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B. Xu

Publications and source records attributed to B. Xu.

At least 37 records · Page 2Linked to original sources

Muon spin rotation and infrared spectroscopy study of $Ba_{1-x}Na_{x}Fe_{2}As_{2}$

The magnetic and superconducting properties of a series of underdoped $Ba_{1-x}Na_{x}Fe_{2}As_{2}$ (BNFA) single crystals with $0.19 \leq x\leq 0.34$ has been investigated with the complementary muon-spin-rotation ($μ$SR) and infrared spectroscopy techniques. The focus has been on the different antiferromagnetic states in the underdoped regime and their competition with superconductivity, especially for the ones with a tetragonal crystal structure and a so-called double-$Q$ magnetic order. Besides the collinear state with a spatially inhomogeneous spin-charge-density wave (i-SCDW) order at $x=0.24$ and $0.26$, that was previously identified in BNFA, we obtained evidence for an orthomagnetic state with a "hedgehog"-type spin vortex crystal (SVC) structure at $x=0.32$ and $0.34$. Whereas in the former i-SCDW state the infrared spectra show no sign of a superconducting response down to the lowest measured temperature of about 10K, in the SVC state there is a strong superconducting response similar to the one at optimum doping. The magnetic order is strongly suppressed here in the superconducting state and at $x=0.34$ there is even a partial re-entrance into a paramagnetic state at $T<<T_c$.

cond-mat.supr-con↗

Superconductivity-induced transverse plasma mode and phonon anomaly in the $c$-axis response of the bilayer compound RbCa$_2$Fe$_4$As$_4$F$_2$

With infrared spectroscopy we studied the out-of-plane ($c$-axis) response of the iron arsenide superconductor ACa$_2$Fe$_4$As$_4$F$_2$ (A = Rb,Cs) which has a bilayer structure similar to the high $T_c$ cuprates YBa$_2$Cu$_3$O$_7$ (YBCO) and Bi$_2$Sr$_2$CaCu$_2$O$_8$ (Bi2212). In analogy to the cuprates, we observe a superconductivity-induced transverse plasma mode (tPM) and a phonon anomaly that are both signatures of local electric field effects that arise from a large difference between the local conductivities in the intra- and inter-bilayer regions. Using a multilayer model developed for the cuprates, we obtain a good description of the $c$-axis response and derive the local conductivities at $T \simeq T_c$ of $σ_1^{\mathrm{bl}}(ω\rightarrow 0) \simeq$ 1\,000 $Ω^{-1}\mathrm{cm}^{-1}$ and $σ_1^{\mathrm{int}}(ω\rightarrow 0) \simeq$ 15 $Ω^{-1}\mathrm{cm}^{-1}$, respectively, that are similar to the ones previously found in underdoped YBCO. Different from the cuprates, we find no evidence of a normal state pseudogap in terms of a partial suppression of the low-energy electronic states that sets in already well above $T_c$. There is also no clear sign of an onset of precursor superconducting pairing correlations well above $T_c \simeq$ 30~K. This highlights that the pseudogap and the precursor superconducting pairing well above $T_c$ are unique features of the cuprates with their strong electronic correlations and, for example, not just the result of a strongly anisotropic electronic response due to the layered crystal structure.

cond-mat.supr-con↗

Electrical spin injection into InGaAs/GaAs quantum wells: a comparison between MgO tunnel barriers grown by sputtering and molecular beam epitaxy methods

An efficient electrical spin injection into an InGaAs/GaAs quantum well light emitting diode is demonstrated thanks to a CoFeB/MgO spin injector. The textured MgO tunnel barrier is fabricated by two different techniques: sputtering and molecular beam epitaxy (MBE). The maximal spin injection efficiency is comparable for both methods. Additionally, the effect of annealing is also investigated for the two types of samples. Both samples show the same trend: an increase of the electroluminescence circular polarization (Pc) with the increase of annealing temperature, followed by a saturation of Pc beyond 350°C annealing. Since the increase of Pc starts well below the crystallization temperature of the full CoFeB bulk layer, this trend could be mainly due to an improvement of chemical structure at the top CoFeB/MgO interface. This study reveals that the control of CoFeB/MgO interface is essential important for an optimal spin injection into semiconductor.

