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B. V. Kheswa

Publications and source records attributed to B. V. Kheswa.

At least 19 recordsLinked to original sources

Statistical properties of $^{133}$Xe and the $^{132}$Xe$(n,γ)$ cross section

$^{133}$Xe is an interesting case for plasma physics to explore nuclear excitation by electron capture, as the process can be studied using statistical properties of $^{133}$Xe. In this work we present results on $^{133}$Xe from the inverse-Oslo method where we extract the nuclear level density and the $γ$-strength function, which is used to calculate the (n,$γ$) cross section on $^{132}$Xe. The $γ$-strength function of $^{133}$Xe can constrain the estimated decay rate from nuclear excitation by electron capture. The $\mathrm{d}(^{132}\mathrm{Xe},\mathrm{p})^{132}\mathrm{Xe}$ reaction was used to create the compound nucleus $^{133}$Xe, which was recorded with an annular particle telescope and a scintillator array consisting of \la and BGO-shielded HPGe Clover detectors. With the inverse-Oslo method, it is possible to study nuclei that are impossible or unable to manufacture targets from, short lived isotopes, or as in this work, noble gases. We present the extracted nuclear level density, and $γ$-strength function for $^{133}$Xe, along with shell-model calculations of the statistical properties of $^{133}$Xe. These are the first statistical properties extracted below 6 MeV for any xenon isotope. We constrain the $^{132}$Xe(n,$γ$) $^{133}$Xe cross section and reaction rate using the TALYS reaction code.

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Nuclear Level Density and $γ$-ray Strength Function of $^{67}\mathrm{Ni}$ and the impact on the i-process

Proton-$γ$ coincidences from $(\mathrm{d},\mathrm{p})$ reactions between a $^{66}\mathrm{Ni}$ beam and a deuterated polyethylene target have been analyzed with the inverse-Oslo method to find the nuclear level density (NLD) and $γ$-ray strength function ($γ$SF) of $^{67}\mathrm{Ni}$. The $^{66}\mathrm{Ni}(n,γ)$ capture cross section has been calculated using the Hauser-Feshbach model in TALYS using the measured NLD and $γ$SF as constraints. The results confirm that the $^{66}\mathrm{Ni}(n,γ)$ reaction acts as a bottleneck when relying on one-zone nucleosynthesis calculations. However, the impact of this reaction is strongly dampened in multi-zone models of low-metallicity AGB stars experiencing i-process nucleosynthesis.

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Gamma-ray emission in proton-induced nuclear reactions on natC and Mylar targets over the incident energy range of Ep = 30-200 MeV. Astrophysical implications

We have measured the gamma-ray line production cross sections in proton-induced nuclear reactions on various target nuclei abundant in astrophysical sites over the incident energy range of Ep = 30 - 200 MeV. We carried out experimental campaigns in joint collaboration at the K = 200 cyclotron of iThemba LABS using a high-energy resolution, high-efficiency detection array composed of 8 Compton-suppressed clover detectors comprising 32 HP-Ge crystals for recording the gamma-ray spectra. In the current paper, we focus on de-excitation lines produced in proton irradiations of natC and Mylar targets. In particular, on the prominent 4.439 and 6.129 MeV lines of $^{12}$C and $^{16}$O which are among the strongest lines emitted in solar flares and in interactions of low-energy cosmic rays with the gas and dust of the inner galaxy. We report new gamma-ray production experimental cross section data for ten nuclear lines that we compare to previous low-energy data sets from the literature, to the predictions of the TALYS code of modern nuclear reactions and to a semi-empirical compilation. In first approach, performing calculations with default input parameters of TALYS we observed substantial deviations between the predicted cross sections and experimental data. Then, using modified optical model potential and nuclear level deformation parameters as input data we generated theoretical excitation functions for the above two main lines fully consistent with experimental data. In contrast, the experimental data sets for the other eight analyzed lines from the two proton-irradiated targets exhibit significant deviations with the predicted cross section values. We also report line-shape experimental data for the line complex observed at $E_g$ = 4.44 MeV in irradiations of the two targets. Finally, we emphasize the astrophysical implications of our results.

