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B. Uchoa

Publications and source records attributed to B. Uchoa.

11 recordsLinked to original sources

Nature of the Topological Transition of the Kitaev Model in [111] Magnetic Field

We investigate the nature of the topological phase transition of the antiferromagnetic Kitaev model on the honeycomb lattice in the presence of a magnetic field along the [111] direction. The field opens a topological gap in the Majorana fermion spectrum and leads to a sequence of topological phase transitions before the field polarised state is reached. At mean field level the gap first closes at the three $M$ points in the Brillouin zone, where the Majorana fermions form Dirac cones, resulting in a change of Chern number by three. An odd number of Dirac fermions in the infrared is unusual and requires Berry curvature compensation in the UV, which occurs via topological, ring-like hybridisation gaps with higher-energy bands. We perform a renormalisation-group analysis of the topological phase transition at the three $M$ points within the Yukawa theory, allowing for intra- and inter-valley fluctuations of the spin-liquid bond operators. We find that the latter lead to a breaking of Lorentz invariance and hence a different universality compared to the standard Ising Gross-Neveu-Yukawa class.

cond-mat.str-el

Observation of Pines' Demon in Sr$_2$RuO$_4$

The characteristic excitation of a metal is its plasmon, which is a quantized collective oscillation of its electron density. In 1956, David Pines predicted that a distinct type of plasmon, dubbed a "demon," could exist in three-dimensional metals containing more than one species of charge carrier. Consisting of out-of-phase movement of electrons in different bands, demons are acoustic, electrically neutral, and do not couple to light, so have never been detected in an equilibrium, three-dimensional metal. Nevertheless, demons are believed to be critical for diverse phenomena including phase transitions in mixed-valence semimetals, optical properties of metal nanoparticles, "soundarons" in Weyl semimetals, and high temperature superconductivity in, for example, metal hydrides. Here, we present evidence for a demon in Sr$_2$RuO$_4$ from momentum-resolved electron energy-loss spectroscopy (M-EELS). Formed of electrons in the $β$ and $γ$ bands, the demon is gapless with a room temperature velocity $v=1.065 \pm 0.12 \times 10^5$ m/s and critical momentum $q_c=0.08$ reciprocal lattice units. Its spectral weight violates low-energy partial sum rules, affirming its neutral character. Our study confirms a 66-year old prediction and suggests that demons may be a pervasive feature of multiband metals.

cond-mat.str-el

Crossover of Charge Fluctuations across the Strange Metal Phase Diagram

A normal metal exhibits a valence plasmon, which is a sound wave in its conduction electron density. The mysterious strange metal is characterized by non-Boltzmann transport and violates most fundamental Fermi liquid scaling laws. A fundamental question is: Do strange metals have plasmons? Using momentum-resolved inelastic electron scattering (M-EELS) we recently showed that, rather than a plasmon, optimally-doped Bi$_{2.1}$Sr$_{1.9}$Ca$_{1.0}$Cu$_{2.0}$O$_{8+x}$ (Bi-2212) exhibits a featureless, temperature-independent continuum with a power-law form over most energy and momentum scales [M. Mitrano, PNAS 115, 5392-5396 (2018)]. Here, we show that this continuum is present throughout the fan-shaped, strange metal region of the phase diagram. Outside this region, dramatic changes in spectral weight are observed: In underdoped samples, spectral weight up to 0.5 eV is enhanced at low temperature, biasing the system towards a charge order instability. The situation is reversed in the overdoped case, where spectral weight is strongly suppressed at low temperature, increasing quasiparticle coherence in this regime. Optimal doping corresponds to the boundary between these two opposite behaviors at which the response is temperature-independent. Our study suggests that plasmons do not exist as well-defined excitations in Bi-2212, and that a featureless continuum is a defining property of the strange metal, which is connected to a peculiar crossover where the spectral weight change undergoes a sign reversal.

cond-mat.str-el

Anomalous density fluctuations in a strange metal

A central mystery in high temperature superconductivity is the origin of the so-called "strange metal," i.e., the anomalous conductor from which superconductivity emerges at low temperature. Measuring the dynamic charge response of the copper-oxides, $χ''(q,ω)$, would directly reveal the collective properties of the strange metal, but it has never been possible to measure this quantity with meV resolution. Here, we present the first measurement of $χ''(q,ω)$ for a cuprate, optimally doped Bi$_2$Sr$_2$CaCu$_2$O$_{8+x}$ ($T_c=91$ K), using momentum-resolved inelastic electron scattering. In the medium energy range 0.1-2 eV relevant to the strange metal, the spectra are dominated by a featureless, temperature- and momentum-independent continuum persisting to the eV energy scale. This continuum displays a simple power law form, exhibiting $q^2$ behavior at low energy and $q^2/ω^2$ behavior at high energy. Measurements of an overdoped crystal ($T_c=50$ K) showed the emergence of a gap-like feature at low temperature, indicating deviation from power law form outside the strange metal regime. Our study suggests the strange metal exhibits a new type of charge dynamics in which excitations are local to such a degree that space and time axes are decoupled.

cond-mat.str-el

Magnetic exchange mechanism for electronic gap opening in graphene

We show within a local self-consistent mean-field treatment that a random distribution of magnetic adatoms can open a robust gap in the electronic spectrum of graphene. The electronic gap results from the interplay between the nature of the graphene sublattice structure and the exchange interaction between adatoms.The size of the gap depends on the strength of the exchange interaction between carriers and localized spins and can be controlled by both temperature and external magnetic field. Furthermore, we show that an external magnetic field creates an imbalance of spin-up and spin-down carriers at the Fermi level, making doped graphene suitable for spin injection and other spintronic applications.

