arXiv subjects

B. J. LeRoy

Publications and source records attributed to B. J. LeRoy.

17 recordsLinked to original sources

arXiv2018

Temperature dependence of interlayer coupling in perpendicular magnetic tunnel junctions with GdOx barriers

Perpendicular magnetic tunnel junctions with GdOX tunneling barriers have shown a unique voltage controllable interlayer magnetic coupling effect. Here we investigate the quality of the GdOX barrier and the coupling mechanism in these junctions by examining the temperature dependence of the tunneling magnetoresistance and the interlayer coupling from room temperature down to 11 K. The barrier is shown to be of good quality with the spin independent conductance only contributing a small portion, 14%, to the total room temperature conductance, similar to AlOX and MgO barriers. The interlayer coupling, however, shows an anomalously strong temperature dependence including sign changes below 80 K. This non-trivial temperature dependence is not described by previous models of interlayer coupling and may be due to the large induced magnetic moment of the Gd ions in the barrier.

cond-mat.mtrl-sci↗

arXiv2013

Gate dependent Raman spectroscopy of graphene on hexagonal boron nitride

Raman spectroscopy, a fast and nondestructive imaging method, can be used to monitor the doping level in graphene devices. We fabricated chemical vapor deposition (CVD) grown graphene on atomically flat hexagonal boron nitride (hBN) flakes and SiO$_2$ substrates. We compared their Raman response as a function of charge carrier density using an ion gel as a top gate. The G peak position, 2D peak position, 2D peak width and the ratio of the 2D peak area to the G peak area show a dependence on carrier density that differs for hBN compared to SiO$_2$. Histograms of two-dimensional mapping are used to compare the fluctuations in the Raman peak properties between the two substrates. The hBN substrate has been found to produce fewer fluctuations at the same charge density owing to its atomically flat surface and reduced charged impurities.

cond-mat.mtrl-sci↗

arXiv2011

STM Spectroscopy of ultra-flat graphene on hexagonal boron nitride

Graphene has demonstrated great promise for future electronics technology as well as fundamental physics applications because of its linear energy-momentum dispersion relations which cross at the Dirac point. However, accessing the physics of the low density region at the Dirac point has been difficult because of the presence of disorder which leaves the graphene with local microscopic electron and hole puddles, resulting in a finite density of carriers even at the charge neutrality point. Efforts have been made to reduce the disorder by suspending graphene, leading to fabrication challenges and delicate devices which make local spectroscopic measurements difficult. Recently, it has been shown that placing graphene on hexagonal boron nitride (hBN) yields improved device performance. In this letter, we use scanning tunneling microscopy to show that graphene conforms to hBN, as evidenced by the presence of Moire patterns in the topographic images. However, contrary to recent predictions, this conformation does not lead to a sizable band gap due to the misalignment of the lattices. Moreover, local spectroscopy measurements demonstrate that the electron-hole charge fluctuations are reduced by two orders of magnitude as compared to those on silicon oxide. This leads to charge fluctuations which are as small as in suspended graphene, opening up Dirac point physics to more diverse experiments than are possible on freestanding devices.

cond-mat.mtrl-sci↗

arXiv2010

Imaging charge density fluctuations in graphene using Coulomb blockade spectroscopy

Using scanning tunneling microscopy, we have imaged local charge density fluctuations in monolayer graphene. By placing a small gold nanoparticle on the end of the STM tip, a charge sensor is created. By raster scanning the tip over the surface and using Coulomb blockade spectroscopy, we map the local charge on the graphene. We observe a series of electron and hole doped puddles with a characteristic length scale of about 20 nm. Theoretical calculations for the correlation length of the puddles based on the number of impurities are in agreement with our measurements.

cond-mat.mes-hall↗

arXiv2010

Lithography-free Fabrication of High Quality Substrate-supported and Freestanding Graphene devices

We present a lithography-free technique for fabrication of clean, high quality graphene devices. This technique is based on evaporation through hard Si shadow masks, and eliminates contaminants introduced by lithographical processes. We demonstrate that devices fabricated by this technique have significantly higher mobility values than those by standard electron beam lithography. To obtain ultra-high mobility devices, we extend this technique to fabricate suspended graphene samples with mobility as high as 120,000 cm^2/Vs.

cond-mat.mes-hall↗

arXiv2009

Spatial mapping of the Dirac point in monolayer and bilayer graphene

We have mapped the Dirac point in exfoliated monolayer and bilayer graphene using spatially resolved scanning tunneling spectroscopy (STS) measurements at low temperature. The Dirac point shifts in energy at different locations in graphene. However, a cross correlation with the topography shows no correlation indicating that topographic features such as ripples are not the primary source of the variation. Rather, we attribute the shift of the Dirac point to random charged impurities located near the graphene. Our findings emphasize the need to advance exfoliated graphene sample preparation to minimize the effect of impurities.

