arXiv subjects

B. W. Southern

Publications and source records attributed to B. W. Southern.

At least 19 recordsLinked to original sources

arXiv2023

Chiral nematic and fluctuation-induced first-order phase transitions in AB-stacked kagome bilayers

We study a Heisenberg-Dzyaloshinskii-Moriya Hamiltonian on AB-stacked kagome bilayers at finite temperature. In a large portion of the parameter space, we observe three transitions upon cooling the system: a crossover from Heisenberg to the XY chiral paramagnet, Kosterlitz-Thouless transition to a chiral nematic phase, and a fluctuation-induced first-order transition to an Ising-like phase. We characterize the properties of phases numerically using Monte Carlo finite-size analysis. To further explain the nature of the observed phase transitions, we develop an analytical coarse-graining procedure that maps the Hamiltonian onto a generalized XY model on a triangular lattice. To leading order, this effective model includes both bilinear and biquadratic interactions and is able to correctly predict the two phase transitions. Lastly, we study the Ising fluctuations at low temperatures and establish that the origin of the first-order transition stems from the quasi-degenerate ring manifold in the momentum space.

cond-mat.stat-mech↗

arXiv2022

Impact of Dzyaloshinskii-Moriya and anisotropic exchange interactions on the cubic kagome antiferromagnets Mn$_3$X and Mn$_3$AB

We perform a symmetry analysis of the ABC-stacked kagome planes of Mn atoms common to the $L1_2$ Mn$_3$X and antiperovskite Mn$_3$AB alloys. In addition to the single-ion-anisotropy and Kitaev-type anisotropic exchange known to stabilize 120° spin structures in these materials, our analysis results in a staggered Dzyaloshinskii-Moriya interaction and further gamma-type anisotropic exchange between nearest-neighbor spins. The presence of these new terms is shown not to affect the energetics of the 120° ground-states which explains their absence in prior minimal magnetic models. We go on to show, however, that their influence becomes apparent when spin-wave excitations are considered. We highlight these effects by calculating inelastic neutron scattering cross-sections to illustrate experimental means of probing the existence and relative strengths of these cloaked interactions.

cond-mat.str-el↗

arXiv2021

Anisotropic magnetic interactions in hexagonal AB-stacked kagome lattice structures: Applications to $\mathrm{Mn}_3\mathrm{X}$ ($\mathrm{X}$ = $\mathrm{Ge}$, $\mathrm{Sn}$, $\mathrm{Ga}$) compounds

$\mathrm{Mn}_3\mathrm{X}$ compounds in which the magnetic $\mathrm{Mn}$ atoms form AB-stacked kagome lattices have received a tremendous amount of attention since the observation of the anomalous Hall effect in $\mathrm{Mn}_3\mathrm{Ge}$ and $\mathrm{Mn}_3\mathrm{Sn}$. Although the magnetic ground state has been known for some time to be an inverse triangular structure with an induced in-plane magnetic moment, there have been several controversies about the minimal magnetic Hamiltonian. We present a general symmetry-based model for these compounds that includes a previously unreported interplane Dzyaloshinskii-Moriya interaction, as well as anisotropic exchange interactions. The latter are shown to compete with the single-ion anisotropy which strongly affects the ground state configurations and elementary spin-wave excitations. Finally, we present the calculated elastic and inelastic neutron scattering intensities and point to experimental assessment of the types of magnetic anisotropy in these compounds that may be important.

cond-mat.str-el↗

arXiv2019

Triangular array of iron-oxide nanoparticles: A simulation study of intra- and inter-particle magnetism

A study of spherical maghemite nanoparticles on a two dimensional triangular array was carried out using a stochastic Landau-Lifshitz-Gilbert (sLLG) approach. The simulation method was first validated with a triangular array of simple dipoles, where results show the expected phase transition to a ferromagnetic state at a finite temperature. The ground state exhibited a continuous degeneracy that was lifted by an order-from-disorder mechanism at infinitesimal temperatures with the appearance of a six-fold planar anisotropy. The nanoparticle array consisted of 7.5 nm diameter maghemite spheres with bulk-like superexchange interactions between Fe-ions in the core, and weaker exchange between surface Fe-ions and a radial anisotropy. The triangular nanoparticle array ordered at the same reduced temperature as the simple dipole array, but exhibited different behaviour at low temperatures due to the surface anisotropy. We find that the vacancies on the octahedral sites in the nanoparticles combine with the surface anisotropy to produce an effective random temperature-dependent anisotropy for each particle. This leads to a reduction in the net magnetization of the nanoparticle array at zero temperature compared to the simple dipole array.

cond-mat.mes-hall↗

arXiv2018

Impact of further-range exchange and cubic anisotropy on magnetic excitations in the fcc kagome antiferromagnet IrMn3

