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B. J. Ramshaw

Publications and source records attributed to B. J. Ramshaw.

At least 55 records · Page 3Linked to original sources

GaN/AlGaN 2DEGs in the quantum regime: Magneto-transport and photoluminescence to 60 tesla

Using high magnetic fields up to 60 T, we report magneto-transport and photoluminescence (PL) studies of a two-dimensional electron gas (2DEG) in a GaN/AlGaN heterojunction grown by molecular-beam epitaxy. Transport measurements demonstrate that the quantum limit can be exceeded (Landau level filling factor $ν< 1$), and show evidence for the $ν=2/3$ fractional quantum Hall state. Simultaneous optical and transport measurements reveal synchronous quantum oscillations of both the PL intensity and longitudinal resistivity in the integer quantum Hall regime. PL spectra directly reveal the dispersion of occupied Landau levels in the 2DEG and therefore the electron mass. These results demonstrate the utility of high (pulsed) magnetic fields for detailed measurements of quantum phenomena in high-density 2DEGs.

cond-mat.mes-hall↗

Thermodynamic Evidence for a Two-Component Superconducting Order Parameter in Sr$_2$RuO$_4$

Sr$_2$RuO$_4$ has stood as the leading candidate for a spin-triplet superconductor for 26 years. Recent NMR experiments have cast doubt on this candidacy, however, and it is difficult to find a theory of superconductivity that is consistent with all experiments. What is needed are symmetry-based experiments that can rule out broad classes of possible superconducting order parameters. Here we use resonant ultrasound spectroscopy to measure the entire symmetry-resolved elastic tensor of Sr$_2$RuO$_4$ through the superconducting transition. We observe a thermodynamic discontinuity in the shear elastic modulus $c_{66}$, requiring that the superconducting order parameter is two-component. A two-component $p$-wave order parameter, such as $p_x+i p_y$, naturally satisfies this requirement. As this order parameter appears to be precluded by recent NMR experiments, we suggest that two other two-component order parameters, namely $\left\{d_{xz},d_{yz}\right\}$ or $\left\{d_{x^2-y^2},g_{xy(x^2-y^2)}\right\}$, are now the prime candidates for the order parameter of Sr$_2$RuO$_4$.

cond-mat.supr-con↗

Scale-Invariance of a Spin Liquid in High Magnetic Fields

In RuCl$_3$, inelastic neutron scattering and Raman spectroscopy reveal a continuum of non-spin-wave excitations that persists to high temperature, suggesting the presence of a spin liquid state on a honeycomb lattice. In the context of the Kitaev model, magnetic fields introduce finite interactions between the elementary excitations, and thus the effects of high magnetic fields - comparable to the spin exchange energy scale - must be explored. Here we report measurements of the magnetotropic coefficient - the second derivative of the free energy with respect to magnetic field orientation - over a wide range of magnetic fields and temperatures. We find that magnetic field and temperature compete to determine the magnetic response in a way that is independent of the large intrinsic exchange interaction energy. This emergent scale-invariant magnetic anisotropy provides evidence for a high degree of exchange frustration that favors the formation of a spin liquid state in RuCl$_3$.

cond-mat.str-el↗

Scale-invariant magnetic anisotropy in RuCl$_3$ at high magnetic fields

In RuCl$_3$, inelastic neutron scattering and Raman spectroscopy reveal a continuum of non-spin-wave excitations that persists to high temperature, suggesting the presence of a spin liquid state on a honeycomb lattice. In the context of the Kitaev model, magnetic fields introduce finite interactions between the elementary excitations, and thus the effects of high magnetic fields - comparable to the spin exchange energy scale - must be explored. Here we report measurements of the magnetotropic coefficient - the second derivative of the free energy with respect to magnetic field orientation - over a wide range of magnetic fields and temperatures. We find that magnetic field and temperature compete to determine the magnetic response in a way that is independent of the large intrinsic exchange interaction energy. This emergent scale-invariant magnetic anisotropy provides evidence for a high degree of exchange frustration that favors the formation of a spin liquid state in RuCl$_3$.

