arXiv subjects

B. M. Sparkes

Publications and source records attributed to B. M. Sparkes.

16 recordsLinked to original sources

arXiv2025

Demonstration of a Mobile Optical Clock Ensemble at Sea

Atomic clocks are at the leading edge of accuracy and precision and are essential for synchronization of distributed critical infrastructure, position, navigation and timing, and scientific applications. There has been a breakthrough in the performance of atomic clocks with the shift from microwave to optical frequency transitions. However, this performance increase has come at the cost of size, complexity and fragility, which has confined optical clocks to laboratories. Here we report on a recent international collaboration where three emerging optical clocks, each based on different operating principles, were trialled at sea. Over weeks of unsupervised naval operation, these clocks demonstrated exceptional reliability and provided frequency stability outputs in optical, microwave and radio-frequency domains. The performance of all three devices was orders of magnitude superior to existing best-in-class commercial solutions over short and medium timescales, marking a significant step toward deploying optical clocks in real-world environments.

physics.atom-ph↗

arXiv2023

Wavefront Curvature in Optical Atomic Beam Clocks

Atomic clocks provide a reproducible basis for our understanding of time and frequency. Recent demonstrations of compact optical clocks, employing thermal atomic beams, have achieved short-term fractional frequency instabilities in the $10^{-16}$, competitive with the best international frequency standards available. However, a serious challenge inherent in compact clocks is the necessarily smaller optical beams, which results in rapid variation in interrogating wavefronts. This can cause inhomogeneous excitation of the thermal beam leading to long term drifts in the output frequency. Here we develop a model for Ramsey-Bordé interferometery using optical fields with curved wavefronts and simulate the $^{40}$Ca beam clock experiment described in [Olson et al., Phys. Rev. Lett. 123, 073202 (2019)]. Olson et al.'s results had shown surprising and unexplained behaviour in the response of the atoms in the interrogation. Our model predicts signals consistent with experimental data and can account for the significant sensitivity to laser geometry that was reported. We find the signal-to-noise ratio is maximised when the laser is uncollimated at the interrogation zones to minimise inhomogeneity, and also identify an optimal waist size determined by both laser inhomogeneity and the velocity distribution of the atomic beam. We investigate the shifts and stability of the clock frequency, showing that the Gouy phase is the primary source of frequency variations arising from laser geometry.

quant-ph↗

arXiv2016

Stimulated Raman Adiabatic Passage for Improved Performance of a Cold Atom Electron and Ion Source

We implement high-efficiency coherent excitation to a Rydberg state using stimulated Raman adiabatic passage in a cold atom electron and ion source. We achieve an efficiency of 60% averaged over the laser excitation volume with a peak efficiency of 82%, a 1.6 times improvement relative to incoherent pulsed-laser excitation. Using pulsed electric field ionization of the Rydberg atoms we create electron bunches with durations of 250 ps. High-efficiency excitation will increase source brightness, crucial for ultrafast electron diffraction experiments, and coherent excitation to high-lying Rydberg states could allow for the reduction of internal bunch heating and the creation of a high-speed single ion source.

physics.atom-ph↗

arXiv2015

Unconditional Room Temperature Quantum Memory

Just as classical information systems require buffers and memory, the same is true for quantum information systems. The potential that optical quantum information processing holds for revolutionising computation and communication is therefore driving significant research into developing optical quantum memory. A practical optical quantum memory must be able to store and recall quantum states on demand with high efficiency and low noise. Ideally, the platform for the memory would also be simple and inexpensive. Here, we present a complete tomographic reconstruction of quantum states that have been stored in the ground states of rubidium in a vapour cell operating at around 80$^o$C. Without conditional measurements, we show recall fidelity up to 98% for coherent pulses containing around one photon. In order to unambiguously verify that our memory beats the quantum no-cloning limit we employ state independent verification using conditional variance and signal transfer coefficients.

quant-ph↗

arXiv2014

Electromagnetically induced transparency and four-wave mixing in a cold atomic ensemble with large optical depth

