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B. R. Fulton

Publications and source records attributed to B. R. Fulton.

At least 19 recordsLinked to original sources

First inverse kinematics study of the $^{22}$Ne$(p,γ)^{23}$Na reaction and its role in AGB star and classical nova nucleosynthesis

The abundances of sodium and oxygen are observed to be anti-correlated in all well-studied globular clusters. Asymptotic giant branch (AGB) stars undergoing hot bottom burning (HBB) are thought to be prime candidates for producing sodium-rich oxygen-poor material and expelling it into the cluster ISM. The 22Ne(p,gamma)23Na reaction has been shown to strongly influence the amount of 23Na produced during HBB. This reaction is also important for classical novae nucleosynthesis, with sensitivity studies showing that the abundances of several isotopes in the Ne-Al region are significantly altered when varying the reaction rate between available compilations. Here we present the first inverse kinematics measurements of key resonances strengths as well as the direct capture S-factor. Together, this study represents the largest centre of mass energy range (149-1222 keV) over which this reaction has been measured in a single experiment. Our results for low-energy resonances at Ecm=149, 181 and 248 keV are in good agreement with recent forward kinematics results; we also find a direct capture S-factor consistent with the literature value of 62 keV.b. However, in the case of the important reference resonance at Ecm = 458 keV we find a strength value of wg=0.44 +/- 0.02 eV, which is significantly lower than recent results. Using our new recommended rate we explore the impact of these results on both AGB star and classical novae nucleosynthesis. In the case of AGB stars we see very little abundance changes with respect to the rate included in the STARLIB-2013. However, we observe changes of up to a factor of 2 in isotopes produced in both the carbon-oxygen (CO) and oxygen-neon (ONe) classical novae models considered here. The 22Ne(p,gamma)23Na reaction rate is now sufficiently well constrained to not significantly contribute toward abundance uncertainties from classical novae nucleosynthesis models.

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A direct measurement of the 17O(a,g)21Ne reaction in inverse kinematics and its impact on heavy element production

During the slow neutron capture process in massive stars, reactions on light elements can both produce and absorb neutrons thereby influencing the final heavy element abundances. At low metallicities, the high neutron capture rate of 16-O can inhibit s-process nucleosynthesis unless the neutrons are recycled via the 17O(a,n)20Ne reaction. The efficiency of this neutron recycling is determined by competition between the 17O(a,n)20Ne and 17O(a,g)21Ne reactions. While some experimental data are available on the former reaction, no data exist for the radiative capture channel at the relevant astrophysical energies. The 17O(a,g)21Ne reaction has been studied directly using the DRAGON recoil separator at the TRIUMF Laboratory. The reaction cross section has been determined at energies between 0.6 and 1.6 MeV Ecm, reaching into the Gamow window for core helium burning for the first time. Resonance strengths for resonances at 0.63, 0.721, 0.81 and 1.122 MeV Ecm have been extracted. The experimentally based reaction rate calculated represents a lower limit, but suggests that significant s-process nucleosynthesis occurs in low metallicity massive stars.

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Initial operation of the recoil mass spectrometer EMMA at the ISAC-II facility of TRIUMF

The Electromagnetic Mass Analyser (EMMA) is a new vacuum-mode recoil mass spectrometer currently undergoing the final stages of commissioning at the ISAC-II facility of TRIUMF. EMMA employs a symmetric configuration of electrostatic and magnetic deflectors to separate the products of nuclear reactions from the beam, focus them in both energy and angle, and disperse them in a focal plane according to their mass/charge (m/q) ratios. The spectrometer was designed to accommodate the gamma-ray detector array TIGRESS around the target position in order to provide spectroscopic information from electromagnetic transitions. EMMA is intended to be used in the measurement of fusion evaporation, radiative capture, and transfer reactions for the study of nuclear structure and astrophysics. Its complement of focal plane detectors facilitates the identification of recoiling nuclei and subsequent recoil decay spectroscopy. Here we describe the facility and report on commissioning efforts.

physics.ins-det

Shell evolution approaching the N=20 island of inversion: structure of 26Na

The levels in 26Na with single particle character have been observed for the first time using the d(25Na,p gamma) reaction at 5 MeV/nucleon. The measured excitation energies and the deduced spectroscopic factors are in good overall agreement with (0+1) hbar-omega shell model calculations performed in a complete spsdfp basis and incorporating a reduction in the N=20 gap. Notably, the 1p3/2 neutron configuration was found to play an enhanced role in the structure of the low-lying negative parity states in 26Na, compared to the isotone 28Al. Thus, the lowering of the 1p3/2 orbital relative to the 0f7/2 occurring in the neighbouring Z=10 and 12 nuclei -- 25,27Ne and 27,29Mg -- is seen also to occur at Z=11 and further strengthens the constraints on the modelling of the transition into the island of inversion.

