arXiv subjects

B. P. Kay

Publications and source records attributed to B. P. Kay.

At least 19 recordsLinked to original sources

arXiv2026

Observation of a dominant $\boldsymbol{0f_{7/2}}$ neutron configuration in the $\boldsymbol{^{32}}$Si $\boldsymbol{J^{\pi}=5^-}$ isomeric state

An yrast, $J^{\pi}=5^-$, spin-trap isomer has been previously identified in $^{32}$Si. The isomeric state decays predominantly via a hindered $E3$ transition [B($E3$) = 0.0841(10)~W.u.], bypassing a nearby $E2$ decay path to the first excited $3^-$ level. The single-neutron aspects of these negative parity levels were investigated via the $^{31}$Si$(d$,$p)^{32}$Si reaction at 9.6~MeV/$u$ using HELIOS and the ATLAS in-flight facility. The $5^-$ state appears as a dominant $\ell=3$ transfer with a relatively large spectroscopic factor, confirming its single-particle $\nu0f_{7/2}$ character. The yrast $3^-$ level had a reduced $\ell=3$ spectroscopic factor of $\approx$ 0.44 compared to that of the $5^-_1$ level. This is similar to the situation observed in nearby $^{34}$S which by contrast has a measured B($E2, 5^-\rightarrow 3^-$) transition strength closer to 1~W.u.. It has been concluded that the hinderance of the $5^-_1\rightarrow 3^-_1$ transition in $^{32}$Si is not primarily due to the differing overlaps in the neutron structure. Instead, the lack of participation by both the protons and the neutrons in the transition is proposed as the transition-strength reduction mechanism.

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arXiv2026

Spectroscopy of $^{11}$Be from the $^{10}$Be($d,p$) reaction measured in inverse kinematics by the AT-TPC in SOLARIS

The spectroscopy of $^{11}$Be is explored using the $^{10}$Be$(d,p)$$^{11}$Be transfer reaction performed in inverse kinematics at $9.6\,\MeV/u$ using the Active Target Time Projection Chamber (AT-TPC) inside the SOLARIS solenoid. This experiment is the first attempt at coupling the AT-TPC with SOLARIS to perform a high luminosity transfer reaction measurement without compromising excitation energy and scattering angle resolutions. The angular momentum transfer for states up to $3.40\,\MeV$ are determined from distorted-wave Born approximation analysis of the measured angular distributions, from which the corresponding spectroscopic factors are deduced. These factors are compared with those from various shell model interactions, and those for the $3.40\,\MeV$ state are consistent with a positive parity assignment. Recent \textit{ab initio} no-core configuration interaction (NCCI) calculations with various nucleon-nucleon interactions are presented for the low-lying positive parity states of $^{11}$Be. The excitation energies produced using the Daejeon16 interaction are in good agreement with those found from both this experiment and the literature, thus supporting a positive parity assignment. The $3.40\,\MeV$ state, if assigned a tentative $J^\pi=3/2^+$, would then correspond to the second excited state of the $K^P=1/2^+$ one-neutron halo ground state rotational band also predicted from such NCCI calculations.

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arXiv2025

Valence $1s-0d$ proton vacancy of the $^{32}$Si ground state

The $^{32}$Si($^3$He,$d$)$^{33}$P reaction was studied in inverse kinematics at 6.3~MeV/$u$. States in $^{33}$P corresponding to the proton $1s-0d$ single-particle orbitals were identified up to $\sim$4.5 MeV in excitation energy. The ($^{3}$He,$d$) spectroscopic factors were determined from Distorted Wave Born Approximation calculations. When combined with complementary neutron-adding data, the $1s-0d$ proton vacancies in the $^{32}$Si ground state were extracted. In conjunction with a re-analysis of data from previous single-particle measurements, the trends in proton and neutron vacancy were explored across the $^{28,30,32,34}$Si isotopes. Both proton and neutron vacancy data show gradual changes in their occupancies. The proton $1s_{1/2}$ orbitals in $^{32}$Si and $^{34}$Si are both consistent with being empty. The ground-state nucleon distributions are described by shell-model calculations constrained to the $1s-0d$ model space.