cond-mat.mtrl-sci↗

Optical Signature of a Crossover from Mott- to Slater-type Gap in Sr$_2$Ir$_{1-x}$Rh$_{x}$O$_{4}$

With optical spectroscopy we provide evidence that the insulator-metal transition in Sr$_2$Ir$_{1-x}$Rh$_{x}$O$_{4}$ occurs close to a crossover from the Mott- to the Slater-type. The Mott-gap at $x = 0$ persists to high temperature and evolves without an anomaly across the Néel temperature, $T_N$. Upon Rh-doping, it collapses rather rapidly and vanishes around $x = 0.055$. Notably, just as the Mott-gap vanishes yet another gap appears that is of the Slater-type and develops right below $T_N$. This Slater-gap is only partial and is accompanied by a reduced scattering rate of the remaining free carriers, similar as in the parent compounds of the iron arsenide superconductors.

cond-mat.str-el↗

Infrared spectroscopy study of the in-plane response of YBa2Cu3O6.6 in magnetic fields up to 30 Tesla

With Terahertz and Infrared spectroscopy we studied the in-plane response of an underdoped YBa2Cu3O6.6 single crystal with Tc=58(1) K in high magnetic fields up to B=30 Tesla applied along the c-axis. Our goal was to investigate the field-induced suppression of superconductivity and to observe the signatures of the three dimensional (3d) incommensurate copper charge density wave (Cu-CDW) which was previously shown to develop at such high magnetic fields. Our study confirms that a B-field in excess of 20 Tesla gives rise to a full suppression of the macroscopic response of the superconducting condensate. However, it reveals surprisingly weak signatures of the 3d Cu-CDW at high magnetic fields. At 30 Tesla there is only a weak reduction of the spectral weight of the Drude-response (by about 3%) that is accompanied by an enhancement of two narrow electronic modes around 90 and 240 cm-1, that are interpreted in terms of pinned phase modes of the CDW along the a- and b-direction, respectively, and of the so-called mid-infrared (MIR) band. The pinned phased modes and the MIR band are strong features already without magnetic field which suggests that prominent but short-ranged and slowly fluctuating (compared to the picosecond IR-time scale) CDW correlations exist all along, i.e., even at zero magnetic field.

cond-mat.supr-con↗

Production of ultra-low radioactivity NaI(Tl) crystals for Dark Matter detectors

Scintillating NaI(Tl) crystals are widely used in a large variety of experimental applications. However, for the use as Dark Matter (DM) detectors, such crystals demand a high level of radio-purity, not achievable by means of standard industrial techniques. One of the main difficulties comes from the presence of potassium that always accompanies sodium in alkali halides. On the other hand, the arguable DM detection by DAMA experiment using NaI(Tl) scintillating crystals requires a reliable verification able to either confirm the existence of DM or rule out the DAMA claim. Ultra-low radioactivity NaI(Tl) crystals, particularly with very low potassium content, are therefore indispensable to overcome the current stalemate in Dark Matter searches. Nonetheless, apart from DAMA-LIBRA experiments, to date, no other experiment has succeeded in building a detector from NaI(Tl) crystals with potassium content of ppb level. This work describes recent results in the preparation of ultra-radio-pure NaI(Tl) crystals using a modified Bridgman method. A double-walled platinum crucible technique has been designed and reliability tests show that 5 ppb of potassium in the NaI(Tl) crystals of 2 and 3 inches in diameter can be achieved starting from NaI powder with potassium content of the order of 10 ppb. The potassium excess is segregated in the tail-side of the as grown ingot where measured potassium concentration is above 20 ppb. The purifying effect of Bridgman growth for larger NaI(Tl) crystals is currently being tested. The work also reports on scintillation parameters of our NaI(Tl) crystals measured in a dedicated setup conceived for naked, hygroscopic crystals. The reproducible and reliable production of ultra-low radioactivity NaI(Tl) crystals reported in this work will hopefully spur the construction of new DM search experiments and, anyway, clarify the controversial DAMA-LIBRA results.

