arXiv subjects

B. J. Ramshaw

Publications and source records attributed to B. J. Ramshaw.

At least 19 recordsLinked to original sources

arXiv2026

Out-of-equilibrium relaxation dynamics of the superconducting order parameter in CsV$_3$Sb$_5$

The application of a time-varying strain field drives a superconducting order parameter out of equilibrium. How the order parameter relaxes back to equilibrium depends both on the structure of the superconducting gap and on the nature of quasiparticle scattering. We report the discovery of an ultrasonic attenuation peak inside the superconducting state of the kagome superconductor CsV$_3$Sb$_5$. This peak is the natural consequence of the order parameter relaxation time matching the ultrasonic drive frequency near $T_{\rm c}$. From the measured frequency dependence of the peak, we extract a microscopic scattering time of $τ_N = 25$ ps. This timescale is two orders of magnitude longer than the elastic scattering time as determined by resistivity measurements, but is comparable to the inelastic scattering time determined by thermal transport. Within the conventional framework of order-parameter relaxation, this implies that elastic scattering is ineffective at relaxing the superconducting condensate, consistent with a sign-preserving $s$-wave state obeying Anderson's theorem.

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arXiv2026

Magnetic field as a dynamic energy scale in quantum-critical CeCoIn$_5$

Whether magnetic field enters the quantum-critical dynamics as a competing energy scale in strange metals remains an open question. Using thermal impedance spectroscopy, we simultaneously measure the electronic specific heat and spin-relaxation dynamics of CeCoIn$_5$. Both properties show scale invariance with temperature and magnetic field, where a single energy scale governs their crossover. Magnetic field thus competes directly with temperature to set the infrared cutoff, establishing it as a dynamic energy scale in the critical dynamics of this strange metal.

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arXiv2026

Symmetry, Sound, and the Quest for Chiral Superconductors

The confirmation of a bulk, topological superconductor is a central goal of modern quantum materials research. Despite decades of searching, no confirmed examples yet exist. A primary difficulty is that most experimental signatures of topological superconductivity are ambiguous and indirect. I review efforts to narrow the search for a chiral topological superconductor using measurements of elastic moduli. In principle, these experiments can provide unambiguous thermodynamic evidence for multi-component superconductivity---a pre-requisite for chiral superconductivity in 2D and quasi-2D materials. Despite the potential strength of this program, the results are still negative. I provide a pedagogical introduction to multi-component order parameters, chiral topological superconductivity, and how superconducting order parameters couple to strain. I discuss ongoing efforts in heavy fermion, iron pnictide, and Kagome superconductors, and suggest routes for speeding up the search process, as well as other experimental tools that should be developed for the pursuit of this goal.

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arXiv2026

Emergence of Fermi-liquid and BCS physics in overdoped cuprates

Cuprates are the paradigmatic `unconventional' superconductors: their critical temperature is much higher than can be expected from phonon-mediated pairing; the superconducting gap has $d$-wave symmetry; and the normal-metallic state appears to be far from a conventional Fermi liquid. These and numerous other experimental facts have led to a consensus that the conventional theory --- the Fermi-liquid-based Bardeen--Cooper--Schrieffer (BCS) theory --- is the wrong starting point for understanding superconductivity in the cuprates. In this Perspective, we propose that, although underdoped cuprates do indeed require a different theoretical framework, there is a crossover with increasing doping to an overdoped regime in which a BCS-like approach is warranted (at energy scales of the order of the superconducting gap and below), provided that the various forms of disorder are accounted for. We summarize key experimental studies of the low-energy properties of overdoped cuprates, identify properties that are and are not compatible with this proposal --- and argue that features that are inconsistent with this approach can in fact be attributed to the expected effects of material disorder. Finally, we provide falsifiable predictions for the behaviour of an `ideal' (disorder-free) overdoped cuprate through which our approach can be tested.