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arXiv2025

Quenching of single-particle strength inferred from nucleon-removal transfer reactions on $^{15}$C

The difference in the proton and neutron separation energies ($\Delta S$) of the weakly bound $^{15}$C ground state is -19.86 MeV, an extreme value. Data from intermediate-energy heavy-ion induced (HI-induced) knockout reactions on nuclei spanning $-20\lesssim\Delta S\lesssim+20$ MeV, suggest that the degree to which single-particle strength is quenched, $R\mathrm{_{s}}$, has a negative correlation with $\Delta S$, decreasing from unity around $-20$~MeV to around 0.2 at $+20$~MeV. For the $^{15}$C ground state ($R_s=0.96(4)$ in HI-induced knockout), contrasting results have recently been obtained via the neutron-adding transfer reaction, which reveal a value of $R_s=0.64(15)$, similar to the value observed at modest $\Delta S$ and more extreme values of $\Delta S$ with reaction probes other than HI knockout. In order to explore the any potential differences between $adding$ and $removing$ processes in transfer reactions at extreme $\Delta S$, single-neutron removal transfer reactions on $^{15}$C were performed at 7.1MeV/u in inverse kinematics. The removal of a valence neutron in 2$s_{1/2}$ orbit using both ($p$,$d$) and ($d$,$t$) reactions shows consistent quenching factors and agrees with those from the neutron-adding reaction. The present results, which can be compared with neutron knockout reaction, suggest that correlations, represented by the quenching factor, show limited dependence on neutron-proton asymmetry under the most extreme asymmetry conditions so far achieved in transfer reactions.

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arXiv2025

Near-threshold dipole strength in {^{10}}Be with isoscalar character

Isoscalar dipole transitions are a distinctive fingerprint of cluster structures. A {1^-} resonance at 7.27(10) MeV, located just below the {\alpha}-emission threshold, has been observed in the deuteron inelastic scattering reactions off 10Be. The deformation lengths of the excited states in 10Be below 9 MeV have been inferred from the differential cross sections using coupled channel calculations. This observed {1^-} resonance has isoscalar characteristics and exhausts approximately 5{\%}-15{\%} of the isoscalar dipole energy-weighted sum rule, providing evidence for pronounced {\alpha} cluster structure in 10Be. The Gamow coupled channel approach supports this interpretation and suggests the near-threshold effect might be playing an important role in this excitation energy domain. The {\alpha}+{\alpha}+n+n four-body calculation reproduces the observed enhanced dipole strength, implying that the four-body cluster structure is essential to describe the {1^-} states in 10Be.

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arXiv2024

Meaurement of spin vs. TKE of $^{144}$Ba produced in spontaneous fission of $^{252}$Cf

We measure the average spin of $^{144}$Ba, a common fragment produced in $^{252}$Cf(sf), as a function of the total kinetic energy (TKE). We combined for the first time a twin Frisch-gridded ionization chamber with a world-class $\gamma$-ray spectrometer that was designed to measure high-multiplicity $\gamma$-ray events, Gammasphere. The chamber, loaded with a $^{252}$Cf(sf) source, provides a fission trigger, the TKE of the fragments, the approximate fragment masses, and the polar angle of the fission axis. Gammasphere provides the total $\gamma$-ray yield, fragment identification through the tagging of decay $\gamma$ rays, and the feeding of rotational bands in the fragments. We determine the dependence of the average spin of $^{144}$Ba on the fragments' TKE by correlating the fragment properties with the distribution of discrete levels that are fed. We find that the average spin only changes by about $0.5$ $\hbar$ across the TKE range of 158-203 MeV. The virtual independence of the spin on TKE suggests that spin is not solely generated through the statistical excitation of rotational modes, and more complex mechanisms are required.

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arXiv2024

Evolution of the nuclear spin-orbit splitting explored via the $^{32}$Si($d$,$p$)$^{33}$Si reaction using SOLARIS

The spin-orbit splitting between neutron 1$p$ orbitals at $^{33}$Si has been deduced using the single-neutron-adding ($d$,$p$) reaction in inverse kinematics with a beam of $^{32}$Si, a long-lived radioisotope. Reaction products were analyzed by the newly implemented SOLARIS spectrometer at the reaccelerated-beam facility at the National Superconducting Cyclotron Laboratory. The measurements show reasonable agreement with shell-model calculations that incorporate modern cross-shell interactions, but they contradict the prediction of proton density depletion based on relativistic mean-field theory. The evolution of the neutron 1$p$-shell orbitals is systematically studied using the present and existing data in the isotonic chains of $N=17$, 19, and 21. In each case, a smooth decrease in the separation of the $1p_{3/2}$-$1p_{1/2}$ orbitals is seen as the respective $p$-orbitals approach zero binding, suggesting that the finite nuclear potential strongly influences the evolution of nuclear structure in this region.

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arXiv2023

Executive Summary of the Topical Program: Nuclear Isomers in the Era of FRIB

We report on the Facility for Rare Isotope Beams (FRIB) Theory Alliance topical program "Nuclear Isomers in the Era of FRIB". We outline the many ways isomers influence and contribute to nuclear science and technology, especially in the four FRIB pillars: properties of rare isotopes, nuclear astrophysics, fundamental symmetries, and applications for the nation and society. We conclude with a resolution stating our recommendation that the nuclear physics community actively pursue isomer research. A white paper is forthcoming.