physics.ins-det↗

Band-selective clean- and dirty-limit superconductivity with nodeless gaps in the bilayer iron-based superconductor CsCa$_2$Fe$_4$As$_4$F$_2$

The optical properties of the new iron-based superconductor CsCa$_2$Fe$_4$As$_4$F$_2$ with $T_c \sim 29$~K have been determined. In the normal state a good description of the low-frequency response is obtained with a superposition of two Drude components of which one has a very low scattering rate (narrow Drude-peak) and the other a rather large one (broad Drude-peak). Well below $T_c \sim 29$~K, a pronounced gap feature is observed which involves a complete suppression of the optical conductivity below $\sim$ 110~cm$^{-1}$ and thus is characteristic of a nodeless superconducting state. The optical response of the broad Drude-component can be described with a dirty-limit Mattis-Bardeen-type response with a single isotropic gap of $2Δ\simeq 14$~meV. To the contrary, the response of the narrow Drude-component is in the ultra-clean-limit and its entire spectral weight is transferred to the zero-frequency $δ(ω)$ function that accounts for the loss-free response of the condensate. These observations provide clear evidence for a band-selective coexistence of clean- and dirty-limit superconductivity with nodeless gaps in CsCa$_2$Fe$_4$As$_4$F$_2$.

cond-mat.supr-con↗

The CLIC Potential for New Physics

The Compact Linear Collider (CLIC) is a mature option for the future of high energy physics. It combines the benefits of the clean environment of $e^+e^-$ colliders with operation at high centre-of-mass energies, allowing to probe scales beyond the reach of the Large Hadron Collider (LHC) for many scenarios of new physics. This places the CLIC project at a privileged spot in between the precision and energy frontiers, with capabilities that will significantly extend knowledge on both fronts at the end of the LHC era. In this report we review and revisit the potential of CLIC to search, directly and indirectly, for physics beyond the Standard Model.

hep-ph↗

Tracking ultrafast photocurrents in the Weyl semimetal TaAs using THz emission spectroscopy

We investigate polarization-dependent ultrafast photocurrents in the Weyl semimetal TaAs using terahertz (THz) emission spectroscopy. Our results reveal that highly directional, transient photocurrents are generated along the non-centrosymmetric c-axis regardless of incident light polarization, while helicity-dependent photocurrents are excited within the ab-plane. This is consistent with earlier static photocurrent experiments, and demonstrates on the basis of both the physical constraints imposed by symmetry and the temporal dynamics intrinsic to current generation and decay that optically induced photocurrents in TaAs are inherent to the underlying crystal symmetry of the transition metal monopnictide family of Weyl semimetals.

cond-mat.str-el↗

Temperature-driven Topological Phase Transition and Intermediate Dirac Semimetal Phase in ZrTe$_5$

We present an infrared spectroscopy study of ZrTe$_5$, which confirms a recent theoretical proposal that this material exhibits a temperature-driven topological quantum phase transition from a weak to a strong topological insulating state with an intermediate Dirac semimetal state around $T_p \simeq$ 138K. Our study details the temperature evolution of the energy gap in the bulk electronic structure. We found that the energy gap closes around $T_p$ where the optical response exhibits characteristic signatures of a Dirac semimetal state, i.e. a linear frequency-dependent optical conductivity extrapolating to the origin (after subtracting a weak Drude response). This finding allows us to reconcile previous diverging reports about the topological nature of ZrTe$_5$ in terms of a variation of $T_p$ that depends on the crystal growth condition.

cond-mat.mtrl-sci↗

Scaling of the Fano effect of the in-plane Fe-As phonon and the superconducting critical temperature in Ba$_{1-x}$K$_{x}$Fe$_{2}$As$_{2}$