Exchange interactions up to fourth nearest neighbor are shown within a classical local-moment Heisenberg approach to be important to model inelastic neutron scattering data on the fcc kagome antiferromagnet IrMn$_3$. Spin wave frequencies are calculated using the torque equation and the magnetic scattering function, $S({\bf Q},ω)$, is determined by a Green's function method, as an extension of our previous work, LeBlanc et al, Phys. Rev. B 90, 144403 (2014). Results are compared with intensity contour data on powder samples of ordered IrMn$_3$, where magnetic Mn ions occupy lattice sites of ABC stacked kagome planes. Values of exchange parameters taken from DFT calculations used in our model provide good agreement with the experimental results only if further-neighbor exchange is included. Estimates of the observed energy gap support the existence of strong cubic anisotropy predicted by DFT calculations.

cond-mat.str-el↗

arXiv2017

Dipolar ferromagnetism in three-dimensional superlattices of nanoparticles

A series of atomistic finite temperature simulations on a model of an FCC lattice of maghemite nanoparticles using the stochastic Landau-Lifshitz-Gilbert (sLLG) equation are presented. The model exhibits a ferromagnetic transition that is in good agreement with theoretical expectations. The simulations also reveal an orientational disorder in the orientational order parameter for $T < 0.5 T_c$ due to pinning of the surface domain walls of the nanoparticles by surface vacancies. The extent of the competition between surface pinning and dipolar interactions provides support for the conjecture that recent measurements on systems of FCC superlattices of iron-oxide nanoparticles provide evidence for dipolar ferromagnetism is discussed.

cond-mat.mes-hall↗

arXiv2015

Monte Carlo simulations of the kagome lattice with magnetic dipolar interactions

The results of extensive Monte Carlo simulations of classical spins on the two-dimensional kagome lattice with only dipolar interactions are presented. In addition to revealing the six-fold degenerate ground state, the nature of the finite-temperature phase transition to long-range magnetic order is discussed. Low temperature states consisting of mixtures of degenerate ground state configurations separated by domain walls can be explained as a result of competing exchange-like and shape anisotropy-like terms in the dipolar coupling. Fluctuations between pairs of degenerate spin configurations are found to persist well into the ordered state as the temperature is lowered until locking in to a low-energy state.

cond-mat.mtrl-sci↗

arXiv2014

Spin waves in the anisotropic fcc kagome antiferromagnet

Spin wave calculations demonstrate that the macroscopic continuous degeneracy associated with the two-dimensional kagome Heisenberg spin lattice persists in the case of the stacked fcc structure giving rise to zero energy modes in three dimensions. The addition of an effective local cubic anisotropy is shown to remove this continuous degeneracy and introduce a gap in the spectrum as well as modify the inelastic scattering function $S({\bf q},ω)$. This scenario supports earlier Monte Carlo simulations which indicate that the phase transition to long range $q=0$ magnetic order is driven to be discontinuous by critical fluctuations associated with the large degeneracy in the absence of anisotropy, but becomes continuous with the addition of anisotropy. The results are relevant to Ir-Mn alloys which are widely used in the magnetic storage industry in thin film form as the antiferromagnetic pinning layer in spin-valve structures.

cond-mat.str-el↗

arXiv2013

Electrical Detection of Direct and Alternating Spin Current Injected from a Ferromagnetic Insulator into a Ferromagnetic Metal

We report room temperature electrical detection of spin injection from a ferromagnetic insulator (YIG) into a ferromagnetic metal (Permalloy, Py). Non-equilibrium spins with both static and precessional spin polarizations are dynamically generated by the ferromagnetic resonance of YIG magnetization, and electrically detected by Py as dc and ac spin currents, respectively. The dc spin current is electrically detected via the inverse spin Hall effect of Py, while the ac spin current is converted to a dc voltage via the spin rectification effect of Py which is resonantly enhanced by dynamic exchange interaction between the ac spin current and the Py magnetization. Our results reveal a new path for developing insulator spintronics, which is distinct from the prevalent but controversial approach of using Pt as the spin current detector.

cond-mat.mtrl-sci↗

arXiv2012

Monte Carlo simulations of magnetic ordering in the fcc Kagome lattice

Monte Carlo simulation results are reported on magnetic ordering in ABC stacked Kagomé layers with fcc symmetry for both XY and Heisenberg models which include exchange interactions with the eight near-neighbors. Well known degeneracies of the 2D system persist in the 3D case and analysis of the numerical data provides strong evidence for a fluctuation-driven first-order transition to well-defined long-range order characterized as the layered $q=0$ (120-degree) spin structure. Effects of varying the inter-layer coupling are also examined. The results are relevant to understanding the role of frustration in IrMn$_3$ alloys widely used by the magnetic storage industry as thin-films in the antiferromagnetic pinning layer in GMR and TMR spin valves. Despite the technological importance of this structure, it has not previously been noted that the magnetic Mn-ions of fcc IrMn$_3$ form Kagomé layers.