cond-mat.str-el

Tailoring Graphene with Metals on Top

We study the effects of metallic doping on the electronic properties of graphene using density functional theory in the local density approximation in the presence of a local charging energy (LDA+U). The electronic properties are sensitive to whether graphene is doped with alkali or transition metals. We estimate the the charge transfer from a single layer of Potassium on top of graphene in terms of the local charging energy of the graphene sheet. The coating of graphene with a non-magnetic layer of Palladium, on the other hand, can lead to a magnetic instability in coated graphene due to the hybridization between the transition-metal and the carbon orbitals.

cond-mat.mtrl-sci

Nodal liquid and s-wave superconductivity in transition metal dichalcogenides

We explore the physical properties of a unified microscopic theory for the coexistence of superconductivity and charge density waves in two-dimensional transition metal dichalcogenides. In the case of particle-hole symmetry the elementary particles are Dirac fermions at the nodes of the charge density wave gap. When particle-hole symmetry is broken electron (hole) pockets are formed around the Fermi surface. The superconducting ground state emerges from the pairing of nodal quasi-particles mediated by acoustic phonons via a piezoelectric coupling. We calculate several properties in the s-wave superconducting phase, including specific heat, ultra-sound absorption, nuclear magnetic relaxation, thermal, and optical conductivities. In the case with particle-hole symmetry, the specific heat jump at the transition deviates strongly from ordinary superconductors. The nuclear magnetic response shows an anomalous anisotropy due to the broken time-reversal symmetry of the superconducting gap, induced by the triple charge density wave state. The loss of lattice inversion symmetry in the charge density wave phase leads to anomalous coherence factors in the optical conductivity and to the appearance of an absorption edge at the optical gap energy. Furthermore, optical and thermal conductivities display anomalous peaks in the infrared when particle-hole symmetry is broken.

cond-mat.supr-con

Magnetic structure and critical behavior of GdRhIn$_{5}$: resonant x-ray diffraction and renormalization group analysis

The magnetic structure and fluctuations of tetragonal GdRhIn5 were studied by resonant x-ray diffraction at the Gd LII and LIII edges, followed by a renormalization group analysis for this and other related Gd-based compounds, namely Gd2IrIn8 and GdIn3. These compounds are spin-only analogs of the isostructural Ce-based heavy-fermion superconductors. The ground state of GdRhIn5 shows a commensurate antiferromagnetic spin structure with propagation vector tau = (0,1/2, 1/2), corresponding to a parallel spin alignment along the a-direction and antiparallel alignment along b and c. A comparison between this magnetic structure and those of other members of the Rm(Co,Rh,Ir)n In3m+2n family (R =rare earth, n = 0, 1; m = 1, 2) indicates that, in general, tau is determined by a competition between first-(J1) and second-neighbor(J2) antiferromagnetic (AFM) interactions. While a large J1 /J2 ratio favors an antiparallel alignment along the three directions (the so-called G-AFM structure), a smaller ratio favors the magnetic structure of GdRhIn5 (C-AFM). In particular, it is inferred that the heavy-fermion superconductor CeRhIn5 is in a frontier between these two ground states, which may explain its non-collinear spiral magnetic structure. The critical behavior of GdRhIn5 close to the paramagnetic transition at TN = 39 K was also studied in detail. A typical second-order transition with the ordered magnetization critical parameter beta = 0.35 was experimentally found, and theoretically investigated by means of a renormalization group analysis.

cond-mat.str-el

Ferromagnetic Domain Walls in finite systems: mean-field critical exponents and applications

The distribution of magnetic moments in finite ferromagnetic bodies was first investigated by Landau and Lifshitz in a famous paper [\textit{Phys. Z. Soviet Union}, \textbf{8}, 153 (1935)], where they obtained the domain structure of a ferromagnetic crystal at low temperatures, in the regime of saturated magnetization. In this article, we investigate the general properties of ferromagnetic domain walls of uniaxial crystals from the view point of the Landau free energy. We present the basic ideas at an introductory level, for non-experts. Extending the formalism to the vicinity of the Curie temperature, where a general qualitative description by the Landau theory of phase transitions can be applied, we find that domain walls tend to suppress the layers, leading to a continuous vanishing of the domain structure with anomalous critical exponents. In the saturated regime, we discuss the role of domain walls in mesoscopic systems and ferromagnetic nanojunctions, relating the observed magnetoresistance with promising applications in the recent area of spintronics.

cond-mat.stat-mech

Electromagnetic Response of Layered Superconductors with Broken Lattice Inversion Symmetry

We investigate the macroscopic effects of charge density waves (CDW) and superconductivity in layered superconducting systems with broken lattice inversion symmetry (allowing for piezoelectricity) such as two dimensional (2D) transition metal dichalcogenides (TMD). We work with the low temperature time dependent Ginzburg-Landau theory and study the coupling of lattice distortions and low energy CDW collective modes to the superconducting order parameter in the presence of electromagnetic fields. We show that superconductivity and piezoelectricity can coexist in these singular metals. Furthermore, our study indicates the nature of the quantum phase transition between a commensurate CDW phase and the stripe phase that has been observed as a function of applied pressure.

cond-mat.supr-con

Commensurability Transition and Stripe Phases in the Ginzburg-Landau Theory

We phenomenologically describe the thermodynamics of charge and spin density waves in doped high-$T_{c}$ oxides. We have explicitly calculated stable non-homogeneous solutions in the incompressible spin driven stripe phase, where stripes are static soliton-like charge density waves (CDW), and in the vicinity of their critical point, where CDW's become harmonic. Our phase diagram points to a commensurability transition separating the low (LI) and high (HI) incommensurable phases. Besides, we demonstrate by rigorous group symmetry arguments that the stripe criticality is compatible with a second order phase transition.

cond-mat.str-el