cond-mat.str-el↗

One-Component Order Parameter in URu$_2$Si$_2$ Uncovered by Resonant Ultrasound Spectroscopy and Machine Learning

The unusual correlated state that emerges in URu$_2$Si$_2$ below T$_{HO}$ = 17.5 K is known as "hidden order" because even basic characteristics of the order parameter, such as its dimensionality (whether it has one component or two), are "hidden". We use resonant ultrasound spectroscopy to measure the symmetry-resolved elastic anomalies across T$_{HO}$. We observe no anomalies in the shear elastic moduli, providing strong thermodynamic evidence for a one-component order parameter. We develop a machine learning framework that reaches this conclusion directly from the raw data, even in a crystal that is too small for traditional resonant ultrasound. Our result rules out a broad class of theories of hidden order based on two-component order parameters, and constrains the nature of the fluctuations from which unconventional superconductivity emerges at lower temperature. Our machine learning framework is a powerful new tool for classifying the ubiquitous competing orders in correlated electron systems.

cond-mat.str-el↗

A proposal for reconciling diverse experiments on the superconducting state in Sr2RuO4

A variety of precise experiments have been carried out to establish the character of the superconducting state in Sr2RuO4. Many of these appear to imply contradictory conclusions concerning the symmetries of this state. Here, we propose that these results can be reconciled if we assume that there is a near-degeneracy between a d_{x^2-y^2} (B_{1g} in group theory nomenclature) and a g_{xy(x^2-y^2)} (A_{2g}) superconducting state. From a weak-coupling perspective, such an accidental degeneracy can occur at a point at which a balance between the on-site and nearest-neighbor repulsions triggers a d-wave to g-wave transition.

cond-mat.supr-con↗

Dirac Fermions and Possible Weak Antilocalization in LaCuSb$_{2}$

Layered heavy-metal square-lattice compounds have recently emerged as potential Dirac fermion materials due to bonding within those sublattices. We report quantum transport and spectroscopic data on the layered Sb square-lattice material LaCuSb$_{2}$. Linearly dispersing band crossings, necessary to generate Dirac fermions, are experimentally observed in the electronic band structure observed using angle-resolved photoemission spectroscopy (ARPES), along with a quasi-two-dimensional Fermi surface. Weak antilocalization that arises from two-dimensional transport is observed in the magnetoresistance, as well as regions of linear dependence, both of which are indicative of topologically non-trivial effects. Measurements of the Shubnikov-de Haas (SdH) quantum oscillations show low effective mass electrons on the order of 0.065$m_{e}$, further confirming the presence of Dirac fermions in this material.

cond-mat.mtrl-sci↗

The strange metal Hall effect connects quantum criticality and superconductivity in an iron-based superconductor

Many unconventional superconductors exhibit a common set of anomalous charge transport properties that characterize them as `strange metals', which provides hope that there is single theory that describes them. However, model-independent connections between the strange metal and superconductivity have remained elusive. In this letter, we show that the Hall effect of the unconventional superconductor BaFe$_2$(As$_{1-x}$P$_x$)$_2$ contains an anomalous contribution arising from the correlations within the strange metal. This term has a distinctive dependence on magnetic field, which allows us to track its behavior across the doping-temperature phase diagram, even under the superconducting dome. These measurements demonstrate that the strange metal Hall component emanates from a quantum critical point and, in the zero temperature limit, decays in proportion to the superconducting critical temperature. This creates a clear and novel connection between quantum criticality and superconductivity, and suggests that similar connections exist in other strange metal superconductors.

