, no matter how small, stabilizes the system which now exhibits {\it two} quantum phase transitions: Normal phase to {\it photon pair} superfluid (PSF) transition and PSF to single particle superfluid (SPSF). The discrete $Z_4$ symmetry of the Hamiltonian spontaneously breaks in two stages: First it breaks partially as the system enters the PSF and then completely breaks when the system finally enters the SPSF phase. We show detailed numerical results supporting this, and map out the ground state phase diagram.

cond-mat.quant-gas↗

arXiv2019

Two-photon Rabi-Hubbard and Jaynes-Cummings-Hubbard models: photon pair superradiance, Mott insulator and normal phases

We study the ground state phase diagrams of two-photon Dicke, the one-dimensional Jaynes-Cummings-Hubbard (JCH), and Rabi-Hubbard (RH) models using mean field, perturbation, quantum Monte Carlo (QMC), and density matrix renormalization group (DMRG) methods. We first compare mean field predictions for the phase diagram of the Dicke model with exact QMC results and find excellent agreement. The phase diagram of the JCH model is then shown to exhibit a single Mott insulator lobe with two excitons per site, a superfluid (SF, superradiant) phase and a large region of instability where the Hamiltonian becomes unbounded. Unlike the one-photon model, there are no higher Mott lobes. Also unlike the one-photon case, the SF phases above and below the Mott are surprisingly different: Below the Mott, the SF is that of photon {\it pairs} as opposed to above the Mott where it is SF of simple photons. The mean field phase diagram of the RH model predicts a transition from a normal to a superradiant phase but none is found with QMC.

cond-mat.other↗