cond-mat.mes-hall↗

arXiv2009

Mapping the Dirac point in gated bilayer graphene

We have performed low temperature scanning tunneling spectroscopy measurements on exfoliated bilayer graphene on SiO2. By varying the back gate voltage we observed a linear shift of the Dirac point and an opening of a band gap due to the perpendicular electric field. In addition to observing a shift in the Dirac point, we also measured its spatial dependence using spatially resolved scanning tunneling spectroscopy. The spatial variation of the Dirac point was not correlated with topographic features and therefore we attribute its shift to random charged impurities.

cond-mat.mes-hall↗

arXiv2009

Spatially resolved spectroscopy of monolayer graphene on SiO2

We have carried out scanning tunneling spectroscopy measurements on exfoliated monolayer graphene on SiO$_2$ to probe the correlation between its electronic and structural properties. Maps of the local density of states are characterized by electron and hole puddles that arise due to long range intravalley scattering from intrinsic ripples in graphene and random charged impurities. At low energy, we observe short range intervalley scattering which we attribute to lattice defects. Our results demonstrate that the electronic properties of graphene are influenced by intrinsic ripples, defects and the underlying SiO$_2$ substrate.

cond-mat.mes-hall↗

arXiv2005

Three-terminal scanning tunneling spectroscopy of suspended carbon nanotubes

We have performed low-temperature scanning tunneling spectroscopy measurements on suspended single-wall carbon nanotubes with a gate electrode allowing three-terminal spectroscopy measurements. These measurements show well-defined Coulomb diamonds as well as side peaks from phonon-assisted tunneling. The side peaks have the same gate voltage dependence as the main Coulomb peaks, directly proving that they are excitations of these states.

cond-mat.mes-hall↗

arXiv2005

Imaging Electron Interferometer

An imaging interferometer was created in a two-dimensional electron gas by reflecting electron waves emitted from a quantum point contact (QPC) with a circular mirror. Images of electron flow obtained with a scanning probe microscope at liquid He temperatures show interference fringes when the mirror is energized. A quantum phase shifter was created by moving the mirror via its gate voltage, and an interferometric spectrometer can be formed by sweeping the tip over many wavelengths. Experiments and theory demonstrate that the interference signal is robust against thermal averaging.

cond-mat.mes-hall↗

arXiv2005

Integration of a gate electrode into carbon nanotube devices for scanning tunneling microscopy

We have developed a fabrication process for incorporating a gate electrode into suspended single-walled carbon nanotube structures for scanning tunneling spectroscopy studies. The nanotubes are synthesized by chemical vapor deposition directly on a metal surface. The high temperature ~800 C involved in the growth process poses challenging issues such as surface roughness and integrity of the structure which are addressed in this work. We demonstrate the effectiveness of the gate on the freestanding part of the nanotubes by performing tunneling spectroscopy that reveals Coulomb blockade diamonds. Our approach enables combined scanning tunneling microscopy and gated electron transport investigations of carbon nanotubes.

cond-mat.mes-hall↗

arXiv2005

Electrical generation and absorption of phonons in carbon nanotubes

The interplay between discrete vibrational and electronic degrees of freedom directly influences the chemical and physical properties of molecular systems. This coupling is typically studied through optical methods such as fluorescence, absorption, and Raman spectroscopy. Molecular electronic devices provide new opportunities for exploring vibration-electronic interactions at the single molecule level. For example, electrons injected from a scanning tunneling microscope tip into a metal can excite vibrational excitations of a molecule in the gap between tip and metal. Here we show how current directly injected into a freely suspended individual single-wall carbon nanotube can be used to excite, detect, and control a specific vibrational mode of the molecule. Electrons inelastically tunneling into the nanotube cause a non-equilibrium occupation of the radial breathing mode, leading to both stimulated emission and absorption of phonons by successive electron tunneling events. We exploit this effect to measure a phonon lifetime on the order of 10 nanoseconds, corresponding to a quality factor well over 10000 for this nanomechanical oscillator.