cond-mat.str-el↗

arXiv2010

Monte Carlo Study of Maghemite Nanoparticles

We consider a simple model of maghemite nanoparticles and study their magnetic properties using Monte Carlo methods. The particles have a spherical geometry with diameters ranging from 3 nm to 8 nm. The interior of the particles consists of core spins with exchange interactions and anisotropy given by the values in the bulk material. The outer layer of the particles consists of surface spins with weaker exchange interactions but an enhanced anisotropy. The thermal behaviour of the total, core and surface magnetizations are calculated as well as the hysteresis loops due to the application of an applied field. The effect of the surface anisotropy on the blocking temperature, the coercive and exchange bias fields is studied.

cond-mat.stat-mech↗

arXiv2006

Short-time dynamics of a family of XY noncollinear magnets

Critical scaling and universality in the short-time dynamics for antiferromagnetic models on a three-dimensional stacked triangular lattice are investigated using Monte Carlo simulation. We have determined the critical point by searching for the best power law for the order parameter as a function of time and measured the critical exponents. Our results indicate that it is possible to distinguish weak first-order from second-order phase transitions and confirm that XY antiferromagnetic systems undergo a (weak) first order phase transition.

cond-mat.stat-mech↗

arXiv2004

Critical properties of a continuous family of XY noncollinear magnets

Monte Carlo methods are used to study a family of three dimensional XY frustrated models interpolating continuously between the stacked triangular antiferromagnets and a variant of this model for which a local rigidity constraint is imposed. Our study leads us to conclude that generically weak first order behavior occurs in this family of models in agreement with a recent nonperturbative renormalization group description of frustrated magnets.

cond-mat.stat-mech↗

arXiv2004

Chiral mixed phase in disordered 3d Heisenberg models

Using Monte Carlo simulations, we compute the spin stiffness of a site-random 3d Heisenberg model with competing ferromagnetic and antiferromagnetic interactions. Our results for the pure limit yield values of the the critical temperature and the critical exponent $ν$ in excellent agreement with previous high precision studies. In the disordered case, a mixed "chiral" phase is found which may be in the same universality class as 3d Heisenberg spin glasses.

cond-mat.stat-mech↗

arXiv2003

Frustrated Heisenberg Antiferromagnets between d=2 and d=3

The antiferromagnetic Heisenberg model on a stacked triangular geometry with a finite number of layers is studied using Monte Carlo methods. A topological phase transition occurs at finite temperature for all film thicknesses. Our results indicate that topological excitations are important for a complete understanding of the critical properties of the model between two and three dimensions.

cond-mat.stat-mech↗

arXiv2003

Damage spreading in two dimensional geometrically frustrated lattices: the triangular and kagome anistropic Heisenberg model

The technique of damage spreading is used to study the phase diagram of the easy axis anisotropic Heisenberg antiferromagnet on two geometrically frustrated lattices. The triangular and kagome systems are built up from triangular units that either share edges or corners respectively. The triangular lattice undergoes two sequential Kosterlitz-Thouless transitions while the kagome lattice undergoes a glassy transition. In both cases, the phase boundaries obtained using damage spreading are in good agreement with those obtained from equilibrium Monte Carlo simulations.

cond-mat.stat-mech↗

arXiv2003

Low Temperature Static and Dynamic Behaviour of the Easy-Axis Heisenberg Antiferromagnet on the Kagome Lattice

The antiferromagnetic Heisenberg model with easy-axis exchange anisotropy on the Kagome lattice is studied by means of Monte Carlo simulations. From equilibrium properties, we find that the values of the critical exponents associated with the magnetization at the critical temperature $T_c$ vary with the magnitude of the anisotropy. On the other hand, the spin-spin autocorrelation functions have a stretched exponential behavior with a power law divergence of the relaxation time at a glass-like temperature $T_g \sim T_c$. From non-equilibrium dynamics at a fixed temperature below $T_g$, aging effects are found which obey the same scaling laws as in spin glasses and polymers.

cond-mat.stat-mech↗

arXiv2003

Off Equilibrium Study of the Fluctuation-Dissipation Relation in the Easy-Axis Heisenberg Antiferromagnet on the Kagome Lattice

Violation of the fluctuation-dissipation theorem (FDT) in a frustrated Heisenberg model on the Kagome lattice is investigated using Monte Carlo simulations. The model exhibits glassy behaviour at low temperatures accompanied by very slow dynamics. Both the spin-spin autocorrelation function and the response to an external magnetic field are studied. Clear evidence of a constant value of the fluctuation dissipation ratio and long range memory effects are observed for the first time in this model. The breakdown of the FDT in the glassy phase follows the predictions of the mean field theory for spin glasses with one-step replica symmetry breaking.

cond-mat.stat-mech↗