arXiv subjects

B. P. P. Mallett

Publications and source records attributed to B. P. P. Mallett.

12 recordsLinked to original sources

arXiv2022

Effective circuit modelling and experimental realization of an ultra-compact self-rectifier flux pump

This paper presents experimental and modelling results of an ultra-compact self-rectifier flux pump energizing a superconducting coil. The device fits inside a volume of 65x65x50~mm and generates up to 320~A dc through the coil and a peak output voltage up to 60~mV. We also develop and present a full electromagnetic effective circuit model of the flux pump and compare its predictions to the experimental results. We show that our model can reproduce accurately the charging of the load coil and that it reproduces the systematic dependence of the maximum load coil current on the input current waveform. The experiments and modelling together show also the importance of dc-flux offsets in the transformer core on the final achievable current through the coil. The miniaturization possible for this class of flux pump and their minimal heat-leak into the cryogenic environment from thermal conduction make them attractive for applications with demanding size, weight and power limitations. Our effective circuit model is a useful tool in the understanding, design and optimization of such flux pumps which will accelerate their progression from research devices to their application.

cond-mat.supr-con↗

arXiv2020

Muon spin rotation and infrared spectroscopy study of $Ba_{1-x}Na_{x}Fe_{2}As_{2}$

The magnetic and superconducting properties of a series of underdoped $Ba_{1-x}Na_{x}Fe_{2}As_{2}$ (BNFA) single crystals with $0.19 \leq x\leq 0.34$ has been investigated with the complementary muon-spin-rotation ($μ$SR) and infrared spectroscopy techniques. The focus has been on the different antiferromagnetic states in the underdoped regime and their competition with superconductivity, especially for the ones with a tetragonal crystal structure and a so-called double-$Q$ magnetic order. Besides the collinear state with a spatially inhomogeneous spin-charge-density wave (i-SCDW) order at $x=0.24$ and $0.26$, that was previously identified in BNFA, we obtained evidence for an orthomagnetic state with a "hedgehog"-type spin vortex crystal (SVC) structure at $x=0.32$ and $0.34$. Whereas in the former i-SCDW state the infrared spectra show no sign of a superconducting response down to the lowest measured temperature of about 10K, in the SVC state there is a strong superconducting response similar to the one at optimum doping. The magnetic order is strongly suppressed here in the superconducting state and at $x=0.34$ there is even a partial re-entrance into a paramagnetic state at $T<<T_c$.

cond-mat.supr-con↗

arXiv2019

Backfolded acoustic phonons in metal-oxide superlattices

We report the observation of low-frequency modes in the Raman spectra of thin-film superlattices of the high-temperature superconductor YBa$ _{2} $Cu$ _{3} $O$ _{7-δ} $ and various manganite perovskites. Our study shows that these modes are caused by the backfolding of acoustic phonons due to the additional periodicity introduced by the superlattice. Such modes were previously only observed for ultra-pure semiconductor superlattices. They can be used to determine the bilayer thickness of the superlattice and its speed of sound. Moreover, we use the spatial resolution of Raman microscopy to map the film thickness inhomogeneity across a sample, making these modes a useful tool to characterize thin-film superlattices.

cond-mat.supr-con↗

arXiv2018

Scaling of the Fano effect of the in-plane Fe-As phonon and the superconducting critical temperature in Ba$_{1-x}$K$_{x}$Fe$_{2}$As$_{2}$

By means of infrared spectroscopy we determine the temperature-doping phase diagram of the Fano effect for the in-plane Fe-As stretching mode in Ba$_{1-x}$K$_{x}$Fe$_{2}$As$_{2}$. The Fano parameter $1/q^2$, which is a measure of the phonon coupling to the electronic particle-hole continuum, shows a remarkable sensitivity to the magnetic/structural orderings at low temperatures. More strikingly, at elevated temperatures in the paramagnetic/tetragonal state we find a linear correlation between $1/q^2$ and the superconducting critical temperature $T_c$. Based on theoretical calculations and symmetry considerations, we identify the relevant interband transitions that are coupled to the Fe-As mode. In particular, we show that a sizable $xy$ orbital component at the Fermi level is fundamental for the Fano effect and possibly also for the superconducting pairing.

cond-mat.supr-con↗

arXiv2017

Infrared ellipsometry study of the photo-generated charge carriers at the (001) and (110) surfaces of SrTiO$_3$ crystals and the interface of corresponding LaAlO$_3$/SrTiO$_3$ heterostructures