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arXiv2023

Direct Determination of Fission-Barrier Heights Using Light-Ion Transfer in Inverse Kinematics

We demonstrate a new technique for obtaining fission data for nuclei away from $β$-stability. These types of data are pertinent to the astrophysical \textit{r-}process, crucial to a complete understanding of the origin of the heavy elements, and for developing a predictive model of fission. These data are also important considerations for terrestrial applications related to power generation and safeguarding. Experimentally, such data are scarce due to the difficulties in producing the actinide targets of interest. The solenoidal-spectrometer technique, commonly used to study nucleon-transfer reactions in inverse kinematics, has been applied to the case of transfer-induced fission as a means to deduce the fission-barrier height, among other variables. The fission-barrier height of $^{239}$U has been determined via the $^{238}$U($d$,$pf$) reaction in inverse kinematics, the results of which are consistent with existing neutron-induced fission data indicating the validity of the technique.

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arXiv2023

Optical potentials for the rare-isotope beam era

We review recent progress and motivate the need for further developments in nuclear optical potentials that are widely used in the theoretical analysis of nucleon elastic scattering and reaction cross sections. In regions of the nuclear chart away from stability, which represent a frontier in nuclear science over the coming decade and which will be probed at new rare-isotope beam facilities worldwide, there is a targeted need to quantify and reduce theoretical reaction model uncertainties, especially with respect to nuclear optical potentials. We first describe the primary physics motivations for an improved description of nuclear reactions involving short-lived isotopes, focusing on its benefits for fundamental science discoveries and applications to medicine, energy, and security. We then outline the various methods in use today to build optical potentials starting from phenomenological, microscopic, and ab initio methods, highlighting in particular the strengths and weaknesses of each approach. We then discuss publicly-available tools and resources facilitating the propagation of recent progresses in the field to practitioners. Finally, we provide a set of open challenges and recommendations for the field to advance the fundamental science goals of nuclear reaction studies in the rare-isotope beam era.

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arXiv2022

Probing the quadrupole transition strength of 15C via deuteron inelastic scattering

Deuteron elastic scattering from 15C and inelastic scattering reactions to the first excited state of 15C were studied using a radioactive beam of 15C in inverse kinematics. The scattered deuterons were measured using HELIOS. The elastic scattering differential cross sections were analyzed using the optical model. A matter deformation length δd = 1.04(11) fm has been extracted from the differential cross sections of inelastic scattering to the first excited state. The ratio of neutron and proton matrix elements Mn/Mp = 3.6(4) has been determined from this quadrupole transition. Neutron effective charges and core-polarization parameters of 15C were determined and discussed. Results from ab-initio no-core configuration interaction calculations were also compared with the experimental observations. This result supports a moderate core decoupling effect of the valence neutron in 15C similarly to its isotone 17O, in line with the interpretation of other neutron-rich carbon isotopes.

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arXiv2022

Instrumentation for correlated prompt $n$-$γ$ emission studies in coincidence with fission fragments

Recent theoretical and experimental results have brought renewed interest and focus on the topic of fission fragment angular momentum. Measurements of neutrons and $γ$ rays in coincidence with fission fragments remain the most valuable tool in the exploration of fission physics. To achieve these scientific goals, we have developed a system that combines a state-of-the-art fission fragment detector and $n$-$γ$ radiation detectors. A new twin Frisch-gridded ionization chamber has been designed and constructed for use with a spontaneous fission source and an array of forty \textit{trans}-stilbene organic scintillators (FS-3) at Argonne National Laboratory. The new ionization chamber design we present in this work aims at minimizing particle attenuation in the chamber walls, and provides a compact apparatus that can be fit inside existing experimental systems. The ionization chamber is capable of measuring fission fragment masses and kinetic energies, whereas the FS-3 provides neutron and gamma-ray multiplicities and spectra. The details of both detector assembly are presented along with the first experimental results of this setup. Planned event-by-event analysis and future experiments are briefly discussed.

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arXiv2022

Study of the Isomeric State in $^{16}$N Using the $^{16}$N$^{g,m}$($d$,$^3$He) Reaction

The isomeric state of $^{16}$N was studied using the $^{16}$N$^{g,m}$($d$,$^3$He)~proton-removal reactions at \mbox{11.8~MeV/$u$} in inverse kinematics. The $^{16}$N beam, of which 24% was in the isomeric state, was produced using the ATLAS in-fight facility and delivered to the HELIOS spectrometer, which was used to analyze the $^{3}$He ions from the ($d$,$^{3}$He) reactions. The simultaneous measurement of reactions on both the ground and isomeric states, reduced the systematic uncertainties from the experiment and in the analysis. A direct and reliable comparison of the relative spectroscopic factors was made based on a Distorted-Wave Born Approximation approach. The experimental results suggest that the isomeric state of $^{16}$N is an excited neutron-halo state. The results can be understood through calculations using a Woods-Saxon potential model, which captures the effects of weak-binding.