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Spectroscopy of $^{19}$Ne for the thermonuclear $^{15}$O($α,γ$)$^{19}$Ne and $^{18}$F($p,α$)$^{15}$O reaction rates

Uncertainties in the thermonuclear rates of the $^{15}$O($α,γ$)$^{19}$Ne and $^{18}$F($p,α$)$^{15}$O reactions affect model predictions of light curves from type I X-ray bursts and the amount of the observable radioisotope $^{18}$F produced in classical novae, respectively. To address these uncertainties, we have studied the nuclear structure of $^{19}$Ne over $E_{x} = 4.0 - 5.1$ MeV and $6.1 - 7.3$ MeV using the $^{19}$F($^{3}$He,t)$^{19}$Ne reaction. We find the $J^π$ values of the 4.14 and 4.20 MeV levels to be consistent with $9/2^{-}$ and $7/2^{-}$ respectively, in contrast to previous assumptions. We confirm the recently observed triplet of states around 6.4 MeV, and find evidence that the state at 6.29 MeV, just below the proton threshold, is either broad or a doublet. Our data also suggest that predicted but yet unobserved levels may exist near the 6.86 MeV state. Higher resolution experiments are urgently needed to further clarify the structure of $^{19}$Ne around the proton threshold before a reliable $^{18}$F($p,α$)$^{15}$O rate for nova models can be determined.

astro-ph.SR

Two-neutron transfer reaction mechanisms in $^{12}$C($^6$He,$^{4}$He)$^{14}$C using a realistic three-body $^{6}$He model

The reaction mechanisms of the two-neutron transfer reaction $^{12}$C($^6$He,$^4$He) have been studied at 30 MeV at the TRIUMF ISAC-II facility using the SHARC charged-particle detector array. Optical potential parameters have been extracted from the analysis of the elastic scattering angular distribution. The new potential has been applied to the study of the transfer angular distribution to the 2$^+_2$ 8.32 MeV state in $^{14}$C, using a realistic 3-body $^6$He model and advanced shell model calculations for the carbon structure, allowing to calculate the relative contributions of the simultaneous and sequential two-neutron transfer. The reaction model provides a good description of the 30 MeV data set and shows that the simultaneous process is the dominant transfer mechanism. Sensitivity tests of optical potential parameters show that the final results can be considerably affected by the choice of optical potentials. A reanalysis of data measured previously at 18 MeV however, is not as well described by the same reaction model, suggesting that one needs to include higher order effects in the reaction mechanism.

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Constraining nova observables: direct measurements of resonance strengths in 33S(p,γ)34Cl

The 33S(p,γ)34Cl reaction is important for constraining predictions of certain isotopic abundances in oxygen-neon novae. Models currently predict as much as 150 times the solar abundance of 33S in oxygen-neon nova ejecta. This overproduction factor may, however, vary by orders of magnitude due to uncertainties in the 33S(p,γ)34Cl reaction rate at nova peak temperatures. Depending on this rate, 33S could potentially be used as a diagnostic tool for classifying certain types of presolar grains. Better knowledge of the 33S(p,γ)34Cl rate would also aid in interpreting nova observations over the S-Ca mass region and contribute to the firm establishment of the maximum endpoint of nova nucleosynthesis. Additionally, the total S elemental abundance which is affected by this reaction has been proposed as a thermometer to study the peak temperatures of novae. Previously, the 33S(p,γ)34Cl reaction rate had only been studied directly down to resonance energies of 432 keV. However, for nova peak temperatures of 0.2-0.4 GK there are 7 known states in 34Cl both below the 432 keV resonance and within the Gamow window that could play a dominant role. Direct measurements of the resonance strengths of these states were performed using the DRAGON recoil separator at TRIUMF. Additionally two new states within this energy region are reported. Several hydrodynamic simulations have been performed, using all available experimental information for the 33S(p,γ)34Cl rate, to explore the impact of the remaining uncertainty in this rate on nucleosynthesis in nova explosions. These calculations give a range of ~ 20-150 for the expected 33S overproduction factor, and a range of ~ 100-450 for the 32S/33S ratio expected in ONe novae.

astro-ph.SR

Is γ-ray emission from novae affected by interference effects in the 18F(p,α)15O reaction?