With infrared (IR) ellipsometry and DC resistance measurements we investigated the photo-doping at the (001) and (110) surfaces of SrTiO$_3$ (STO) single crystals and at the corresponding interfaces of LaAlO$_3$/SrTiO$_3$ (LAO/STO) heterostructures. In the bare STO crystals we find that the photo-generated charge carriers, which accumulate near the (001) surface, have a similar depth profile and sheet carrier concentration as the confined electrons that were previously observed in LAO/STO (001) heterostructures. A large fraction of these photo-generated charge carriers persist at low temperature at the STO (001) surface even after the UV light has been switched off again. These persistent charge carriers seem to originate from oxygen vacancies that are trapped at the structural domain boundaries which develop below the so-called antiferrodistortive transition at T* = 105 K. This is most evident from a corresponding photo-doping study of the DC transport in STO (110) crystals for which the concentration of these domain boundaries can be modified by applying a weak uniaxial stress. The oxygen vacancies and their trapping by defects are also the source of the electrons that are confined to the interface of LAO/STO (110) heterostructures which likely do not have a polar discontinuity as in LAO/STO (001). In the former, the trapping and clustering of the oxygen vacancies also has a strong influence on the anisotropy of the charge carrier mobility. We show that this anisotropy can be readily varied and even inverted by various means, such as a gentle thermal treatment, UV irradiation, or even a weak uniaxial stress. Our experiments suggest that extended defects, which develop over long time periods (of weeks to months), can strongly influence the response of the confined charge carriers at the LAO/STO (110) interface.

cond-mat.str-el↗

arXiv2016

Possible very high transition temperatures in the infinite-layer ACuO$ _{2} $ cuprate superconductor for A={Mg, Ca, Sr, Ba}: A DFT study

We show from a bond valence sum correlation that very high superconducting $ T_{c} $ values should be found in optimally hole-doped infinite-layer ACuO$ _{2} $ cuprates - up to 160~K for A = Ba. The projected increase in $ T_{c} $ across the series arises from "internal pressure" effects as A runs from Mg to Ba. We then use density functional theory to investigate these pressure effects on the band structure in an attempt to understand this progressive increase in $ T_{c} $. Where these materials have been synthesised we find good agreement between our calculated structural parameters and the experimental ones. We find that internal pressure associated with increasing ion size does indeed enhance the superconducting energy gap, as observed, via modifications to the electronic dispersion. Furthermore, in our calculations, pressure alters the dispersion independently of how it is applied (internal or external) so that the superconducting energy gap correlates with the unit-cell volume and a Fermi-surface shape-parameter describing ratio of next-nearest-neighbor to nearest-neighbor hopping integrals. We infer an energy scale for the pairing interaction of the order of 1~eV, well above the magnetic energy scale.

cond-mat.supr-con↗

arXiv2016

Granular superconductivity and magnetic-field-driven recovery of macroscopic coherence in a cuprate/manganite multilayer

We show that in Pr$ _{0.5} $La$ _{0.2} $Ca$ _{0.3} $MnO$ _{3} $/YBa$ _{2} $Cu$ _{3} $O$ _{7} $ (PLCMO/YBCO) multilayers the low temperature state of YBCO is very resistive and resembles the one of a granular superconductor or a frustrated Josephson-junction network. Notably, a coherent superconducting response can be restored with a large magnetic field which also suppresses the charge-orbital order in PLCMO. This coincidence suggests that the granular superconducting state of YBCO is induced by the charge-orbital order of PLCMO. The coupling mechanism and the nature of the induced inhomogeneous state in YBCO remain to be understood.

cond-mat.supr-con↗

arXiv2016

Muon spin rotation and infrared spectroscopy study of magnetism and superconductivity in Ba$ _{1-x} $K$ _{x} $Fe$ _{2} $As$ _{2} $

Using muon spin rotation and infrared spectroscopy we study the relation between magnetism and superconductivity in Ba$ _{1-x} $K$ _{x} $Fe$ _{2} $As$ _{2} $ single crystals from the underdoped to the slightly overdoped regime. We find that the Fe magnetic moment is only moderately suppressed in most of the underdoped region where it decreases more slowly than the Néel-temperature, $ T^{\mathrm{N}} $. This applies for both the total Fe moment obtained from muon spin rotation and for the itinerant component that is deduced from the spectral weight of the spin-density-wave pair breaking peak in the infrared response. In the moderately underdoped region, superconducting and static magnetic orders co-exist on the nano-scale and compete for the same electronic states. The static magnetic moment disappears rather sharply near optimal doping, however, in the slightly overdoped region there is still an enhancement or slowing down of spin fluctuations in the superconducting state. Similar to the gap magnitude reported from specific heat measurements, the superconducting condensate density is nearly constant in the optimally- and slightly overdoped region, but exhibits a rather pronounced decrease on the underdoped side. Several of these observations are similar to the phenomenology in the electron doped counterpart Ba(Fe$ _{1-y} $Co$ _{y} $)$ _{2} $As$ _{2} $.