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arXiv2026

Thermodynamic Discovery of Tetracriticality and Emergent Multicomponent Superconductivity in UTe$_2$

The candidate topological superconductor UTe$_2$ exhibits a complex phase diagram with multiple superconducting states, yet the nature of their coexistence has remained a central mystery. In particular, the apparent intersection of two second-order phase boundaries at a ``triple point'' in the pressure-temperature phase diagram is thermodynamically forbidden, suggesting either hidden phase transitions or a fundamental misunderstanding of the superconductivity in UTe$_2$. Here, we use pulse-echo ultrasound to resolve this puzzle by discovering a new phase boundary that is characterized by a unique ``upward jump" in the sound velocity -- direct thermodynamic evidence for a phase transition where superconducting order is lost upon cooling. Our results establish $\left(P^{\star},T^{\star}\right)$ as a tetracritical point, beyond which the ambient and pressure-induced superconducting order parameters form a multi-component state. We use the measured phase diagram to demonstrate that strong competition between the two superconducting order parameters drives the loss of order on cooling, and leads to phase locking that suppresses superconducting fluctuations. These findings provide the definitive magnetic field-temperature-pressure phase diagram of UTe$_2$, and establish a thermodynamic foundation for multi-component -- and potentially topological -- superconductivity.

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arXiv2026

Universal Planckian relaxation in the strange metal state of the cuprates

A major puzzle in high-$T_{\rm c}$ superconductivity is the origin of the ``Planckian'' relaxation rate $1/τ$ underlying the linear-in-temperature resistivity in the strange-metal state, which persists up to very high temperatures. Implicit in theoretical discussions is the assumption that $1/τ$ must be universal. Experimentally, it is unclear, however, how such universality can be reconciled with the observed strong doping dependence of the resistivity over a wide doping range. We show, through an analysis of a large body of optical conductivity and electrical resistivity data, that a universal $1/τ$ requires only that the square optical plasma frequency $ω_{\rm opt}^2(p)$ scales linearly with $p$ across the entire doping range, as is observed experimentally. We further argue that this can be understood via a Gutzwiller factor in doped Mott insulators of the form proposed by Anderson [\emph{Science} \textbf{235}, 1196 (1987)].

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arXiv2026

Scale-invariant magnetic anisotropy in $α$-RuCl$_3$: A quantum Monte Carlo study

We compute the rotational anisotropy of the free energy of $α$-RuCl$_3$ in an external magnetic field. This quantity, known as the magnetotropic susceptibility, $k$, relates to the second derivative of the free energy with respect to the angle of rotation. We have used approximation-free, auxiliary-field quantum Monte Carlo simulations for a realistic model of $α$-RuCl$_3$ and optimized the path integral to alleviate the negative sign problem. This allows us to reach temperatures down to $30~\mathrm{K}$, an energy scale below the dominant Kitaev coupling. We demonstrate that the magnetotropic spin susceptibility in this model of $α$-RuCl$_3$ displays scaling behavior $k = T f(B/T)$ at high temperatures. Once the uniform susceptibility departs from the Curie law (i.e., at the energy scale of the exchange interactions), it appears to transition to an emergent scalinglike behavior, characterized by a different function $f$ at lower temperatures, stemming from the locality of torque fluctuations. We observe a remarkable numerical match between experiment and simulations and we also find qualitative agreement with the pure Kitaev model. In comparison, for the XXZ Heisenberg Hamiltonian, the scaling $k = T f(B/T)$ breaks down at a temperature scale where the uniform spin susceptibility deviates from the Curie law and never reemerges at low temperatures.

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arXiv2026

Phonon Hall Viscosity and the Intrinsic Thermal Hall Effect of $α$-RuCl$_3$

The thermal Hall effect has been observed in a wide variety of magnetic insulators, yet its origins remains controversial. While some studies attribute the effect to intrinsic mechanism, such as heat carriers with Berry curvature, others propose extrinsic mechanisms, such as heat carriers scattering off crystal defects. Even the nature of the heat carriers is unknown: magnons, phonons, and fractionalized spin excitations have all been proposed. Resolving these issues is essential for the study of quantum spin liquids, and particularly for $α$-RuCl$_3$, where a quantized thermal Hall effect has been attributed to Majorana edge modes. Here, we use ultrasonic measurements of the acoustic Faraday effect to demonstrate that the phonons in $α$-RuCl$_3$ have Hall viscosity -- a non-dissipative viscosity that rotates phonon polarizations and deflects phonon heat currents. We show that phonon Hall viscosity produces an intrinsic thermal Hall effect that quantitatively accounts for a significant fraction of the measured thermal Hall effect in $α$-RuCl$_3$: the thermal Hall effect in $α$-RuCl$_3$ is due to phonons \textit{and} it is intrinsic. More broadly, we demonstrate that the acoustic Faraday effect is a powerful tool for detecting phonon Hall viscosity and the associated phonon Berry curvature, offering a new way to uncover and study exotic states of matter that elude conventional experiments.