cond-mat.mes-hall↗

arXiv2004

Thermal Electron Wavepacket Interferometry: Derivation and New Results

A novel formal equivalence between thermal averages of coherent properties (e.g. conductance), and time averages of a single wavepacket arises for Fermi gasses and certain geometries. In the case of one open channel in a quantum point contact (QPC), only one wavepacket history, with wavepacket width equal to thermal length, completely determines thermally averaged conductance. The formal equivalence moreover allows very simple physical interpretations of interference features surviving under thermal averaging. Simply put, pieces of thermal wavepacket returning to the QPC along independent paths must arrive at the same time in order to interfere. Remarkably, one immediate result of this approach is that higher temperature leads to narrower wavepackets and therefore better resolution of events in the time domain. In effect, experiments at 4.2 K are performing time gated experiments at better than a gigahertz. Experiments involving thermally averaged ballistic conductance in 2DEGS are presented as an application of this picture.

cond-mat.mes-hall↗

arXiv2004

Scanning Tunneling Spectroscopy of Suspended Single-Wall Carbon Nanotubes

We have performed low-temperature STM measurements on single-wall carbon nanotubes that are freely suspended over a trench. The nanotubes were grown by CVD on a Pt substrate with predefined trenches etched into it. Atomic resolution was obtained on the freestanding portions of the nanotubes. Spatially resolved spectroscopy on the suspended portion of both metallic and semiconducting nanotubes was also achieved, showing a Coulomb-staircase behavior superimposed on the local density of states. The spacing of the Coulomb blockade peaks changed with tip position reflecting a changing tip-tube capacitance.

cond-mat.mes-hall↗

arXiv2002

Imaging coherent electron wave flow in a two-dimensional electron gas

We measure the energy distribution of electrons passing through a two-dimensional electron gas using a scanning probe microscope. We present direct spatial images of coherent electron wave flow from a quantum point contact formed in a GaAs/AlGaAs two-dimensional electron gas using a liquid He cooled SPM. A negative voltage is placed on the tip, which creates a small region of depleted electrons that backscatters electron waves. Oscillating the voltage on the tip and locking into this frequency gives the spatial derivative of electron flow perpendicular to the direction of current flow. We show images of electron flow using this method. By measuring the amount of electrons backscattered as a function of the voltage applied to the tip, the energy distribution of electrons is measured.

cond-mat.mes-hall↗

arXiv2002

Imaging Coherent Electron Flow

Images of electron flow through a two-dimensional electron gas from a quantum point contact (QPC) can be obtained at liquid He temperatures using scanning probe microscopy (SPM). A negatively charged SPM tip depletes the electron gas immediately below it and decreases the conductance by backscattering electrons. Images of electron flow are obtained by recording the conductance as the tip is scanned over the sample. These images show angular patterns that are characteristic of electron flow through individual modes of the QPC, as well as well-defined branches at longer distances. The addition of a prism formed by a triangular gate bends electron paths as the electron density is reduced under the prism by an applied gate voltage. Under the conditions of the experiment, electron-electron scattering is the dominant inelastic process. By observing how the amplitude of backscattered electrons in images of electron flow decreases with added electron energy, we are able to determine the average length and time necessary for inelastic scattering. A dc voltage Vo applied across the QPC accelerates electrons so that their energy is greater than the Fermi energy before inelastic scattering occurs. The signal is observed to decrease in amplitude and eventually disappear at distances from the QPC that decrease progressively as Vo is increased.

cond-mat.mes-hall↗

arXiv2000

Coherent Branched Flow in a Two-Dimensional Electron Gas

Semiconductor nanostructures based on two dimensional electron gases (2DEGs) have the potential to provide new approaches to sensing, information processing, and quantum computation. Much is known about electron transport in 2DEG nanostructures and many remarkable phenomena have been discovered (e.g. weak localization, quantum chaos, universal conductance fluctuations)1,2 - yet a fundamental aspect of these devices, namely how electrons move through them, has never been clarified. Important details about the actual pattern of electron flow are not specified by statistical measures such as the mean free path. Scanned probe microscope (SPM) measurements allow spatial investigations of nanostructures, and it has recently become possible to directly image electron flow through 2DEG devices using newly developed SPM techniques3-13. Here we present SPM images of electron flow from a quantum point contact (QPC) which show unexpected dynamical channeling - the electron flow forms persistent, narrow, branching channels rather than smoothly spreading fans. Theoretical study of this flow, including electron scattering by impurities and donor atoms, shows that the channels are not due to deep valleys in the potential, but rather are caused by the indirect cumulative effect of small angle scattering. Surprisingly, the channels are decorated by interference fringes well beyond where the simplest thermal averaging arguments suggest they should be found. These findings may have important implications for 2DEG physics and for the design of future nanostructure devices.

cond-mat.mes-hall↗