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New experimental constraint on the $^{185}$W($n,γ$)$^{186}$W cross section

In this work, we present new data on the $^{182,183,184}$W($γ,n$) cross sections, utilizing a quasi-monochromatic photon beam produced at the NewSUBARU synchrotron radiation facility. Further, we have extracted the nuclear level density and $γ$-ray strength function of $^{186}$W from data on the $^{186}$W($α,α^\primeγ$)$^{186}$W reaction measured at the Oslo Cyclotron Laboratory. Combining previous measurements on the $^{186}$W($γ,n$) cross section with our new $^{182,183,184}$W($γ,n$) and ($α,α^\primeγ$)$^{186}$W data sets, we have deduced the $^{186}$W $γ$-ray strength function in the range of $1 < E_γ< 6$ MeV and $7 < E_γ< 14$ MeV. Our data are used to extract the level density and $γ$-ray strength functions needed as input to the nuclear-reaction code \textsf{TALYS}, providing an indirect, experimental constraint for the $^{185}$W($n,γ$)$^{186}$W cross section and reaction rate. Compared to the recommended Maxwellian-averaged cross section (MACS) in the KADoNiS-1.0 data base, our results are on average lower for the relevant energy range $k_B T \in [5,100]$ keV, and we provide a smaller uncertainty for the MACS. The theoretical values of Bao \textit{et al.} and the cross section experimentally constrained on photoneutron data of Sonnabend \textit{et al.} are significantly higher than our result. The lower value by Mohr \textit{et al.} is in very good agreement with our deduced MACS. Our new results could have implications for the $s$-process and in particular the predicted $s$-process production of $^{186,187}$Os nuclei.

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Evolution of the $γ$-ray strength function in neodymium isotopes

The experimental gamma-ray strength functions (gamma-SFs) of 142,144-151Nd have been studied for gamma-ray energies up to the neutron separation energy. The results represent a unique set of gamma-SFs for an isotopic chain with increasing nuclear deformation. The data reveal how the low-energy enhancement, the scissors mode and the pygmy dipole resonance evolve with nuclear deformation and mass number. The data indicate that the mechanisms behind the low-energy enhancement and the scissors mode are decoupled from each other.

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Statistical properties of the well deformed $^{153,155}$Sm nuclei and the scissors resonance

The Nuclear Level Densities (NLDs) and the $γ$-ray Strength Functions ($γ$SFs) of $^{153,155}$Sm have been extracted from (d,p$γ$) coincidences using the Oslo method. The experimental NLD of $^{153}$Sm is higher than the NLD of $^{155}$Sm, in accordance with microscopic calculations. The $γ$SFs of $^{153,155}$Sm are in fair agreement with QRPA calculations based on the D1M Gogny interaction. An enhancement is observed in the $γ$SF for both $^{153,155}$Sm nuclei around 3 MeV in excitation energy and is attributed to the M1 Scissors Resonance (SR). Their integrated strengths were found to be in the range 1.3 - 2.1 and 4.4 - 6.4 $μ^{2}_{N}$ for $^{153}$Sm and $^{155}$Sm, respectively. The strength of the SR for $^{155}$Sm is comparable to those for deformed even-even Sm isotopes from nuclear resonance fluorescence measurements, while that of $^{153}$Sm is lower than expected.

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Strong enhancement of level densities in the crossover from spherical to deformed neodymium isotopes

Understanding the evolution of level densities in the crossover from spherical to well-deformed nuclei has been a long-standing problem in nuclear physics. We measure nuclear level densities for a chain of neodymium isotopes $^{142,144-151}$Nd which exhibit such a crossover. These results represent to date the most complete data set of nuclear level densities for an isotopic chain between neutron shell-closure and towards mid-shell. We observe a strong increase of the level densities along the chain with an overall increase by a factor of $\approx 170$ at an excitation energy of 7.5 MeV and saturation around mass 150. Level densities calculated by the shell model Monte Carlo (SMMC) are in excellent agreement with these experimental results. Based on our experimental and theoretical findings, we offer an explanation of the observed mass dependence of the level densities in terms of the intrinsic single-particle level density and the collective enhancement.

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Spectroscopy of low spin states in 157Dy: Search for evidence of enhanced octupole correlations

Low-spin states of 157Dy have been studied using the JUROGAM II array, following the 155Gd (α, 2n) reaction at a beam energy of 25 MeV. The level scheme of 157Dy has been expanded with four new bands. Rotational structures built on the [523]5/2- and [402]3/2+ neutron orbitals constitute new additions to the level scheme as do many of the inter- and intra-band transitions. This manuscript also reports the observation of cross I- to (I-1)- and I- to (I-1)+ E1 dipole transitions inter-linking structures built on the [523]5/2- (band 5) and [402]3/2+ (band 7) neutron orbitals. These interlacing band structures are interpreted as the bands of parity doublets with simplex quantum number s = -i related to possible octupole correlations.

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First candidates for γ vibrational bands built on the [505]11/2- neutron orbital in odd-A Dy isotopes

Rotational structures have been measured using the Jurogam II and GAMMASPHERE arrays at low spin following the 155Gd(α,2n)157Dy and 148Nd(12C, 5n)155Dy reactions at 25 and 65 MeV, respectively. We report high-K bands, which are conjectured to be the first candidates of a Kπ= 2+ γ vibrational band, built on the [505]11/2- neutron orbital, in both odd-A 155, 157Dy isotopes. The coupling of the first excited K=0+ states or the so-called \b{eta} vibrational bands at 661 and 676 keV in 154Dy and 156Dy to the [505]11/2- orbital, to produce a Kπ=11/2- band, was not observed in both 155Dy and 157Dy, respectively. The implication of these findings on the interpretation of the first excited 0+ states in the core nuclei 154Dy and 156Dy are also discussed.

