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B. M. Reinhard

Publications and source records attributed to B. M. Reinhard.

2 recordsLinked to original sources

Dominant chiral optical forces in vicinity of optical nanofibers

Transverse spin angular momentum (SAM) of light and associated transverse chiral optical forces have received tremendous attention recently as the latter may lead to an optical separation of chiral biomolecules. In this context, the relative magnitude of chiral and non-chiral forces represents a challenge for the implementation of chiral separation schemes. In this work we demonstrate that, by spatially separating the maxima of transverse spin density from the gradient of field intensity, it is possible to dominate chiral-specific components of the force over non-chiral ones. To that end, we study optical nanofibers and nanowires as a candidate for such scheme and demonstrate that in their vicinity, chiral optical forces can emerge that are stronger than gradient and scattering forces. This finding may be of significance in the design of improved optical separation schemes for chiral biomolecules.

physics.optics

Enhanced Electromagnetic Chirality by Locally Excited Surface Plasmon Polaritons

The possibility to enhance chiral light-matter interactions through plasmonic nanostructures provides entirely new opportunities for greatly improving the detection limits of chiroptical spectroscopies down to the single molecule level. The most pronounced of these chiral interactions occur in the ultraviolet (UV) range of the electromagnetic spectrum, which is difficult to access with conventional localized plasmon resonance based sensors. Although Surface Plasmon Polaritons (SPPs) on noble metal films can sustain resonances in the desired spectral range, their transverse magnetic nature has been an obstacle for enhancing chiroptical effects. Here we demonstrate, both analytically and numerically, that SPPs excited by near-field sources can exhibit rich and non-trivial chiral characteristics. In particular, we show that the excitation of SPPs by a chiral source not only results in a locally enhanced optical chirality but also achieves manifold enhancement of net optical chirality. Our finding that SPPs facilitate a plasmonic enhancement of optical chirality in the UV part of the spectrum is of great interest in chiral bio-sensing.

physics.optics