cond-mat.str-el↗

A key role of correlation effects in the Lifshitz transition in Sr$_2$RuO$_4$

Uniaxial pressure applied along an Ru-Ru bond direction induces an elliptical distortion of the largest Fermi surface of Sr$_2$RuO$_4$, eventually causing a Fermi surface topological transition, also known as a Lifshitz transition, into an open Fermi surface. There are various anomalies in low-temperature properties associated with this transition, including maxima in the superconducting critical temperature and in resistivity. In the present paper, we report new measurements, employing new uniaxial stress apparatus and new measurements of the low-temperature elastic moduli, of the strain at which this Lifshitz transition occurs: a longitudinal strain $\varepsilon_{xx}$ of $(-0.44\pm0.06)\cdot10^{-2}$, which corresponds to a B$_{1g}$ strain $\varepsilon_{xx} - \varepsilon_{yy}$ of $(-0.66\pm0.09)\cdot10^{-2}$. This is considerably smaller than the strain corresponding to a Lifshitz transition in density functional theory calculations, even if the spin-orbit coupling is taken into account. Using dynamical mean-field theory we show that electronic correlations reduce the critical strain. It turns out that the orbital anisotropy of the local Coulomb interaction on the Ru site is furthermore important to bring this critical strain close to the experimental number, and thus well into the experimentally accessible range of strains.

cond-mat.str-el↗

Chiral spin-order in some purported Kitaev spin-liquid compounds

We examine recent magnetic torque measurements in two compounds, $γ$-Li$_2$IrO$_3$ and RuCl$_3$, which have been discussed as possible realizations of the Kitaev model. The analysis of the reported discontinuity in torque, as an external magnetic field is rotated across the $c-$axis in both crystals, suggests that they have a translationally-invariant chiral spin-order of the from $<{\bf S}_i. ({\bf S}_j ~\times ~ {\bf S}_k)> \ne 0$ in the ground state and persisting over a very wide range of magnetic field and temperature. An extra-ordinary $|B|B^2$ dependence of the torque for small fields, beside the usual $B^2$ part, is predicted due to the chiral spin-order, and found to be consistent with experiments upon further analysis of the data. Other experiments such as inelastic scattering and thermal Hall effect and several questions raised by the discovery of chiral spin-order, including its topological consequences are discussed.

cond-mat.str-el↗

Spatially modulated heavy-fermion superconductivity in CeIrIn5

The ability to spatially modulate the electronic properties of solids has led to landmark discoveries in condensed matter physics as well as new electronic applications. Although crystals of strongly correlated metals exhibit a diverse set of electronic ground states, few approaches to spatially modulating their properties exist. Here we demonstrate spatial control over the superconducting state in mesoscale samples of the canonical heavy-fermion superconductor CeIrIn5. We use a focused ion beam (FIB) to pattern crystals on the microscale, which tailors the strain induced by differential thermal contraction into specific areas of the device. The resulting non-uniform strain fields induce complex patterns of superconductivity due to the strong dependence of the transition temperature on the strength and direction of strain. Electrical transport and magnetic imaging of devices with different geometry show that the obtained spatial modulation of superconductivity agrees with predictions based on finite element simulations. These results present a generic approach to manipulating electronic order on micrometer length scales in strongly correlated matter.

cond-mat.supr-con↗

Scale-invariant magnetoresistance in a cuprate superconductor

The anomalous metallic state in high-temperature superconducting cuprates is masked by the onset of superconductivity near a quantum critical point. Use of high magnetic fields to suppress superconductivity has enabled a detailed study of the ground state in these systems. Yet, the direct effect of strong magnetic fields on the metallic behavior at low temperatures is poorly understood, especially near critical doping, $x=0.19$. Here we report a high-field magnetoresistance study of thin films of \LSCO cuprates in close vicinity to critical doping, $0.161\leq x\leq0.190$. We find that the metallic state exposed by suppressing superconductivity is characterized by a magnetoresistance that is linear in magnetic field up to the highest measured fields of $80$T. The slope of the linear-in-field resistivity is temperature-independent at very high fields. It mirrors the magnitude and doping evolution of the linear-in-temperature resistivity that has been ascribed to Planckian dissipation near a quantum critical point. This establishes true scale-invariant conductivity as the signature of the strange metal state in the high-temperature superconducting cuprates.