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Measurement and analysis of nuclear $γ$-ray production cross sections in proton interactions with Mg, Si and Fe nuclei abundant in astrophysical sites over the incident energy range $E=30-66$ MeV

Gamma-ray production cross section excitation functions have been measured for $30$, $42$, $54$ and $66$ MeV proton beams accelerated onto targets of astrophysical interest, $^{nat}$C, C + O (Mylar), $^{nat}$Mg, $^{nat}$Si and $^{56}$Fe, at the Sector Separated Cyclotron (SSC) of iThemba LABS (near Cape Town, South Africa). The AFRODITE array equipped with 8 Compton suppressed HPGe clover detectors was used to record $γ$-ray data. For known, intense $γ$-ray lines the previously reported experimental data measured up to $E_{p}\simeq$ $25$ MeV at the Washington and Orsay tandem accelerators were extended to higher proton energies. Our experimental data for the last 3 targets are reported here and discussed with respect to previous data and the Murphy \textit{et al.} compilation [ApJS 183, 142 (2009)], as well as to predictions of the nuclear reaction code TALYS. The overall agreement between theory and experiment obtained in first-approach calculations using default input parameters of TALYS has been appreciably improved by using modified optical model potential (OMP), deformation, and level density parameters. The OMP parameters have been extracted from theoretical fits to available experimental elastic/inelastic nucleon scattering angular distribution data by means of the coupled-channels reaction code OPTMAN. Experimental data for several new $γ$-ray lines are also reported and discussed. The astrophysical implications of our results are emphasised.

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Nuclear level densities and $γ$-ray strength functions of $^{87}\mathrm{Kr}$ -- First application of the Oslo Method in inverse kinematics

The $γ$-ray strength function ($γ$SF) and nuclear level density (NLD) have been extracted for the first time from inverse kinematic reactions with the Oslo Method. This novel technique allows measurements of these properties across a wide range of previously inaccessible nuclei. Proton-$γ$ coincidence events from the $\mathrm{d}(^{86}\mathrm{Kr}, \mathrm{p}γ)^{87}\mathrm{Kr}$ reaction were measured at iThemba LABS and the $γ$SF and NLD in $^{87}\mathrm{Kr}$ obtained. The low-energy region of the $γ$SF is compared to Shell Model calculations which suggest this region to be dominated by M1 strength. The $γ$SF and NLD are used as input parameters to Hauser-Feshbach calculations to constrain $(\mathrm{n},γ)$ cross sections of nuclei using the TALYS reaction code. These results are compared to $^{86}\mathrm{Kr}(n,γ)$ data from direct measurements.

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$γ$-ray Strength Function for Barium Isotopes

Photoneutron cross sections were measured for $^{137}$Ba and $^{138}$Ba at energies below two-neutron threshold using quasi-monochromatic $γ$-ray beams produced in laser Compton-scattering at the NewSUBARU synchrotron radiation facility. The photoneutron data are used to constrain the $γ$-ray strength function on the basis of the Hartree-Fock-Bogolyubov plus quasi-particle random phase approximation using the Gogny D1M interaction. Supplementing the experimentally constrained $γ$-ray strength function with the zero-limit E1 and M1 contributions which are unique to the deexcitation mode, we discuss radiative neutron capture cross sections relevant to the s-process nucleosynthesis of barium isotopes in the vicinity of the neutron magic number 82.

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Nuclear level densities and gamma-ray strength functions of $^{180,181,182}$Ta

Particle-$γ$ coincidence experiments were performed at the Oslo Cyclotron Laboratory with the $^{181}$Ta(d,X) and $^{181}$Ta($^{3}$He,X) reactions, to measure the nuclear level densities (NLDs) and $γ$-ray strength functions ($γ$SFs) of $^{180, 181, 182}$Ta using the Oslo method. The Back-shifted Fermi-Gas, Constant Temperature plus Fermi Gas, and Hartree-Fock-Bogoliubov plus Combinatorial models where used for the absolute normalisations of the experimental NLDs at the neutron separation energies. The NLDs and $γ$SFs are used to calculate the corresponding $^{181}$Ta(n,$γ$) cross sections and these are compared to results from other techniques. The energy region of the scissors resonance strength is investigated and from the data and comparison to prior work it is concluded that the scissors strength splits into two distinct parts. This splitting may allow for the determination of triaxiality and a $γ$ deformation of $14.9^{\circ} \pm 1.8^{\circ}$ was determined for $^{181}$Ta.