The 18F(p,α)15O reaction rate is crucial for constraining model predictions of the γ-ray observable radioisotope 18F produced in novae. The determination of this rate is challenging due to particular features of the level scheme of the compound nucleus, 19Ne, which result in interference effects potentially playing a significant role. The dominant uncertainty in this rate arises from interference between Jπ=3/2+ states near the proton threshold (Sp = 6.411 MeV) and a broad Jπ=3/2+ state at 665 keV above threshold. This unknown interference term results in up to a factor of 40 uncertainty in the astrophysical S-factor at nova temperatures. Here we report a new measurement of states in this energy region using the 19F(3He,t)19Ne reaction. In stark contrast with previous assumptions we find at least 3 resonances between the proton threshold and Ecm=50 keV, all with different angular distributions. None of these are consistent with Jπ= 3/2+ angular distributions. We find that the main uncertainty now arises from the unknown proton-width of the 48 keV resonance, not from possible interference effects. Hydrodynamic nova model calculations performed indicate that this unknown width affects 18F production by at least a factor of two in the model considered.

astro-ph.SR

Measurement of the 18Ne(a,p_0)21Na reaction cross section in the burning energy region for X-ray bursts

The 18Ne(a,p)21Na reaction provides one of the main HCNO-breakout routes into the rp-process in X-ray bursts. The 18Ne(a,p_0)21Na reaction cross section has been determined for the first time in the Gamow energy region for peak temperatures T=2GK by measuring its time-reversal reaction 21Na(p,a)18Ne in inverse kinematics. The astrophysical rate for ground-state to ground-state transitions was found to be a factor of 2 lower than Hauser-Feshbach theoretical predictions. Our reduced rate will affect the physical conditions under which breakout from the HCNO cycles occurs via the 18Ne(a,p)21Na reaction.

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Single-Proton Removal Reaction Study of 16B

The low-lying level structure of the unbound system $^{16}$B has been investigated via single-proton removal from a 35 MeV/nucleon $^{17}$C beam. The coincident detection of the beam velocity $^{15}$B fragment and neutron allowed the relative energy of the in-flight decay of $^{16}$B to be reconstructed. The resulting spectrum exhibited a narrow peak some 85 keV above threshold. It is argued that this feature corresponds to a very narrow ($Γ\ll $100 keV) resonance, or an unresolved multiplet, with a dominant $π(p_{3/2})^{-1} \otimes ν(d_{5/2}^3)_{J=3/2^+}$ + $π(p_{3/2})^{-1} \otimes ν(d_{5/2}^2,s_{1/2})_{J=3/2^+}$ configuration which decays by d-wave neutron emission.

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First results on double beta decay modes of Cd, Te and Zn isotopes with the COBRA experiment

Four 1cm^3 CdZnTe semiconductor detectors were operated in the Gran Sasso National Laboratory to explore the feasibility of such devices for double beta decay searches as proposed for the COBRA experiment. The research involved background studies accompanied by measurements of energy resolution performed at the surface. Energy resolutions sufficient to reduce the contribution of two-neutrino double beta decay events to a negligible level for a large scale experiment have already been achieved and further improvements are expected. Using activity measurements of contaminants in all construction materials a background model was developed with the help of Monte Carlo simulations and major background sources were identified. A total exposure of 4.34 kg.days of underground data has been accumulated allowing a search for neutrinoless double beta decay modes of seven isotopes found in CdZnTe. Half-life limits (90% C.L.) are presented for decays to ground and excited states. Four improved lower limits have been obtained, including zero neutrino double electron capture transitions of Zn64 and Te120 to the ground state, which are 1.19*10^{17} years and 2.68*10^{15} years respectively.

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B(E1) Strengths from Coulomb Excitation of 11Be

The $B$(E1;$1/2^+\to1/2^-$) strength for $^{11}$Be has been extracted from intermediate energy Coulomb excitation measurements, over a range of beam energies using a new reaction model, the extended continuum discretized coupled channels (XCDCC) method. In addition, a measurement of the excitation cross section for $^{11}$Be+$^{208}$Pb at 38.6 MeV/nucleon is reported. The $B$(E1) strength of 0.105(12) e$^2$fm$^2$ derived from this measurement is consistent with those made previously at 60 and 64 MeV/nucleon, i n contrast to an anomalously low result obtained at 43 MeV/nucleon. By coupling a multi-configuration description of the projectile structure with realistic reaction theory, the XCDCC model provides for the first time a fully quantum mechanical description of Coulomb excitation. The XCDCC calculations reveal that the excitation process involves significant contributions from nuclear, continuum, and higher-order effects. An analysis of the present and two earlier intermediate energy measurements yields a combined B(E1) strength of 0.105(7) e$^2$fm$^2$. This value is in good agreement with the value deduced independently from the lifetime of the $1/2^-$ state in $^{11}$Be, and has a comparable p recision.

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Structure of 12Be: intruder d-wave strength at N=8

The breaking of the N=8 shell-model magic number in the 12Be ground state has been determined to include significant occupancy of the intruder d-wave orbital. This is in marked contrast with all other N=8 isotones, both more and less exotic than 12Be. The occupancies of the 0 hbar omega neutron p1/2-orbital and the 1 hbar omega, neutron d5/2 intruder orbital were deduced from a measurement of neutron removal from a high-energy 12Be beam leading to bound and unbound states in 11Be.