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arXiv2022

Quenching of Single-Particle Strength in A=15 Nuclei

Absolute cross sections for the addition of $s$- and $d$-wave neutrons to $^{14}$C and $^{14}$N have been determined simultaneously via the ($d$,$p$) reaction at 10 MeV/u. The difference between the neutron and proton separation energies, $ΔS$, is around $-20$ MeV for the $^{14}$C$+$$n$ system and $+8$ MeV for $^{14}$N$+$$n$. The population of the $1s_{1/2}$ and $0d_{5/2}$ orbitals for both systems is reduced by a factor of approximately 0.5 compared to the independent single-particle model, or about 0.6 when compared to the shell model. This finding strongly contrasts with results deduced from intermediate-energy knockout reactions between similar nuclei on targets of $^{9}$Be and $^{12}$C. The simultaneous technique used removes many systematic uncertainties.

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arXiv2022

Evidence of a near-threshold resonance in $^{11}$B relevant to the $β$-delayed proton emission of $^{11}$Be

A narrow near-threshold proton-emitting resonance (Ex = 11.4 MeV, J$^π$ = 1/2$^{+}$ and $Γ_{p}$ = 4.4 keV) was directly observed in $^{11}$B via proton resonance scattering. This resonance was previously inferred in the $β$-delayed proton emission of the neutron halo nucleus $^{11}$Be. The good agreement between both experimental results serves as a ground to confirm the existence of such exotic decay and the particular behavior of weakly bound nuclei coupled to the continuum. $R$-matrix analysis shows a sizable partial decay width for both, proton and $α$ emission channels.

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arXiv2022

First direct measurement of the $^{13}$N($α$,$p$)$^{16}$O reaction relevant for core-collapse supernovae nucleosynthesis

Understanding the explosion mechanism of a core-collapse supernova (CCSN) is important to accurately model CCSN scenarios for different progenitor stars using model-observation comparisons. The uncertainties of various nuclear reaction rates relevant for CCSN scenarios strongly affect the accuracy of these stellar models. Out of these reactions, the $^{13}$N($α$,$p$)$^{16}$O reaction has been found to affect various stages of a CCSN at varying temperatures. This work presents the first direct measurement of the $^{13}$N($α$,$p$)$^{16}$O reaction performed using a 34.6 MeV beam of radioactive $^{13}$N ions and the active-target detector MUSIC (MUlti-Sampling Ionization Chamber) at Argonne National Laboratory. The resulting total $^{13}$N($α$,$p$)$^{16}$O reaction cross sections from this measurement in the center-of-mass energy range of 3.26 - 6.02 MeV are presented and compared with calculations using the Hauser-Feshbach formalism. Uncertainties in the reaction rate have been dramatically reduced at CCSN temperatures.

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arXiv2022

In-flight production of an isomeric beam of $^{16}$N

An in-flight beam of $^{16}$N was produced via the single-neutron adding ($d$,$p$) reaction in inverse kinematics at the recently upgraded Argonne Tandem Linear Accelerator System (ATLAS) in-flight system. The amount of the $^{16}$N beam which resided in its excited 0.120-MeV $J^π=0^-$ isomeric state (T$_{1/2}\approx5$ $μ$s) was determined to be 40(5)% at a reaction energy of 7.9(3) MeV/$u$, and 24(2)% at a reaction energy of 13.2(2) MeV/$u$. The isomer measurements took place at an experimental station $\approx30$ m downstream of the production target and utilized an Al beam-stopping foil and a HPGe Clover detector. Composite $^{16}$N beam rate determinations were made at the experimental station and the focal plane of the Argonne in-flight radioactive ion-beam separator (RAISOR) with Si $Δ$E-E telescopes. A Distorted Wave Born Approximation (DWBA) approach was coupled with the known spectroscopic information on $^{16}$N in order to estimate the relative $^{16}$N isomer yields and composite $^{16}$N beam rates. In addition to the observed reaction-energy dependence of the isomer fraction, a large sensitivity to angular acceptance of the recoils was also observed.

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arXiv2021

Single-Nucleon Energies Changing with Nucleon Number

The broad range of accumulated experimental data on the binding energies for single-particle states in nuclei is examined as a function of the constituent number of neutrons and protons and an unexpectedly simple pattern emerges. The dependence of the energies of neutron states on the number of constituent protons, or of proton states on the number of neutrons, are very similar to each other and the sign reflects the well-known strong attraction. For the same kind of nucleons changing as in the state -- energies for neutron states with neutron number changing or proton states with protons -- the dependence is at least a factor of four weaker in magnitude and slightly repulsive, except when the changing nucleons are only within the same orbit as the state. The systematics of the accumulated data are presented with a minimum of use made of model assumptions.

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