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B. J. Coombes

Publications and source records attributed to B. J. Coombes.

13 recordsLinked to original sources

Resolving anomalous collectivity in the $4_1^+$ to $2_1^+$ transition of $^{58}$Fe

The low-excitation states of atomic nuclei in the region around the $N = Z = 28$ shell closure are generally well described by the shell model. Most experimental observables in the iron isotopes $^{56}$Fe, $^{58}$Fe, and $^{60}$Fe ($Z = 26$; $N=30$, $32$, $34$) support a shell-model description. However, the lifetimes of the $4_1^+$ state in $^{58}$Fe in the literature result in a reduced transition strength that deviates markedly from shell-model predictions. There are three independent measurements, all in agreement and all based on the Doppler Shift Attenuation Method (DSAM) or Doppler-Broadened Line Shape method (DBLS). In this work, Coulomb-excitation measurements were performed on $^{56}$Fe and $^{58}$Fe beams to determine the ratios $B(E2; 4_1^+ \to 2_1^+)/B(E2; 2_1^+ \to 0_1^+)$. Thus, $B(E2; 4_1^+ \to 2_1^+)$ is determined relative to the known $B(E2; 2_1^+ \to 0_1^+)$ values. For $^{56}$Fe, $B(E2; 4_1^+ \to 2_1^+) = 23(4)$ W.u., agreeing with the adopted value. However, for $^{58}$Fe, the $B(E2; 4_1^+ \to 2_1^+)$ values obtained (for the various combinations of matrix element signs that could not be firmly established) are all significantly lower than the value derived from the previous lifetime measurements, and are in accord with shell-model calculations. The 1978 DSAM measurement of Bolotin et al., Nucl. Phys. A 311, 75 (1978), has been re-examined. The discrepancy between that measurement and the Coulomb-excitation measurement can be ascribed to the Lindhard-Scharff-Schiøtt (LSS) electronic stopping powers adopted for the DSAM analysis, which considerably overestimate contemporary values. Evidently, lifetime measurements from that era that are based on LSS stopping powers should be used with caution. The revised lifetime data, incorporating current stopping powers, are compared with shell-model calculations.

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Coulomb excitation of $^{124}$Te: Emerging collectivity and persisting seniority structure in the $6_1^+$ level

The low-lying energy spectra of even-even tellurium isotopes near midshell have long been interpreted as `textbook' examples of vibrational collective motion. However, in many cases electric-quadrupole observables, which are a particularly sensitive probe of collectivity, remain undetermined. Coulomb-excitation measurements were performed to measure transition strengths connecting the ground and low-excitation states in $^{124}$Te. This isotope lies at a transitional point between collective structure near the neutron midshell and seniority structures near the $N=82$ shell. A transition strength, $B(E2; 6_1^+ \to 4_1^+)$, of 27(9)~W.u. was measured for the $6^+_1\rightarrow4^+_1$ transition for the first time in this nucleus; this value is significantly below that expected for a spherical vibrator, as well as other collective models. We examine the transition strengths in $^{124}$Te and its neighbors by comparison with large-basis shell-model calculations and by comparison with General Collective Model (GCM) fits. A GCM description of $^{120}$Te agrees with experimental $E2$ transition strengths, but no comparable description of $^{124}$Te is possible with the GCM. In contrast, there is remarkably good agreement between the $B(E2; 6_1^+ \to 4_1^+)$ values and shell-model calculations for $^{124-134}$Te. It appears that, despite approaching midshell, $^{124}$Te retains a seniority structure for the $6^+_1$ level, i.e. a significant $π0g_{7/2}^2$ contribution. This persistence of the shell structure at the $6^+_1$ state is in contrast to the $B(E2)$ values of the lower-excitation $2^+_1$ and $4^+_1$ states in $^{124}$Te, and neighboring $^{120}$Te and $^{122}$Te, for which the collectivity becomes enhanced as more neutrons are removed from $N=82$.