By means of infrared spectroscopy we determine the temperature-doping phase diagram of the Fano effect for the in-plane Fe-As stretching mode in Ba$_{1-x}$K$_{x}$Fe$_{2}$As$_{2}$. The Fano parameter $1/q^2$, which is a measure of the phonon coupling to the electronic particle-hole continuum, shows a remarkable sensitivity to the magnetic/structural orderings at low temperatures. More strikingly, at elevated temperatures in the paramagnetic/tetragonal state we find a linear correlation between $1/q^2$ and the superconducting critical temperature $T_c$. Based on theoretical calculations and symmetry considerations, we identify the relevant interband transitions that are coupled to the Fe-As mode. In particular, we show that a sizable $xy$ orbital component at the Fermi level is fundamental for the Fano effect and possibly also for the superconducting pairing.

cond-mat.supr-con↗

Optical study of Dirac fermions and related phonon anomalies in antiferromagnetic compound CaFeAsF

We performed optical studies on CaFeAsF single crystals, a parent compound of the 1111-type iron-based superconductors that undergoes a structural phase transition from tetragonal to orthorhombic at $T_s$ = 121 K and a magnetic one to a spin density wave (SDW) state at $T_N$ = 110 K. In the low temperature optical conductivity spectrum, after the subtraction of a narrow Drude peak, we observe a pronounced singularity around 300 cm$^{-1}$ that separates two regions of quasilinear conductivity. We outline that these characteristic absorption features are signatures of Dirac fermions, similar to what was previously reported for the BaFe$_2$As$_2$ system [1]. In support of this interpretation, we show that for the latter system this singular feature disappears rapidly upon electron and hole doping, as expected if it arises from a van Hove singularity in-between two Dirac cones. Finally, we show that one of the infrared-active phonon modes (the Fe-As mode at 250 cm$^{-1}$) develops a strongly asymmetric line shape in the SDW state and note that this behaviour can be explained in terms of a strong coupling with the Dirac fermions.

cond-mat.supr-con↗

Electrical initialization of electron and nuclear spins in a single quantum dot at zero magnetic field

The emission of circularly polarized light from a single quantum dot relies on the injection of carriers with well-defined spin polarization. Here we demonstrate single dot electroluminescence (EL) with a circular polarization degree up to 35% at zero applied magnetic field. The injection of spin polarized electrons is achieved by combining ultrathin CoFeB electrodes on top of a spin-LED device with p-type InGaAs quantum dots in the active region. We measure an Overhauser shift of several $μ$eV at zero magnetic field for the positively charged exciton (trion X$^+$) EL emission, which changes sign as we reverse the injected electron spin orientation. This is a signature of dynamic polarization of the nuclear spins in the quantum dot induced by the hyperfine interaction with the electrically injected electron spin. This study paves the way for electrical control of nuclear spin polarization in a single quantum dot without any external magnetic field.

cond-mat.mes-hall↗

Infrared probe of the gap evolution across the phase diagram of Ba$_{1-x}$K$_{x}$Fe$_{2}$As$_{2}$

We measured the optical conductivity of superconducting single crystals of Ba$_{1-x}$K$_{x}$Fe$_{2}$As$_{2}$ with $x$ ranging from 0.40 (optimal doping, $T_c = 39$ K) down to 0.20 (underdoped, $T_c = 16$ K), where a magnetic order coexists with superconductivity. In the normal state, the low-frequency optical conductivity can be described by an incoherent broad Drude component and a coherent narrow Drude component: the broad one is doping-independent, while the narrow one shows strong scattering in the heavily underdoped compound. In the superconducting state, the formation of the condensate leads to a low-frequency suppression of the optical conductivity spectral weight. In the heavily underdoped region, the superfluid density is significantly suppressed, and the weight of unpaired carriers rapidly increases. We attribute these results to changes in the superconducting gap across the phase diagram, which could show a nodal-to-nodeless transition due to the strong interplay between magnetism and superconductivity in underdoped Ba$_{1-x}$K$_{x}$Fe$_{2}$As$_{2}$.