cond-mat.supr-con↗

arXiv2016

Anisotropy of the infrared-active phonon modes in the mono-domain state of tetragonal SrTiO3 (110)

With infrared and terahertz ellipsometry we investigated the anisotropy of the infrared active phonon modes in SrTiO3 (110) single crystals in the tetragonal state below the so-called antiferrodistortive transition at T* = 105 K. In particular, we show that the anisotropy of the oscillator strength of the so-called R-mode, which becomes weakly infrared active below T*, is a valuable indicator for the orientation of the structural domains. Our results reveal that a mono-domain state with the tetragonal axis (c-axis) parallel to the [001] direction can be created by applying a moderate uniaxial stress of about 2.3 MPa along the [1-10] direction (with a mechanical clamp). The resulting, intrinsic splitting of the infrared-active phonon modes is reported.

cond-mat.mtrl-sci↗

arXiv2016

X-ray absorption study of the ferromagnetic Cu moment at the $\mathbf{{YBa_2Cu_3O_7}/{La_{2/3}Ca_{1/3}MnO_3}}$ interface and the variation of its exchange interaction with the Mn moment

With x-ray absorption spectroscopy and polarized neutron reflectometry we studied how the magnetic proximity effect at the interface between the cuprate high-$T_C$ superconductor $\mathrm{YBa_2Cu_3O_7}$ (YBCO) and the ferromagnet $\mathrm{La_{2/3}Ca_{1/3}MnO_3}$ (LCMO) is related to the electronic and magnetic properties of the LCMO layers. In particular, we explored how the magnitude of the ferromagnetic Cu moment on the YBCO side depends on the strength of the antiferromagnetic (AF) exchange coupling with the Mn moment on the LCMO side. We found that the Cu moment remains sizeable if the AF coupling with the Mn moments is strongly reduced or even entirely suppressed. The ferromagnetic order of the Cu moments thus seems to be intrinsic to the interfacial CuO$_2$ planes and related to a weakly ferromagnetic intra-planar exchange interaction. The latter is discussed in terms of the partial occupation of the Cu $3d_{3z^2-r^2}$ orbitals, which occurs in the context of the so-called orbital reconstruction of the interfacial Cu ions.

cond-mat.mtrl-sci↗

arXiv2015

Muon-spin-rotation study of the magnetic structure in the tetragonal antiferromagnetic state of weakly underdoped Ba$ _{1-x} $K$ _{x} $Fe$ _{2} $As$ _{2} $

With muon spin rotation ($ μ$SR) we studied the transition between the orthorhombic antiferromagnetic (o-AF) and the tetragonal antiferromagnetic (t-AF) states of a weakly underdoped Ba$ _{1-x} $K$ _{x} $Fe$ _{2} $As$ _{2} $ single crystal. We observed some characteristic changes of the magnitude and the orientation of the magnetic field at the muon site which, due to the fairly high point symmetry of the latter, allow us to identify the magnetic structure of the t-AF state. It is the so-called, inhomogeneous double-$\mathbf{Q}$ magnetic structure with $ c $-axis oriented moments which has a vanishing magnetic moment on half of the Fe sites.

cond-mat.supr-con↗

arXiv2013

Dielectric versus magnetic pairing mechanisms in high-temperature cuprate superconductors investigated using Raman scattering

We suggest, and demonstrate, a systematic approach to the study of cuprate superconductors, namely, progressive change of ion size in order to systematically alter the interaction strength and other key parameters. R(Ba,Sr)$_2$Cu$_3$O$_y$ (R={La, ... Lu,Y}) is such a system where potentially obscuring structural changes are minimal. We thereby systematically alter both dielectric and magnetic properties. Dielectric fluctuation is characterized by ionic polarizability while magnetic fluctuation is characterized by exchange interactions measurable by Raman scattering. The range of transition temperatures is 70 to 107 K and we find that these correlate only with the dielectric properties, a behavior which persists with external pressure. The ultimate significance may remain to be proven but it highlights the role of dielectric screening in the cuprates and adds support to a previously proposed novel pairing mechanism involving exchange of quantized waves of electronic polarization.

cond-mat.supr-con↗