cond-mat.str-el↗

Quantum limit transport and destruction of the Weyl nodes in TaAs

Weyl fermions are a new ingredient for correlated states of electronic matter. A key difficulty has been that real materials also contain non-Weyl quasiparticles, and disentangling the experimental signatures has proven challenging. We use magnetic fields up to 95 tesla to drive the Weyl semimetal TaAs far into its quantum limit (QL), where only the purely chiral 0th Landau levels (LLs) of the Weyl fermions are occupied. We find the electrical resistivity to be nearly independent of magnetic field up to 50 tesla: unusual for conventional metals but consistent with the chiral anomaly for Weyl fermions. Above 50 tesla we observe a two-order-of-magnitude increase in resistivity, indicating that a gap opens in the chiral LLs. Above 80 tesla we observe strong ultrasonic attenuation below 2 kelvin, suggesting a mesoscopically-textured state of matter. These results point the way to inducing new correlated states of matter in the QL of Weyl semimetals.

cond-mat.str-el↗

Anisotropy in the Magnetoresistance Scaling of BaFe$_2$(As$_{1-x}$P$_{x}$)$_2$

Theories of the strange metal, the parent state of many high temperature superconductors, invariably involve an important role for correlations in the spin and charge degrees of freedom. The most distinctive signature of this state in the charge transport sector is a resistance that varies linearly in temperature, but this phenomenon does not clearly point to one mechanism as temperature is a scalar quantity that influences every possible mechanism for momentum relaxation. In a previous work we identified an unusual scaling relationship between magnetic field and temperature in the in-plane resistivity of the unconventional superconductor BaFe$_2$(As$_{1-x}$P$_{x}$)$_2$, providing an opportunity to use the vector nature of the magnetic field to acquire additional clues about the mechanisms responsible for scattering in the strange metal state. Here we extend this work by investigating other components of the conductivity tensor under different orientations of the magnetic field. We find that the scaling phenomenon involves only the out-of-plane component of the magnetic field and is, strikingly, independent of the direction of the applied current. This suggests that the origin of the strange magnetotransport is in the action of the magnetic field on the correlated behavior of spin and charge degrees of freedom, rather than on the simple cyclotron motion of individual quasiparticles.

cond-mat.str-el↗

Resonant torsion magnetometry in anisotropic quantum materials

Unusual behavior of quantum materials commonly arises from their effective low-dimensional physics, which reflects the underlying anisotropy in the spin and charge degrees of freedom. Torque magnetometry is a highly sensitive technique to directly quantify the anisotropy in quantum materials, such as the layered high-T$_c$ superconductors, anisotropic quantum spin-liquids, and the surface states of topological insulators. Here we introduce the magnetotropic coefficient $k=\partial^2 F/\partial θ^2$, the second derivative of the free energy F with respect to the angle $θ$ between the sample and the applied magnetic field, and report a simple and effective method to experimentally detect it. A sub-$μ$g crystallite is placed at the tip of a commercially available atomic force microscopy cantilever, and we show that $k$ can be quantitatively inferred from a shift in the resonant frequency under magnetic field. While related to the magnetic torque $τ=\partial F/\partial θ$, $k$ takes the role of torque susceptibility, and thus provides distinct insights into anisotropic materials akin to the difference between magnetization and magnetic susceptibility. The thermodynamic coefficient $k$ is discontinuous at second-order phase transitions and subject to Ehrenfest relations with the specific heat and magnetic susceptibility. We apply this simple yet quantitative method on the exemplary cases of the Weyl-semimetal NbP and the spin-liquid candidate RuCl$_3$, yet it is broadly applicable in quantum materials research.

cond-mat.str-el↗

Uncovering Weyl Fermions in the Quantum Limit of NbP

The Fermi surface topology of a Weyl semimetal (WSM) depends strongly on the position of the chemical potential. If it resides close to the band touching points (Weyl nodes), as it does in TaAs, separate Fermi surfaces of opposite chirality emerge, leading to novel phenomena such as the chiral magnetic effect. If the chemical potential lies too far from the nodes, however, the chiral Fermi surfaces merge into a single large Fermi surface with no net chirality. This is realized in the WSM NbP, where the Weyl nodes lie far below the Fermi energy and where the transport properties in low magnetic fields show no evidence of chiral Fermi surfaces. Here we show that the behavior of NbP in high magnetic fields is nonetheless dominated by the presence of the Weyl nodes. Torque magnetometry up to 60 tesla reveals a change in the slope of $τ/B$ at the quantum limit B$^\star$ ($\approx 32\,\rm{T}$), where the chemical potential enters the $n=0$ Landau level. Numerical simulations show that this behaviour results from the magnetic field pulling the chemical potential to the chiral $n=0$ Landau level belonging to the Weyl nodes. These results show that high magnetic fields can uncover topological singularities in the underlying band structure of a potential WSM, and can recover topologically non-trivial experimental properties, even when the position of the chemical potential precludes their observation in zero magnetic field.

