A low-temperature setup for lock-in technique based dynamic magnetoelectric coupling measurements
Magnetoelectric (ME) phenomena in emerging material classes, such as two-dimensional van der Waals (vdW) magnets and Single-Molecule Magnets (SMMs), hold immense promise for next-generation cryogenic memory and quantum technologies. However, ME coupling in these systems predominantly manifests at low temperatures, making a sensitive, cryo-compatible ME characterization techniques critical. To address this requirement, we report the design, validation, and performance of a custom closed-cycle refrigerator-based setup for dynamic lock-in ME coupling measurements across 20-300 K under dc magnetic fields up to 7.5 kOe. Key design considerations for mitigating parasitic inductive background signals are also presented. The setup was validated on a CoFe2O4-BaTiO3 (CFO-BTO) particulate composite, reproducing the characteristic room-temperature butterfly ME loop with a maximum ME coefficient value of 0.23 mV/cm-Oe at ~ 3 kOe. Temperature-dependent measurements resolved ME anomalies at ~ 200 K and 280 K, coinciding with the rhombohedral-orthorhombic and orthorhombic-tetragonal structural transitions of BaTiO3, and were corroborated by simultaneous dielectric measurements on the same sample without cryostat reconfiguration. The instrument enables reliable ME and dielectric characterization down to 20 K, making it well suited for probing weak magnetoelectric coupling and phase transitions in multiferroic composites and quantum materials.