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Evolution of the nuclear spin-orbit splitting explored via the $^{32}$Si($d$,$p$)$^{33}$Si reaction using SOLARIS

The spin-orbit splitting between neutron 1$p$ orbitals at $^{33}$Si has been deduced using the single-neutron-adding ($d$,$p$) reaction in inverse kinematics with a beam of $^{32}$Si, a long-lived radioisotope. Reaction products were analyzed by the newly implemented SOLARIS spectrometer at the reaccelerated-beam facility at the National Superconducting Cyclotron Laboratory. The measurements show reasonable agreement with shell-model calculations that incorporate modern cross-shell interactions, but they contradict the prediction of proton density depletion based on relativistic mean-field theory. The evolution of the neutron 1$p$-shell orbitals is systematically studied using the present and existing data in the isotonic chains of $N=17$, 19, and 21. In each case, a smooth decrease in the separation of the $1p_{3/2}$-$1p_{1/2}$ orbitals is seen as the respective $p$-orbitals approach zero binding, suggesting that the finite nuclear potential strongly influences the evolution of nuclear structure in this region.

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Shape polarization in the tin isotopes near $N=60$ from precision $g$-factor measurements on short-lived $11/2^-$ isomers

The $g$ factors of $11/2^-$ isomers in semimagic $^{109}$Sn and $^{111}$Sn (isomeric lifetimes $τ= 2.9(3)$ ns and $τ= 14.4(7)$ ns, respectively) were measured by an extension of the Time Differential Perturbed Angular Distribution technique, which uses \LaBr detectors and the hyperfine fields of a gadolinium host to achieve precise measurements in a new regime of short-lived isomers. The results, $g(11/2^-; {^{109}\textrm{Sn}}) = -0.186(8)$ and $g(11/2^-; {^{111}\textrm{Sn}}) = -0.214(4)$, are significantly lower in magnitude than those of the $11/2^-$ isomers in the heavier isotopes and depart from the value expected for a near pure neutron $h_{11/2}$ configuration. Broken-symmetry density functional theory calculations applied to the sequence of $11/2^-$ states reproduce the magnitude and location of this deviation. The $g(11/2^-)$ values are affected by shape core polarization; the odd $0h_{11/2}$ neutron couples to $J^π=2^+,4^+,6^+...$ configurations in the weakly-deformed effective core, causing a decrease in the $g$-factor magnitudes.

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Direct measurement of hexacontatetrapole, $\textbf{E6}$ γ decay from $^{\textbf{53m}}$Fe

The only proposed observation of a discrete, hexacontatetrapole ($E6$) transition in nature occurs from the T$_{1/2}$ = 2.54(2)-minute decay of $^{53m}$Fe. However, there are conflicting claims concerning its $γ$-decay branching ratio, and a rigorous interrogation of $γ$-ray sum contributions is lacking. Experiments performed at the Australian Heavy Ion Accelerator Facility were used to study the decay of $^{53m}$Fe. For the first time, sum-coincidence contributions to the weak $E6$ and $M5$ decay branches have been firmly quantified using complementary experimental and computational methods. Agreement across the different approaches confirms the existence of the real $E6$ transition; the $M5$ branching ratio and transition rate have also been revised. Shell model calculations performed in the full $pf$ model space suggest that the effective proton charge for high-multipole, $E4$ and $E6$, transitions is quenched to approximately two-thirds of the collective $E2$ value. Correlations between nucleons may offer an explanation of this unexpected phenomenon, which is in stark contrast to the collective nature of lower-multipole, electric transitions observed in atomic nuclei.

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Hyperfine fields at $^{66}$Ga, $^{67,69}$Ge implanted into iron and gadolinium hosts at 6 K, and applications to g-factor measurements

Isomers in $^{66}$Ga, $^{67}$Ge, and $^{69}$Ge were recoil-implanted into ferromagnetic hosts of iron and gadolinium at $\approx 6$~K, and the hyperfine magnetic fields were determined by Time Differential Perturbed Angular Distribution (TDPAD) measurements. The hyperfine field strengths at $\approx 6$~K are compared to the results of previous higher-temperature measurements and the amplitudes of the $R(t)$ functions are compared to empirical expectations. The results show that gadolinium can be a suitable host for high-precision in-beam $g$-factor measurements. The results of new $g$-factor measurements for isomers in $^{66}$Ga and $^{67}$Ge are $g(^{66}$Ga$,7^{-}) = +0.126(4)$, supporting a $[π_{f5/2} \otimes νg_{9/2}]_{7^-}$ configuration assignment, and $g(^{67}$Ge$,\frac{9}{2}^{+})=-0.1932(22)$, derived from a new measurement of the ratio $g(^{67}\mathrm{Ge})/g(^{69}\mathrm{Ge}) = 0.869(9)$. These values are in agreement with previous results. The $R(t)$ amplitudes indicate that the nuclear alignment produced in the isomeric states was significantly lower than the empirically expected $σ/I \approx 0.35$.