cond-mat.str-el↗

Pseudogap temperature $T^\star$ of cuprate superconductors from the Nernst effect

We use the Nernst effect to delineate the boundary of the pseudogap phase in the temperature-doping phase diagram of cuprate superconductors. New data for the Nernst coefficient $ν(T)$ of YBa$_{2}$Cu$_{3}$O$_{y}$ (YBCO), La$_{1.8-x}$Eu$_{0.2}$Sr$_x$CuO$_4$ (Eu-LSCO) and La$_{1.6-x}$Nd$_{0.4}$Sr$_x$CuO$_4$ (Nd-LSCO) are presented and compared with previous data including La$_{2-x}$Sr$_x$CuO$_4$ (LSCO). The temperature $T_ν$ at which $ν/T$ deviates from its high-temperature behaviour is found to coincide with the temperature at which the resistivity deviates from its linear-$T$ dependence, which we take as the definition of the pseudogap temperature $T^\star$- in agreement with gap opening detected in ARPES data. We track $T^\star$ as a function of doping and find that it decreases linearly vs $p$ in all four materials, having the same value in the three LSCO-based cuprates, irrespective of their different crystal structures. At low $p$, $T^\star$ is higher than the onset temperature of the various orders observed in underdoped cuprates, suggesting that these orders are secondary instabilities of the pseudogap phase. A linear extrapolation of $T^\star(p)$ to $p=0$ yields $T^\star(p\to 0)\simeq T_N(0)$, the Néel temperature for the onset of antiferromagnetic order at $p=0$, suggesting that there is a link between pseudogap and antiferromagnetism. With increasing $p$, $T^\star(p)$ extrapolates linearly to zero at $p\simeq p_{\rm c2}$, the critical doping below which superconductivity emerges at high doping, suggesting that the conditions which favour pseudogap formation also favour pairing. We also use the Nernst effect to investigate how far superconducting fluctuations extend above $T_{\rm c}$, as a function of doping, and find that a narrow fluctuation regime tracks $T_{\rm c}$, and not $T^\star$. This confirms that the pseudogap phase is not a form of precursor superconductivity.

cond-mat.supr-con↗

Electronic in-plane symmetry breaking at field-tuned quantum criticality in CeRhIn5

Electronic nematics are exotic states of matter where electronic interactions break a rotational symmetry of the underlying lattice, in analogy to the directional alignment without translational order in nematic liquid crystals. Intriguingly such phases appear in the copper- and iron-based superconductors, and their role in establishing high-temperature superconductivity remains an open question. Nematicity may take an active part, cooperating or competing with superconductivity, or may appear accidentally in such systems. Here we present experimental evidence for a phase of nematic character in the heavy fermion superconductor CeRhIn5. We observe a field-induced breaking of the electronic tetragonal symmetry of in the vicinity of an antiferromagnetic (AFM) quantum phase transition at Hc~50T. This phase appears in out-of-plane fields of H*~28T and is characterized by substantial in-plane resistivity anisotropy. The anisotropy can be aligned by a small in-plane field component, with no apparent connection to the underlying crystal structure. Furthermore no anomalies are observed in the magnetic torque, suggesting the absence of metamagnetic transitions in this field range. These observations are indicative of an electronic nematic character of the high field state in CeRhIn5. The appearance of nematic behavior in a phenotypical heavy fermion superconductor highlights the interrelation of nematicity and unconventional superconductivity, suggesting nematicity to be a commonality in such materials.

cond-mat.str-el↗