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arXiv2026

Vanishing Phase Stiffness and Fluctuation-Dominated Superconductivity: Evidence for Inter-Band Pairing in UTe$_2$

Superconductivity in three dimensions is almost universally governed by Ginzburg-Landau mean field theory, with critical fluctuations typically confined to within a few percent of the transition temperature ($T_{\rm c}$). We report that the heavy-Fermion superconductor UTe$_2$ exhibits a fluctuation regime that extends over a temperature range as wide as $T_{\rm c}$ itself -- the largest observed for any three-dimensional superconductor. Through ultrasound measurements of the elastic moduli and sound attenuation, we find that UTe$_2$ transitions from a mean-field-like state at ambient pressure to a fluctuation dominated state at higher pressures. This regime is marked by elastic softening and an increase in sound attenuation that onsets well above $T_{\rm c}$, with the attenuation remaining anomalously high deep in the superconducting state. Our analysis shows that these features stem from an extremely low superfluid phase stiffness. This results in a kinetic inductance as high as that of granular aluminum, but achieved in the clean limit. We propose that this exotic state is driven by dominant inter-band pairing mediated by ferromagnetic fluctuations, leading to "local" cooper pairs with a coherence length of only a few lattice constants.

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arXiv2025

Expert Evaluation of LLM World Models: A High-$T_c$ Superconductivity Case Study

Large Language Models (LLMs) show great promise as a powerful tool for scientific literature exploration. However, their effectiveness in providing scientifically accurate and comprehensive answers to complex questions within specialized domains remains an active area of research. Using the field of high-temperature cuprates as an exemplar, we evaluate the ability of LLM systems to understand the literature at the level of an expert. We construct an expert-curated database of 1,726 scientific papers that covers the history of the field, and a set of 67 expert-formulated questions that probe deep understanding of the literature. We then evaluate six different LLM-based systems for answering these questions, including both commercially available closed models and a custom retrieval-augmented generation (RAG) system capable of retrieving images alongside text. Experts then evaluate the answers of these systems against a rubric that assesses balanced perspectives, factual comprehensiveness, succinctness, and evidentiary support. Among the six systems two using RAG on curated literature outperformed existing closed models across key metrics, particularly in providing comprehensive and well-supported answers. We discuss promising aspects of LLM performances as well as critical short-comings of all the models. The set of expert-formulated questions and the rubric will be valuable for assessing expert level performance of LLM based reasoning systems.

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arXiv2025

Multipolar Fermi Surface Deformations in Sr$_2$RuO$_4$ Probed by Resistivity and Sound Attenuation: A Window into Electron Viscosity and the Collision Operator

Recent developments in electron hydrodynamics have demonstrated the importance of considering the full structure of the electron-electron scattering operator, which encodes a sequence of lifetimes, one for each component of the Fermi surface deformation in a multipolar expansion. In this context, the dipolar lifetime is measured by resistivity, whereas the quadrupolar component probes the viscosity and can be measured in the bulk via sound attenuation. We introduce a framework to extract the collision operator of an arbitrary metal by combining resistivity and sound attenuation measurements with a realistic calculation of the scattering operator that includes multiband and Umklapp effects. The collision operator allows for the prediction of a plethora of properties, including the non-local conductivity, and can be used to predict hydrodynamic behavior for bulk metals. As a first application, we apply this framework to Sr$_2$RuO$_4$ in a temperature range where electron-electron scattering is dominant. We find quantitative agreement between our model and the temperature dependence of both the resistivity and the sound attenuation, we find the quadrupolar (B1g) relaxation rate to be 30% higher than the dipolar one due to the presence of hot spots on the $γ$ band, and we predict a strongly anisotropic viscosity arising from the $α$ and $β$ bands.