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Pulse Shape Discrimination of low-energy nuclear and electron recoils for improved particle identification in NaI:Tl

The scintillation mechanism in NaI:Tl crystals produces different pulse shapes that are dependent on the incoming particle type. The time distribution of scintillation light from nuclear recoil events decays faster than for electron recoil events and this difference can be categorised using various Pulse Shape Discrimination (PSD) techniques. In this study, we measured nuclear and electron recoils in a NaI:Tl crystal, with electron equivalent energies between 2 and 40 keV. We report on a new PSD approach, based on an event-type likelihood; this outperforms the charge-weighted mean-time, which is the conventional metric for PSD in NaI:Tl. Furthermore, we show that a linear combination of the two methods improves the discrimination power at these energies.

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Electric monopole transition from the superdeformed band in $^{40}$Ca

The electric monopole ($E0$) transition strength $ρ^2$ for the transition connecting the third 0$^+$ level, a "superdeformed" band head, to the "spherical" 0$^+$ ground state in doubly magic $^{40}$Ca has been determined via $e^+e^-$ pair-conversion spectroscopy. The measured value, $ρ^2(E0; 0^+_3 \to 0^+_1)~=~2.3(5)\times10^{-3}$, is the smallest $ρ^2(E0; 0^+ \to 0^+)$ found in $A<50$ nuclei. In contrast, the $E0$ transition strength to the ground state observed from the second 0$^+$ state, a band head of "normal" deformation, is an order of magnitude larger, $ρ^2(E0; 0^+_2 \to 0^+_1)~=~25.9(16)\times~10^{-3}$, which shows significant mixing between these two states. Large-Scale Shell Model (LSSM) calculations were performed to understand the microscopic structure of the excited states, and the configuration mixing between them; experimental $ρ^2$ values in $^{40}$Ca and neighboring isotopes were well reproduced by the LSSM calculations. The unusually small $ρ^2(E0; 0^+_3 \to 0^+_1)$ value is due to destructive interference in the mixing of shape-coexisting structures, which are based on several different multiparticle-multihole excitations. This observation goes beyond the usual treatment of $E0$ strengths, where two-state shape mixing cannot result in destructive interference.

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Improved precision on the experimental E0 decay branching ratio of the Hoyle state

Stellar carbon synthesis occurs exclusively via the $3α$ process, in which three $α$ particles fuse to form $^{12}$C in the excited Hoyle state, followed by electromagnetic decay to the ground state. The Hoyle state is above the $α$ threshold, and the rate of stellar carbon production depends on the radiative width of this state. The radiative width cannot be measured directly, and must instead be deduced by combining three separately measured quantities. One of these quantities is the $E0$ decay branching ratio of the Hoyle state, and the current $10$\% uncertainty on the radiative width stems mainly from the uncertainty on this ratio. The $E0$ branching ratio was deduced from a series of pair conversion measurements of the $E0$ and $E2$ transitions depopulating the $0^+_2$ Hoyle state and $2^+_1$ state in $^{12}$C, respectively. The excited states were populated by the $^{12}$C$(p,p^\prime)$ reaction at 10.5 MeV beam energy, and the pairs were detected with the electron-positron pair spectrometer, Super-e, at the Australian National University. The deduced branching ratio required knowledge of the proton population of the two states, as well as the alignment of the $2^+_1$ state in the reaction. For this purpose, proton scattering and $γ$-ray angular distribution experiments were also performed. An $E0$ branching ratio of $Γ^{E0}_π/Γ=8.2(5)\times10^{-6}$ was deduced in the current work, and an adopted value of $Γ^{E0}_π/Γ=7.6(4)\times10^{-6}$ is recommended based on a weighted average of previous literature values and the new result. The new recommended value for the $E0$ branching ratio is about 14% larger than the previous adopted value of $Γ^{E0}_π/Γ=6.7(6)\times10^{-6}$, while the uncertainty has been reduced from 9% to 5%.

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Emerging nuclear collectivity in $^{124-130}$Te

The emergence of nuclear collectivity near doubly-magic $^{132}$Sn was explored along the stable, even-even $^{124-130}$Te isotopes. Preliminary measurements of the $B(E2;4^{+}_{1}\rightarrow2^{+}_{1})$ transition strengths are reported from Coulomb excitation experiments primarily aimed at measuring the $g$ factors of the $4^{+}_{1}$ states. Isotopically enriched Te targets were excited by 198-205 MeV $^{58}$Ni beams. A comparison of transition strengths obtained is made to large-scale shell-model calculations with successes and limitations discussed.