We report on the delay of optical pulses using electromagnetically induced transparency in an ensemble of cold atoms with an optical depth exceeding 500. To identify the regimes in which four-wave mixing impacts on EIT behaviour, we conduct the experiment in both rubidium 85 and rubidium 87. Comparison with theory shows excellent agreement in both isotopes. In rubidium 87, negligible four-wave mixing was observed and we obtained one pulse-width of delay with 50% efficiency. In rubidium 85, four-wave-mixing contributes to the output. In this regime we achieve a delay-bandwidth product of 3.7 at 50% efficiency, allowing temporally multimode delay, which we demonstrate by compressing two pulses into the memory medium.

quant-ph↗

arXiv2013

Time- and frequency-domain polariton interference

We present experimental observations of interference between an atomic spin coherence and an optical field in a Λ-type gradient echo memory. The interference is mediated by a strong classical field that couples a weak probe field to the atomic coherence through a resonant Raman transition. Interference can be observed between a prepared spin coherence and another propagating optical field, or between multiple Λ transitions driving a single spin coherence. In principle, the interference in each scheme can yield a near unity visibility.

quant-ph↗

arXiv2013

Gradient echo memory in an ultra-high optical depth cold atomic ensemble

Quantum memories are an integral component of quantum repeaters - devices that will allow the extension of quantum key distribution to communication ranges beyond that permissible by passive transmission. A quantum memory for this application needs to be highly efficient and have coherence times approaching a millisecond. Here we report on work towards this goal, with the development of a $^{87}$Rb magneto-optical trap with a peak optical depth of 1000 for the D2 $F=2 \rightarrow F'=3$ transition using spatial and temporal dark spots. With this purpose-built cold atomic ensemble to implement the gradient echo memory (GEM) scheme. Our data shows a memory efficiency of $80\pm 2$% and coherence times up to 195 $μ$s, which is a factor of four greater than previous GEM experiments implemented in warm vapour cells.

quant-ph↗

arXiv2012

Storage and Manipulation of Light Using a Raman Gradient Echo Process

The Gradient Echo Memory (GEM) scheme has potential to be a suitable protocol for storage and retrieval of optical quantum information. In this paper, we review the properties of the $Λ$-GEM method that stores information in the ground states of three-level atomic ensembles via Raman coupling. The scheme is versatile in that it can store and re-sequence multiple pulses of light. To date, this scheme has been implemented using warm rubidium gas cells. There are different phenomena that can influence the performance of these atomic systems. We investigate the impact of atomic motion and four-wave mixing and present experiments that show how parasitic four-wave mixing can be mitigated. We also use the memory to demonstrate preservation of pulse shape and the backward retrieval of pulses.

quant-ph↗

arXiv2012

Precision spectral manipulation: a demonstration using a coherent optical memory

The ability to coherently spectrally manipulate quantum information has the potential to improve qubit rates across quantum channels and find applications in optical quantum computing. In this paper we present experiments that use a multi-element solenoid combined with the three-level gradient echo memory scheme to perform precision spectral manipulation of optical pulses. These operations include bandwidth and frequency manipulation, spectral filtering of separate frequency components, as well as time-delayed interference between pulses with both the same, and different, frequencies. These operations have potential uses in quantum information applications.

quant-ph↗

arXiv2011

Memory-Enhanced Noiseless Cross Phase Modulation

Using a gradient echo memory, we experimentally demonstrate cross phase modulation (XPM) between two optical pulses; one stored and one freely propagating through the memory medium. We explain how this idea can be extended to enable substantial nonlinear interaction between two single photons that are both stored in the memory. We present semi-classical and quantum simulations along with a proposed experimental scheme to demonstrate the feasibility of achieving large XPM at single photon level.

quant-ph↗

arXiv2011

Photon number discrimination without a photon counter and its application to reconstructing non-Gaussian states

The non-linearity of a conditional photon-counting measurement can be used to `de-Gaussify' a Gaussian state of light. Here we present and experimentally demonstrate a technique for photon number resolution using only homodyne detection. We then apply this technique to inform a conditional measurement; unambiguously reconstructing the statistics of the non-Gaussian one and two photon subtracted squeezed vacuum states. Although our photon number measurement relies on ensemble averages and cannot be used to prepare non-Gaussian states of light, its high efficiency, photon number resolving capabilities, and compatibility with the telecommunications band make it suitable for quantum information tasks relying on the outcomes of mean values.

