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B. J. Verhaar

Publications and source records attributed to B. J. Verhaar.

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Stability of rubidium molecules in the lowest triplet state

Experiments involving ultracold molecules require sufficiently long lifetimes, which can be very short for excited rovibrational states in the molecular potentials. For alkali atoms such as rubidium, a lowest rovibrational molecular state can both be found in the electronic singlet and triplet configurations. The molecular singlet ground state is absolutely stable. However, the lowest triplet state can decay to a deeper bound singlet molecule due to a radiative decay mechanism that involves the interatomic spin-orbit interaction. We investigate this mechanism, and find the lifetime of rubidium molecules in the lowest triplet rovibrational state to be about 21 minutes.

cond-mat.quant-gas

Predicting scattering properties of ultracold atoms: adiabatic accumulated phase method and mass scaling

Ultracold atoms are increasingly used for high precision experiments that can be utilized to extract accurate scattering properties. This calls for a stronger need to improve on the accuracy of interatomic potentials, and in particular the usually rather inaccurate inner-range potentials. A boundary condition for this inner range can be conveniently given via the accumulated phase method. However, in this approach one should satisfy two conditions, which are in principle conflicting, and the validity of these approximations comes under stress when higher precision is required. We show that a better compromise between the two is possible by allowing for an adiabatic change of the hyperfine mixing of singlet and triplet states for interatomic distances smaller than the separation radius. A mass scaling approach to relate accumulated phase parameters in a combined analysis of isotopically related atom pairs is described in detail and its accuracy is estimated, taking into account both Born-Oppenheimer and WKB breakdown. We demonstrate how numbers of singlet and triplet bound states follow from the mass scaling.

cond-mat.other

Feshbach resonances with large background scattering length: interplay with open-channel resonances

Feshbach resonances are commonly described by a single-resonance Feshbach model, and open-channel resonances are not taken into account explicitly. However, an open-channel resonance near threshold limits the range of validity of this model. Such a situation exists when the background scattering length is much larger than the range of the interatomic potential. The open-channel resonance introduces strong threshold effects not included in the single-resonance description. We derive an easy-to-use analytical model that takes into account both the Feshbach resonance and the open-channel resonance. We apply our model to $^{85}$Rb, which has a large background scattering length, and show that the agreement with coupled-channels calculations is excellent. The model can be readily applied to other atomic systems with a large background scattering length, such as $^6$Li and $^{133}$Cs. Our approach provides full insight into the underlying physics of the interplay between open-channel (or potential) resonances and Feshbach resonances.

cond-mat.other

Metastable neon collisions: anisotropy and scattering length

In this paper we investigate the effective scattering length $a$ of spin-polarized Ne*. Due to its anisotropic electrostatic interaction, its scattering length is determined by five interaction potentials instead of one, even in the spin-polarized case, a unique property among the Bose condensed species and candidates. Because the interaction potentials of Ne* are not known accurately enough to predict the value of the scattering length, we investigate the behavior of $a$ as a function of the five phase integrals corresponding to the five interaction potentials. We find that the scattering length has five resonances instead of only one and cannot be described by a simple gas-kinetic approach or the DIS approximation. However, the probability for finding a positive or large value of the scattering length is not enhanced compared to the single potential case. The complex behavior of $a$ is studied by comparing a quantum mechanical five-channel numerical calculation to simpler two-channel models. We find that the induced dipole-dipole interaction is responsible for coupling between the different |Ω> states, resulting in an inhomogeneous shift of the resonance positions and widths in the quantum mechanical calculation as compared to the DIS approach. The dependence of the resonance positions and widths on the input potentials turns out to be rather straightforward. The existence of two bosonic isotopes of Ne* enables us to choose the isotope with the most favorable scattering length for efficient evaporative cooling towards the Bose-Einstein Condensation transition, greatly enhancing the feasibility to reach this transition.

physics.atom-ph

Radio-Frequency Spectroscopy of Ultracold Fermions

Radio-frequency techniques were used to study ultracold fermions. We observed the absence of mean-field "clock" shifts, the dominant source of systematic error in current atomic clocks based on bosonic atoms. This is a direct consequence of fermionic antisymmetry. Resonance shifts proportional to interaction strengths were observed in a three-level system. However, in the strongly interacting regime, these shifts became very small, reflecting the quantum unitarity limit and many-body effects. This insight into an interacting Fermi gas is relevant for the quest to observe superfluidity in this system.

cond-mat.soft

Feshbach resonances in rubidium 87: Precision measurement and analysis

More than 40 Feshbach resonances in rubidium 87 are observed in the magnetic field range between 0.5 and 1260 G for various spin mixtures in the lower hyperfine ground state. The Feshbach resonances are observed by monitoring the atom loss, and their positions are determined with an accuracy of 30 mG. In a detailed analysis, the resonances are identified and an improved set of model parameters for the rubidium interatomic potential is deduced. The elastic width of the broadest resonance at 1007 G is predicted to be significantly larger than the magnetic field resolution of the apparatus. This demonstrates the potential for applications based on tuning the scattering length.

cond-mat.stat-mech

Inter-isotope determination of ultracold rubidium interactions from three high-precision experiments

Combining the measured binding energies of four of the most weakly bound rovibrational levels of the $^{87}$Rb$_2$ molecule with the results of two other recent high-precision rubidium experiments, we obtain exceptionally strong constraints on the atomic interaction parameters in a highly model independent analysis. The comparison of $^{85}$Rb and $^{87}$Rb data, where the two isotopes are related by a mass scaling procedure, plays a crucial role. Using the consistent picture of the interactions that thus arises we are led to predictions for scattering lengths, clock shifts, Feshbach resonance fields and widths with an unprecedented level of accuracy. To demonstrate this, we predict two Feshbach resonances in mixed-spin scattering channels at easily accessible magnetic field strengths, which we expect to play a role in the damping of coherent spin oscillations.

cond-mat.soft

Limit on suppression of ionization in metastable neon traps due to long-range anisotropy

This paper investigates the possibility of suppressing the ionization rate in a magnetostatic trap of metastable neon atoms by spin-polarizing the atoms. Suppression of the ionization is critical for the possibility of reaching Bose-Einstein condensation with such atoms. We estimate the relevant long-range interactions for the system, consisting of electric quadrupole-quadrupole and dipole-induced dipole terms, and develop short-range potentials based on the Na_2 singlet and triplet potentials. The auto-ionization widths of the system are also calculated. With these ingredients we calculate the ionization rate for spin-polarized and for spin-isotropic samples, caused by anisotropy of the long-range interactions. We find that spin-polarization may allow for four orders of magnitude suppression of the ionization rate for Ne. The results depend sensitively on a precise knowledge of the interaction potentials, however, pointing out the need for experimental input. The same model gives a suppression ratio close to unity for metastable xenon in accordance with experimental results, due to a much increased anisotropy in this case.

physics.atom-ph