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First-excited state $g$ factors in the stable, even Ge and Se isotopes

Transient-field $g$-factor measurements in inverse kinematics were performed for the first-excited states of the stable, even isotopes of Ge and Se. The $g$ factors of $^{74}$Ge and $^{74}$Se were measured simultaneously using a cocktail beam, which eliminates most possible sources of systematic error in a relative $g$-factor measurement. The results are $g(^{74}{\rm Se})/g(^{74}{\rm Ge})=1.34(7)$, $g(^{70}{\rm Ge})/g(^{74}{\rm Ge}) = 1.16(15)$, $g(^{72}{\rm Ge})/g(^{74}{\rm Ge})=0.92(13)$, $g(^{76}{\rm Ge})/g(^{74}{\rm Ge})=0.88(5)$, $g(^{76}{\rm Se})/g(^{74}{\rm Se})=0.96(7)$, $g(^{78}{\rm Se})/g(^{74}{\rm Se})=0.82(5)$, $g(^{80}{\rm Se})/g(^{74}{\rm Se})=0.99(7)$ and $g(^{82}{\rm Se})/g(^{74}{\rm Se})=1.19(6)$. The measured $g$-factor ratios are in agreement with ratios from previous measurements, despite considerable variation in previous reported absolute values. The absolute values of the $g$ factors remain uncertain, however the Rutgers parametrization was used to set the transient-field strength and then compare the experimental $g$ factors with shell-model calculations based on the JUN45 and jj44b interactions. Modest agreement was found between experiment and theory for both interactions. The shell model calculations indicate that the $g(2^+_1)$ values and trends are determined largely by the balance of the spin carried by orbital motion of the protons.

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Spectroscopy and excited-state $g$~factors in weakly collective ${^{111}}$Cd: confronting collective and microscopic models

The even cadmium isotopes near the neutron midshell have long been considered good examples of vibrational nuclei. However, the vibrational nature of these nuclei has been questioned based on E2 transition rates that are not consistent with vibrational excitations. In the neighbouring odd-mass nuclei, the g factors of the low-excitation collective states have been shown to be more consistent with a deformed rotational core than a vibrational core. Beyond the comparison of vibrational versus rotational models, recent advances in computational power have made shell-model calculations feasible for Cd isotopes, which may give insights into the emergence and nature of collectivity in the Cd isotopes. Collective excitations in the A ~ 100 region were studied through magnetic moments and electromagnetic transitions in 111Cd. The spectroscopy of 111Cd has been studied following Coulomb excitation. Angular correlation measurements, transient-field g-factor measurements and lifetime measurements by the Doppler-broadened line shape method were performed. The structure of the nucleus was explored in relation to particle-vibration versus particle-rotor interpretations. Large-scale shell-model calculations were performed with the SR88MHJM Hamiltonian. Excited-state g factors have been measured, spin assignments examined and lifetimes determined. Attention was given to the reported $5/2^{+}$ 753-keV and $3/2^{+}$ 755-keV states. The $3/2^{+}$ 755-keV level was not observed; evidence is presented that the reported $3/2^+$ state was a misidentification of the $5/2^{+}$ 753-keV state. It is shown that the g factors and level structure of 111Cd are not readily explained by the particle-vibration model. A particle-rotor approach has both successes and limitations. The shell-model approach successfully reproduces much of the known low-excitation structure in 111Cd.

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Perturbed angular distributions with LaBr$_3$ detectors: the $g$ factor of the first ${10^+}$ state in $^{110}$Cd revisited

The Time Differential Perturbed Angular Distribution technique with LaBr$_3$ detectors has been applied to the $I^π= \frac{11}{2}^-$ isomeric state ($E_x = 846$ keV, $τ=107$~ns) in $^{107}$Cd, which was populated and recoil-implanted into a gadolinium host following the $^{98}$Mo($^{12}$C, $3n$)$^{107}$Cd reaction. The static hyperfine field strength of Cd recoil implanted into gadolinium was thus measured, together with the fraction of nuclei implanted into field-free sites, under similar conditions as pertained for a previous implantation perturbed angular distribution $g$-factor measurement on the $I^π= 10^+$ state in $^{110}$Cd. The $^{110}$Cd $g(10^+)$ value was thereby re-evaluated, bringing it into agreement with the value expected for a seniority-two $νh_{\frac{11}{2}}$ configuration.

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