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arXiv2025

Giant transverse magnetic fluctuations at the edge of re-entrant superconductivity in UTe$_{2}$

UTe$_{2}$ exhibits the remarkable phenomenon of re-entrant superconductivity, whereby the zero-resistance state reappears above 40 tesla after being suppressed with a field of around 10 tesla. One potential pairing mechanism, invoked in the related re-entrant superconductors UCoGe and URhGe, involves transverse fluctuations of a ferromagnetic order parameter. However, the requisite ferromagnetic order - present in both UCoGe and URhGe - is absent in UTe$_{2}$, and magnetization measurements show no sign of strong fluctuations. Here, we measure the magnetotropic susceptibility of UTe$_{2}$ across two field-angle planes. This quantity is sensitive to the magnetic susceptibility in a direction transverse to the applied magnetic field - a quantity that is not accessed in conventional magnetization measurements. We observe a very large decrease in the magnetotropic susceptibility over a broad range of field orientations, indicating a large increase in the transverse magnetic susceptibility. The three superconducting phases of UTe$_{2}$, including the high-field re-entrant phase, surround this region of enhanced susceptibility in the field-angle phase diagram. The strongest transverse susceptibility is found near the critical end point of the high-field metamagnetic transition, suggesting that quantum critical fluctuations of a field-induced magnetic order parameter may be responsible for the large transverse susceptibility, and may provide a pairing mechanism for field-induced superconductivity in UTe$_{2}$.

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arXiv2024

Electronic band structure of a superconducting nickelate probed by the Seebeck coefficient in the disordered limit

Superconducting nickelates are a new family of strongly correlated electron materials with a phase diagram closely resembling that of superconducting cuprates. While analogy with the cuprates is natural, very little is known about the metallic state of the nickelates, making these comparisons difficult. We probe the electronic dispersion of thin-film superconducting 5-layer ($n=5$) and metallic 3-layer ($n=3$) nickelates by measuring the Seebeck coefficient, $S$. We find a temperature-independent and negative $S/T$ for both $n=5$ and $n=3$ nickelates. These results are in stark contrast to the strongly temperature-dependent $S/T$ measured at similar electron filling in the cuprate La$_{1.36}$Nd$_{0.4}$Sr$_{0.24}$CuO$_4$. The electronic structure calculated from density functional theory can reproduce the temperature dependence, sign, and amplitude of $S/T$ in the nickelates using Boltzmann transport theory. This demonstrates that the electronic structure obtained from first-principles calculations provides a reliable description of the Fermiology of superconducting nickelates, and suggests that, despite indications of strong electronic correlations, there are well-defined quasiparticles in the metallic state. Finally, we explain the differences in the Seebeck coefficient between nickelates and cuprates as originating in strong dissimilarities in impurity concentrations. Our study demonstrates that the high elastic scattering limit of the Seebeck coefficient reflects only the underlying band structure of a metal, analogous to the high magnetic field limit of the Hall coefficient. This opens a new avenue for Seebeck measurements to probe the electronic band structures of relatively disordered quantum materials.

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arXiv2024

Absence of a Bulk Thermodynamic Phase Transition to a Density Wave Phase in UTe2

Competing and intertwined orders are ubiquitous in strongly correlated electron systems, such as the charge, spin, and superconducting orders in the high-Tc cuprates. Recent scanning tunneling microscopy (STM) measurements provide evidence for a charge density wave (CDW) that coexists with superconductivity in the heavy Fermion metal UTe2. This CDW persists up to at least 7.5 K and, as a CDW breaks the translational symmetry of the lattice, its disappearance is necessarily accompanied by thermodynamic phase transition. Here, we report high-precision thermodynamic measurements of the elastic moduli of UTe2. We observe no signature of a phase transition in the elastic moduli down to a level of 1 part in 10^7, strongly implying the absence of bulk CDW order in UTe2. We suggest that the CDW and associated pair density wave (PDW) observed by STM may be confined to the surface of UTe2.