cond-mat.supr-con↗

Determining Cosmology for a Nonlocal Realization of MOND

We numerically determine the cosmological branch of the free function in a nonlocal metric-based modification of gravity which provides a relativistic generalization of Milgrom's Modified Newtonian Dynamics. We are able to reproduce the $Λ$CDM expansion history over virtually all of cosmic history, including the era of radiation domination during Big Bang Nucleosynthesis, the era of matter domination during Recombination, and most of the era of vacuum energy domination. The very late period of $0 \leq z < 0.0880$, during which the model deviates from the $Λ$CDM expansion history, is interesting because it causes the current value of the Hubble parameter to be about 4.5\% larger than it would be for the $Λ$CDM model. This may resolve the tension between inferences of $H_0$ which are based on data from large redshift and inferences based on Hubble plots.

gr-qc↗

Temperature-tunable Fano resonance induced by strong coupling between Weyl fermions and phonons in TaAs

Strong coupling between discrete phonon and continuous electron-hole pair excitations can give rise to a pronounced asymmetry in the phonon line shape, known as the Fano resonance. This effect has been observed in a variety of systems, such as stripe-phase nickelates, graphene and high-$T_{c}$ superconductors. Here, we reveal explicit evidence for strong coupling between an infrared-active $A_1$ phonon and electronic transitions near the Weyl points (Weyl fermions) through the observation of a Fano resonance in the recently discovered Weyl semimetal TaAs. The resultant asymmetry in the phonon line shape, conspicuous at low temperatures, diminishes continuously as the temperature increases. This anomalous behavior originates from the suppression of the electronic transitions near the Weyl points due to the decreasing occupation of electronic states below the Fermi level ($E_{F}$) with increasing temperature, as well as Pauli blocking caused by thermally excited electrons above $E_{F}$. Our findings not only elucidate the underlying mechanism governing the tunable Fano resonance, but also open a new route for exploring exotic physical phenomena through the properties of phonons in Weyl semimetals.

cond-mat.str-el↗

Optical observation of spin-density-wave fluctuations in Ba122 iron-based superconductors

In iron-based superconductors, a spin-density-wave (SDW) magnetic order is suppressed with doping and unconventional superconductivity appears in close proximity to the SDW instability. The optical response of the SDW order shows clear gap features: substantial suppression in the low-frequency optical conductivity, alongside a spectral weight transfer from low to high frequencies. Here, we study the detailed temperature dependence of the optical response in three different series of the Ba122 system [Ba$_{1-x}$K$_{x}$Fe$_{2}$As$_{2}$, Ba(Fe$_{1-x}$Co$_{x}$)$_{2}$As$_{2}$ and BaFe$_{2}$(As$_{1-x}$P$_{x}$)$_{2}$]. Intriguingly, we found that the suppression of the low-frequency optical conductivity and spectral weight transfer appear at a temperature $T^{\ast}$ much higher than the SDW transition temperature $T_{SDW}$. Since this behavior has the same optical feature and energy scale as the SDW order, we attribute it to SDW fluctuations. Furthermore, $T^{\ast}$ is suppressed with doping, closely following the doping dependence of the nematic fluctuations detected by other techniques. These results suggest that the magnetic and nematic orders have an intimate relationship, in favor of the magnetic-fluctuation-driven nematicity scenario in iron-based superconductors.

cond-mat.supr-con↗

Spin-flop transition and magnetic phase diagram in CaCo$_{2}$As$_{2}$ revealed by torque measurements

The magnetic properties of CaCo$_{2}$As$_{2}$ single crystal was systematically studied by using dc magnetization and magnetic torque measurements. A paramagnetic to antiferromagnetic transition occurs at $T_N$ = 74 K with Co spins being aligned parallel to the c axis. For $H \parallel c$, a field-induced spin-flop transition was observed below $T_N$ and a magnetic transition from antiferromagnetic to paramagnetic was inferred from the detailed analysis of magnetization and magnetic torque. Finally, we summarize the magnetic phase diagram of CaCo$_{2}$As$_{2}$ based on our results in the \emph{H-T} plane.

cond-mat.supr-con↗