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Photoneutron cross sections for Ni isotopes: Toward understanding $(n,γ)$ cross sections relevant to the weak s-process nucleosynthesis

Photoneutron cross sections were measured for $^{58}$Ni, $^{60}$Ni, $^{61}$Ni, and $^{64}$Ni at energies between the one-neutron and two-neutron thresholds using quasi-monochromatic $γ$-ray beams produced in laser Compton-scattering at the NewSUBARU synchrotron radiation facility. The new photoneutron data are used to extract the $γ$-ray strength function above the neutron threshold complementing the information obtained by the Oslo method below the threshold. We discuss radiative neutron capture cross sections and the Maxwellian-averaged cross sections for Ni isotopes including $^{63}$Ni, a branching point nucleus along the weak s-process path. The cross sections are calculated with the experimentally constrained $γ$-ray strength functions from the Hartree-Fock-Bogolyubov plus quasi-particle-random phase approximation based on the Gogny D1M interaction for both $E1$ and $M1$ components and supplemented with the $M1$ upbend.

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Experimental $γ$-decay strength in $^{59, 60}$Ni compared with microscopic calculations

Nuclear level densities and $γ$-ray strength functions have been extracted for $^{59, 60}\rm{Ni}$, using the Oslo method on data sets from the $^{60}$Ni($^{3}$He,$^{3}$He$^{\prime}γ$)$^{60}$Ni and $^{60}$Ni($^{3}$He,$αγ$)$^{59}$Ni reactions. Above the neutron separation energy, S$_n$, we have measured the $γ$-ray strength functions for $^{61}$Ni and $^{60}$Ni in photoneutron experiments. The low-energy part of the $^{59,60}$Ni $γ$-ray strength functions show an increase for decreasing $γ$ energies. The experimental $γ$-ray strength functions are compared with $M1$ $γ$-ray strength functions calculated within the shell model. The $E1$ $γ$-ray strength function of $^{60}$Ni has been calculated using the QTBA framework. The QTBA calculations describe the data above $E_γ\approx$ 7 MeV, while the shell-model calculations agree qualitatively with the low energy part of the $γ$-ray strength function. Hence, we give a plausible explanation of the observed shape of the $γ$-decay strength.

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Low-energy enhancement and fluctuations of $γ$-ray strength functions in $^{56,57}$Fe: test of the Brink-Axel hypothesis

Nuclear level densities and $γ$-ray strength functions of $^{56,57}$Fe have been extracted from proton-$γ$ coincidences. A low-energy enhancement in the $γ$-ray strength functions up to a factor of 30 over common theoretical E1 models is confirmed. Angular distributions of the low-energy enhancement in $^{57}$Fe indicate its dipole nature, in agreement with findings for $^{56}$Fe. The high statistics and the excellent energy resolution of the large-volume LaBr$_{3}$(Ce) detectors allowed for a thorough analysis of $γ$ strength as function of excitation energy. Taking into account the presence of strong Porter-Thomas fluctuations, there is no indication of any significant excitation-energy dependence in the $γ$-ray strength function, in support of the generalized Brink-Axel hypothesis.

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Nature of low-lying electric dipole resonance excitations in 74Ge

Isospin properties of dipole excitations in 74 Ge are investigated using the (α,α'γ) reaction and compared to (γ,γ) data. The results indicate that the dipole excitations in the energy region of 6 to 9 MeV adhere to the scenario of the recently found splitting of the region of dipole excitations into two separated parts: one at low energy, being populated by both isoscalar and isovector probes, and the other at high energy, excited only by the electromagnetic probe. Relativistic quasiparticle time blocking approximation (RQTBA) calculations show a reduction in the isoscalar E1 strength with an increase in excitation energy, which is consistent with the measurement.

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Low-energy enhancement in the γ-ray strength functions of $^{73,74}$Ge

The $γ$-ray strength functions and level densities of $^{73,74}$Ge have been extracted up to the neutron separation energy S$_n$ from particle-$γ$ coincidence data using the Oslo method. Moreover, the $γ$-ray strength function of $^{74}$Ge above S$_n$ has been determined from photo-neutron measurements, hence these two experiments cover the range of E$_γ\approx$ 1-13 MeV for $^{74}$Ge. The obtained data show that both $^{73,74}$Ge display an increase in strength at low $γ$ energies. The experimental $γ$-ray strength functions are compared with $M1$ strength functions deduced from average $B(M1)$ values calculated within the shell model for a large number of transitions. The observed low-energy enhancements in $^{73,74}$Ge are adopted in the calculations of the $^{72,73}$Ge(n,$γ$) cross sections, where there are no direct experimental data. Calculated reaction rates for more neutron-rich germanium isotopes are shown to be strongly dependent on the presence of the low-energy enhancement.

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