quant-ph↗

arXiv2011

A Scalable, Self-Analyzing Digital Locking System for use on Quantum Optics Experiments

Digital control of optics experiments has many advantages over analog control systems, specifically in terms of scalability, cost, flexibility, and the integration of system information into one location. We present a digital control system, freely available for download online, specifically designed for quantum optics experiments that allows for automatic and sequential re-locking of optical components. We show how the inbuilt locking analysis tools, including a white-noise network analyzer, can be used to help optimize individual locks, and verify the long term stability of the digital system. Finally, we present an example of the benefits of digital locking for quantum optics by applying the code to a specific experiment used to characterize optical Schrodinger cat states.

physics.ins-det↗

arXiv2010

High efficiency coherent optical memory with warm rubidium vapour

By harnessing aspects of quantum mechanics, communication and information processing could be radically transformed. Promising forms of quantum information technology include optical quantum cryptographic systems and computing using photons for quantum logic operations. As with current information processing systems, some form of memory will be required. Quantum repeaters, which are required for long distance quantum key distribution, require optical memory as do deterministic logic gates for optical quantum computing. In this paper we present results from a coherent optical memory based on warm rubidium vapour and show 87% efficient recall of light pulses, the highest efficiency measured to date for any coherent optical memory. We also show storage recall of up to 20 pulses from our system. These results show that simple warm atomic vapour systems have clear potential as a platform for quantum memory.

quant-ph↗

arXiv2010

An AC Stark Gradient Echo Memory in Cold Atoms

The burgeoning fields of quantum computing and quantum key distribution have created a demand for a quantum memory. The gradient echo memory scheme is a quantum memory candidate for light storage that can boast efficiencies approaching unity, as well as the flexibility to work with either two or three level atoms. The key to this scheme is the frequency gradient that is placed across the memory. Currently the three level implementation uses a Zeeman gradient and warm atoms. In this paper we model a new gradient creation mechanism - the ac Stark effect - to provide an improvement in the flexibility of gradient creation and field switching times. We propose this scheme in concert with a move to cold atoms (~1 mK). These temperatures would increase the storage times possible, and the small ensemble volumes would enable large ac Stark shifts with reasonable laser power. We find that memory bandwidths on the order of MHz can be produced with experimentally achievable laser powers and trapping volumes, with high precision in gradient creation and switching times on the order of nanoseconds possible. By looking at the different decoherence mechanisms present in this system we determine that coherence times on the order of 10s of milliseconds are possible, as are delay-bandwidth products of approximately 50 and efficiencies over 90%.

quant-ph↗

arXiv2010

Precision spectral manipulation of optical pulses using a coherent photon echo memory

Photon echo schemes are excellent candidates for high efficiency coherent optical memory. They are capable of high-bandwidth multi-pulse storage, pulse resequencing and have been shown theoretically to be compatible with quantum information applications. One particular photon echo scheme is the gradient echo memory (GEM). In this system, an atomic frequency gradient is induced in the direction of light propagation leading to a Fourier decomposition of the optical spectrum along the length of the storage medium. This Fourier encoding allows precision spectral manipulation of the stored light. In this letter, we show frequency shifting, spectral compression, spectral splitting, and fine dispersion control of optical pulses using GEM.

quant-ph↗

arXiv2008

Photon echoes generated by reversing magnetic field gradients in a rubidium vapour

We propose a photon echo quantum memory scheme using detuned Raman coupling to long lived ground states. In contrast to previous 3-level schemes based on controlled reversible inhomogeneous broadening that use sequences of $π$-pulses, the scheme does not require accurate control of the coupling dynamics to the ground states. We present a proof of principle experimental realization of our proposal using rubidium atoms in a warm vapour cell. The Raman resonance line is broadened using a magnetic field that varies linearly along the direction of light propagation. Inverting the magnetic field gradient rephases the atomic dipoles and re-emits the light pulse in the forward direction.

quant-ph↗