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arXiv2024

Quantum Fluctuations Suppress the Critical Fields in BaCo$_2$(AsO$_4$)$_2$

Early efforts to realize exotic quantum ground states in frustrated magnets focused on frustration arising from the lattice geometry alone. Attention has shifted to bond-dependent anisotropic interactions, as well as further-neighbor interactions, on non-geometrically-frustrated lattices due to their greater versatility. The honeycomb magnet BaCo$_2$(AsO$_4$)$_2$ recently emerged as a candidate host for both bond-dependent (e.g. Kitaev) and third-neighbor ($J_3$) interactions, and has become a model experimental system due to its relatively low levels of disorder. Understanding the relative importance of different exchange interactions holds the key to achieving novel ground states, such as quantum spin liquids. Here, we use the magnetotropic susceptibility to map out the intermediate and high-field phase diagram of BaCo$_2$(AsO$_4$)$_2$ as a function of the out-of-plane magnetic field direction at $T = 1.6$ K. We show that the experimental data are qualitatively consistent with classical Monte Carlo results of the XXZ-$J_1$-$J_3$ model with small Kitaev and off-diagonal exchange couplings included. However, the calculated critical fields are systematically larger than the experimental values. Infinite-DMRG computations on the quantum model reveal that quantum corrections from a nearby ferromagnetic state are likely responsible for the suppressed critical fields. Together, our experiment and theory analyses demonstrate that, while quantum fluctuations play an important role in determining the phase diagram, most of the physics of BaCo$_2$(AsO$_4$)$_2$ can be understood in terms of the classical dynamics of long-range ordered states, leaving little room for the possibility of a quantum spin liquid.

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arXiv2024

Resonant Ultrasound Spectroscopy for Irregularly-Shaped Samples and its Application to Uranium Ditelluride

Resonant ultrasound spectroscopy (RUS) is a powerful technique for measuring the full elastic tensor of a given material in a single experiment. Previously, this technique was limited to regularly-shaped samples such as rectangular parallelepipeds, spheres, and cylinders. We demonstrate a new method for determining the elastic moduli of irregularly-shaped samples, extending the applicability of RUS to a much larger set of materials. We apply this new approach to the recently-discovered unconventional superconductor UTe$_2$ and provide its elastic tensor at both 300 and 4 kelvin.

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arXiv2024

Elastocaloric evidence for a multicomponent superconductor stabilized within the nematic state in Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$

The iron-based high-$T_c$ superconductors exhibit rich phase diagrams with intertwined phases, including magnetism, nematicity and superconductivity. The superconducting $T_c$ in many of these materials is maximized in the regime of strong nematic fluctuations, making the role of nematicity in influencing the superconductivity a topic of intense research. Here, we use the AC elastocaloric effect (ECE) to map out the phase diagram of Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ near optimal doping. The ECE signature at $T_c$ on the overdoped side, where superconductivity condenses without any nematic order, is quantitatively consistent with other thermodynamic probes that indicate a single-component superconducting state. In contrast, on the slightly underdoped side, where superconductivity condenses within the nematic phase, ECE reveals a second thermodynamic transition proximate to and below $T_c$. We rule out magnetism and re-entrant tetragonality as the origin of this transition, and find that our observations strongly suggest a phase transition into a multicomponent superconducting state. This implies the existence of a sub-dominant pairing instability that competes strongly with the dominant $s^\pm$ instability. Our results thus motivate a re-examination of the pairing state and its interplay with nematicity in this extensively studied iron-based superconductor, while also demonstrating the power of ECE in uncovering strain-tuned phase diagrams of quantum materials.

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arXiv2023

Single-Component Superconductivity in UTe$_2$ at Ambient Pressure

The microscopic mechanism of Cooper pairing in a superconductor leaves its fingerprint on the symmetry of the order parameter. UTe$_2$ has been inferred to have a multi-component order parameter that entails exotic effects like time reversal symmetry breaking. However, recent experimental observations in newer-generation samples have raised questions about this interpretation, pointing to the need for a direct experimental probe of the order parameter symmetry. Here, we use pulse-echo ultrasound to measure the elastic moduli of UTe$_2$ in samples that exhibit both one and two superconducting transitions. We demonstrate the absence of thermodynamic discontinuities in the shear elastic moduli of both single- and double-transition samples, providing direct evidence that UTe$_2$ has a single-component superconducting order parameter. We further show that superconductivity is highly sensitive to compression strain along the $a$ and $c$ axes, but insensitive to strain along the $b$ axis. This leads us to suggest a single-component, odd-parity order parameter -- specifically the B$_{2u}$ order parameter -- as most compatible with our data.

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