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The 7Be(d,p)2alpha cross section at Big Bang energies and the primordial 7Li abundance

The WMAP satellite, devoted to the observations of the anisotropies of the Cosmic Microwave Background (CMB) radiation, has recently provided a determination of the baryonic density of the Universe with unprecedented precision. Using this, Big Bang Nucleosynthesis (BBN) calculations predict a primordial 7Li abundance which is a factor 2-3 higher than that observed in galactic halo dwarf stars. It has been argued that this discrepancy could be resolved if the 7Be(d,p)2alpha reaction rate is around a factor of 100 larger than has previously been considered. We have now studied this reaction, for the first time at energies appropriate to the Big Bang environment, at the CYCLONE radioactive beam facility at Louvain-la-Neuve. The cross section was found to be a factor of 10 smaller than derived from earlier measurements. It is concluded therefore that nuclear uncertainties cannot explain the discrepancy between observed and predicted primordial 7Li abundances, and an alternative astrophysical solution must be investigated.

astro-ph

Three-centre cluster structure in 11C and 11B

Studies of the 16O(9Be,alpha 7Be)14C, 7Li(9Be,alpha 7Li)5He and 7Li(9Be,alpha alpha t)5He reactions at E(beam)=70 and 55 MeV have been performed using resonant particle spectroscopy techniques. The 11C excited states decaying into alpha+7Be(gs) are observed between 8.5 and 13.5 MeV. The alpha+7Li(gs), alpha+7Li*(4.652 MeV) and t+8Be(gs) decays of 11B excited states between 9 and 19 MeV are observed. The decay processes are used to indicate the possible three-centre 2alpha+3He (2alpha+3H) cluster structure of observed states. This cluster structure is more prominent in the positive-parity states, where two rotational bands with large deformations are suggested. Excitations of some of the observed T=1/2 resonances coincide with the energies of previously measured T=3/2 isobaric analogs of the 11Be states,indicating that these states may have mixed isospin.

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alpha-decay of excited states in 11C and 11B

Studies of the 16O(9Be,alpha7Be)14C and 7Li(9Be,alpha7Li)5He reactions at E{beam}=70 MeV have been performed using resonant particle spectroscopy techniques. The 11C excited states decaying into alpha+7Be(gs) are observed at 8.65, 9.85, 10.7 and 12.1 MeV as well as possible states at 12.6 and 13.4 MeV. This result is the first observation of alpha-decay for excited states above 9 MeV. The alpha+7Li(gs) decay of 11B excited states at 9.2, 10.3, 10.55, 11.2, (11.4), 11.8, 12.5,(13.0), 13.1, (14.0), 14.35, (17.4) and (18.6) MeV is observed. The decay processes are used to indicate the possible three-centre 2alpha+3He(3H) cluster structure of observed states. Two rotational bands corresponding to very deformed structures are suggested for the positive-parity states. Excitations of some observed T=1/2 resonances coincide with the energies of T=3/2 states which are the isobaric analogs of the lowest 11Be states. Some of these states may have mixed isospin.

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Reevaluation of the $^{22}$Na(p,$γ$) reaction rate: Implications for the detection of $^{22}$Na gamma rays from novae

Understanding the processes which create and destroy $^{22}$Na is important for diagnosing classical nova outbursts. Conventional $^{22}$Na(p,$γ$) studies are complicated by the need to employ radioactive targets. In contrast, we have formed the particle-unbound states of interest through the heavy-ion fusion reaction, $^{12}$C($^{12}$C,n)$^{23}$Mg and used the Gammasphere array to investigate their radiative decay branches. Detailed spectroscopy was possible and the $^{22}$Na(p,$γ$) reaction rate has been re-evaluated. New hydrodynamical calculations incorporating the upper and lower limits on the new rate suggest a reduction in the yield of $^{22}$Na with respect to previous estimates, implying a reduction in the maximum detectability distance for $^{22}$Na $γ$ rays from novae.

astro-ph

Cluster structure of 13C probed via the 7Li(9Be,13C*->9Be+alpha) reaction

A study of the 7Li(9Be,4He9Be)3H reaction at E{beam}=70 MeV has been performed using resonant particle spectroscopy techniques and provides a measurement of alpha-decaying states in 13C. Excited states are observed at 12.0, 13.4, 14.1, 14.6, 15.2, 16.8, 17.9, 18.7, 21.3 and 23.9 MeV. This study provides the first measurement of the three highest energy states. Angular distribution measurements have been performed and have been employed to indicate the transferred angular momentum for the populated states. These data are compared with recent speculations of the presence of chain-like structures in 13C.

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